Articles | Volume 10, issue 1
https://doi.org/10.5194/amt-10-167-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/amt-10-167-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Altitude registration of limb-scattered radiation
Leslie Moy
CORRESPONDING AUTHOR
Science Systems and Applications, Inc. (SSAI), 10210 Greenbelt Road, Suite 600, Lanham, Maryland 20706, USA
Pawan K. Bhartia
NASA Goddard Space Flight Center, Greenbelt, Maryland, USA
Glen Jaross
NASA Goddard Space Flight Center, Greenbelt, Maryland, USA
Robert Loughman
Hampton University, Hampton, Virginia, USA
Natalya Kramarova
Science Systems and Applications, Inc. (SSAI), 10210 Greenbelt Road, Suite 600, Lanham, Maryland 20706, USA
Zhong Chen
Science Systems and Applications, Inc. (SSAI), 10210 Greenbelt Road, Suite 600, Lanham, Maryland 20706, USA
Ghassan Taha
GESTAR, Columbia, Maryland, USA
Grace Chen
Science Systems and Applications, Inc. (SSAI), 10210 Greenbelt Road, Suite 600, Lanham, Maryland 20706, USA
Philippe Xu
Science Applications International Corporation (SAIC), Lanham, Maryland, USA
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Atmos. Meas. Tech., 11, 2837–2861, https://doi.org/10.5194/amt-11-2837-2018, https://doi.org/10.5194/amt-11-2837-2018, 2018
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The Ozone Mapping and Profiler Suite (OMPS) Limb Profiler (LP) is a newly designed research sensor aiming to continue high vertical resolution ozone records from space-borne sensors. In summer 2017 all LP measurements were processed with the new version 2.5 algorithm. In this paper we provide a description of the key changes implemented in the new algorithm and evaluate the quality of ozone retrievals by comparing with independent satellite profile measurements (MLS, ACE-FTS and OSIRIS).
Selena Zhang, Susan Solomon, Chris D. Boone, and Ghassan Taha
Atmos. Chem. Phys., 24, 11727–11736, https://doi.org/10.5194/acp-24-11727-2024, https://doi.org/10.5194/acp-24-11727-2024, 2024
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This paper investigates the vertical impacts of the anomalous 2023 Canadian wildfire season using multiple satellite instruments. Our results highlight that despite a record-breaking area burned, only a small amount of smoke managed to enter the stratosphere. This shows that the conditions for deep convection were rarely met in the 2023 wildfire season, suggesting that even a massive area burned is not necessarily an indicator of stratospheric perturbations.
Michael D. Himes, Ghassan Taha, Daniel Kahn, Tong Zhu, and Natalya A. Kramarova
EGUsphere, https://doi.org/10.5194/egusphere-2024-1823, https://doi.org/10.5194/egusphere-2024-1823, 2024
This preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).
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The Ozone Mapping and Profiler Suite's Limb Profiler (OMPS LP) provides near-global coverage and information about how aerosols from volcanic eruptions and major wildfires are vertically distributed through the atmosphere. We developed a machine learning method to characterize aerosols using OMPS LP measurements about 60 times faster than the current approach. This near-real-time characterization can be used to ensure aviation flight paths avoid dangerous conditions.
Heesung Chong, Gonzalo González Abad, Caroline R. Nowlan, Christopher Chan Miller, Alfonso Saiz-Lopez, Rafael P. Fernandez, Hyeong-Ahn Kwon, Zolal Ayazpour, Huiqun Wang, Amir H. Souri, Xiong Liu, Kelly Chance, Ewan O'Sullivan, Jhoon Kim, Ja-Ho Koo, William R. Simpson, François Hendrick, Richard Querel, Glen Jaross, Colin Seftor, and Raid M. Suleiman
Atmos. Meas. Tech., 17, 2873–2916, https://doi.org/10.5194/amt-17-2873-2024, https://doi.org/10.5194/amt-17-2873-2024, 2024
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We present a new bromine monoxide (BrO) product derived using radiances measured from OMPS-NM on board the Suomi-NPP satellite. This product provides nearly a decade of global stratospheric and tropospheric column retrievals, a feature that is currently rare in publicly accessible datasets. Both stratospheric and tropospheric columns from OMPS-NM demonstrate robust performance, exhibiting good agreement with ground-based observations collected at three stations (Lauder, Utqiagvik, and Harestua).
