Articles | Volume 15, issue 15
https://doi.org/10.5194/amt-15-4623-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-15-4623-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
15 Aug 2022
Research article |
| 15 Aug 2022
| 15 Aug 2022
Evaluation of the High Altitude Lidar Observatory (HALO) methane retrievals during the summer 2019 ACT-America campaign
Rory A. Barton-Grimley
CORRESPONDING AUTHOR
NASA Langley Research Center, Hampton, VA, USA
NASA Langley Research Center, Hampton, VA, USA
Susan A. Kooi
Science Systems and Applications, Inc., Hampton, VA, USA
James E. Collins
Science Systems and Applications, Inc., Hampton, VA, USA
David B. Harper
NASA Langley Research Center, Hampton, VA, USA
Anthony Notari
NASA Langley Research Center, Hampton, VA, USA
Joseph Lee
Science Systems and Applications, Inc., Hampton, VA, USA
Joshua P. DiGangi
NASA Langley Research Center, Hampton, VA, USA
Yonghoon Choi
Science Systems and Applications, Inc., Hampton, VA, USA
Kenneth J. Davis
Department of Meteorology and Atmospheric Science, and Earth and
Environmental Systems Institute, The Pennsylvania State University,
University Park, PA, USA
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Taiwo Ajayi, Yonghoon Choi, Ewan C. Crosbie, Joshua P. DiGangi, Glenn S. Diskin, Marta A. Fenn, Richard A. Ferrare, Johnathan W. Hair, Miguel Ricardo A. Hilario, Chris A. Hostetler, Simon Kirschler, Richard H. Moore, Taylor J. Shingler, Michael A. Shook, Cassidy Soloff, Kenneth L. Thornhill, Christiane Voigt, Edward L. Winstead, Luke D. Ziemba, and Armin Sorooshian
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Ewan Crosbie, Luke D. Ziemba, Michael A. Shook, Taylor Shingler, Johnathan W. Hair, Armin Sorooshian, Richard A. Ferrare, Brian Cairns, Yonghoon Choi, Joshua DiGangi, Glenn S. Diskin, Chris Hostetler, Simon Kirschler, Richard H. Moore, David Painemal, Claire Robinson, Shane T. Seaman, K. Lee Thornhill, Christiane Voigt, and Edward Winstead
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Joshua L. Laughner, Geoffrey C. Toon, Joseph Mendonca, Christof Petri, Sébastien Roche, Debra Wunch, Jean-Francois Blavier, David W. T. Griffith, Pauli Heikkinen, Ralph F. Keeling, Matthäus Kiel, Rigel Kivi, Coleen M. Roehl, Britton B. Stephens, Bianca C. Baier, Huilin Chen, Yonghoon Choi, Nicholas M. Deutscher, Joshua P. DiGangi, Jochen Gross, Benedikt Herkommer, Pascal Jeseck, Thomas Laemmel, Xin Lan, Erin McGee, Kathryn McKain, John Miller, Isamu Morino, Justus Notholt, Hirofumi Ohyama, David F. Pollard, Markus Rettinger, Haris Riris, Constantina Rousogenous, Mahesh Kumar Sha, Kei Shiomi, Kimberly Strong, Ralf Sussmann, Yao Té, Voltaire A. Velazco, Steven C. Wofsy, Minqiang Zhou, and Paul O. Wennberg
Earth Syst. Sci. Data, 16, 2197–2260, https://doi.org/10.5194/essd-16-2197-2024, https://doi.org/10.5194/essd-16-2197-2024, 2024
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Hiren T. Jethva, Omar Torres, Richard A. Ferrare, Sharon P. Burton, Anthony L. Cook, David B. Harper, Chris A. Hostetler, Jens Redemann, Vinay Kayetha, Samuel LeBlanc, Kristina Pistone, Logan Mitchell, and Connor J. Flynn
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We introduce a novel synergy algorithm applied to ORALCES airborne measurements of above-cloud aerosol optical depth and UV–Vis satellite observations from OMI and MODIS to retrieve spectral aerosol single-scattering albedo of lofted layers of carbonaceous smoke aerosols over clouds. The development of the proposed aerosol–cloud algorithm implies a possible synergy of CALIOP and OMI–MODIS passive sensors to deduce a global product of AOD and SSA of absorbing aerosols above clouds.
Eva-Lou Edwards, Yonghoon Choi, Ewan C. Crosbie, Joshua P. DiGangi, Glenn S. Diskin, Claire E. Robinson, Michael A. Shook, Edward L. Winstead, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 24, 3349–3378, https://doi.org/10.5194/acp-24-3349-2024, https://doi.org/10.5194/acp-24-3349-2024, 2024
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We investigate Cl− depletion in sea salt particles over the northwest Atlantic from December 2021 to June 2022 using an airborne dataset. Losses of Cl− are greatest in May and least in December–February and March. Inorganic acidic species can account for all depletion observed for December–February, March, and June near Bermuda but none in May. Quantifying Cl− depletion as a percentage captures seasonal trends in depletion but fails to convey the effects it may have on atmospheric oxidation.
Luis F. Millán, Matthew D. Lebsock, Ken B. Cooper, Jose V. Siles, Robert Dengler, Raquel Rodriguez Monje, Amin Nehrir, Rory A. Barton-Grimley, James E. Collins, Claire E. Robinson, Kenneth L. Thornhill, and Holger Vömel
Atmos. Meas. Tech., 17, 539–559, https://doi.org/10.5194/amt-17-539-2024, https://doi.org/10.5194/amt-17-539-2024, 2024
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In this study, we describe and validate a new technique in which three radar tones are used to estimate the water vapor inside clouds and precipitation. This instrument flew on board NASA's P-3 aircraft during the Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Snowstorms (IMPACTS) campaign and the Synergies Of Active optical and Active microwave Remote Sensing Experiment (SOA2RSE) campaign.
Georgios I. Gkatzelis, Matthew M. Coggon, Chelsea E. Stockwell, Rebecca S. Hornbrook, Hannah Allen, Eric C. Apel, Megan M. Bela, Donald R. Blake, Ilann Bourgeois, Steven S. Brown, Pedro Campuzano-Jost, Jason M. St. Clair, James H. Crawford, John D. Crounse, Douglas A. Day, Joshua P. DiGangi, Glenn S. Diskin, Alan Fried, Jessica B. Gilman, Hongyu Guo, Johnathan W. Hair, Hannah S. Halliday, Thomas F. Hanisco, Reem Hannun, Alan Hills, L. Gregory Huey, Jose L. Jimenez, Joseph M. Katich, Aaron Lamplugh, Young Ro Lee, Jin Liao, Jakob Lindaas, Stuart A. McKeen, Tomas Mikoviny, Benjamin A. Nault, J. Andrew Neuman, John B. Nowak, Demetrios Pagonis, Jeff Peischl, Anne E. Perring, Felix Piel, Pamela S. Rickly, Michael A. Robinson, Andrew W. Rollins, Thomas B. Ryerson, Melinda K. Schueneman, Rebecca H. Schwantes, Joshua P. Schwarz, Kanako Sekimoto, Vanessa Selimovic, Taylor Shingler, David J. Tanner, Laura Tomsche, Krystal T. Vasquez, Patrick R. Veres, Rebecca Washenfelder, Petter Weibring, Paul O. Wennberg, Armin Wisthaler, Glenn M. Wolfe, Caroline C. Womack, Lu Xu, Katherine Ball, Robert J. Yokelson, and Carsten Warneke
Atmos. Chem. Phys., 24, 929–956, https://doi.org/10.5194/acp-24-929-2024, https://doi.org/10.5194/acp-24-929-2024, 2024
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This study reports emissions of gases and particles from wildfires. These emissions are related to chemical proxies that can be measured by satellite and incorporated into models to improve predictions of wildfire impacts on air quality and climate.
Miguel Ricardo A. Hilario, Avelino F. Arellano, Ali Behrangi, Ewan C. Crosbie, Joshua P. DiGangi, Glenn S. Diskin, Michael A. Shook, Luke D. Ziemba, and Armin Sorooshian
Atmos. Meas. Tech., 17, 37–55, https://doi.org/10.5194/amt-17-37-2024, https://doi.org/10.5194/amt-17-37-2024, 2024
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Wet scavenging strongly influences aerosol lifetime and interactions but is a large uncertainty in global models. We present a method to identify meteorological variables relevant for estimating wet scavenging. During long-range transport over the tropical western Pacific, relative humidity and the frequency of humid conditions are better predictors of scavenging than precipitation. This method can be applied to other regions, and our findings can inform scavenging parameterizations in models.
Qian Xiao, Jiaoshi Zhang, Yang Wang, Luke D. Ziemba, Ewan Crosbie, Edward L. Winstead, Claire E. Robinson, Joshua P. DiGangi, Glenn S. Diskin, Jeffrey S. Reid, K. Sebastian Schmidt, Armin Sorooshian, Miguel Ricardo A. Hilario, Sarah Woods, Paul Lawson, Snorre A. Stamnes, and Jian Wang
Atmos. Chem. Phys., 23, 9853–9871, https://doi.org/10.5194/acp-23-9853-2023, https://doi.org/10.5194/acp-23-9853-2023, 2023
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Using recent airborne measurements, we show that the influences of anthropogenic emissions, transport, convective clouds, and meteorology lead to new particle formation (NPF) under a variety of conditions and at different altitudes in tropical marine environments. NPF is enhanced by fresh urban emissions in convective outflow but is suppressed in air masses influenced by aged urban emissions where reactive precursors are mostly consumed while particle surface area remains relatively high.
