Articles | Volume 16, issue 15
https://doi.org/10.5194/amt-16-3653-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-16-3653-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
08 Aug 2023
Research article |
| 08 Aug 2023
| 08 Aug 2023
Concept, absolute calibration, and validation of a new benchtop laser imaging polar nephelometer
Alireza Moallemi
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
now at: Extreme Environments Research Lab (EPFL), School of Architecture, Civil and Environmental Engineering, EPFL, Sion, Switzerland
Robin L. Modini
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
Benjamin T. Brem
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
Barbara Bertozzi
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
Philippe Giaccari
Micos Engineering GmbH, 8600 Dübendorf, Switzerland
Laboratory of Atmospheric Chemistry, Paul Scherrer Institute (PSI), 5232 Villigen, Switzerland
Related authors
No articles found.
Cuiqi Zhang, Xiaoli Shen, Justin Jacquot, Larissa Lacher, Selvakumar Vishnupriya, Benjamin T. Brem, Robin L. Modini, Nora Nowak, Michael Sprenger, Martin Steinbacher, Stephan Henne, Martine Collaud Coen, Franz Conen, Kristina Höhler, Ottmar Möhler, Martin Gysel-Beer, Daniel J. Cziczo, and Zamin A. Kanji
EGUsphere, https://doi.org/10.5194/egusphere-2026-5645, https://doi.org/10.5194/egusphere-2026-5645, 2026
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
Clouds play a key role in weather and climate, but the particles that trigger cloud ice formation are difficult to identify directly. By simulating clouds in a cloud chamber and particle measurements at a mountain station, we found that mineral dust was the main trigger of cloud ice formation. Dust from local construction and transported from higher atmospheric layers both contributed. The study shows that both human activities and atmospheric processes can influence cloud formation.
Arlett Díaz-Zurita, Simone Brunamonti, Alexander Haefele, Martine Collaud Coen, Giovanni Martucci, Benjamin Tobias Brem, Martin Gysel-Beer, Hassan Lyamani, Gloria Titos, Daniel Pérez-Ramírez, Christoph Hüglin, Lucas Alados-Arboledas, Alejandro Keller, Frank Gunther Wienhold, Maxime Hervo, and Francisco Navas-Guzmán
EGUsphere, https://doi.org/10.5194/egusphere-2026-4361, https://doi.org/10.5194/egusphere-2026-4361, 2026
Short summary
Short summary
This study provides a unique framework for assessing aerosol hygroscopicity by combining Raman lidar observations with vertically resolved in situ measurements from the balloon-borne Compact Backscatter Aerosol Detector coupled with Vaisala RS41 radiosondes and ground-based tandem nephelometers. The three approaches showed good agreement. Raman lidar identified more than 200 hygroscopic aerosol layers, constituting one of the largest datasets available for statistical investigations.
Akriti Masoom, Stelios Kazadzis, Robin Lewis Modini, Martin Gysel-Beer, Julian Gröbner, Martine Collaud Coen, Francisco Navas-Guzman, Natalia Kouremeti, Benjamin Tobias Brem, Nora Kristina Nowak, Giovanni Martucci, and Maxime Hervo
Atmos. Chem. Phys., 26, 10801–10834, https://doi.org/10.5194/acp-26-10801-2026, https://doi.org/10.5194/acp-26-10801-2026, 2026
Short summary
Short summary
This article aims at providing details on the spectral aerosol properties observed during 2023 Canadian wildfire plume transport and exploring the synergism between remote sensing and in situ measurements for investigating the cause of the occurrence of the observations of spectral aerosol properties.
Julian Weng, Yufang Hao, Benjamin T. Brem, Tianqu Cui, Peeyush Khare, Lubna Dada, Kaspar R. Daellenbach, Sophie Darfeuil, Gaëlle Uzu, Jean-Luc Jaffrezo, Martin Steinbacher, Stefan Reimann, Thaleia Gkraikou, Konstantina Oikonomou, Jean Sciare, Martine Collaud Coen, Claudia Mohr, Andre S. H. Prévôt, Martin Gysel-Beer, Imad El Haddad, and Patrik Winiger
EGUsphere, https://doi.org/10.5194/egusphere-2026-3660, https://doi.org/10.5194/egusphere-2026-3660, 2026
Short summary
Short summary
Long-term observations at the Jungfraujoch High Altitude Research Station show that, alongside air mass transport, sustained oxidative processing shaped by atmospheric water vapor plays a central role in driving aerosol loading and composition. Combining detailed aerosol chemical characterization with process-level insights, we provide important observational benchmarks for improving atmospheric model performance in the remote free troposphere, where uncertainties remain particularly high.
Martina Mazzini, Diego Aliaga, Janne Lamphilati, Martin Gysel-Beer, Benjamin Tobias Brem, Robin Lewis Modini, Dominic Heslin-Rees, Tareq Hussein, Marco Zanatta, Paolo Cristofanelli, Federico Bianchi, Markku Kulmala, and Angela Marinoni
Atmos. Chem. Phys., 26, 8893–8912, https://doi.org/10.5194/acp-26-8893-2026, https://doi.org/10.5194/acp-26-8893-2026, 2026
Short summary
Short summary
This study investigates particle number size distribution at two high-altitude European stations to better understand the mechanisms driving new particle formation (NPF) in the free troposphere. Interestingly, despite a consistently higher background of freshly nucleated particles at Jungfraujoch, NPF events were more frequent and intense at Monte Cimone, which also shows higher formation and growth rates, likely due to the proximity of the polluted planetary boundary layer from the Po Valley.
Kunfeng Gao, Romanos Foskinis, Marilena Gidarakou, Kalliopi Violaki, Guangyu Li, Benjamin Tobias Brem, Sophie Erb, Bernard Clot, Marie-José Graber, Branko Sikoparjja, Predrag Matavulj, Dusan Licina, Cuiqi Zhang, Benoît Crouzy, Alexandros Papayannis, Zamin A. Kanji, and Athanasios Nenes
EGUsphere, https://doi.org/10.5194/egusphere-2026-2699, https://doi.org/10.5194/egusphere-2026-2699, 2026
Short summary
Short summary
This study identified bioaerosols (>85%) as the dominant source for ice nucleating particles in mixed-phase clouds at a semi-rural site in central Europe, using a combination of in-situ, remote sensing and airmass modelling analysis. We developed a bioaerosol-aware ice nucleating particle parameterization that outperformed existing dust-only schemes across multiple field datasets. These findings improve representation of bioaerosol–cloud interactions and reduce uncertainty in climate feedback.
