Articles | Volume 16, issue 22
https://doi.org/10.5194/amt-16-5697-2023
https://doi.org/10.5194/amt-16-5697-2023
Research article
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28 Nov 2023
Research article | Highlight paper |  | 28 Nov 2023

Ground-to-UAV, laser-based emissions quantification of methane and acetylene at long standoff distances

Kevin C. Cossel, Eleanor M. Waxman, Eli Hoenig, Daniel Hesselius, Christopher Chaote, Ian Coddington, and Nathan R. Newbury

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Cited articles

Alfieri, S., Amato, U., Carfora, M. F., Esposito, M., and Magliulo, V.: Quantifying trace gas emissions from composite landscapes: A mass-budget approach with aircraft measurements, Atmos. Environ., 44, 1866–1876, https://doi.org/10.1016/j.atmosenv.2010.02.026, 2010. 
Amediek, A., Ehret, G., Fix, A., Wirth, M., Büdenbender, C., Quatrevalet, M., Kiemle, C., and Gerbig, C.: CHARM-F – a new airborne integrated-path differential-absorption lidar for carbon dioxide and methane observations: measurement performance and quantification of strong point source emissions, Appl. Opt., 56, 5182, https://doi.org/10.1364/AO.56.005182, 2017. 
Bai, M., Loh, Z., Griffith, D. W. T., Turner, D., Eckard, R., Edis, R., Denmead, O. T., Bryant, G. W., Paton-Walsh, C., Tonini, M., McGinn, S. M., and Chen, D.: Performance of open-path lasers and Fourier transform infrared spectroscopic systems in agriculture emissions research, Atmos. Meas. Tech., 15, 3593–3610, https://doi.org/10.5194/amt-15-3593-2022, 2022. 
Bailey, D. M., Adkins, E. M., and Miller, J. H.: An open-path tunable diode laser absorption spectrometer for detection of carbon dioxide at the Bonanza Creek Long-Term Ecological Research Site near Fairbanks, Alaska, Appl. Phys. B, 123, 245, https://doi.org/10.1007/s00340-017-6814-8, 2017. 
Bell, C., Rutherford, J., Brandt, A., Sherwin, E., Vaughn, T., and Zimmerle, D.: Single-blind determination of methane detection limits and quantification accuracy using aircraft-based LiDAR, Elementa Science of the Anthropocene, 10, 00080, https://doi.org/10.1525/elementa.2022.00080, 2022. 
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Executive editor
As the Editor states does this manuscript describe application of long-path absorption spectroscopy to detection of gas leak plumes. The technique uses an unmanned aerial vehicle (UAV) carrying a retroreflector as the endpoint of the absorption path, which allows for rapid discovery of plume location and quantification of plume cross section for emissions rate determination. The technique works at a safe standoff distance and through the use of the UAV doesn't need two fixed end locations. It would be of interest to many seeking to find and quantify gas leaks, which is important for safety and minimizing greenhouse gas and reactive gas emissions.
Short summary
Measurements of the emission rate of a gas or gases from point and area sources are important in a range of monitoring applications. We demonstrate a method for rapid quantification of the emission rate of multiple gases using a spatially scannable open-path sensor. The open-path spectrometer measures the total column density of gases between the spectrometer and a retroreflector mounted on an uncrewed aerial vehicle (UAV). By scanning the UAV altitude, we can determine the total gas emissions.
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