Armin Sorooshian, Mikhail D. Alexandrov, Adam D. Bell, Ryan Bennett, Grace Betito, Sharon P. Burton, Megan E. Buzanowicz, Brian Cairns, Eduard V. Chemyakin, Gao Chen, Yonghoon Choi, Brian L. Collister, Anthony L. Cook, Andrea F. Corral, Ewan C. Crosbie, Bastiaan van Diedenhoven, Joshua P. DiGangi, Glenn S. Diskin, Sanja Dmitrovic, Eva-Lou Edwards, Marta A. Fenn, Richard A. Ferrare, David van Gilst, Johnathan W. Hair, David B. Harper, Miguel Ricardo A. Hilario, Chris A. Hostetler, Nathan Jester, Michael Jones, Simon Kirschler, Mary M. Kleb, John M. Kusterer, Sean Leavor, Joseph W. Lee, Hongyu Liu, Kayla McCauley, Richard H. Moore, Joseph Nied, Anthony Notari, John B. Nowak, David Painemal, Kasey E. Phillips, Claire E. Robinson, Amy Jo Scarino, Joseph S. Schlosser, Shane T. Seaman, Chellappan Seethala, Taylor J. Shingler, Michael A. Shook, Kenneth A. Sinclair, William L. Smith Jr., Douglas A. Spangenberg, Snorre A. Stamnes, Kenneth L. Thornhill, Christiane Voigt, Holger Vömel, Andrzej P. Wasilewski, Hailong Wang, Edward L. Winstead, Kira Zeider, Xubin Zeng, Bo Zhang, Luke D. Ziemba, and Paquita Zuidema
Earth Syst. Sci. Data, 15, 3419–3472, https://doi.org/10.5194/essd-15-3419-2023, https://doi.org/10.5194/essd-15-3419-2023, 2023
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The NASA Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) produced a unique dataset for research into aerosol–cloud–meteorology interactions. HU-25 Falcon and King Air aircraft conducted systematic and spatially coordinated flights over the northwest Atlantic Ocean. This paper describes the ACTIVATE flight strategy, instrument and complementary dataset products, data access and usage details, and data application notes.
Daniel J. Varon, Daniel J. Jacob, Benjamin Hmiel, Ritesh Gautam, David R. Lyon, Mark Omara, Melissa Sulprizio, Lu Shen, Drew Pendergrass, Hannah Nesser, Zhen Qu, Zachary R. Barkley, Natasha L. Miles, Scott J. Richardson, Kenneth J. Davis, Sudhanshu Pandey, Xiao Lu, Alba Lorente, Tobias Borsdorff, Joannes D. Maasakkers, and Ilse Aben
Atmos. Chem. Phys., 23, 7503–7520, https://doi.org/10.5194/acp-23-7503-2023, https://doi.org/10.5194/acp-23-7503-2023, 2023
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We use TROPOMI satellite observations to quantify weekly methane emissions from the US Permian oil and gas basin from May 2018 to October 2020. We find that Permian emissions are highly variable, with diverse economic and activity drivers. The most important drivers during our study period were new well development and natural gas price. Permian methane intensity averaged 4.6 % and decreased by 1 % per year.
Zachary Barkley, Kenneth Davis, Natasha Miles, Scott Richardson, Aijun Deng, Benjamin Hmiel, David Lyon, and Thomas Lauvaux
Atmos. Chem. Phys., 23, 6127–6144, https://doi.org/10.5194/acp-23-6127-2023, https://doi.org/10.5194/acp-23-6127-2023, 2023
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Using methane monitoring instruments attached to towers, we measure methane concentrations and quantify methane emissions coming from the Marcellus and Permian oil and gas basins. In the Marcellus, emissions were 3 times higher than the state inventory across the entire monitoring period. In the Permian, we see a sharp decline in emissions aligning with the onset of the COVID-19 pandemic. Tower observational networks can be utilized in other basins for long-term monitoring of emissions.
Laura Tomsche, Felix Piel, Tomas Mikoviny, Claus J. Nielsen, Hongyu Guo, Pedro Campuzano-Jost, Benjamin A. Nault, Melinda K. Schueneman, Jose L. Jimenez, Hannah Halliday, Glenn Diskin, Joshua P. DiGangi, John B. Nowak, Elizabeth B. Wiggins, Emily Gargulinski, Amber J. Soja, and Armin Wisthaler
Atmos. Chem. Phys., 23, 2331–2343, https://doi.org/10.5194/acp-23-2331-2023, https://doi.org/10.5194/acp-23-2331-2023, 2023
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Ammonia (NH3) is an important trace gas in the atmosphere and fires are among the poorly investigated sources. During the 2019 Fire Influence on Regional to Global Environments and Air Quality (FIREX-AQ) aircraft campaign, we measured gaseous NH3 and particulate ammonium (NH4+) in smoke plumes emitted from 6 wildfires in the Western US and 66 small agricultural fires in the Southeastern US. We herein present a comprehensive set of emission factors of NH3 and NHx, where NHx = NH3 + NH4+.
Hao Guo, Clare M. Flynn, Michael J. Prather, Sarah A. Strode, Stephen D. Steenrod, Louisa Emmons, Forrest Lacey, Jean-Francois Lamarque, Arlene M. Fiore, Gus Correa, Lee T. Murray, Glenn M. Wolfe, Jason M. St. Clair, Michelle Kim, John Crounse, Glenn Diskin, Joshua DiGangi, Bruce C. Daube, Roisin Commane, Kathryn McKain, Jeff Peischl, Thomas B. Ryerson, Chelsea Thompson, Thomas F. Hanisco, Donald Blake, Nicola J. Blake, Eric C. Apel, Rebecca S. Hornbrook, James W. Elkins, Eric J. Hintsa, Fred L. Moore, and Steven C. Wofsy
Atmos. Chem. Phys., 23, 99–117, https://doi.org/10.5194/acp-23-99-2023, https://doi.org/10.5194/acp-23-99-2023, 2023
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We have prepared a unique and unusual result from the recent ATom aircraft mission: a measurement-based derivation of the production and loss rates of ozone and methane over the ocean basins. These are the key products of chemistry models used in assessments but have thus far lacked observational metrics. It also shows the scales of variability of atmospheric chemical rates and provides a major challenge to the atmospheric models.
Pamela S. Rickly, Hongyu Guo, Pedro Campuzano-Jost, Jose L. Jimenez, Glenn M. Wolfe, Ryan Bennett, Ilann Bourgeois, John D. Crounse, Jack E. Dibb, Joshua P. DiGangi, Glenn S. Diskin, Maximilian Dollner, Emily M. Gargulinski, Samuel R. Hall, Hannah S. Halliday, Thomas F. Hanisco, Reem A. Hannun, Jin Liao, Richard Moore, Benjamin A. Nault, John B. Nowak, Jeff Peischl, Claire E. Robinson, Thomas Ryerson, Kevin J. Sanchez, Manuel Schöberl, Amber J. Soja, Jason M. St. Clair, Kenneth L. Thornhill, Kirk Ullmann, Paul O. Wennberg, Bernadett Weinzierl, Elizabeth B. Wiggins, Edward L. Winstead, and Andrew W. Rollins
Atmos. Chem. Phys., 22, 15603–15620, https://doi.org/10.5194/acp-22-15603-2022, https://doi.org/10.5194/acp-22-15603-2022, 2022
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Biomass burning sulfur dioxide (SO2) emission factors range from 0.27–1.1 g kg-1 C. Biomass burning SO2 can quickly form sulfate and organosulfur, but these pathways are dependent on liquid water content and pH. Hydroxymethanesulfonate (HMS) appears to be directly emitted from some fire sources but is not the sole contributor to the organosulfur signal. It is shown that HMS and organosulfur chemistry may be an important S(IV) reservoir with the fate dependent on the surrounding conditions.
Ewan Crosbie, Luke D. Ziemba, Michael A. Shook, Claire E. Robinson, Edward L. Winstead, K. Lee Thornhill, Rachel A. Braun, Alexander B. MacDonald, Connor Stahl, Armin Sorooshian, Susan C. van den Heever, Joshua P. DiGangi, Glenn S. Diskin, Sarah Woods, Paola Bañaga, Matthew D. Brown, Francesca Gallo, Miguel Ricardo A. Hilario, Carolyn E. Jordan, Gabrielle R. Leung, Richard H. Moore, Kevin J. Sanchez, Taylor J. Shingler, and Elizabeth B. Wiggins
Atmos. Chem. Phys., 22, 13269–13302, https://doi.org/10.5194/acp-22-13269-2022, https://doi.org/10.5194/acp-22-13269-2022, 2022
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The linkage between cloud droplet and aerosol particle chemical composition was analyzed using samples collected in a polluted tropical marine environment. Variations in the droplet composition were related to physical and dynamical processes in clouds to assess their relative significance across three cases that spanned a range of rainfall amounts. In spite of the pollution, sea salt still remained a major contributor to the droplet composition and was preferentially enhanced in rainwater.
Eva-Lou Edwards, Jeffrey S. Reid, Peng Xian, Sharon P. Burton, Anthony L. Cook, Ewan C. Crosbie, Marta A. Fenn, Richard A. Ferrare, Sean W. Freeman, John W. Hair, David B. Harper, Chris A. Hostetler, Claire E. Robinson, Amy Jo Scarino, Michael A. Shook, G. Alexander Sokolowsky, Susan C. van den Heever, Edward L. Winstead, Sarah Woods, Luke D. Ziemba, and Armin Sorooshian
Atmos. Chem. Phys., 22, 12961–12983, https://doi.org/10.5194/acp-22-12961-2022, https://doi.org/10.5194/acp-22-12961-2022, 2022
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This study compares NAAPS-RA model simulations of aerosol optical thickness (AOT) and extinction to those retrieved with a high spectral resolution lidar near the Philippines. Agreement for AOT was good, and extinction agreement was strongest below 1500 m. Substituting dropsonde relative humidities into NAAPS-RA did not drastically improve agreement, and we discuss potential reasons why. Accurately modeling future conditions in this region is crucial due to its susceptibility to climate change.
Ilann Bourgeois, Jeff Peischl, J. Andrew Neuman, Steven S. Brown, Hannah M. Allen, Pedro Campuzano-Jost, Matthew M. Coggon, Joshua P. DiGangi, Glenn S. Diskin, Jessica B. Gilman, Georgios I. Gkatzelis, Hongyu Guo, Hannah A. Halliday, Thomas F. Hanisco, Christopher D. Holmes, L. Gregory Huey, Jose L. Jimenez, Aaron D. Lamplugh, Young Ro Lee, Jakob Lindaas, Richard H. Moore, Benjamin A. Nault, John B. Nowak, Demetrios Pagonis, Pamela S. Rickly, Michael A. Robinson, Andrew W. Rollins, Vanessa Selimovic, Jason M. St. Clair, David Tanner, Krystal T. Vasquez, Patrick R. Veres, Carsten Warneke, Paul O. Wennberg, Rebecca A. Washenfelder, Elizabeth B. Wiggins, Caroline C. Womack, Lu Xu, Kyle J. Zarzana, and Thomas B. Ryerson
Atmos. Meas. Tech., 15, 4901–4930, https://doi.org/10.5194/amt-15-4901-2022, https://doi.org/10.5194/amt-15-4901-2022, 2022
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Understanding fire emission impacts on the atmosphere is key to effective air quality management and requires accurate measurements. We present a comparison of airborne measurements of key atmospheric species in ambient air and in fire smoke. We show that most instruments performed within instrument uncertainties. In some cases, further work is needed to fully characterize instrument performance. Comparing independent measurements using different techniques is important to assess their accuracy.