Leonie Bernet, Benjamin T. Brem, Nicolas Bukowiecki, Stephan Henne, Jörg Klausen, Mathew Mutuku, David Njiru, Patricia Nying'uro, Christoph Zellweger, and Martin Steinbacher
Atmos. Chem. Phys., 26, 6741–6762, https://doi.org/10.5194/acp-26-6741-2026, https://doi.org/10.5194/acp-26-6741-2026, 2026
Short summary
Short summary
Long-term atmospheric measurements are crucial to understanding climate change but remain scarce across Africa. We monitored atmospheric species at Mt. Kenya from 2020 to 2024. Our data reveal equatorial seasonal and daily variability and show that models miss local patterns. Emissions at Mt. Kenya mainly come from households, industry, and agriculture, though with large uncertainties. These findings stress the need for more ground stations to improve climate models and emission estimates.
Martine Collaud Coen, Benjamin Tobias Brem, Martin Gysel-Beer, Robin Modini, Stephan Henne, Martin Steinbacher, Davide Putero, Maria I. Gini, and Kostantinos Eleftheriadis
Atmos. Chem. Phys., 26, 1623–1645, https://doi.org/10.5194/acp-26-1623-2026, https://doi.org/10.5194/acp-26-1623-2026, 2026
Short summary
Short summary
Saharan dust (SD) is transported over long distances by large-scale atmospheric circulation, reaching the Jungfraujoch high-altitude station 30 to 150 times per year. This study analyses the influence of instrument types on the SD detection using the single scattering albedo spectral dependence. This optical method is then compared to those based on size distribution and back-trajectories. The 23-year climatology of dust frequency and mass as well as the source sensitivity are also examined.
Marilena Gidarakou, Alexandros Papayannis, Kunfeng Gao, Panagiotis Gidarakos, Benoît Crouzy, Romanos Foskinis, Sophie Erb, Benjamin T. Brem, Cuiqi Zhang, Gian Lieberherr, Martine Collaud Coen, Branko Sikoparija, Zamin A. Kanji, Bernard Clot, Bertrand Calpini, Eugenia Giagka, and Athanasios Nenes
Atmos. Chem. Phys., 26, 923–945, https://doi.org/10.5194/acp-26-923-2026, https://doi.org/10.5194/acp-26-923-2026, 2026
Short summary
Short summary
Vertical profiles of pollen and biomass burning particles were obtained at a semi-rural site at the MeteoSwiss station near Payerne (Switzerland) using a novel multi-channel elastic-fluorescence lidar system combined with in situ measurements during the spring 2023 wildfires and pollination season during the PERICLES (PayernE lidaR and Insitu detection of fluorescent bioaerosol and dust partiCLES and their cloud impacts) campaign.
Lubna Dada, Benjamin T. Brem, Lidia-Marta Amarandi-Netedu, Martine Collaud Coen, Nikolaos Evangeliou, Christoph Hueglin, Nora Nowak, Robin Modini, Martin Steinbacher, and Martin Gysel-Beer
Aerosol Research, 3, 315–336, https://doi.org/10.5194/ar-3-315-2025, https://doi.org/10.5194/ar-3-315-2025, 2025
Short summary
Short summary
We investigated the sources of ultrafine particles (UFPs) in Payerne, Switzerland, highlighting the significant role of secondary processes in elevating UFP concentrations to levels comparable to urban areas. As the first study in rural midland Switzerland to analyze new particle formation events and secondary contributions, it offers key insights for air quality regulation and the role of agriculture in Switzerland and central Europe.
Tiantian Wang, Jun Zhang, Houssni Lamkaddam, Kun Li, Ka Yuen Cheung, Lisa Kattner, Erlend Gammelsæter, Michael Bauer, Zachary C. J. Decker, Deepika Bhattu, Rujin Huang, Rob L. Modini, Jay G. Slowik, Imad El Haddad, Andre S. H. Prevot, and David M. Bell
Atmos. Chem. Phys., 25, 2707–2724, https://doi.org/10.5194/acp-25-2707-2025, https://doi.org/10.5194/acp-25-2707-2025, 2025
Short summary
Short summary
Our study analyzes real-time emissions of organic vapors from solid fuel combustion. Using the mass spectrometer, we tested various fuels, finding higher emission factors for organic vapors from wood burning. Intermediate-volatility organic compounds constituted a significant fraction of emissions in solid fuel combustion. Statistical tests identified unique potential markers. Our insights benefit air quality, climate, and health, aiding accurate emission assessments.
Imad El Haddad, Danielle Vienneau, Kaspar R. Daellenbach, Robin Modini, Jay G. Slowik, Abhishek Upadhyay, Petros N. Vasilakos, David Bell, Kees de Hoogh, and Andre S. H. Prevot
Atmos. Chem. Phys., 24, 11981–12011, https://doi.org/10.5194/acp-24-11981-2024, https://doi.org/10.5194/acp-24-11981-2024, 2024
Short summary
Short summary
This opinion paper explores how advances in aerosol science inform our understanding of the health impacts of outdoor particulate pollution. We advocate for a shift in the way we target PM pollution, focusing on the most harmful anthropogenic emissions. We highlight key observations, modelling developments, and emission measurements needed to achieve this shift.
Valeria Mardoñez-Balderrama, Griša Močnik, Marco Pandolfi, Robin L. Modini, Fernando Velarde, Laura Renzi, Angela Marinoni, Jean-Luc Jaffrezo, Isabel Moreno R., Diego Aliaga, Federico Bianchi, Claudia Mohr, Martin Gysel-Beer, Patrick Ginot, Radovan Krejci, Alfred Wiedensohler, Gaëlle Uzu, Marcos Andrade, and Paolo Laj
Atmos. Chem. Phys., 24, 12055–12077, https://doi.org/10.5194/acp-24-12055-2024, https://doi.org/10.5194/acp-24-12055-2024, 2024
Short summary
Short summary
Levels of black carbon (BC) are scarcely reported in the Southern Hemisphere, especially in high-altitude conditions. This study provides insight into the concentration level, variability, and optical properties of BC in La Paz and El Alto and at the Chacaltaya Global Atmosphere Watch Station. Two methods of source apportionment of absorption were tested and compared showing traffic as the main contributor to absorption in the urban area, in addition to biomass and open waste burning.
