Articles | Volume 10, issue 3
https://doi.org/10.5194/amt-10-1017-2017
https://doi.org/10.5194/amt-10-1017-2017
Research article
 | 
15 Mar 2017
Research article |  | 15 Mar 2017

A new Differential Optical Absorption Spectroscopy instrument to study atmospheric chemistry from a high-altitude unmanned aircraft

Jochen Stutz, Bodo Werner, Max Spolaor, Lisa Scalone, James Festa, Catalina Tsai, Ross Cheung, Santo F. Colosimo, Ugo Tricoli, Rasmus Raecke, Ryan Hossaini, Martyn P. Chipperfield, Wuhu Feng, Ru-Shan Gao, Eric J. Hintsa, James W. Elkins, Fred L. Moore, Bruce Daube, Jasna Pittman, Steven Wofsy, and Klaus Pfeilsticker

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Cited articles

Aliwell, S., Van Roozendael, M., Johnston, P., Richter, A., Wagner, T., Arlander, D., Burrows, J., Fish, D., Jones, R., Tørnkvist, K., Lambert, J.-C., Pfeilsticker, K., and Pundt, I.: Analysis for BrO in zenith-sky spectra: An intercomparison exercise for analysis improvement, J. Geophys. Res., 107, 1–20, https://doi.org/10.1029/2001JD000329, 2002.
Baidar, S., Oetjen, H., Coburn, S., Dix, B., Ortega, I., Sinreich, R., and Volkamer, R.: The CU Airborne MAX-DOAS instrument: vertical profiling of aerosol extinction and trace gases, Atmos. Meas. Tech., 6, 719–739, https://doi.org/10.5194/amt-6-719-2013, 2013.
Bauer, R., Rozanov, A., McLinden, C. A., Gordley, L. L., Lotz, W., Russell III, J. M., Walker, K. A., Zawodny, J. M., Ladstätter-Weißenmayer, A., Bovensmann, H., and Burrows, J. P.: Validation of SCIAMACHY limb NO2 profiles using solar occultation measurements, Atmos. Meas. Tech., 5, 1059–1084, https://doi.org/10.5194/amt-5-1059-2012, 2012.
Bogumil, K., Orphal, J., Homann, T., Voigt, S., Spietz, P., Fleischmann, O., Vogel, A., Hartmann, M., Kromminga, H., Bovensmann, H., Frerick, J., and Burrows, J.: Measurements of molecular absorption spectra with the SCIAMACHY pre-flight model: Instrument characterization and reference data for atmospheric remote-sensing in the 230–2380 nm region, J. Photochem. Photobio. A, 157, 167–184, https://doi.org/10.1016/S1010-6030(03)00062-5, 2003.
Brune, W. H., Toohey, D. W., Anderson, J. G., Starr, W. L., Vedder, J. F., and Danielsen, E. F.: In situ northern mid-latitude observations of ClO, O3, and BrO in the wintertime lower stratosphere, Science, 242, 558–562, 1988.
Short summary
A new limb-scanning Differential Optical Absorption Spectroscopy (DOAS) instrument was developed for NASA’s Global Hawk unmanned aerial system during the Airborne Tropical TRopopause EXperiment to study trace gases in the tropical tropopause layer. A new technique that uses in situ and DOAS O3 observations together with radiative transfer calculations allows the retrieval of mixing ratios from the slant column densities of BrO and NO2 at high accuracies of 0.5 ppt and 15 ppt, respectively.