Harshvardhan Harshvardhan, Richard Ferrare, Sharon Burton, Johnathan Hair, Chris Hostetler, David Harper, Anthony Cook, Marta Fenn, Amy Jo Scarino, Eduard Chemyakin, and Detlef Müller
Atmos. Chem. Phys., 22, 9859–9876, https://doi.org/10.5194/acp-22-9859-2022, https://doi.org/10.5194/acp-22-9859-2022, 2022
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The evolution of aerosol in biomass burning smoke plumes that travel over marine clouds off the Atlantic coast of central Africa was studied using measurements made by a lidar deployed on a high-altitude aircraft. The main finding was that the physical properties of aerosol do not change appreciably once the plume has left land and travels over the ocean over a timescale of 1 to 2 d. Almost all particles in the plume are of radius less than 1 micrometer and spherical in shape.
Linghan Zeng, Jack Dibb, Eric Scheuer, Joseph M. Katich, Joshua P. Schwarz, Ilann Bourgeois, Jeff Peischl, Tom Ryerson, Carsten Warneke, Anne E. Perring, Glenn S. Diskin, Joshua P. DiGangi, John B. Nowak, Richard H. Moore, Elizabeth B. Wiggins, Demetrios Pagonis, Hongyu Guo, Pedro Campuzano-Jost, Jose L. Jimenez, Lu Xu, and Rodney J. Weber
Atmos. Chem. Phys., 22, 8009–8036, https://doi.org/10.5194/acp-22-8009-2022, https://doi.org/10.5194/acp-22-8009-2022, 2022
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Wildfires emit aerosol particles containing brown carbon material that affects visibility and global climate and is toxic. Brown carbon is poorly characterized due to measurement limitations, and its evolution in the atmosphere is not well known. We report on aircraft measurements of brown carbon from large wildfires in the western United States. We compare two methods for measuring brown carbon and study the evolution of brown carbon in the smoke as it moved away from the burning regions.
Vanessa C. Monteiro, Natasha L. Miles, Scott J. Richardson, Zachary Barkley, Bernd J. Haupt, David Lyon, Benjamin Hmiel, and Kenneth J. Davis
Earth Syst. Sci. Data, 14, 2401–2417, https://doi.org/10.5194/essd-14-2401-2022, https://doi.org/10.5194/essd-14-2401-2022, 2022
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We describe a network of five ground-based in situ towers, equipped to measure concentrations of methane, carbon dioxide, hydrogen sulfide, and the isotopic ratio of methane, in the Permian Basin, United States. The main goal is to use methane concentrations with atmospheric models to determine methane emissions from one of the Permian sub-basins. These datasets can improve emissions estimations, leading to best practices in the oil and natural gas industry, and policies for emissions reduction.
Liqiao Lei, Timothy A. Berkoff, Guillaume Gronoff, Jia Su, Amin R. Nehrir, Yonghua Wu, Fred Moshary, and Shi Kuang
Atmos. Meas. Tech., 15, 2465–2478, https://doi.org/10.5194/amt-15-2465-2022, https://doi.org/10.5194/amt-15-2465-2022, 2022
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Aerosol extinction in the UVB (280–315 nm) is difficult to retrieve using simple lidar techniques due to the lack of lidar ratios at those wavelengths. The 2018 Long Island Sound Tropospheric Ozone Study (LISTOS) in the New York City region provided the opportunity to characterize the lidar ratio for UVB aerosol retrieval for the Langley Mobile Ozone Lidar (LMOL). A 292 nm aerosol product comparison between the NASA Langley High Altitude Lidar Observatory (HALO) and LMOL was also carried out.
Brian J. Carroll, Amin R. Nehrir, Susan A. Kooi, James E. Collins, Rory A. Barton-Grimley, Anthony Notari, David B. Harper, and Joseph Lee
Atmos. Meas. Tech., 15, 605–626, https://doi.org/10.5194/amt-15-605-2022, https://doi.org/10.5194/amt-15-605-2022, 2022
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HALO is a recently developed lidar system that demonstrates new technologies and advanced algorithms for profiling water vapor as well as aerosol and cloud properties. The high-resolution, high-accuracy measurements have unique advantages within the suite of atmospheric instrumentation, such as directly trading water vapor measurement resolution for precision. This paper provides the methodology and first water vapor results, showing agreement with in situ and spaceborne sounder measurements.
David F. Baker, Emily Bell, Kenneth J. Davis, Joel F. Campbell, Bing Lin, and Jeremy Dobler
Geosci. Model Dev., 15, 649–668, https://doi.org/10.5194/gmd-15-649-2022, https://doi.org/10.5194/gmd-15-649-2022, 2022
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The OCO-2 satellite measures many closely spaced column-averaged CO2 values around its orbit. To give these data proper weight in flux inversions, their error correlations must be accounted for. Here we lay out a 1-D error model with correlations that die out exponentially along-track to do so. A correlation length scale of ∼20 km is derived from column CO2 measurements from an airborne lidar flown underneath OCO-2 for use in this model. The model's performance is compared to previous ones.
Dongwook Kim, Changmin Cho, Seokhan Jeong, Soojin Lee, Benjamin A. Nault, Pedro Campuzano-Jost, Douglas A. Day, Jason C. Schroder, Jose L. Jimenez, Rainer Volkamer, Donald R. Blake, Armin Wisthaler, Alan Fried, Joshua P. DiGangi, Glenn S. Diskin, Sally E. Pusede, Samuel R. Hall, Kirk Ullmann, L. Gregory Huey, David J. Tanner, Jack Dibb, Christoph J. Knote, and Kyung-Eun Min
Atmos. Chem. Phys., 22, 805–821, https://doi.org/10.5194/acp-22-805-2022, https://doi.org/10.5194/acp-22-805-2022, 2022
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CHOCHO was simulated using a 0-D box model constrained by measurements during the KORUS-AQ mission. CHOCHO concentration was high in large cities, aromatics being the most important precursors. Loss path to aerosol was the highest sink, contributing to ~ 20 % of secondary organic aerosol formation. Our work highlights that simple CHOCHO surface uptake approach is valid only for low aerosol conditions and more work is required to understand CHOCHO solubility in high-aerosol conditions.
Jin Liao, Glenn M. Wolfe, Reem A. Hannun, Jason M. St. Clair, Thomas F. Hanisco, Jessica B. Gilman, Aaron Lamplugh, Vanessa Selimovic, Glenn S. Diskin, John B. Nowak, Hannah S. Halliday, Joshua P. DiGangi, Samuel R. Hall, Kirk Ullmann, Christopher D. Holmes, Charles H. Fite, Anxhelo Agastra, Thomas B. Ryerson, Jeff Peischl, Ilann Bourgeois, Carsten Warneke, Matthew M. Coggon, Georgios I. Gkatzelis, Kanako Sekimoto, Alan Fried, Dirk Richter, Petter Weibring, Eric C. Apel, Rebecca S. Hornbrook, Steven S. Brown, Caroline C. Womack, Michael A. Robinson, Rebecca A. Washenfelder, Patrick R. Veres, and J. Andrew Neuman
Atmos. Chem. Phys., 21, 18319–18331, https://doi.org/10.5194/acp-21-18319-2021, https://doi.org/10.5194/acp-21-18319-2021, 2021
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Formaldehyde (HCHO) is an important oxidant precursor and affects the formation of O3 and other secondary pollutants in wildfire plumes. We disentangle the processes controlling HCHO evolution from wildfire plumes sampled by NASA DC-8 during FIREX-AQ. We find that OH abundance rather than normalized OH reactivity is the main driver of fire-to-fire variability in HCHO secondary production and estimate an effective HCHO yield per volatile organic compound molecule oxidized in wildfire plumes.
Zachary C. J. Decker, Michael A. Robinson, Kelley C. Barsanti, Ilann Bourgeois, Matthew M. Coggon, Joshua P. DiGangi, Glenn S. Diskin, Frank M. Flocke, Alessandro Franchin, Carley D. Fredrickson, Georgios I. Gkatzelis, Samuel R. Hall, Hannah Halliday, Christopher D. Holmes, L. Gregory Huey, Young Ro Lee, Jakob Lindaas, Ann M. Middlebrook, Denise D. Montzka, Richard Moore, J. Andrew Neuman, John B. Nowak, Brett B. Palm, Jeff Peischl, Felix Piel, Pamela S. Rickly, Andrew W. Rollins, Thomas B. Ryerson, Rebecca H. Schwantes, Kanako Sekimoto, Lee Thornhill, Joel A. Thornton, Geoffrey S. Tyndall, Kirk Ullmann, Paul Van Rooy, Patrick R. Veres, Carsten Warneke, Rebecca A. Washenfelder, Andrew J. Weinheimer, Elizabeth Wiggins, Edward Winstead, Armin Wisthaler, Caroline Womack, and Steven S. Brown
Atmos. Chem. Phys., 21, 16293–16317, https://doi.org/10.5194/acp-21-16293-2021, https://doi.org/10.5194/acp-21-16293-2021, 2021
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To understand air quality impacts from wildfires, we need an accurate picture of how wildfire smoke changes chemically both day and night as sunlight changes the chemistry of smoke. We present a chemical analysis of wildfire smoke as it changes from midday through the night. We use aircraft observations from the FIREX-AQ field campaign with a chemical box model. We find that even under sunlight typical
nighttimechemistry thrives and controls the fate of key smoke plume chemical processes.
Charles A. Brock, Karl D. Froyd, Maximilian Dollner, Christina J. Williamson, Gregory Schill, Daniel M. Murphy, Nicholas J. Wagner, Agnieszka Kupc, Jose L. Jimenez, Pedro Campuzano-Jost, Benjamin A. Nault, Jason C. Schroder, Douglas A. Day, Derek J. Price, Bernadett Weinzierl, Joshua P. Schwarz, Joseph M. Katich, Siyuan Wang, Linghan Zeng, Rodney Weber, Jack Dibb, Eric Scheuer, Glenn S. Diskin, Joshua P. DiGangi, ThaoPaul Bui, Jonathan M. Dean-Day, Chelsea R. Thompson, Jeff Peischl, Thomas B. Ryerson, Ilann Bourgeois, Bruce C. Daube, Róisín Commane, and Steven C. Wofsy
Atmos. Chem. Phys., 21, 15023–15063, https://doi.org/10.5194/acp-21-15023-2021, https://doi.org/10.5194/acp-21-15023-2021, 2021
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The Atmospheric Tomography Mission was an airborne study that mapped the chemical composition of the remote atmosphere. From this, we developed a comprehensive description of aerosol properties that provides a unique, global-scale dataset against which models can be compared. The data show the polluted nature of the remote atmosphere in the Northern Hemisphere and quantify the contributions of sea salt, dust, soot, biomass burning particles, and pollution particles to the haziness of the sky.