Franziska Vogel, Michael P. Adams, Larissa Lacher, Polly B. Foster, Grace C. E. Porter, Barbara Bertozzi, Kristina Höhler, Julia Schneider, Tobias Schorr, Nsikanabasi S. Umo, Jens Nadolny, Zoé Brasseur, Paavo Heikkilä, Erik S. Thomson, Nicole Büttner, Martin I. Daily, Romy Fösig, Alexander D. Harrison, Jorma Keskinen, Ulrike Proske, Jonathan Duplissy, Markku Kulmala, Tuukka Petäjä, Ottmar Möhler, and Benjamin J. Murray
Atmos. Chem. Phys., 24, 11737–11757, https://doi.org/10.5194/acp-24-11737-2024, https://doi.org/10.5194/acp-24-11737-2024, 2024
Short summary
Short summary
Primary ice formation in clouds strongly influences their properties; hence, it is important to understand the sources of ice-nucleating particles (INPs) and their variability. We present 2 months of INP measurements in a Finnish boreal forest using a new semi-autonomous INP counting device based on gas expansion. These results show strong variability in INP concentrations, and we present a case that the INPs we observe are, at least some of the time, of biological origin.
Timothy A. Sipkens, Joel C. Corbin, Brett Smith, Stéphanie Gagné, Prem Lobo, Benjamin T. Brem, Mark P. Johnson, and Gregory J. Smallwood
Atmos. Meas. Tech., 17, 4291–4302, https://doi.org/10.5194/amt-17-4291-2024, https://doi.org/10.5194/amt-17-4291-2024, 2024
Short summary
Short summary
Carbonaceous particles, such as soot, contribute to climate forcing, air pollution, and human health impacts. Thermal–optical analysis is a calibration standard used to measure these particles, but significant differences have been observed in the measurements across identical instruments. We report on the reproducibility of these measurements for aircraft emissions, which range from 8.0 % of the nominal value for organic carbon to 17 % for elemental carbon.
Larissa Lacher, Michael P. Adams, Kevin Barry, Barbara Bertozzi, Heinz Bingemer, Cristian Boffo, Yannick Bras, Nicole Büttner, Dimitri Castarede, Daniel J. Cziczo, Paul J. DeMott, Romy Fösig, Megan Goodell, Kristina Höhler, Thomas C. J. Hill, Conrad Jentzsch, Luis A. Ladino, Ezra J. T. Levin, Stephan Mertes, Ottmar Möhler, Kathryn A. Moore, Benjamin J. Murray, Jens Nadolny, Tatjana Pfeuffer, David Picard, Carolina Ramírez-Romero, Mickael Ribeiro, Sarah Richter, Jann Schrod, Karine Sellegri, Frank Stratmann, Benjamin E. Swanson, Erik S. Thomson, Heike Wex, Martin J. Wolf, and Evelyn Freney
Atmos. Chem. Phys., 24, 2651–2678, https://doi.org/10.5194/acp-24-2651-2024, https://doi.org/10.5194/acp-24-2651-2024, 2024
Short summary
Short summary
Aerosol particles that trigger ice formation in clouds are important for the climate system but are very rare in the atmosphere, challenging measurement techniques. Here we compare three cloud chambers and seven methods for collecting aerosol particles on filters for offline analysis at a mountaintop station. A general good agreement of the methods was found when sampling aerosol particles behind a whole air inlet, supporting their use for obtaining data that can be implemented in models.
Christina Spitieri, Maria Gini, Martin Gysel-Beer, and Konstantinos Eleftheriadis
Atmos. Chem. Phys., 23, 235–249, https://doi.org/10.5194/acp-23-235-2023, https://doi.org/10.5194/acp-23-235-2023, 2023
Short summary
Short summary
The paper provides insights into the hygroscopic properties and state of mixing of atmospheric aerosol through 1 year of measurements of key microphysical parameters in the suburbs of the most densely populated city of Greece, Athens, in the eastern Mediterranean, which is considered an important climate change hotspot. The results can be used for the prediction of cloud condensation nuclei and quantification of the influence of ambient relative humidity on light scattering by aerosol particles.
Alireza Moallemi, Rob L. Modini, Tatyana Lapyonok, Anton Lopatin, David Fuertes, Oleg Dubovik, Philippe Giaccari, and Martin Gysel-Beer
Atmos. Meas. Tech., 15, 5619–5642, https://doi.org/10.5194/amt-15-5619-2022, https://doi.org/10.5194/amt-15-5619-2022, 2022
Short summary
Short summary
Aerosol properties (size distributions, refractive indices) can be retrieved from in situ, angularly resolved light scattering measurements performed with polar nephelometers. We apply an established framework to assess the aerosol property retrieval potential for different instrument configurations, target applications, and assumed prior knowledge. We also demonstrate how a reductive greedy algorithm can be used to determine the optimal placements of the angular sensors in a polar nephelometer.
Christian Tatzelt, Silvia Henning, André Welti, Andrea Baccarini, Markus Hartmann, Martin Gysel-Beer, Manuela van Pinxteren, Robin L. Modini, Julia Schmale, and Frank Stratmann
Atmos. Chem. Phys., 22, 9721–9745, https://doi.org/10.5194/acp-22-9721-2022, https://doi.org/10.5194/acp-22-9721-2022, 2022
Short summary
Short summary
We present the abundance and origin of cloud-relevant aerosol particles in the preindustral-like conditions of the Southern Ocean (SO) during austral summer. Cloud condensation nuclei (CCN) and ice-nucleating particles (INP) were measured during a circum-Antarctic scientific cruise with in situ instrumentation and offline filter measurements, respectively. Transport processes were found to play an equally important role as local sources for both the CCN and INP population of the SO.