Yi Wang, Mark Schoeberl, and Ghassan Taha
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-267, https://doi.org/10.5194/amt-2023-267, 2024
Revised manuscript not accepted
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The OMPS-LP satellite instrument assesses aerosol scattering in the atmospheric limb. Using a dual-wavelength extinction coefficient algorithm, we extract stratospheric aerosol vertical profiles from OMPS-LP data. Our study addresses uncertainties and validates these profiles against in-situ balloon data and SAGE-III/ISS retrievals. Investigating the Raikoke and Hunga Tonga-Hunga Ha'apai eruptions, we analyze the evolution of aerosol size and concentration, confirming our method's reliability.
Yi Wang, Mark Schoeberl, Ghassan Taha, Daniel Zawada, and Adam Bourassa
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-36, https://doi.org/10.5194/amt-2023-36, 2023
Revised manuscript not accepted
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The OMPS-LP satellite instrument measures aerosol scattering properties across the atmospheric limb. Adopting an algorithm that uses extinction at two wavelengths, we retrieve vertical profiles of particle size and concentration. We demonstrate that these profiles are consistent with in-situ balloon and SAGE-III/ISS satellite measurements. We also show how aerosol size and concentration evolve during Reikoke and Hunga Tonga-Hunga Ha'apai eruptions.
Sarah A. Strode, Ghassan Taha, Luke D. Oman, Robert Damadeo, David Flittner, Mark Schoeberl, Christopher E. Sioris, and Ryan Stauffer
Atmos. Meas. Tech., 15, 6145–6161, https://doi.org/10.5194/amt-15-6145-2022, https://doi.org/10.5194/amt-15-6145-2022, 2022
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We use a global atmospheric chemistry model simulation to generate scaling factors that account for the daily cycle of NO2 and ozone. These factors facilitate comparisons between sunrise and sunset observations from SAGE III/ISS and observations from other instruments. We provide the scaling factors as monthly zonal means for different latitudes and altitudes. We find that applying these factors yields more consistent comparisons between observations from SAGE III/ISS and other instruments.
Quintus Kleipool, Nico Rozemeijer, Mirna van Hoek, Jonatan Leloux, Erwin Loots, Antje Ludewig, Emiel van der Plas, Daley Adrichem, Raoul Harel, Simon Spronk, Mark ter Linden, Glen Jaross, David Haffner, Pepijn Veefkind, and Pieternel F. Levelt
Atmos. Meas. Tech., 15, 3527–3553, https://doi.org/10.5194/amt-15-3527-2022, https://doi.org/10.5194/amt-15-3527-2022, 2022
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A new collection-4 dataset for the Ozone Monitoring Instrument (OMI) mission has been established to supersede the current collection-3 level-1b (L1b) data, produced with a newly developed L01b data processor based on the TROPOspheric Monitoring Instrument (TROPOMI) L01b processor. The collection-4 L1b data have a similar output format to the TROPOMI L1b data for easy connection of the data series. Many insights from the TROPOMI algorithms, as well as from OMI collection-3 usage, were included.
Nick Gorkavyi, Nickolay Krotkov, Can Li, Leslie Lait, Peter Colarco, Simon Carn, Matthew DeLand, Paul Newman, Mark Schoeberl, Ghassan Taha, Omar Torres, Alexander Vasilkov, and Joanna Joiner
Atmos. Meas. Tech., 14, 7545–7563, https://doi.org/10.5194/amt-14-7545-2021, https://doi.org/10.5194/amt-14-7545-2021, 2021
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The 21 June 2019 eruption of the Raikoke volcano produced significant amounts of volcanic aerosols (sulfate and ash) and sulfur dioxide (SO2) gas that penetrated into the lower stratosphere. We showed that the amount of SO2 decreases with a characteristic period of 8–18 d and the peak of sulfate aerosol lags the initial peak of SO2 by 1.5 months. We also examined the dynamics of an unusual stratospheric coherent circular cloud of SO2 and aerosol observed from 18 July to 22 September 2019.