Hao Guo, Clare M. Flynn, Michael J. Prather, Sarah A. Strode, Stephen D. Steenrod, Louisa Emmons, Forrest Lacey, Jean-Francois Lamarque, Arlene M. Fiore, Gus Correa, Lee T. Murray, Glenn M. Wolfe, Jason M. St. Clair, Michelle Kim, John Crounse, Glenn Diskin, Joshua DiGangi, Bruce C. Daube, Roisin Commane, Kathryn McKain, Jeff Peischl, Thomas B. Ryerson, Chelsea Thompson, Thomas F. Hanisco, Donald Blake, Nicola J. Blake, Eric C. Apel, Rebecca S. Hornbrook, James W. Elkins, Eric J. Hintsa, Fred L. Moore, and Steven Wofsy
Atmos. Chem. Phys., 21, 13729–13746, https://doi.org/10.5194/acp-21-13729-2021, https://doi.org/10.5194/acp-21-13729-2021, 2021
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The NASA Atmospheric Tomography (ATom) mission built a climatology of the chemical composition of tropospheric air parcels throughout the middle of the Pacific and Atlantic oceans. The level of detail allows us to reconstruct the photochemical budgets of O3 and CH4 over these vast, remote regions. We find that most of the chemical heterogeneity is captured at the resolution used in current global chemistry models and that the majority of reactivity occurs in the
hottest20 % of parcels.
Min Huang, James H. Crawford, Joshua P. DiGangi, Gregory R. Carmichael, Kevin W. Bowman, Sujay V. Kumar, and Xiwu Zhan
Atmos. Chem. Phys., 21, 11013–11040, https://doi.org/10.5194/acp-21-11013-2021, https://doi.org/10.5194/acp-21-11013-2021, 2021
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This study evaluates the impact of satellite soil moisture data assimilation on modeled weather and ozone fields at various altitudes above the southeastern US during the summer. It emphasizes the importance of soil moisture in the understanding of surface ozone pollution and upper tropospheric chemistry, as well as air pollutants’ source–receptor relationships between the US and its downwind areas.
Christina J. Williamson, Agnieszka Kupc, Andrew Rollins, Jan Kazil, Karl D. Froyd, Eric A. Ray, Daniel M. Murphy, Gregory P. Schill, Jeff Peischl, Chelsea Thompson, Ilann Bourgeois, Thomas B. Ryerson, Glenn S. Diskin, Joshua P. DiGangi, Donald R. Blake, Thao Paul V. Bui, Maximilian Dollner, Bernadett Weinzierl, and Charles A. Brock
Atmos. Chem. Phys., 21, 9065–9088, https://doi.org/10.5194/acp-21-9065-2021, https://doi.org/10.5194/acp-21-9065-2021, 2021
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Aerosols in the stratosphere influence climate by scattering and absorbing sunlight and through chemical reactions occurring on the particles’ surfaces. We observed more nucleation mode aerosols (small aerosols, with diameters below 12 nm) in the mid- and high-latitude lowermost stratosphere (8–13 km) in the Northern Hemisphere (NH) than in the Southern Hemisphere. The most likely cause of this is aircraft emissions, which are concentrated in the NH at similar altitudes to our observations.
Kristopher M. Bedka, Amin R. Nehrir, Michael Kavaya, Rory Barton-Grimley, Mark Beaubien, Brian Carroll, James Collins, John Cooney, G. David Emmitt, Steven Greco, Susan Kooi, Tsengdar Lee, Zhaoyan Liu, Sharon Rodier, and Gail Skofronick-Jackson
Atmos. Meas. Tech., 14, 4305–4334, https://doi.org/10.5194/amt-14-4305-2021, https://doi.org/10.5194/amt-14-4305-2021, 2021
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This paper demonstrates the Doppler Aerosol WiNd (DAWN) lidar and High Altitude Lidar Observatory (HALO) measurement capabilities across a range of atmospheric conditions, compares DAWN and HALO measurements with Aeolus satellite Doppler wind lidar to gain an initial perspective of Aeolus performance, and discusses how atmospheric dynamic processes can be resolved and better understood through simultaneous observations of wind, water vapour, and aerosol profile observations.
Tao Zheng, Sha Feng, Kenneth J. Davis, Sandip Pal, and Josep-Anton Morguí
Geosci. Model Dev., 14, 3037–3066, https://doi.org/10.5194/gmd-14-3037-2021, https://doi.org/10.5194/gmd-14-3037-2021, 2021
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Carbon dioxide is the most important greenhouse gas. We develop the numerical model that represents carbon dioxide transport in the atmosphere. This model development is based on the MPAS model, which has a variable-resolution capability. The purpose of developing carbon dioxide transport in MPAS is to allow for high-resolution transport model simulation that is not limited by the lateral boundaries. It will also form the base for a future development of MPAS-based carbon inversion system.
David R. Lyon, Benjamin Hmiel, Ritesh Gautam, Mark Omara, Katherine A. Roberts, Zachary R. Barkley, Kenneth J. Davis, Natasha L. Miles, Vanessa C. Monteiro, Scott J. Richardson, Stephen Conley, Mackenzie L. Smith, Daniel J. Jacob, Lu Shen, Daniel J. Varon, Aijun Deng, Xander Rudelis, Nikhil Sharma, Kyle T. Story, Adam R. Brandt, Mary Kang, Eric A. Kort, Anthony J. Marchese, and Steven P. Hamburg
Atmos. Chem. Phys., 21, 6605–6626, https://doi.org/10.5194/acp-21-6605-2021, https://doi.org/10.5194/acp-21-6605-2021, 2021
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The Permian Basin (USA) is the world’s largest oil field. We use tower- and aircraft-based approaches to measure how methane emissions in the Permian Basin changed throughout 2020. In early 2020, 3.3 % of the region’s gas was emitted; then in spring 2020, the loss rate temporarily dropped to 1.9 % as oil price crashed. We find this short-term reduction to be a result of reduced well development, less gas flaring, and fewer abnormal events despite minimal reductions in oil and gas production.
Miguel Ricardo A. Hilario, Ewan Crosbie, Michael Shook, Jeffrey S. Reid, Maria Obiminda L. Cambaliza, James Bernard B. Simpas, Luke Ziemba, Joshua P. DiGangi, Glenn S. Diskin, Phu Nguyen, F. Joseph Turk, Edward Winstead, Claire E. Robinson, Jian Wang, Jiaoshi Zhang, Yang Wang, Subin Yoon, James Flynn, Sergio L. Alvarez, Ali Behrangi, and Armin Sorooshian
Atmos. Chem. Phys., 21, 3777–3802, https://doi.org/10.5194/acp-21-3777-2021, https://doi.org/10.5194/acp-21-3777-2021, 2021
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This study characterizes long-range transport from major Asian pollution sources into the tropical northwest Pacific and the impact of scavenging on these air masses. We combined aircraft observations, HYSPLIT trajectories, reanalysis, and satellite retrievals to reveal distinct composition and size distribution profiles associated with specific emission sources and wet scavenging. The results of this work have implications for international policymaking related to climate and health.
Johannes Schneider, Ralf Weigel, Thomas Klimach, Antonis Dragoneas, Oliver Appel, Andreas Hünig, Sergej Molleker, Franziska Köllner, Hans-Christian Clemen, Oliver Eppers, Peter Hoppe, Peter Hoor, Christoph Mahnke, Martina Krämer, Christian Rolf, Jens-Uwe Grooß, Andreas Zahn, Florian Obersteiner, Fabrizio Ravegnani, Alexey Ulanovsky, Hans Schlager, Monika Scheibe, Glenn S. Diskin, Joshua P. DiGangi, John B. Nowak, Martin Zöger, and Stephan Borrmann
Atmos. Chem. Phys., 21, 989–1013, https://doi.org/10.5194/acp-21-989-2021, https://doi.org/10.5194/acp-21-989-2021, 2021
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During five aircraft missions, we detected aerosol particles containing meteoric material in the lower stratosphere. The stratospheric measurements span a latitude range from 15 to 68° N, and we find that at potential temperature levels of more than 40 K above the tropopause; particles containing meteoric material occur at similar abundance fractions across latitudes and seasons. We conclude that meteoric material is efficiently distributed between high and low latitudes by isentropic mixing.
Xueying Yu, Dylan B. Millet, Kelley C. Wells, Daven K. Henze, Hansen Cao, Timothy J. Griffis, Eric A. Kort, Genevieve Plant, Malte J. Deventer, Randall K. Kolka, D. Tyler Roman, Kenneth J. Davis, Ankur R. Desai, Bianca C. Baier, Kathryn McKain, Alan C. Czarnetzki, and A. Anthony Bloom
Atmos. Chem. Phys., 21, 951–971, https://doi.org/10.5194/acp-21-951-2021, https://doi.org/10.5194/acp-21-951-2021, 2021
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Methane concentrations have doubled since 1750. The US Upper Midwest is a key region contributing to such trends, but sources are poorly understood. We collected and analyzed aircraft data to resolve spatial and timing biases in wetland and livestock emission estimates and uncover errors in inventory treatment of manure management. We highlight the importance of intensive agriculture for the regional and US methane budgets and the potential for methane mitigation through improved management.
Laura M. Judd, Jassim A. Al-Saadi, James J. Szykman, Lukas C. Valin, Scott J. Janz, Matthew G. Kowalewski, Henk J. Eskes, J. Pepijn Veefkind, Alexander Cede, Moritz Mueller, Manuel Gebetsberger, Robert Swap, R. Bradley Pierce, Caroline R. Nowlan, Gonzalo González Abad, Amin Nehrir, and David Williams
Atmos. Meas. Tech., 13, 6113–6140, https://doi.org/10.5194/amt-13-6113-2020, https://doi.org/10.5194/amt-13-6113-2020, 2020
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This paper evaluates Sentinel-5P TROPOMI v1.2 NO2 tropospheric columns over New York City using data from airborne mapping spectrometers and a network of ground-based spectrometers (Pandora) collected in 2018. These evaluations consider impacts due to cloud parameters, a priori profile assumptions, and spatial and temporal variability. Overall, TROPOMI tropospheric NO2 columns appear to have a low bias in this region.