Ivo Beck, Hélène Angot, Andrea Baccarini, Lubna Dada, Lauriane Quéléver, Tuija Jokinen, Tiia Laurila, Markus Lampimäki, Nicolas Bukowiecki, Matthew Boyer, Xianda Gong, Martin Gysel-Beer, Tuukka Petäjä, Jian Wang, and Julia Schmale
Atmos. Meas. Tech., 15, 4195–4224, https://doi.org/10.5194/amt-15-4195-2022, https://doi.org/10.5194/amt-15-4195-2022, 2022
Short summary
Short summary
We present the pollution detection algorithm (PDA), a new method to identify local primary pollution in remote atmospheric aerosol and trace gas time series. The PDA identifies periods of contaminated data and relies only on the target dataset itself; i.e., it is independent of ancillary data such as meteorological variables. The parameters of all pollution identification steps are adjustable so that the PDA can be tuned to different locations and situations. It is available as open-access code.
Cyril Brunner, Benjamin T. Brem, Martine Collaud Coen, Franz Conen, Martin Steinbacher, Martin Gysel-Beer, and Zamin A. Kanji
Atmos. Chem. Phys., 22, 7557–7573, https://doi.org/10.5194/acp-22-7557-2022, https://doi.org/10.5194/acp-22-7557-2022, 2022
Short summary
Short summary
Microscopic particles called ice-nucleating particles (INPs) are essential for ice crystals to form in clouds. INPs are a tiny proportion of atmospheric aerosol, and their abundance is poorly constrained. We study how the concentration of INPs changes diurnally and seasonally at a mountaintop station in central Europe. Unsurprisingly, a diurnal cycle is only found when considering air masses that have had lower-altitude ground contact. The highest INP concentrations occur in spring.
Zoé Brasseur, Dimitri Castarède, Erik S. Thomson, Michael P. Adams, Saskia Drossaart van Dusseldorp, Paavo Heikkilä, Kimmo Korhonen, Janne Lampilahti, Mikhail Paramonov, Julia Schneider, Franziska Vogel, Yusheng Wu, Jonathan P. D. Abbatt, Nina S. Atanasova, Dennis H. Bamford, Barbara Bertozzi, Matthew Boyer, David Brus, Martin I. Daily, Romy Fösig, Ellen Gute, Alexander D. Harrison, Paula Hietala, Kristina Höhler, Zamin A. Kanji, Jorma Keskinen, Larissa Lacher, Markus Lampimäki, Janne Levula, Antti Manninen, Jens Nadolny, Maija Peltola, Grace C. E. Porter, Pyry Poutanen, Ulrike Proske, Tobias Schorr, Nsikanabasi Silas Umo, János Stenszky, Annele Virtanen, Dmitri Moisseev, Markku Kulmala, Benjamin J. Murray, Tuukka Petäjä, Ottmar Möhler, and Jonathan Duplissy
Atmos. Chem. Phys., 22, 5117–5145, https://doi.org/10.5194/acp-22-5117-2022, https://doi.org/10.5194/acp-22-5117-2022, 2022
Short summary
Short summary
The present measurement report introduces the ice nucleation campaign organized in Hyytiälä, Finland, in 2018 (HyICE-2018). We provide an overview of the campaign settings, and we describe the measurement infrastructure and operating procedures used. In addition, we use results from ice nucleation instrument inter-comparison to show that the suite of these instruments deployed during the campaign reports consistent results.
Dalrin Ampritta Amaladhasan, Claudia Heyn, Christopher R. Hoyle, Imad El Haddad, Miriam Elser, Simone M. Pieber, Jay G. Slowik, Antonio Amorim, Jonathan Duplissy, Sebastian Ehrhart, Vladimir Makhmutov, Ugo Molteni, Matti Rissanen, Yuri Stozhkov, Robert Wagner, Armin Hansel, Jasper Kirkby, Neil M. Donahue, Rainer Volkamer, Urs Baltensperger, Martin Gysel-Beer, and Andreas Zuend
Atmos. Chem. Phys., 22, 215–244, https://doi.org/10.5194/acp-22-215-2022, https://doi.org/10.5194/acp-22-215-2022, 2022
Short summary
Short summary
We use a combination of models for gas-phase chemical reactions and equilibrium gas–particle partitioning of isoprene-derived secondary organic aerosols (SOAs) informed by dark ozonolysis experiments conducted in the CLOUD chamber. Our predictions cover high to low relative humidities (RHs) and quantify how SOA mass yields are enhanced at high RH as well as the impact of inorganic seeds of distinct hygroscopicities and acidities on the coupled partitioning of water and semi-volatile organics.
Cyril Brunner, Benjamin T. Brem, Martine Collaud Coen, Franz Conen, Maxime Hervo, Stephan Henne, Martin Steinbacher, Martin Gysel-Beer, and Zamin A. Kanji
Atmos. Chem. Phys., 21, 18029–18053, https://doi.org/10.5194/acp-21-18029-2021, https://doi.org/10.5194/acp-21-18029-2021, 2021
Short summary
Short summary
Special microscopic particles called ice-nucleating particles (INPs) are essential for ice crystals to form in the atmosphere. INPs are sparse and their atmospheric concentration and properties are not well understood. Mineral dust particles make up a significant fraction of INPs but how much remains unknown. Here, we address this knowledge gap by studying periods when mineral particles are present in large quantities at a mountaintop station in central Europe.
Gian Lieberherr, Kevin Auderset, Bertrand Calpini, Bernard Clot, Benoît Crouzy, Martin Gysel-Beer, Thomas Konzelmann, José Manzano, Andrea Mihajlovic, Alireza Moallemi, David O'Connor, Branko Sikoparija, Eric Sauvageat, Fiona Tummon, and Konstantina Vasilatou
Atmos. Meas. Tech., 14, 7693–7706, https://doi.org/10.5194/amt-14-7693-2021, https://doi.org/10.5194/amt-14-7693-2021, 2021
Short summary
Short summary
Today there is no standard procedure to validate bioaerosol and pollen monitors. Three instruments were tested, focusing on detecting particles of different sizes. Only one instrument was able to detect the smallest particles (0.5 µm Ø), whereas the others performed best at the largest tested particles (10 µm Ø). These results are the first step towards a standardised validation procedure. The need for a reference counting method for larger particles (pollen grains: 10–200 µm Ø) was emphasised.