Jerald R. Ziemke, Gordon J. Labow, Natalya A. Kramarova, Richard D. McPeters, Pawan K. Bhartia, Luke D. Oman, Stacey M. Frith, and David P. Haffner
Atmos. Meas. Tech., 14, 6407–6418, https://doi.org/10.5194/amt-14-6407-2021, https://doi.org/10.5194/amt-14-6407-2021, 2021
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Seasonal and interannual ozone profile climatologies are produced from combined MLS and MERRA-2 GMI ozone for the general public. Both climatologies extend from pole to pole at altitudes of 0–80 km (1 km spacing) for the time record from 1970 to 2018. These climatologies are important for use as a priori information in satellite ozone retrieval algorithms, as validation of other measured and model-simulated ozone, and in radiative transfer studies of the atmosphere.
Sampa Das, Peter R. Colarco, Luke D. Oman, Ghassan Taha, and Omar Torres
Atmos. Chem. Phys., 21, 12069–12090, https://doi.org/10.5194/acp-21-12069-2021, https://doi.org/10.5194/acp-21-12069-2021, 2021
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Interactions of extreme fires with weather systems can produce towering smoke plumes that inject aerosols at very high altitudes (> 10 km). Three such major injections, largest at the time in terms of emitted aerosol mass, took place over British Columbia, Canada, in August 2017. We model the transport and impacts of injected aerosols on the radiation balance of the atmosphere. Our model results match the satellite-observed plume transport and residence time at these high altitudes very closely.
Daniel Zawada, Ghislain Franssens, Robert Loughman, Antti Mikkonen, Alexei Rozanov, Claudia Emde, Adam Bourassa, Seth Dueck, Hannakaisa Lindqvist, Didier Ramon, Vladimir Rozanov, Emmanuel Dekemper, Erkki Kyrölä, John P. Burrows, Didier Fussen, and Doug Degenstein
Atmos. Meas. Tech., 14, 3953–3972, https://doi.org/10.5194/amt-14-3953-2021, https://doi.org/10.5194/amt-14-3953-2021, 2021
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Satellite measurements of atmospheric composition often rely on computer tools known as radiative transfer models to model the propagation of sunlight within the atmosphere. Here we have performed a detailed inter-comparison of seven different radiative transfer models in a variety of conditions. We have found that the models agree remarkably well, at a level better than previously reported. This result provides confidence in our understanding of atmospheric radiative transfer.
Ghassan Taha, Robert Loughman, Tong Zhu, Larry Thomason, Jayanta Kar, Landon Rieger, and Adam Bourassa
Atmos. Meas. Tech., 14, 1015–1036, https://doi.org/10.5194/amt-14-1015-2021, https://doi.org/10.5194/amt-14-1015-2021, 2021
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This work describes the newly released OMPS LP aerosol extinction profile multi-wavelength Version 2.0 algorithm and dataset. It is shown that the V2.0 aerosols exhibit significant improvements in OMPS LP retrieval performance in the Southern Hemisphere and at lower altitudes. The new product is compared to the SAGE III/ISS, OSIRIS and CALIPSO missions and shown to be of good quality and suitable for scientific studies.
Corinna Kloss, Gwenaël Berthet, Pasquale Sellitto, Felix Ploeger, Ghassan Taha, Mariam Tidiga, Maxim Eremenko, Adriana Bossolasco, Fabrice Jégou, Jean-Baptiste Renard, and Bernard Legras
Atmos. Chem. Phys., 21, 535–560, https://doi.org/10.5194/acp-21-535-2021, https://doi.org/10.5194/acp-21-535-2021, 2021
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The year 2019 was particularly rich for the stratospheric aerosol layer due to two volcanic eruptions (at Raikoke and Ulawun) and wildfire events. With satellite observations and models, we describe the exceptionally complex situation following the Raikoke eruption. The respective plume overwhelmed the Northern Hemisphere stratosphere in terms of aerosol load and resulted in the highest climate impact throughout the past decade.