Petter Weibring, Dirk Richter, James G. Walega, Alan Fried, Joshua DiGangi, Hannah Halliday, Yonghoon Choi, Bianca Baier, Colm Sweeney, Ben Miller, Kenneth J. Davis, Zachary Barkley, and Michael D. Obland
Atmos. Meas. Tech., 13, 6095–6112, https://doi.org/10.5194/amt-13-6095-2020, https://doi.org/10.5194/amt-13-6095-2020, 2020
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The present study describes an autonomously operated instrument for high-precision (20–40 parts per trillion in 1 s) measurements of ethane during actual airborne operations on a small aircraft platform (NASA's King Air B200). This paper discusses the dynamic nature of airborne performance due to various aircraft-induced perturbations, methods devised to identify such events, and solutions we have enacted to circumvent these perturbations.
Lei Zhu, Gonzalo González Abad, Caroline R. Nowlan, Christopher Chan Miller, Kelly Chance, Eric C. Apel, Joshua P. DiGangi, Alan Fried, Thomas F. Hanisco, Rebecca S. Hornbrook, Lu Hu, Jennifer Kaiser, Frank N. Keutsch, Wade Permar, Jason M. St. Clair, and Glenn M. Wolfe
Atmos. Chem. Phys., 20, 12329–12345, https://doi.org/10.5194/acp-20-12329-2020, https://doi.org/10.5194/acp-20-12329-2020, 2020
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We develop a validation platform for satellite HCHO retrievals using in situ observations from 12 aircraft campaigns. The platform offers an alternative way to quickly assess systematic biases in HCHO satellite products over large domains and long periods, facilitating optimization of retrieval settings and the minimization of retrieval biases. Application to the NASA operational HCHO product indicates that relative biases range from −44.5 % to +112.1 % depending on locations and seasons.
Hirofumi Ohyama, Isamu Morino, Voltaire A. Velazco, Theresa Klausner, Gerry Bagtasa, Matthäus Kiel, Matthias Frey, Akihiro Hori, Osamu Uchino, Tsuneo Matsunaga, Nicholas M. Deutscher, Joshua P. DiGangi, Yonghoon Choi, Glenn S. Diskin, Sally E. Pusede, Alina Fiehn, Anke Roiger, Michael Lichtenstern, Hans Schlager, Pao K. Wang, Charles C.-K. Chou, Maria Dolores Andrés-Hernández, and John P. Burrows
Atmos. Meas. Tech., 13, 5149–5163, https://doi.org/10.5194/amt-13-5149-2020, https://doi.org/10.5194/amt-13-5149-2020, 2020
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Column-averaged dry-air mole fractions of CO2 and CH4 measured by a solar viewing portable Fourier transform spectrometer (EM27/SUN) were validated with in situ profile data obtained during the transfer flights of two aircraft campaigns. Atmospheric dynamical properties based on ERA5 and WRF-Chem were used as criteria for selecting the best aircraft profiles for the validation. The resulting air-mass-independent correction factors for the EM27/SUN data were 0.9878 for CO2 and 0.9829 for CH4.
Kirk Knobelspiesse, Henrique M. J. Barbosa, Christine Bradley, Carol Bruegge, Brian Cairns, Gao Chen, Jacek Chowdhary, Anthony Cook, Antonio Di Noia, Bastiaan van Diedenhoven, David J. Diner, Richard Ferrare, Guangliang Fu, Meng Gao, Michael Garay, Johnathan Hair, David Harper, Gerard van Harten, Otto Hasekamp, Mark Helmlinger, Chris Hostetler, Olga Kalashnikova, Andrew Kupchock, Karla Longo De Freitas, Hal Maring, J. Vanderlei Martins, Brent McBride, Matthew McGill, Ken Norlin, Anin Puthukkudy, Brian Rheingans, Jeroen Rietjens, Felix C. Seidel, Arlindo da Silva, Martijn Smit, Snorre Stamnes, Qian Tan, Sebastian Val, Andrzej Wasilewski, Feng Xu, Xiaoguang Xu, and John Yorks
Earth Syst. Sci. Data, 12, 2183–2208, https://doi.org/10.5194/essd-12-2183-2020, https://doi.org/10.5194/essd-12-2183-2020, 2020
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The Aerosol Characterization from Polarimeter and Lidar (ACEPOL) field campaign is a resource for the next generation of spaceborne multi-angle polarimeter (MAP) and lidar missions. Conducted in the fall of 2017 from the Armstrong Flight Research Center in Palmdale, California, four MAP instruments and two lidars were flown on the high-altitude ER-2 aircraft over a variety of scene types and ground assets. Data are freely available to the public and useful for algorithm development and testing.
Wenfu Tang, Benjamin Gaubert, Louisa Emmons, Yonghoon Choi, Joshua P. DiGangi, Glenn S. Diskin, Xiaomei Xu, Cenlin He, Helen Worden, Simone Tilmes, Rebecca Buchholz, Hannah S. Halliday, and Avelino F. Arellano
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-864, https://doi.org/10.5194/acp-2020-864, 2020
Revised manuscript not accepted
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A specific demonstration of the potential use of correlative information from carbon monoxide to refine estimates of regional carbon dioxide emissions from fossil fuel combustion.
Cited articles
Abshire, J. B., Ramanathan, A. K., Riris, H., Allan, G. R., Sun, X., Hasselbrack, W. E., Mao, J., Wu, S., Chen, J., Numata, K., Kawa, S. R., Yang, M. Y. M., and DiGangi, J.: Airborne measurements of CO2 column concentrations made with a pulsed IPDA lidar using a multiple-wavelength-locked laser and HgCdTe APD detector, Atmos. Meas. Tech., 11, 2001–2025, https://doi.org/10.5194/amt-11-2001-2018, 2018.
Alvarez, R. A., Zavala-Araiza, D., Lyon, D. R., Allen, D. T., Barkley, Z. R.,
Brandt, A. R., Davis, K. J., Herndon, S. C., Jacob, D. J., Karion, A., and Kort, E. A.: Assessment of methane emissions from the US oil and gas supply
chain, Science, 361, 186–188, 2018.
Amediek, A., Sun, X., and Abshire, J. B.: Analysis of Range Measurements From
a Pulsed Airborne CO2 Integrated Path Differential Absorption Lidar, IEEE T. Geosci. Remote, 51, 2498–2504, 2013.
Amediek, A., Ehret, G., Fix, A., Wirth, M., Büdenbender, C., Quatrevalet, M., Kiemle, C., and Gerbig, C.: CHARM-F – a new airborne integrated-path differential-absorption lidar for carbon dioxide and methane observations: measurement performance and quantification of strong point source emissions, Appl. Optics, 56, 5182–5197, 2017.
Amediek, A., Fix, A., Ehret, G., Caron, J., and Durand, Y.: Airborne lidar reflectance measurements at 1.57 µm in support of the A-SCOPE mission for atmospheric CO2, Atmos. Meas. Tech., 2, 755–772, https://doi.org/10.5194/amt-2-755-2009, 2009.
Andrews, A. E., Kofler, J. D., Trudeau, M. E., Williams, J. C., Neff, D. H., Masarie, K. A., Chao, D. Y., Kitzis, D. R., Novelli, P. C., Zhao, C. L., Dlugokencky, E. J., Lang, P. M., Crotwell, M. J., Fischer, M. L., Parker, M. J., Lee, J. T., Baumann, D. D., Desai, A. R., Stanier, C. O., De Wekker, S. F. J., Wolfe, D. E., Munger, J. W., and Tans, P. P.: CO2, CO, and CH4 measurements from tall towers in the NOAA Earth System Research Laboratory's Global Greenhouse Gas Reference Network: instrumentation, uncertainty analysis, and recommendations for future high-accuracy greenhouse gas monitoring efforts, Atmos. Meas. Tech., 7, 647–687, https://doi.org/10.5194/amt-7-647-2014, 2014.
Barkley, Z. R., Lauvaux, T., Davis, K. J., Fried, A., Weibring, P., Richter, D., Walega, J. G., DiGangi, J., Ehrman, S. H., Ren, X., and Dickerson, R. R.:
Estimating methane emissions from underground coal and natural gas production in southwestern Pennsylvania, Geophys. Res. Lett., 46, 4531–4540, 2019a.
Barkley, Z. R., Davis, K. J., Feng, S., Balashov, N., Fried, A., DiGangi, J., Choi, Y., and Halliday, H. S.: Forward Modeling and Optimization of Methane Emissions in the South Central United States Using Aircraft Transects Across Frontal Boundaries, Geophys. Res. Lett., 46, 13564–13573, 2019b.
Barkley, Z. R., Davis, K. J., Feng, S., Cui, Y. Y., Fried, A., Weibring, P.,
Richter, D., Walega, J. G., Miller, S. M., Eckl, M., Roiger, A., Fiehn, A., and Kostinek, J.: Analysis of oil and gas ethane and methane emissions in the
southcentral and eastern United States using four seasons of continuous
aircraft ethane measurements, J. Geophys. Res.-Atmos., 126, e2020JD034194, https://doi.org/10.1029/2020JD034194, 2021.
Bedka, K. M., Nehrir, A. R., Kavaya, M., Barton-Grimley, R., Beaubien, M., Carroll, B., Collins, J., Cooney, J., Emmitt, G. D., Greco, S., Kooi, S., Lee, T., Liu, Z., Rodier, S., and Skofronick-Jackson, G.: Airborne lidar observations of wind, water vapor, and aerosol profiles during the NASA Aeolus calibration and validation (Cal/Val) test flight campaign, Atmos. Meas. Tech., 14, 4305–4334, https://doi.org/10.5194/amt-14-4305-2021, 2021.
Bell, E., O'Dell, C. W., Davis, K. J., Campbell, J., Browell, E., Scott
Denning, A., Dobler, J., Erxleben, W., Fan, T. F., Kooi, S., and Lin, B.:
Evaluation of OCO-2 X variability at local and synoptic scales using lidar
and in situ observations from the ACT-America campaigns, J. Geophys. Res.-Atmos., 125, e2019JD031400, https://doi.org/10.1029/2019JD031400, 2020.
Bousquet, P., Ciais, P., Miller, J. B., Dlugokencky, E. J., Hauglustaine,
D. A., Prigent, C., Van der Werf, G. R., Peylin, P., Brunke, E. G., Carouge, C., and Langenfelds, R. L.: Contribution of anthropogenic and natural sources to atmospheric methane variability, Nature, 443, 439–443, 2006.
