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AMT | Articles | Volume 13, issue 5
Atmos. Meas. Tech., 13, 2397–2411, 2020
https://doi.org/10.5194/amt-13-2397-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
Atmos. Meas. Tech., 13, 2397–2411, 2020
https://doi.org/10.5194/amt-13-2397-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.

Research article 15 May 2020

Research article | 15 May 2020

Nitrate radical generation via continuous generation of dinitrogen pentoxide in a laminar flow reactor coupled to an oxidation flow reactor

Andrew T. Lambe et al.

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Cited articles

Asaf, D., Tas, E., Pedersen, D., Peleg, M., and Luria, M.: Long-Term Measurements of NO3 Radical at a Semiarid Urban Site: 2. Seasonal Trends and Loss Mechanisms, Environ. Sci. Technol., 44, 5901–5907, https://doi.org/10.1021/es100967z, 2010. a, b, c
Atkinson, R.: Kinetics and Mechanisms of the Gas-Phase Reactions of the NO3 Radical with Organic Compounds, J. Phys. Chem. Ref. Data, 20, 459–507, https://doi.org/10.1063/1.555887, 1991. a, b
Atkinson, R., Arey, J., Zielinska, B., and Aschmann, S. M.: Kinetics and nitro-products of the gas-phase OH and NO3 radical-initiated reactions of naphthalene-d8, fluoranthene-d10, and pyrene, Int. J. Chem., 22, 999–1014, https://doi.org/10.1002/kin.550220910, 1990. a
Atkinson, R., Tuazon, E. C., Bridier, I., and Arey, J.: Reactions of NO3-naphthalene adducts with O2 and NO2, Int. J. Chem. Kinet., 26, 605–614, https://doi.org/10.1002/kin.550260603, 1994. a
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We present a new method to continuously generate N2O5 in the gas phase that is injected into a reactor where it decomposes to generate nitrate radicals (NO3). To assess the applicability of the method towards different chemical systems, we present experimental and model characterization of the integrated NO3 exposure and other metrics as a function of operating conditions. We demonstrate the method by characterizing secondary organic aerosol particles generated from the β-pinene + NO3 reaction.
We present a new method to continuously generate N2O5 in the gas phase that is injected into a...
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