Omar Torres, Hiren Jethva, Changwoo Ahn, Glen Jaross, and Diego G. Loyola
Atmos. Meas. Tech., 13, 6789–6806, https://doi.org/10.5194/amt-13-6789-2020, https://doi.org/10.5194/amt-13-6789-2020, 2020
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TROPOMI measures the quantity of small suspended particles (aerosols). We describe initial results of aerosol measurements using a NASA algorithm that retrieves the UV aerosol index, aerosol optical depth, and single-scattering albedo. An evaluation of derived products using sun-photometer observations shows close agreement. We also use these results to discuss important biomass burning and wildfire events around the world that got the attention of scientists and news media alike.
Clark J. Weaver, Pawan K. Bhartia, Dong L. Wu, Gordon J. Labow, and David E. Haffner
Atmos. Meas. Tech., 13, 5715–5723, https://doi.org/10.5194/amt-13-5715-2020, https://doi.org/10.5194/amt-13-5715-2020, 2020
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Currently, we do not know whether clouds will accelerate or moderate climate. We look to the past and ask whether cloudiness has changed over the last 4 decades. Using a suite of nine satellite instruments, we need to ensure that the first satellite, which was launched in 1980 and died in 1991, observed the same measurement as the eight other satellite instruments used in the record. If the instruments were measuring length and observing a 1.00 m long stick, they would all see 0.99 to 1.01 m.
Zhong Chen, Pawan K. Bhartia, Omar Torres, Glen Jaross, Robert Loughman, Matthew DeLand, Peter Colarco, Robert Damadeo, and Ghassan Taha
Atmos. Meas. Tech., 13, 3471–3485, https://doi.org/10.5194/amt-13-3471-2020, https://doi.org/10.5194/amt-13-3471-2020, 2020
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The scope of the paper is the evaluation of stratospheric aerosols derived from the OMPS/LP instrument via comparison with independent datasets from the SAGE III/ISS instrument. Results show very good agreement for extinction profiles between an altitude of 19 and 27 km, to within ±25 %, and show systematic differences (LP-SAGE III/ISS) above 28 km and below 19 km (greater than ±25 %).
Stacey M. Frith, Pawan K. Bhartia, Luke D. Oman, Natalya A. Kramarova, Richard D. McPeters, and Gordon J. Labow
Atmos. Meas. Tech., 13, 2733–2749, https://doi.org/10.5194/amt-13-2733-2020, https://doi.org/10.5194/amt-13-2733-2020, 2020
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We use the NASA GEOS-GMI chemistry climate model to construct a climatology of stratospheric ozone diurnal variations as a function of latitude, pressure and month, which can be used in a variety of data analysis tasks involving ozone observations made at different times of the day. The climatology compares well with previous modeling simulations and available observations, and to the authors' knowledge is the first characterization of the diurnal cycle available for general ozone data analyses.
Ernest Nyaku, Robert Loughman, Pawan K. Bhartia, Terry Deshler, Zhong Chen, and Peter R. Colarco
Atmos. Meas. Tech., 13, 1071–1087, https://doi.org/10.5194/amt-13-1071-2020, https://doi.org/10.5194/amt-13-1071-2020, 2020
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This paper shows the importance of the nature of the aerosol phase function used in the retrieval of the stratospheric aerosol extinction from limb scattering measurements. The aerosol phase function is derived from the parameters using either a unimodal lognormal or gamma aerosol size distribution. These two distributions were fitted to the same aerosol concentration measurements at two altitudes, and depending on the nature of the measurements, each distribution shows its strengths.