Sebastian Landwehr, Michele Volpi, F. Alexander Haumann, Charlotte M. Robinson, Iris Thurnherr, Valerio Ferracci, Andrea Baccarini, Jenny Thomas, Irina Gorodetskaya, Christian Tatzelt, Silvia Henning, Rob L. Modini, Heather J. Forrer, Yajuan Lin, Nicolas Cassar, Rafel Simó, Christel Hassler, Alireza Moallemi, Sarah E. Fawcett, Neil Harris, Ruth Airs, Marzieh H. Derkani, Alberto Alberello, Alessandro Toffoli, Gang Chen, Pablo Rodríguez-Ros, Marina Zamanillo, Pau Cortés-Greus, Lei Xue, Conor G. Bolas, Katherine C. Leonard, Fernando Perez-Cruz, David Walton, and Julia Schmale
Earth Syst. Dynam., 12, 1295–1369, https://doi.org/10.5194/esd-12-1295-2021, https://doi.org/10.5194/esd-12-1295-2021, 2021
Short summary
Short summary
The Antarctic Circumnavigation Expedition surveyed a large number of variables describing the dynamic state of ocean and atmosphere, freshwater cycle, atmospheric chemistry, ocean biogeochemistry, and microbiology in the Southern Ocean. To reduce the dimensionality of the dataset, we apply a sparse principal component analysis and identify temporal patterns from diurnal to seasonal cycles, as well as geographical gradients and
hotspotsof interaction. Code and data are open access.
Clémence Rose, Martine Collaud Coen, Elisabeth Andrews, Yong Lin, Isaline Bossert, Cathrine Lund Myhre, Thomas Tuch, Alfred Wiedensohler, Markus Fiebig, Pasi Aalto, Andrés Alastuey, Elisabeth Alonso-Blanco, Marcos Andrade, Begoña Artíñano, Todor Arsov, Urs Baltensperger, Susanne Bastian, Olaf Bath, Johan Paul Beukes, Benjamin T. Brem, Nicolas Bukowiecki, Juan Andrés Casquero-Vera, Sébastien Conil, Konstantinos Eleftheriadis, Olivier Favez, Harald Flentje, Maria I. Gini, Francisco Javier Gómez-Moreno, Martin Gysel-Beer, Anna Gannet Hallar, Ivo Kalapov, Nikos Kalivitis, Anne Kasper-Giebl, Melita Keywood, Jeong Eun Kim, Sang-Woo Kim, Adam Kristensson, Markku Kulmala, Heikki Lihavainen, Neng-Huei Lin, Hassan Lyamani, Angela Marinoni, Sebastiao Martins Dos Santos, Olga L. Mayol-Bracero, Frank Meinhardt, Maik Merkel, Jean-Marc Metzger, Nikolaos Mihalopoulos, Jakub Ondracek, Marco Pandolfi, Noemi Pérez, Tuukka Petäjä, Jean-Eudes Petit, David Picard, Jean-Marc Pichon, Veronique Pont, Jean-Philippe Putaud, Fabienne Reisen, Karine Sellegri, Sangeeta Sharma, Gerhard Schauer, Patrick Sheridan, James Patrick Sherman, Andreas Schwerin, Ralf Sohmer, Mar Sorribas, Junying Sun, Pierre Tulet, Ville Vakkari, Pieter Gideon van Zyl, Fernando Velarde, Paolo Villani, Stergios Vratolis, Zdenek Wagner, Sheng-Hsiang Wang, Kay Weinhold, Rolf Weller, Margarita Yela, Vladimir Zdimal, and Paolo Laj
Atmos. Chem. Phys., 21, 17185–17223, https://doi.org/10.5194/acp-21-17185-2021, https://doi.org/10.5194/acp-21-17185-2021, 2021
Short summary
Short summary
Aerosol particles are a complex component of the atmospheric system the effects of which are among the most uncertain in climate change projections. Using data collected at 62 stations, this study provides the most up-to-date picture of the spatial distribution of particle number concentration and size distribution worldwide, with the aim of contributing to better representation of aerosols and their interactions with clouds in models and, therefore, better evaluation of their impact on climate.
Lucía Caudillo, Birte Rörup, Martin Heinritzi, Guillaume Marie, Mario Simon, Andrea C. Wagner, Tatjana Müller, Manuel Granzin, Antonio Amorim, Farnoush Ataei, Rima Baalbaki, Barbara Bertozzi, Zoé Brasseur, Randall Chiu, Biwu Chu, Lubna Dada, Jonathan Duplissy, Henning Finkenzeller, Loïc Gonzalez Carracedo, Xu-Cheng He, Victoria Hofbauer, Weimeng Kong, Houssni Lamkaddam, Chuan P. Lee, Brandon Lopez, Naser G. A. Mahfouz, Vladimir Makhmutov, Hanna E. Manninen, Ruby Marten, Dario Massabò, Roy L. Mauldin, Bernhard Mentler, Ugo Molteni, Antti Onnela, Joschka Pfeifer, Maxim Philippov, Ana A. Piedehierro, Meredith Schervish, Wiebke Scholz, Benjamin Schulze, Jiali Shen, Dominik Stolzenburg, Yuri Stozhkov, Mihnea Surdu, Christian Tauber, Yee Jun Tham, Ping Tian, António Tomé, Steffen Vogt, Mingyi Wang, Dongyu S. Wang, Stefan K. Weber, André Welti, Wang Yonghong, Wu Yusheng, Marcel Zauner-Wieczorek, Urs Baltensperger, Imad El Haddad, Richard C. Flagan, Armin Hansel, Kristina Höhler, Jasper Kirkby, Markku Kulmala, Katrianne Lehtipalo, Ottmar Möhler, Harald Saathoff, Rainer Volkamer, Paul M. Winkler, Neil M. Donahue, Andreas Kürten, and Joachim Curtius
Atmos. Chem. Phys., 21, 17099–17114, https://doi.org/10.5194/acp-21-17099-2021, https://doi.org/10.5194/acp-21-17099-2021, 2021
Short summary
Short summary
We performed experiments in the CLOUD chamber at CERN at low temperatures to simulate new particle formation in the upper free troposphere (at −30 ºC and −50 ºC). We measured the particle and gas phase and found that most of the compounds present in the gas phase are detected as well in the particle phase. The major compounds in the particles are C8–10 and C18–20. Specifically, we showed that C5 and C15 compounds are detected in a mixed system with isoprene and α-pinene at −30 ºC, 20 % RH.