Bousquet, P., Ringeval, B., Pison, I., Dlugokencky, E. J., Brunke, E.-G., Carouge, C., Chevallier, F., Fortems-Cheiney, A., Frankenberg, C., Hauglustaine, D. A., Krummel, P. B., Langenfelds, R. L., Ramonet, M., Schmidt, M., Steele, L. P., Szopa, S., Yver, C., Viovy, N., and Ciais, P.: Source attribution of the changes in atmospheric methane for 2006–2008, Atmos. Chem. Phys., 11, 3689–3700, https://doi.org/10.5194/acp-11-3689-2011, 2011.
Browell, E. V., Ismail, S., and Grant, W. B.: Differential absorption lidar
(DIAL) measurements from air and space, Appl. Phys. B, 67, 399–410, 1998.
Bruhwiler, L., Dlugokencky, E., Masarie, K., Ishizawa, M., Andrews, A., Miller, J., Sweeney, C., Tans, P., and Worthy, D.: CarbonTracker-CH4: an assimilation system for estimating emissions of atmospheric methane, Atmos. Chem. Phys., 14, 8269–8293, https://doi.org/10.5194/acp-14-8269-2014, 2014.
Campbell, J. F., Lin, B., Dobler, J., Pal, S., Davis, K., Obland, M. D.,
Erxleben, W., McGregor, D., O'Dell, C., Bell, E., and Weir, B.: Field
evaluation of column CO2 retrievals from intensity-modulated continuous-wave
differential absorption lidar measurements during the ACT-America campaign, Earth Space Sci., 7, e2019EA000847, https://doi.org/10.1029/2019EA000847, 2020.
Carroll, B. J., Nehrir, A. R., Kooi, S. A., Collins, J. E., Barton-Grimley, R. A., Notari, A., Harper, D. B., and Lee, J.: Differential absorption lidar measurements of water vapor by the High Altitude Lidar Observatory (HALO): retrieval framework and first results, Atmos. Meas. Tech., 15, 605–626, https://doi.org/10.5194/amt-15-605-2022, 2022.
Cassé, V., Gibert, F., Edouart, D., Chomette, O., and Crevoisier, C.:
Optical energy variability induced by speckle: The cases of MERLIN and
CHARM-F IPDA lidar, Atmosphere, 10, 540, https://doi.org/10.3390/atmos10090540, 2019.
Cui, Y. Y., Brioude, J., McKeen, S. A., Angevine, W. M., Kim, S. W., Frost,
G. J., Ahmadov, R., Peischl, J., Bousserez, N., Liu, Z., and Ryerson, T. B.:
Top-down estimate of methane emissions in California using a mesoscale
inverse modeling technique: The South Coast Air Basin, J. Geophys. Res.-Atmos., 120, 6698–6711, 2015.
Cusworth, D. H., Duren, R. M., Thorpe, A. K., Olson-Duvall, W., Heckler, J.,
Chapman, J. W., Eastwood, M. L., Helmlinger, M. C., Green, R. O., Asner, G. P., and Dennison, P. E.: Intermittency of large methane emitters in the Permian Basin, Environ. Sci. Tech. Let., 8, 567–573, 2021.
Davis, K. J., Browell, E. V., Feng, S., Lauvaux, T., Obland, M. D., Pal, S.,
Baier, B. C., Baker, D. F., Baker, I. T., Barkley, Z. R., and Bowman, K. W.: The atmospheric carbon and transport (ACT)-America mission, B. Am. Meteorol. Soc., 102, E1714–E1734, 2021.
Dean, J. F., Middelburg, J. J., Röckmann, T., Aerts, R., Blauw, L. G.,
Egger, M., Jetten, M. S., de Jong, A. E., Meisel, O. H., Rasigraf, O., and
Slomp, C. P.: Methane feedbacks to the global climate system in a warmer
world, Rev. Geophys., 56, 207–250, 2018.
Delahaye, T., Landsheere, X., Pangui, E., Huet, F., Hartmann, J. M., and Tran, H.: Measurements of H2O broadening coefficients of infrared methane lines, J. Quant. Spectrosc. Ra., 173, 40–48, 2016a.
Delahaye, T., Maxwell, S. E., Reed, Z. D., Lin, H., Hodges, J. T., Sung, K.,
Devi, V. M., Warneke, T., Spietz, P., and Tran, H.: Precise methane absorption measurements in the 1.64 µm spectral region for the MERLIN mission, J. Geophys. Res.-Atmos., 121, 7360–7370, 2016b.
Delahaye, T., Ghysels, M., Hodges, J. T., Sung, K., Armante, R., and Tran, H.: Measurement and modeling of air-broadened methane absorption in the MERLIN spectral region at low temperatures, J. Geophys. Res.-Atmos., 124, 3556–3564, 2019.
DiGangi, J. P., Choi, Y., Nowak, J. B., Halliday, H. S., Yang, M. M., Baier, B. C., and Sweeney, C.: ACT-America: L2 In Situ Atmospheric CO2, CO, CH4, and O3 Concentrations, Eastern USA, ORNL DAAC [data set], Oak Ridge, Tennessee, USA, https://doi.org/10.3334/ORNLDAAC/1556, 2018.
DiGangi, J. P., Choi, Y., Nowak, J. B., Halliday, H. S., Diskin, G. S., Feng,
S., Barkley, Z. R., Lauvaux, T., Pal, S., Davis, K. J. and Baier, B. C.: Seasonal variability in local carbon dioxide biomass burning sources over
central and eastern US using airborne in situ enhancement ratios, J. Geophys. Res.-Atmos., 126, e2020JD034525, https://doi.org/10.1029/2020JD034525, 2021.
Dobler, J. T., Harrison, F. W., Browell, E. V., Lin, B., McGregor, D., Kooi,
S., Choi, Y., and Ismail, S.: Atmospheric CO2 column measurements with an
airborne intensity-modulated continuous wave 1.57 µm fiber laser
lidar, Appl. Optics, 52, 2874–2892, 2013.
Dufour, E. and Bréon, F. M.: Spaceborne estimate of atmospheric CO2
column by use of the differential absorption method: error analysis, Appl. Optics, 42, 3595–3609, 2003.
Ehhalt, D., Prather, M., Dentener, F., Derwent, R., Dlugokencky, Edward J.,
Holland, E., Isaksen, I., Katima, J., Kirchhoff, V., Matson, P., Midgley, P.,
Wang, M., Berntsen, T., Bey, I., Brasseur, G., Buja, L., Collins, W. J., Daniel, J. S., DeMore, W. B., Derek, N., Dickerson, R., Etheridge, D., Feichter, J., Fraser, P., Friedl, R., Fuglestvedt, J., Gauss, M., Grenfell, L., Grübler, A., Harris, N., Hauglustaine, D., Horowitz, L., Jackman, C., Jacob, D., Jaeglé, L., Jain, A., Kanakidou, M., Karlsdottir, S., Ko, M., Kurylo, M., Lawrence, M., Logan, J. A., Manning, M., Mauzerall, D., McConnell, J., Mickley, L. J., Montzka, S., Muller, J. F., Olivier, J., Pickering, K., Pitari, G., Roelofs, G.-J., Rogers, H., Rognerud, B., Smith, Steven J., Solomon, S., Staehelin, J., Steele, P., Stevenson, D. S., Sundet, J., Thompson, A., van Weele, M., von Kuhlmann, R., Wang, Y., Weisenstein, D. K., Wigley, T. M., Wild, O., Wuebbles, D. J., Yantosca, R., Joos, F., and McFarland, M.: Atmospheric Chemistry and Greenhouse Gases, United States, chapter 4, https://www.ipcc.ch/report/ar3/wg1/chapter-4-atmospheric-chemistry-and-greenhouse-gases/
(last access: 13 July 2022), 2001.
Ehret, G., Kiemle, C., Wirth, M., Amediek, A., Fix, A., and Houweling, S.:
Space-borne remote sensing of CO2, CH4, and N2O by integrated path
differential absorption lidar: a sensitivity analysis, Appl. Phys. B, 90, 593–608, 2008.
Ehret, G., Bousquet, P., Pierangelo, C., Alpers, M., Millet, B., Abshire,
J. B., Bovensmann, H., Burrows, J. P., Chevallier, F., Ciais, P., and
Crevoisier, C.: MERLIN: A French-German space lidar mission dedicated to
atmospheric methane, Remote Sens., 9, 1052, https://doi.org/10.3390/rs9101052, 2017.
Feng, S., Lauvaux, T., Keller, K., Davis, K. J., Rayner, P., Oda, T., and
Gurney, K. R.: A road map for improving the treatment of uncertainties in
high-resolution regional carbon flux inverse estimates, Geophys. Res. Lett., 46, 13461–13469, 2019a.
Feng, S., Lauvaux, T., Davis, K. J., Keller, K., Zhou, Y., Williams, C.,
Schuh, A. E., Liu, J., and Baker, I.: Seasonal characteristics of model
uncertainties from biogenic fluxes, transport, and large-scale boundary
inflow in atmospheric CO2 simulations over North America, J. Geophys. Res.-Atmos., 124, 14325–14346, 2019b.
Fernald, F. G.: Analysis of atmospheric lidar observations: some comments, Appl. Optics, 23, 652–653, 1984.
Fitzpatrick, F., Hansell, J., Shuman, T., and Young, J.: Laser transmitter development for a methane DIAL system, in: Novel Optical Systems, Methods, and Applications XXII, SPIE, Vol. 11105, p. 111050U, https://doi.org/10.1117/12.2532032, 2019.
Fix, A., Quatrevalet, M., Amediek, A., and Wirth, M.: Energy calibration of
integrated path differential absorption lidars, Appl. Optics, 57, 7501–7514, 2018.
Fix, A., Amediek, A., Ehret, G., Quatrevalet, M., Wirth, M., Galkowski, M., and Gerbig, C.: On the prospects of using the cloud slicing technique in
integrated path differential absorption lidars, in: 16th
International Workshop on Greenhouse Gas Measurements from Space, 2–5 June 2020,
https://cdn.eventsforce.net/files/ef-xnn67yq56ylu/website/9/3_701__andreas_fix_-_short_on_the_prospects_of_using_the_cloud_slicing_technique_in_integrated_path_differential_absorption_lidars.pdf, last access: 30 March 2022), 2020.
Frankenberg, C., Aben, Bergamaschi, P., Dlugokencky, E. J., Van
Hees, R., Houweling, S., Van Der Meer, P., Snel, R., and Tol, P.: Global
column-averaged methane mixing ratios from 2003 to 2009 as derived from
SCIAMACHY: Trends and variability, J. Geophys. Res., 116, D04302, https://doi.org/10.1029/2010JD014849, 2011.