Corinna Kloss, Gwenaël Berthet, Pasquale Sellitto, Felix Ploeger, Silvia Bucci, Sergey Khaykin, Fabrice Jégou, Ghassan Taha, Larry W. Thomason, Brice Barret, Eric Le Flochmoen, Marc von Hobe, Adriana Bossolasco, Nelson Bègue, and Bernard Legras
Atmos. Chem. Phys., 19, 13547–13567, https://doi.org/10.5194/acp-19-13547-2019, https://doi.org/10.5194/acp-19-13547-2019, 2019
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With satellite measurements and transport models, we show that a plume resulting from strong Canadian fires in July/August 2017 was not only distributed throughout the northern/higher latitudes, but also reached the faraway tropics, aided by the circulation of Asian monsoon anticyclone. The regional climate impact in the wider Asian monsoon area in September exceeds the impact of the Asian tropopause aerosol layer by a factor of ~ 3 and compares to that of an advected moderate volcanic eruption.
Bradford L. Fisher, Nickolay A. Krotkov, Pawan K. Bhartia, Can Li, Simon A. Carn, Eric Hughes, and Peter J. T. Leonard
Atmos. Meas. Tech., 12, 5137–5153, https://doi.org/10.5194/amt-12-5137-2019, https://doi.org/10.5194/amt-12-5137-2019, 2019
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This article describes a new discrete wavelength algorithm, MS_SO2, which has been used operationally to retrieve global daily volcanic SO2 vertical column densities and the UV volcanic ash index from the Total Ozone Mapping Spectrometer (TOMS) data collected by NASA’s Nimbus-7 satellite from 1978 to 1991. We examine the sensitivity of the algorithm to the detection of SO2, evaluate potential sources of error and compare results from MS_SO2 with the Principal Component Analysis (PCA) algorithm.
Jerry R. Ziemke, Luke D. Oman, Sarah A. Strode, Anne R. Douglass, Mark A. Olsen, Richard D. McPeters, Pawan K. Bhartia, Lucien Froidevaux, Gordon J. Labow, Jacquie C. Witte, Anne M. Thompson, David P. Haffner, Natalya A. Kramarova, Stacey M. Frith, Liang-Kang Huang, Glen R. Jaross, Colin J. Seftor, Mathew T. Deland, and Steven L. Taylor
Atmos. Chem. Phys., 19, 3257–3269, https://doi.org/10.5194/acp-19-3257-2019, https://doi.org/10.5194/acp-19-3257-2019, 2019
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Both a 38-year merged satellite record of tropospheric ozone from TOMS/OMI/MLS/OMPS and a MERRA-2 GMI model simulation show large increases of 6–7 Dobson units from the Near East to India–East Asia and eastward over the Pacific. These increases in tropospheric ozone are attributed to increases in pollution over the region over the last several decades. Secondary 38-year increases of 4–5 Dobson units with both GMI model and satellite measurements occur over central African–tropical Atlantic.
Zhong Chen, Pawan K. Bhartia, Robert Loughman, Peter Colarco, and Matthew DeLand
Atmos. Meas. Tech., 11, 6495–6509, https://doi.org/10.5194/amt-11-6495-2018, https://doi.org/10.5194/amt-11-6495-2018, 2018
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We describe the derivation of an improved aerosol size distribution (ASD) for the OMPS/LP retrieval algorithm. The new ASD uses a gamma function distribution that is derived from CARMA-calculated results. The new ASD also explains the spectral dependence of LP-measured radiances well. Initial comparisons with collocated extinction profiles retrieved at 676 nm from the SAGE III/ISS instrument show a significant improvement in agreement for the LP retrievals.
Alexander Vasilkov, Eun-Su Yang, Sergey Marchenko, Wenhan Qin, Lok Lamsal, Joanna Joiner, Nickolay Krotkov, David Haffner, Pawan K. Bhartia, and Robert Spurr
Atmos. Meas. Tech., 11, 4093–4107, https://doi.org/10.5194/amt-11-4093-2018, https://doi.org/10.5194/amt-11-4093-2018, 2018
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We discuss a new cloud algorithm that retrieves effective cloud fraction and cloud altitude and pressure from the oxygen dimer absorption band at 477 nm. The algorithm accounts for how changes in the sun–satellite geometry affect the surface reflection. The cloud fraction and pressure are used as inputs to the OMI algorithm that retrieves a pollutant gas called nitrogen dioxide. Impacts of the application of the newly developed cloud algorithm on the OMI nitrogen dioxide retrieval are discussed.