Larissa Lacher, Hans-Christian Clemen, Xiaoli Shen, Stephan Mertes, Martin Gysel-Beer, Alireza Moallemi, Martin Steinbacher, Stephan Henne, Harald Saathoff, Ottmar Möhler, Kristina Höhler, Thea Schiebel, Daniel Weber, Jann Schrod, Johannes Schneider, and Zamin A. Kanji
Atmos. Chem. Phys., 21, 16925–16953, https://doi.org/10.5194/acp-21-16925-2021, https://doi.org/10.5194/acp-21-16925-2021, 2021
Short summary
Short summary
We investigate ice-nucleating particle properties at Jungfraujoch during the 2017 joint INUIT/CLACE field campaign, to improve the knowledge about those rare particles in a cloud-relevant environment. By quantifying ice-nucleating particles in parallel to single-particle mass spectrometry measurements, we find that mineral dust and aged sea spray particles are potential candidates for ice-nucleating particles. Our findings are supported by ice residual analysis and source region modeling.
Sebastian Düsing, Albert Ansmann, Holger Baars, Joel C. Corbin, Cyrielle Denjean, Martin Gysel-Beer, Thomas Müller, Laurent Poulain, Holger Siebert, Gerald Spindler, Thomas Tuch, Birgit Wehner, and Alfred Wiedensohler
Atmos. Chem. Phys., 21, 16745–16773, https://doi.org/10.5194/acp-21-16745-2021, https://doi.org/10.5194/acp-21-16745-2021, 2021
Short summary
Short summary
The work deals with optical properties of aerosol particles in dried and atmospheric states. Based on two measurement campaigns in the rural background of central Europe, different measurement approaches were compared with each other, such as modeling based on Mie theory and direct in situ or remote sensing measurements. Among others, it was shown that the aerosol extinction-to-backscatter ratio is relative humidity dependent, and refinement with respect to the model input parameters is needed.
Cited articles
Ahern, A. T., Erdesz, F., Wagner, N. L., Brock, C. A., Lyu, M., Slovacek, K., Moore, R. H., Wiggins, E. B., and Murphy, D. M.: Laser imaging nephelometer for aircraft deployment, Atmos. Meas. Tech., 15, 1093–1105, https://doi.org/10.5194/amt-15-1093-2022, 2022.
Barkey, B., Paulson, S. E., and Chung, A.: Genetic algorithm inversion of
dual polarization polar nephelometer data to determine aerosol refractive
index, Aerosol Sci. Tech., 41, 751–760, https://doi.org/10.1080/02786820701432640, 2007.
Barkey, B., Paulson, S., and Liou, K. N.: Polar nephelometers for light
scattering by ice crystals and aerosols: design and measurements, in: Light
Scattering Reviews, Vol. 6, edited by: Kokhanovsky, A. A., Springer Berlin
Heidelberg, Berlin, Heidelberg, 3–37,
https://doi.org/10.1007/978-3-642-15531-4_1, 2012.
Bian, Y., Zhao, C., Xu, W., Zhao, G., Tao, J., and Kuang, Y.: Development and validation of a CCD-laser aerosol detective system for measuring the ambient aerosol phase function, Atmos. Meas. Tech., 10, 2313–2322, https://doi.org/10.5194/amt-10-2313-2017, 2017.
Boiger, R., Modini, R. L., Moallemi, A., Degen, D., Adelmann, A., and
Gysel-Beer, M.: Retrieval of aerosol properties from in situ, multi-angle
light scattering measurements using invertible neural networks. J. Aerosol
Sci., 163, 105977, https://doi.org/10.1016/j.jaerosci.2022.105977, 2022.
Bohren, C. F. and Huffman, D. R.: Absorption and scattering of light by
small particles, Wiley-VCH, Weinheim, 530 pp., ISBN 9780471293408, 2004.
Boucher, O.: Atmospheric Aerosols, Springer Netherlands, Dordrecht,
https://doi.org/10.1007/978-94-017-9649-1, 2015.
Boucher, O., Randall, D., Artaxo, P., Bretherton, C., Feingold, G., Forster, P., Kerminen, V.-M., Kondo, Y., Liao, H., Lohmann, U., Rasch, P., Satheesh, S. K., Sherwood, S., Stevens, B., and Zhang, X. Y.: Clouds and
aerosols, in: Climate Change 2013: the physical science basis. Contribution
of Working Group I to the Fifth Assessment Report of the Intergovernmental
Panel on Climate Change, edited by: Stocker, T. F., Qin, D., Plattner, G.-K., Tignor, M., Allen, S. K., Doschung, J., Nauels, A., Xia, Y., Bex, V., and Midgley, P. M., Cambridge University Press, 571–657, https://doi.org/10.1017/CBO9781107415324.016, 2014.
Cohen, A. J., Brauer, M., Burnett, R., Anderson, H. R., Frostad, J., Estep,
K., Balakrishnan, K., Brunekreef, B., Dandona, L., Dandona, R., Feigin, V.,
Freedman, G., Hubbell, B., Jobling, A., Kan, H., Knibbs, L., Liu, Y.,
Martin, R., Morawska, L., Pope, C. A., Shin, H., Straif, K., Shaddick, G.,
Thomas, M., van Dingenen, R., van Donkelaar, A., Vos, T., Murray, C. J. L.,
and Forouzanfar, M. H.: Estimates and 25-year trends of the global burden of
disease attributable to ambient air pollution: an analysis of data from the
Global Burden of Diseases Study 2015, Lancet, 389, 1907–1918,
https://doi.org/10.1016/S0140-6736(17)30505-6, 2017.
Dick, W. D., Ziemann, P. J., and McMurry, P. H.: Multiangle light-scattering
measurements of refractive index of submicron atmospheric particles, Aerosol
Sci. Tech., 41, 549–569, https://doi.org/10.1080/02786820701272012, 2007.