Gelaro, R., McCarty, W., Suárez, M. J., Todling, R., Molod, A., Takacs,
L., Randles, C. A., Darmenov, A., Bosilovich, M. G., Reichle, R., and Wargan,
K.: The modern-era retrospective analysis for research and applications,
version 2 (MERRA-2), J. Climate, 30, 5419–5454, 2017.
Gibert, F., Flamant, P. H., Bruneau, D., and Loth, C.: Two-micrometer
heterodyne differential absorption lidar measurements of the atmospheric CO2 mixing ratio in the boundary layer, Appl. Optics, 45, 4448–4458, 2006.
Gibert, F., Flamant, P. H., Cuesta, J., and Bruneau, D: Vertical 2-µm heterodyne differential absorption lidar measurements of mean CO2 mixing ratio in the troposphere, J. Atmos. Ocean. Tech., 25, 1477–1497, 2008.
Gordon, I. E., Rothman, L. S., Hill, C., Kochanov, R. V., Tan, Y., Bernath,
P. F., Birk, M., Boudon, V., Campargue, A., Chance, K. V., and Drouin, B. J.:
The HITRAN2016 molecular spectroscopic database, J. Quant. Spectrosc. Ra., 203, 3–69, 2017.
Grant, W. B.: Effect of differential spectral reflectance on DIAL
measurements using topographic targets, Appl. Optics, 21, 2390–2394, 1982.
Hair, J. W., Hostetler, C. A., Cook, A. L., Harper, D. B., Ferrare, R. A., Mack, T. L., Welch, W., Izquierdo, L. R., and Hovis, F. E.: Airborne high spectral resolution lidar for profiling aerosol optical properties, Appl. Optics, 47, 6734–6752, 2008.
Hastings, D. A. and Dunbar, P.: Development & assessment of the global
land one-km base elevation digital elevation model (GLOBE), Group, 4, 218–221, 1998.
Heimburger, A. M., Harvey, R. M., Shepson, P. B., Stirm, B. H., Gore, C.,
Turnbull, J., Cambaliza, M. O., Salmon, O. E., Kerlo, A. E. M., Lavoie, T. N., and Davis, K. J.: Assessing the optimized precision of the aircraft mass balance method for measurement of urban greenhouse gas emission rates through
averaging, Elementa: Science of the Anthropocene, 5, 26, https://doi.org/10.1525/elementa.134, 2017.
Hu, H., Landgraf, J., Detmers, R., Borsdorff, T., Aan de Brugh, J., Aben,
I., Butz, A., and Hasekamp, O.: Toward global mapping of methane with
TROPOMI: First results and intersatellite comparison to GOSAT, Geophys. Res. Lett., 45, 3682–3689, 2018.
Ismail, S. and Browell, E. V.: Airborne and spaceborne lidar measurements of
water vapor profiles: a sensitivity analysis, Appl. Optics, 28, 3603–3615, 1989.
Jacob, D. J., Turner, A. J., Maasakkers, J. D., Sheng, J., Sun, K., Liu, X., Chance, K., Aben, I., McKeever, J., and Frankenberg, C.: Satellite observations of atmospheric methane and their value for quantifying methane emissions, Atmos. Chem. Phys., 16, 14371–14396, https://doi.org/10.5194/acp-16-14371-2016, 2016.
Jervis, D., McKeever, J., Durak, B. O. A., Sloan, J. J., Gains, D., Varon, D. J., Ramier, A., Strupler, M., and Tarrant, E.: The GHGSat-D imaging spectrometer, Atmos. Meas. Tech., 14, 2127–2140, https://doi.org/10.5194/amt-14-2127-2021, 2021.
Judd, L. M., Al-Saadi, J. A., Szykman, J. J., Valin, L. C., Janz, S. J., Kowalewski, M. G., Eskes, H. J., Veefkind, J. P., Cede, A., Mueller, M., Gebetsberger, M., Swap, R., Pierce, R. B., Nowlan, C. R., Abad, G. G., Nehrir, A., and Williams, D.: Evaluating Sentinel-5P TROPOMI tropospheric NO2 column densities with airborne and Pandora spectrometers near New York City and Long Island Sound, Atmos. Meas. Tech., 13, 6113–6140, https://doi.org/10.5194/amt-13-6113-2020, 2020.
Karion, A., Callahan, W., Stock, M., Prinzivalli, S., Verhulst, K. R., Kim, J., Salameh, P. K., Lopez-Coto, I., and Whetstone, J.: Greenhouse gas observations from the Northeast Corridor tower network, Earth Syst. Sci. Data, 12, 699–717, https://doi.org/10.5194/essd-12-699-2020, 2020.
Kiemle, C., Quatrevalet, M., Ehret, G., Amediek, A., Fix, A., and Wirth, M.: Sensitivity studies for a space-based methane lidar mission, Atmos. Meas. Tech., 4, 2195–2211, https://doi.org/10.5194/amt-4-2195-2011, 2011.
Lin, B., Nehrir, A. R., Harrison, F. W., Browell, E. V., Ismail, S., Obland,
M. D., Campbell, J., Dobler, J., Meadows, B., Fan, T. F., and Kooi, S.:
Atmospheric CO2 column measurements in cloudy conditions using
intensity-modulated continuous-wave lidar at 1.57 micron, Opt. Express, 23, A582–A593, 2015.
Lin, J. C., Bares, R., Fasoli, B., Garcia, M., Crosman, E., and Lyman, S.:
Declining methane emissions and steady, high leakage rates observed over
multiple years in a western US oil/gas production basin, Scientific Reports, 11, 1–12, 2021.
Lopez-Coto, I., Ren, X., Salmon, O. E., Karion, A., Shepson, P. B., Dickerson, R. R., Stein, A., Prasad, K., and Whetstone, J. R.: Wintertime CO2, CH4, and CO emissions estimation for the Washington, DC–Baltimore metropolitan area using an inverse modeling technique, Environ. Sci. Technol., 54, 2606–2614, 2020.
Lu, X., Jacob, D. J., Wang, H., Maasakkers, J. D., Zhang, Y., Scarpelli, T. R., Shen, L., Qu, Z., Sulprizio, M. P., Nesser, H., Bloom, A. A., Ma, S., Worden, J. R., Fan, S., Parker, R. J., Boesch, H., Gautam, R., Gordon, D., Moran, M. D., Reuland, F., Villasana, C. A. O., and Andrews, A.: Methane emissions in the United States, Canada, and Mexico: evaluation of national methane emission inventories and 2010–2017 sectoral trends by inverse analysis of in situ (GLOBALVIEWplus CH4 ObsPack) and satellite (GOSAT) atmospheric observations, Atmos. Chem. Phys., 22, 395–418, https://doi.org/10.5194/acp-22-395-2022, 2022.
Lyon, D. R., Hmiel, B., Gautam, R., Omara, M., Roberts, K. A., Barkley, Z. R., Davis, K. J., Miles, N. L., Monteiro, V. C., Richardson, S. J., Conley, S., Smith, M. L., Jacob, D. J., Shen, L., Varon, D. J., Deng, A., Rudelis, X., Sharma, N., Story, K. T., Brandt, A. R., Kang, M., Kort, E. A., Marchese, A. J., and Hamburg, S. P.: Concurrent variation in oil and gas methane emissions and oil price during the COVID-19 pandemic, Atmos. Chem. Phys., 21, 6605–6626, https://doi.org/10.5194/acp-21-6605-2021, 2021.
Maasakkers, J. D., Jacob, D. J., Sulprizio, M. P., Turner, A. J., Weitz, M.,
Wirth, T., Hight, C., DeFigueiredo, M., Desai, M., Schmeltz, R., and
Hockstad, L.: Gridded national inventory of US methane emissions, Environ. Sci. Technol., 50, 13123–13133, 2016.
McKain, K., Down, A., Raciti, S. M., Budney, J., Hutyra, L. R., Floerchinger,
C., Herndon, S. C., Nehrkorn, T., Zahniser, M. S., Jackson, R. B., and Phillips, N.: Methane emissions from natural gas infrastructure and use in the urban region of Boston, Massachusetts, P. Natl. Acad. Sci. USA, 112, 1941–1946, 2015.
Menzies, R. T. and Tratt, D. M.: Differential laser absorption spectrometry
for global profiling of tropospheric carbon dioxide: selection of optimum
sounding frequencies for high-precision measurements, Appl. Optics, 42, 6569–6577, 2003.
Myhre, G., D. Shindell, F.-M. Bréon, W. Collins, J. Fuglestvedt, J.
Huang, D. Koch, J.-F. Lamarque, D. Lee, B. Mendoza, T. Nakajima, A. Robock,
G. Stephens, T. Takemura and H. Zhang, 2013: Anthropogenic and Natural
Radiative Forcing, in: Climate Change 2013: The Physical Science Basis.
Contribution of Working Group I to the Fifth Assessment Report of the
Intergovernmental Panel on Climate Change, edited by: Stocker, T. F., Qin, D., Plattner, G.-K., Tignor, M., Allen, S. K., Boschung, J., Nauels, A., Xia, Y., Bex, V., and Midgley, P. M., Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, https://doi.org/10.1017/CBO9781107415324.008, 2013.
NASEM (National Academies of Sciences, Engineering, and Medicine): Thriving on Our Changing Planet: A Decadal Strategy for Earth Observation from Space, The National Academies Press, Washington, DC, https://doi.org/10.17226/24938, 2018.
Nehrir, A. R., Repasky, K. S., Carlsten, J. L., Obland, M. D., and Shaw, J. A.: Water vapor profiling using a widely tunable, amplified diode-laser-based
differential absorption lidar (DIAL), J. Atmos. Ocean. Tech., 26, 733–745, 2009.
Nehrir, A. R., Kiemle, C., Lebsock, M. D., Kirchengast, G., Buehler, S. A.,
Löhnert, U., Liu, C. L., Hargrave, P. C., Barrera-Verdejo, M., and Winker, D. M.: Emerging technologies and synergies for airborne and space-based measurements of water vapor profiles, Surv. Geophys., 38, 1445–1482, 2017.
Nehrir, A., Notari, A., Harper, D., Fitzpatrick, F., Collins, J., Kooi, S.,
Antill, C., Hare, R., Barton-Grimley, R. A., Hair, J., Ferrare, R.,
Hostetler, C., and Welch, W.: The High Altitude Lidar Observatory (HALO): A
multi-function lidar and technology test-bed for airborne and space-based
measurements of water vapor and methane, NASA Earth Science Technology Office, http://www.estotechnology.us/techportfolio/pdf/additionalInfo/1914_Nehrir/Nehrir_ESTF2018_A1P2.pdf (last access: 13 July 2022), 2018.