Natalya A. Kramarova, Pawan K. Bhartia, Glen Jaross, Leslie Moy, Philippe Xu, Zhong Chen, Matthew DeLand, Lucien Froidevaux, Nathaniel Livesey, Douglas Degenstein, Adam Bourassa, Kaley A. Walker, and Patrick Sheese
Atmos. Meas. Tech., 11, 2837–2861, https://doi.org/10.5194/amt-11-2837-2018, https://doi.org/10.5194/amt-11-2837-2018, 2018
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The Ozone Mapping and Profiler Suite (OMPS) Limb Profiler (LP) is a newly designed research sensor aiming to continue high vertical resolution ozone records from space-borne sensors. In summer 2017 all LP measurements were processed with the new version 2.5 algorithm. In this paper we provide a description of the key changes implemented in the new algorithm and evaluate the quality of ozone retrievals by comparing with independent satellite profile measurements (MLS, ACE-FTS and OSIRIS).
Omar Torres, Pawan K. Bhartia, Hiren Jethva, and Changwoo Ahn
Atmos. Meas. Tech., 11, 2701–2715, https://doi.org/10.5194/amt-11-2701-2018, https://doi.org/10.5194/amt-11-2701-2018, 2018
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Since about three years after the launch the Ozone Monitoring Instrument (OMI) on the EOS-Aura satellite, the sensor’s viewing capability has been affected by what is believed to be an internal obstruction that has reduced OMI’s spatial coverage. It currently affects about half of the instrument’s 60 viewing positions. In this work we carry out an analysis to assess the effect of the reduced spatial coverage on the monthly average values of retrieved parameters.
Robert Loughman, Pawan K. Bhartia, Zhong Chen, Philippe Xu, Ernest Nyaku, and Ghassan Taha
Atmos. Meas. Tech., 11, 2633–2651, https://doi.org/10.5194/amt-11-2633-2018, https://doi.org/10.5194/amt-11-2633-2018, 2018
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The Ozone Mapping and Profiler Suite (OMPS) Limb Profiler (LP) Version 1 algorithm retrieves aerosol extinction profiles at 675 nm by iteration, based on comparisons between the measured and calculated radiance profiles (assuming an aerosol size distribution). The most significant error source is uncertainty about the aerosol phase function. Horizontal variations in aerosol extinction may also limit the quality of the retrieved aerosol extinction profiles.
Pieternel F. Levelt, Joanna Joiner, Johanna Tamminen, J. Pepijn Veefkind, Pawan K. Bhartia, Deborah C. Stein Zweers, Bryan N. Duncan, David G. Streets, Henk Eskes, Ronald van der A, Chris McLinden, Vitali Fioletov, Simon Carn, Jos de Laat, Matthew DeLand, Sergey Marchenko, Richard McPeters, Jerald Ziemke, Dejian Fu, Xiong Liu, Kenneth Pickering, Arnoud Apituley, Gonzalo González Abad, Antti Arola, Folkert Boersma, Christopher Chan Miller, Kelly Chance, Martin de Graaf, Janne Hakkarainen, Seppo Hassinen, Iolanda Ialongo, Quintus Kleipool, Nickolay Krotkov, Can Li, Lok Lamsal, Paul Newman, Caroline Nowlan, Raid Suleiman, Lieuwe Gijsbert Tilstra, Omar Torres, Huiqun Wang, and Krzysztof Wargan
Atmos. Chem. Phys., 18, 5699–5745, https://doi.org/10.5194/acp-18-5699-2018, https://doi.org/10.5194/acp-18-5699-2018, 2018
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The aim of this paper is to highlight the many successes of the Ozone Monitoring Instrument (OMI) spanning more than 13 years. Data from OMI have been used in a wide range of applications. Due to its unprecedented spatial resolution, in combination with daily global coverage, OMI plays a unique role in measuring trace gases important for the ozone layer, air quality, and climate change. OMI data continue to be used for new research and applications.