Dolgos, G. and Martins, J. V.: Polarized Imaging Nephelometer for in situ
airborne measurements of aerosol light scattering, Opt. Express, 22,
21972–21990, https://doi.org/10.1364/OE.22.021972, 2014.
Dubovik, O., Herman, M., Holdak, A., Lapyonok, T., Tanré, D., Deuzé, J. L., Ducos, F., Sinyuk, A., and Lopatin, A.: Statistically optimized inversion algorithm for enhanced retrieval of aerosol properties from spectral multi-angle polarimetric satellite observations, Atmos. Meas. Tech., 4, 975–1018, https://doi.org/10.5194/amt-4-975-2011, 2011.
Dubovik, O., Lapyonok, T., Litvinov, P., Herman, M., Fuertes, D., Ducos, F.,
Torres, B., Derimian, Y., Huang, X., Lopatin, A., Chaikovsky, A.,
Aspetsberger, M., and Federspiel, C.: GRASP: a versatile algorithm for
characterizing the atmosphere, SPIE Newsroom,
https://doi.org/10.1117/2.1201408.005558, 2014.
Dubovik, O., Li, Z., Mishchenko, M. I., Tanré, D., Karol, Y., Bojkov,
B., Cairns, B., Diner, D. J., Espinosa, W. R., Goloub, P., Gu, X., Hasekamp,
O., Hong, J., Hou, W., Knobelspiesse, K. D., Landgraf, J., Li, L., Litvinov,
P., Liu, Y., Lopatin, A., Marbach, T., Maring, H., Martins, V., Meijer, Y.,
Milinevsky, G., Mukai, S., Parol, F., Qiao, Y., Remer, L., Rietjens, J.,
Sano, I., Stammes, P., Stamnes, S., Sun, X., Tabary, P., Travis, L. D.,
Waquet, F., Xu, F., Yan, C., and Yin, D.: Polarimetric remote sensing of
atmospheric aerosols: Instruments, methodologies, results, and perspectives,
J. Quant. Spectrosc. Ra., 224, 474–511, https://doi.org/10.1016/j.jqsrt.2018.11.024, 2019.
Dubovik, O., Fuertes, D., Litvinov, P., Lopatin, A., Lapyonok, T., Doubovik,
I., Xu, F., Ducos, F., Chen, C., Torres, B., Derimian, Y., Li, L.,
Herreras-Giralda, M., Herrera, M., Karol, Y., Matar, C., Schuster, G. L.,
Espinosa, R., Puthukkudy, A., Li, Z., Fischer, J., Preusker, R., Cuesta, J.,
Kreuter, A., Cede, A., Aspetsberger, M., Marth, D., Bindreiter, L., Hangler,
A., Lanzinger, V., Holter, C., and Federspiel, C.: A comprehensive
description of multi-term LSM for applying multiple a priori constraints in
problems of atmospheric remote sensing: GRASP Algorithm, Concept, and
Applications, Front. Remote Sens., 2, 706851, https://doi.org/10.3389/frsen.2021.706851, 2021.
Espinosa, W. R., Remer, L. A., Dubovik, O., Ziemba, L., Beyersdorf, A., Orozco, D., Schuster, G., Lapyonok, T., Fuertes, D., and Martins, J. V.: Retrievals of aerosol optical and microphysical properties from Imaging Polar Nephelometer scattering measurements, Atmos. Meas. Tech., 10, 811–824, https://doi.org/10.5194/amt-10-811-2017, 2017.
Espinosa, W. R., Martins, J. V., Remer, L. A., Dubovik, O., Lapyonok, T.,
Fuertes, D., Puthukkudy, A., Orozco, D., Ziemba, L., Thornhill, K. L., and
Levy, R.: Retrievals of aerosol size distribution, spherical fraction, and
complex refractive index from airborne in situ angular light scattering and
absorption measurements, J. Geophys. Res.-Atmos., 124, 7997–8024,
https://doi.org/10.1029/2018JD030009, 2019.
GRASP-SAS: Platform for GRASP open source code, GRASP OPEN [code], https://www.grasp-open.com/ (last access: 25 May 2022), 2015.
Holben, B. N., Eck, T. F., Slutsker, I., Tanré, D., Buis, J. P., Setzer,
A., Vermote, E., Reagan, J. A., Kaufman, Y. J., Nakajima, T., Lavenu, F.,
Jankowiak, I., and Smirnov, A.: AERONET – a federated instrument network and
data archive for aerosol characterization, Remote Sens. Environ., 66, 1–16,
https://doi.org/10.1016/S0034-4257(98)00031-5, 1998.
Horvath, H., Alados Arboledas, L., and Olmo Reyes, F. J.: Angular scattering of the Sahara dust aerosol, Atmos. Chem. Phys., 18, 17735–17744, https://doi.org/10.5194/acp-18-17735-2018, 2018.
Hu, Q., Qiu, Z., Hong, J., and Chen, D.: A polarized scanning nephelometer
for measurement of light scattering of an ensemble-averaged matrix of
aerosol particles, J. Quant. Spectrosc. Ra., 261, 107497,
https://doi.org/10.1016/j.jqsrt.2020.107497, 2021.
Kasarova, S. N., Sultanova, N. G., Ivanov, C. D., and Nikolov, I. D.:
Analysis of the dispersion of optical plastic materials, Opt. Mater., 29,
1481–1490, https://doi.org/10.1016/j.optmat.2006.07.010, 2007.
Li, R., Tang, G., Ding, J., Logan, T., Brooks, S. D., Collins, D. R., Yang,
P., and Kattawar, G. W.: Laboratory measurements of light scattering
properties of kaolinite dust at 532 nm, Aerosol Sci. Tech., 52, 666–678,
https://doi.org/10.1080/02786826.2018.1444729, 2018.
Ma, X., Lu, J. Q., Brock, R. S., Jacobs, K. M., Yang, P., and Hu, X.-H.:
Determination of complex refractive index of polystyrene microspheres from
370 to 1610 nm, Phys. Med. Biol., 48, 4165–4172,
https://doi.org/10.1088/0031-9155/48/24/013, 2003.