Nisbet, E. G., Dlugokencky, E. J., and Bousquet, P.: Methane on the rise – again, Science, 343, 493–495, 2014.
Nisbet, E. G., Dlugokencky, E. J., Manning, M. R., Lowry, D., Fisher, R. E.,
France, J. L., Michel, S. E., Miller, J. B., White, J. W. C., Vaughn, B., and
Bousquet, P.: Rising atmospheric methane: 2007–2014 growth and isotopic
shift, Global Biogeochem. Cy., 30, 1356–1370, 2016.
Pal, S. and Davis, K. J.: ACT-America Campaign Catalog, ORNL DAAC, Oak Ridge, Tennessee, USA [data set], https://doi.org/10.3334/ORNLDAAC/1862, 2021.
Plant, G., Kort, E. A., Floerchinger, C., Gvakharia, A., Vimont, I., and
Sweeney, C.: Large fugitive methane emissions from urban centers along the
U.S. East Coast, Geophys. Res. Lett., 46, 8500–8507, https://doi.org/10.1029/2019GL082635, 2019.
Ramanathan, A. K., Mao, J., Abshire, J. B., and Allan, G. R.: Remote sensing
measurements of the CO2 mixing ratio in the planetary boundary layer using
cloud slicing with airborne lidar, Geophys. Res. Lett., 42, 2055–2062, 2015.
Refaat, T. F., Ismail, S., Nehrir, A. R., Hair, J. W., Crawford, J. H., Leifer, I., and Shuman, T.: Performance evaluation of a 1.6-µm methane DIAL system from ground, aircraft and UAV platforms, Opt. Express, 21, 30415–30432, 2013.
Refaat, T. F., Petros, M., Singh, U. N., Antill, C. W., and Remus, R. G.:
High-Precision and High-Accuracy Column Dry-Air Mixing Ratio Measurement of
Carbon Dioxide Using Pulsed 2-µm IPDA Lidar, IEEE T. Geosci. Remote, 58, 5804–5819, 2020.
Richardson, S. J., Miles, N. L., Davis, K. J., Lauvaux, T., and Martins, D.:
Tower measurement network of in situ CO2, CO, and CH4 surface in situ measurement network in support of the Indianapolis FLUX (INFLUX) Experiment, Elementa: Science of the Anthropocene, 5, 59, https://doi.org/10.1525/elementa.140, 2017.
Riris, H., Numata, K., Li, S., Wu, S., Ramanathan, A., Dawsey, M., Mao, J.,
Kawa, R., and Abshire, J. B.: Airborne measurements of atmospheric methane
column abundance using a pulsed integrated-path differential absorption
lidar, Appl. Optics, 51, 8296–8305, 2012.
Riris, H., Numata, K., Wu, S., Gonzalez, B., Rodriguez, M., Scott, S., Kawa, S., and Mao, J.: Methane optical density measurements with an integrated path
differential absorption lidar from an airborne platform, J. Appl. Remote Sens., 11, 034001, https://doi.org/10.1117/1.JRS.11.034001, 2017.
Scarino, A. J., Obland, M. D., Fast, J. D., Burton, S. P., Ferrare, R. A., Hostetler, C. A., Berg, L. K., Lefer, B., Haman, C., Hair, J. W., Rogers, R. R., Butler, C., Cook, A. L., and Harper, D. B.: Comparison of mixed layer heights from airborne high spectral resolution lidar, ground-based measurements, and the WRF-Chem model during CalNex and CARES, Atmos. Chem. Phys., 14, 5547–5560, https://doi.org/10.5194/acp-14-5547-2014, 2014.
Schaefer, H., Fletcher, S. E. M., Veidt, C., Lassey, K. R., Brailsford, G. W., Bromley, T. M., Dlugokencky, E. J., Michel, S. E., Miller, J. B., Levin, I., and Lowe, D. C.: A 21st-century shift from fossil-fuel to biogenic methane emissions indicated by 13CH4, Science, 352, 80–84, 2016.
Schotland, R. M.: The Determination of the Vertical Profile of Atmospheric
Gases by Means of a Ground Based Optical Radar, in: Proceeding of the Third
Symposium on Remote Sensing of Environment, University of Michigan, Ann Arbor, October, 1964.
Schotland, R. M.: Errors in the lidar measurement of atmospheric gases by
differential absorption, J. Appl. Meteorol., 13, 71–77, 1974.
Schuldt, K. N., Mund, J., Luijkx, I. T., et al.: Multi-laboratory compilation of atmospheric carbon dioxide data for the period 1957–2020;
obspack_co2_1_GLOBALVIEWplus_v7.0_2021-08-18, NOAA Global Monitoring Laboratory [data set], https://doi.org/10.25925/20210801, 2021.
Sun, X., Abshire, J. B., Beck, J. D., Mitra, P., Reiff, K., and Yang, G.:
HgCdTe avalanche photodiode detectors for airborne and spaceborne lidar at
infrared wavelengths, Opt. Express, 25, 16589–16602, 2017.
Tellier, Y., Pierangelo, C., Wirth, M., Gibert, F., and Marnas, F.: Averaging bias correction for the future space-borne methane IPDA lidar mission MERLIN, Atmos. Meas. Tech., 11, 5865–5884, https://doi.org/10.5194/amt-11-5865-2018, 2018.
Varon, D. J., Jacob, D. J., Jervis, D., and McKeever, J.: Quantifying
time-averaged methane emissions from individual coal mine vents with
GHGSat-D satellite observations, Environ. Sci. Technol., 54, 10246–10253, 2020.
Vasilchenko, S., Tran, H., Mondelain, D., Kassi, S., and Campargue, A.:
Accurate absorption spectroscopy of water vapor near 1.64 µm in
support of the MEthane Remote LIdar missioN (MERLIN), J. Quant. Spectrosc. Ra., 235, 332–342, 2019.
Veefkind, J. P., Aben, I., McMullan, K., Förster, H., De Vries, J.,
Otter, G., Claas, J., Eskes, H. J., De Haan, J. F., Kleipool, Q., and Van
Weele, M.: TROPOMI on the ESA Sentinel-5 Precursor: A GMES mission for
global observations of the atmospheric composition for climate, air quality
and ozone layer applications, Remote Sens. Environ., 120, 70–83, 2012.
Verhulst, K. R., Karion, A., Kim, J., Salameh, P. K., Keeling, R. F., Newman, S., Miller, J., Sloop, C., Pongetti, T., Rao, P., Wong, C., Hopkins, F. M., Yadav, V., Weiss, R. F., Duren, R. M., and Miller, C. E.: Carbon dioxide and methane measurements from the Los Angeles Megacity Carbon Project – Part 1: calibration, urban enhancements, and uncertainty estimates, Atmos. Chem. Phys., 17, 8313–8341, https://doi.org/10.5194/acp-17-8313-2017, 2017.
Wecht, K. J., Jacob, D. J., Frankenberg, C., Jiang, Z., and Blake, D. R.:
Mapping of North American methane emissions with high spatial resolution by
inversion of SCIAMACHY satellite data, J. Geophys. Res.-Atmos., 119, 7741–7756, 2014a.
Wecht, K. J., Jacob, D. J., Sulprizio, M. P., Santoni, G. W., Wofsy, S. C., Parker, R., Bösch, H., and Worden, J.: Spatially resolving methane emissions in California: constraints from the CalNex aircraft campaign and from present (GOSAT, TES) and future (TROPOMI, geostationary) satellite observations, Atmos. Chem. Phys., 14, 8173–8184, https://doi.org/10.5194/acp-14-8173-2014, 2014b.
Wei, Y., Shrestha, R., Pal, S., Gerken, T., Feng, S., McNelis, J., Singh,
D., Thornton, M. M., Boyer, A. G., Shook, M. A., and Chen, G.: Atmospheric
Carbon and Transport – America (ACT-America) data sets: Description,
management, and delivery, Earth Space Sci., 8, e2020EA001634, https://doi.org/10.1029/2020EA001634, 2021.
Yang, M. M., Barrick, J. D., Sweeney, C., DiGangi, J. P., and Bennett, J. R.: ACT-America: L1 Meteorological and Aircraft Navigational Data, ORNL DAAC [data set], Oak Ridge, Tennessee, USA, https://doi.org/10.3334/ORNLDAAC/1574, 2018.
Yokota, T., Yoshida, Y., Eguchi, N., Ota, Y., Tanaka, T., Watanabe, H., and
Maksyutov, S.: Global concentrations of CO2 and CH4 retrieved from GOSAT: First preliminary results, Sola, 5, 160–163, 2009.
Yu, X., Millet, D. B., Wells, K. C., Henze, D. K., Cao, H., Griffis, T. J., Kort, E. A., Plant, G., Deventer, M. J., Kolka, R. K., Roman, D. T., Davis, K. J., Desai, A. R., Baier, B. C., McKain, K., Czarnetzki, A. C., and Bloom, A. A.: Aircraft-based inversions quantify the importance of wetlands and livestock for Upper Midwest methane emissions, Atmos. Chem. Phys., 21, 951–971, https://doi.org/10.5194/acp-21-951-2021, 2021.
Zhang, Y., Gautam, R., Pandey, S., Omara, M., Maasakkers, J. D., Sadavarte,
P., Lyon, D., Nesser, H., Sulprizio, M. P., Varon, D. J., and Zhang, R.: Quantifying methane emissions from the largest oil-producing basin in the
United States from space, Sci. Adv., 6, eaaz5120, https://doi.org/10.1126/sciadv.aaz5120, 2020.
Zhang, Y., Jacob, D. J., Lu, X., Maasakkers, J. D., Scarpelli, T. R., Sheng, J.-X., Shen, L., Qu, Z., Sulprizio, M. P., Chang, J., Bloom, A. A., Ma, S., Worden, J., Parker, R. J., and Boesch, H.: Attribution of the accelerating increase in atmospheric methane during 2010–2018 by inverse analysis of GOSAT observations, Atmos. Chem. Phys., 21, 3643–3666, https://doi.org/10.5194/acp-21-3643-2021, 2021.
Short summary
HALO is a multi-functional lidar that measures CH4 columns and profiles of H2O mixing ratio and aerosol/cloud optical properties. HALO supports carbon cycle, weather dynamics, and radiation science suborbital research and is a technology testbed for future space-based differential absorption lidar missions. In 2019 HALO collected CH4 columns and aerosol/cloud profiles during the ACT-America campaign. Here we assess HALO's CH4 accuracy and precision compared to co-located in situ observations.
HALO is a multi-functional lidar that measures CH4 columns and profiles of H2O mixing ratio and...