Jungbin Mok, Nickolay A. Krotkov, Omar Torres, Hiren Jethva, Zhanqing Li, Jhoon Kim, Ja-Ho Koo, Sujung Go, Hitoshi Irie, Gordon Labow, Thomas F. Eck, Brent N. Holben, Jay Herman, Robert P. Loughman, Elena Spinei, Seoung Soo Lee, Pradeep Khatri, and Monica Campanelli
Atmos. Meas. Tech., 11, 2295–2311, https://doi.org/10.5194/amt-11-2295-2018, https://doi.org/10.5194/amt-11-2295-2018, 2018
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Measuring aerosol absorption from the shortest ultraviolet (UV) to the near-infrared (NIR) wavelengths is important for studies of climate, tropospheric photochemistry, human health, and agricultural productivity. We estimate the accuracy and demonstrate consistency of aerosol absorption retrievals from different instruments, after accounting for spectrally varying surface albedo and gaseous absorption.
Zhong Chen, Pawan K. Bhartia, Robert Loughman, and Peter Colarco
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2018-4, https://doi.org/10.5194/amt-2018-4, 2018
Revised manuscript has not been submitted
Jerald R. Ziemke, Sarah A. Strode, Anne R. Douglass, Joanna Joiner, Alexander Vasilkov, Luke D. Oman, Junhua Liu, Susan E. Strahan, Pawan K. Bhartia, and David P. Haffner
Atmos. Meas. Tech., 10, 4067–4078, https://doi.org/10.5194/amt-10-4067-2017, https://doi.org/10.5194/amt-10-4067-2017, 2017
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We combine satellite measurements of ozone and cloud properties from the Aura OMI and MLS instruments for 2004–2016 to measure ozone in the mid–upper levels of deep convective clouds. Our results ascribe upward injection of low boundary layer ozone (varying from low to high amounts) as a major driver of the measured concentrations of ozone in thick clouds. Our OMI/MLS generated ozone product is made available to the public for use in science applications.
Viktoria F. Sofieva, Erkki Kyrölä, Marko Laine, Johanna Tamminen, Doug Degenstein, Adam Bourassa, Chris Roth, Daniel Zawada, Mark Weber, Alexei Rozanov, Nabiz Rahpoe, Gabriele Stiller, Alexandra Laeng, Thomas von Clarmann, Kaley A. Walker, Patrick Sheese, Daan Hubert, Michel van Roozendael, Claus Zehner, Robert Damadeo, Joseph Zawodny, Natalya Kramarova, and Pawan K. Bhartia
Atmos. Chem. Phys., 17, 12533–12552, https://doi.org/10.5194/acp-17-12533-2017, https://doi.org/10.5194/acp-17-12533-2017, 2017
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We present a merged dataset of ozone profiles from several satellite instruments: SAGE II, GOMOS, SCIAMACHY, MIPAS, OSIRIS, ACE-FTS and OMPS. For merging, we used the latest versions of the original ozone datasets.
The merged SAGE–CCI–OMPS dataset is used for evaluating ozone trends in the stratosphere through multiple linear regression. Negative ozone trends in the upper stratosphere are observed before 1997 and positive trends are found after 1997.