Manfred, K. M., Washenfelder, R. A., Wagner, N. L., Adler, G., Erdesz, F., Womack, C. C., Lamb, K. D., Schwarz, J. P., Franchin, A., Selimovic, V., Yokelson, R. J., and Murphy, D. M.: Investigating biomass burning aerosol morphology using a laser imaging nephelometer, Atmos. Chem. Phys., 18, 1879–1894, https://doi.org/10.5194/acp-18-1879-2018, 2018.
Mishchenko, M. I., Cairns, B., Kopp, G., Schueler, C. F., Fafaul, B. A.,
Hansen, J. E., Hooker, R. J., Itchkawich, T., Maring, H. B., and Travis, L.
D.: Accurate monitoring of terrestrial aerosols and total solar irradiance:
introducing the glory mission, B. Am. Meteorol. Soc., 88, 677–692,
https://doi.org/10.1175/BAMS-88-5-677, 2007.
Moallemi, A., Modini, R. L., Lapyonok, T., Lopatin, A., Fuertes, D., Dubovik, O., Giaccari, P., and Gysel-Beer, M.: Information content and aerosol property retrieval potential for different types of in situ polar nephelometer data, Atmos. Meas. Tech., 15, 5619–5642, https://doi.org/10.5194/amt-15-5619-2022, 2022.
Moallemi, A., Modini, R. L., Giaccari, P., Brem, B. T., Bertozzi, B., and Gysel-Beer, M.: Data archive for the peer-reviewed journal article “Concept, absolute calibration and validation of a new, bench-top laser imaging polar nephelometer”, Version 1, Zenodo [data set], https://doi.org/10.5281/zenodo.8021082, 2023.
Muñoz, O., Moreno, F., Guirado, D., Dabrowska, D. D., Volten, H., and
Hovenier, J. W.: The Amsterdam–Granada Light Scattering Database, J. Quant.
Spectrosc. Ra., 113, 565–574, https://doi.org/10.1016/j.jqsrt.2012.01.014, 2012.
Myhre, G., Shindell, D., Bréon, F. M., Collins, W., Fuglestvedt, J., Huang, J., Koch, D., Lamarque, J. F., Lee, D., Mendoza, B., Nakajima, T., Robock, A., Stephens. G., Takemura, T., and Zhang, H.: Climate
Change 2013: the physical science basis. Contribution of Working Group I to
the Fifth Assessment Report of the Intergovernmental Panel on Climate
Change, edited by: Stocker, T. F., Qin, D., Plattner, G.-K., Tignor, M., Allen, S. K., Doschung, J., Nauels, A., Xia, Y., Bex, V., and Midgley, P. M., 659–740, https://doi.org/10.1017/CBO9781107415324.018 , 2014.
Nakagawa, M., Nakayama, T., Sasago, H., Ueda, S., Venables, D. S., and
Matsumi, Y.: Design and characterization of a novel single-particle polar
nephelometer, Aerosol Sci. Tech., 50, 392–404,
https://doi.org/10.1080/02786826.2016.1155105, 2016.
Omar, A. H., Winker, D. M., Vaughan, M. A., Hu, Y., Trepte, C. R., Ferrare,
R. A., Lee, K.-P., Hostetler, C. A., Kittaka, C., Rogers, R. R., Kuehn, R.
E., and Liu, Z.: The CALIPSO automated aerosol classification and lidar
ratio selection algorithm, J. Atmos. Ocean. Tech., 26, 1994–2014,
https://doi.org/10.1175/2009JTECHA1231.1, 2009.
Pettersson, A., Lovejoy, E. R., Brock, C. A., Brown, S. S., and
Ravishankara, A. R.: Measurement of aerosol optical extinction at with
pulsed cavity ring down spectroscopy, J. Aerosol Sci., 35, 995–1011,
https://doi.org/10.1016/j.jaerosci.2004.02.008, 2004.
Prahl, S.: Miepython, GitHub [code], https://github.com/scottprahl/miepython (last access: 1 August 2022), 2022.
Schafer, J. S., Eck, T. F., Holben, B. N., Thornhill, K. L., Ziemba, L. D., Sawamura, P., Moore, R. H., Slutsker, I., Anderson, B. E., Sinyuk, A., Giles, D. M., Smirnov, A., Beyersdorf, A. J., and Winstead, E. L.: Intercomparison of aerosol volume size distributions derived from AERONET ground-based remote sensing and LARGE in situ aircraft profiles during the 2011–2014 DRAGON and DISCOVER-AQ experiments, Atmos. Meas. Tech., 12, 5289–5301, https://doi.org/10.5194/amt-12-5289-2019, 2019.
Schuster, G. L., Espinosa, W. R., Ziemba, L. D., Beyersdorf, A. J.,
Rocha-Lima, A., Anderson, B. E., Martins, J. V., Dubovik, O., Ducos, F.,
Fuertes, D., Lapyonok, T., Shook, M., Derimian, Y., and Moore, R. H.: A
laboratory experiment for the statistical evaluation of aerosol retrieval
(STEAR) algorithms, Remote Sensing, 11, 498, https://doi.org/10.3390/rs11050498, 2019.
Tavakoli, F. and Olfert, J. S.: An instrument for the classification of
aerosols by particle relaxation time: theoretical models of the aerodynamic
aerosol classifier, Aerosol Sci. Technol., 47, 916–926,
https://doi.org/10.1080/02786826.2013.802761, 2013.
Verhaege, C., Shcherbakov, V., and Personne, P.: Retrieval of complex
refractive index and size distribution of spherical particles from
Dual-Polarization Polar Nephelometer data, J. Quant. Spectrosc. Ra., 110, 1690–1697, https://doi.org/10.1016/j.jqsrt.2009.01.004, 2009.
Waldram, J. M.: Measurement of the photometric properties of the upper
atmosphere, Transactions of the Illuminating Engineering Society, 10, 147–187, https://doi.org/10.1177/147715354501000801, 1945.
Short summary
Polarimetric data, i.e., the angular and polarization dependence of light scattering by aerosols, contain ample information on optical and microphysical properties. Retrieval of these properties is a central approach in aerosol remote sensing. We present a description, calibration, validation, and a first application of a new benchtop polar nephelometer, which provides in situ polarimetric measurements of an aerosol. Such data facilitate agreement between retrieval results and independent data.
Polarimetric data, i.e., the angular and polarization dependence of light scattering by...
