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AMT | Articles | Volume 13, issue 4
Atmos. Meas. Tech., 13, 2035–2056, 2020
https://doi.org/10.5194/amt-13-2035-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
Atmos. Meas. Tech., 13, 2035–2056, 2020
https://doi.org/10.5194/amt-13-2035-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.

Research article 22 Apr 2020

Research article | 22 Apr 2020

High-humidity tandem differential mobility analyzer for accurate determination of aerosol hygroscopic growth, microstructure, and activity coefficients over a wide range of relative humidity

Eugene F. Mikhailov and Sergey S. Vlasenko

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Cited articles

Andreae, M. O. and Rosenfeld, D.: Aerosol-cloud-precipitation interactions. Part 1. The nature and sources of cloud-active aerosols, Earth-Sci. Rev., 89, 13–41, https://doi.org/10.1016/j.earscirev.2008.03.001, 2008. 
Aumann, E. and Hildemann, L. M.: Measuring and modeling the composition and temperature-dependence of surface tension for organic solutions, Atmos. Environ., 44, 329–337, https://doi.org/10.1016/j.atmosenv.2009.10.033, 2010. 
Biskos, G., Paulsen, D., Russell, L. M., Buseck, P. R., and Martin, S. T.: Prompt deliquescence and efflorescence of aerosol nanoparticles, Atmos. Chem. Phys., 6, 4633–4642, https://doi.org/10.5194/acp-6-4633-2006, 2006. 
Brechtel, F. J. and Kreidenweis, S. M.: Predicting particle critical supersaturation from hygroscopic growth measurements in the humidified TDMA. Part II: Laboratory and Ambient Studies, J. Atmos. Sci. 57, 1872–1887, https://doi.org/10.1175/1520-0469(2000)057<1854:PPCSFH>2.0.CO;2, 2000. 
Brockmann, J. E. and Rader, D. J.: APS response to nonspherical particles and experimental determination of dynamic shape factor, Aerosol Sci. Technol., 13, 162–172, https://doi.org/10.1080/02786829008959434, 1990. 
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Here we present the high-humidity tandem differential hygroscopicity analyzer (HHTDMA) and a new method to measure the hygroscopic growth of aerosol particles with in situ restructuring to minimize the influence of particle shape. Our results demonstrate that the HHTDMA system described in this work allows us to determine the thermodynamic characteristics of aqueous solutions with an accuracy close to that obtained by bulk methods.
Here we present the high-humidity tandem differential hygroscopicity analyzer (HHTDMA) and a new...
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