Wolfgang Steinbrecht, Lucien Froidevaux, Ryan Fuller, Ray Wang, John Anderson, Chris Roth, Adam Bourassa, Doug Degenstein, Robert Damadeo, Joe Zawodny, Stacey Frith, Richard McPeters, Pawan Bhartia, Jeannette Wild, Craig Long, Sean Davis, Karen Rosenlof, Viktoria Sofieva, Kaley Walker, Nabiz Rahpoe, Alexei Rozanov, Mark Weber, Alexandra Laeng, Thomas von Clarmann, Gabriele Stiller, Natalya Kramarova, Sophie Godin-Beekmann, Thierry Leblanc, Richard Querel, Daan Swart, Ian Boyd, Klemens Hocke, Niklaus Kämpfer, Eliane Maillard Barras, Lorena Moreira, Gerald Nedoluha, Corinne Vigouroux, Thomas Blumenstock, Matthias Schneider, Omaira García, Nicholas Jones, Emmanuel Mahieu, Dan Smale, Michael Kotkamp, John Robinson, Irina Petropavlovskikh, Neil Harris, Birgit Hassler, Daan Hubert, and Fiona Tummon
Atmos. Chem. Phys., 17, 10675–10690, https://doi.org/10.5194/acp-17-10675-2017, https://doi.org/10.5194/acp-17-10675-2017, 2017
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Thanks to the 1987 Montreal Protocol and its amendments, ozone-depleting chlorine (and bromine) in the stratosphere has declined slowly since the late 1990s. Improved and extended long-term ozone profile observations from satellites and ground-based stations confirm that ozone is responding as expected and has increased by about 2 % per decade since 2000 in the upper stratosphere, around 40 km altitude. At lower altitudes, however, ozone has not changed significantly since 2000.
Guanyu Huang, Xiong Liu, Kelly Chance, Kai Yang, Pawan K. Bhartia, Zhaonan Cai, Marc Allaart, Gérard Ancellet, Bertrand Calpini, Gerrie J. R. Coetzee, Emilio Cuevas-Agulló, Manuel Cupeiro, Hugo De Backer, Manvendra K. Dubey, Henry E. Fuelberg, Masatomo Fujiwara, Sophie Godin-Beekmann, Tristan J. Hall, Bryan Johnson, Everette Joseph, Rigel Kivi, Bogumil Kois, Ninong Komala, Gert König-Langlo, Giovanni Laneve, Thierry Leblanc, Marion Marchand, Kenneth R. Minschwaner, Gary Morris, Michael J. Newchurch, Shin-Ya Ogino, Nozomu Ohkawara, Ankie J. M. Piters, Françoise Posny, Richard Querel, Rinus Scheele, Frank J. Schmidlin, Russell C. Schnell, Otto Schrems, Henry Selkirk, Masato Shiotani, Pavla Skrivánková, René Stübi, Ghassan Taha, David W. Tarasick, Anne M. Thompson, Valérie Thouret, Matthew B. Tully, Roeland Van Malderen, Holger Vömel, Peter von der Gathen, Jacquelyn C. Witte, and Margarita Yela
Atmos. Meas. Tech., 10, 2455–2475, https://doi.org/10.5194/amt-10-2455-2017, https://doi.org/10.5194/amt-10-2455-2017, 2017
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It is essential to understand the data quality of +10-year OMI ozone product and impacts of the “row anomaly” (RA). We validate the OMI Ozone Profile (PROFOZ) product from Oct 2004 to Dec 2014 against ozonesonde observations globally. Generally, OMI has good agreement with ozonesondes. The spatiotemporal variation of retrieval performance suggests the need to improve OMI’s radiometric calibration especially during the post-RA period to maintain the long-term stability.
V. M. Erik Schenkeveld, Glen Jaross, Sergey Marchenko, David Haffner, Quintus L. Kleipool, Nico C. Rozemeijer, J. Pepijn Veefkind, and Pieternel F. Levelt
Atmos. Meas. Tech., 10, 1957–1986, https://doi.org/10.5194/amt-10-1957-2017, https://doi.org/10.5194/amt-10-1957-2017, 2017
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The Ozone Monitoring Instrument (OMI) has been flying on NASA’s EOS Aura satellite since July 15, 2004. It has measured the concentration of trace gasses in the atmosphere, like ozone, NO2 and SO2. This article describes the trend in performance and calibration parameters of OMI during 12 years of flight. The degradation of the CCD detectors, solar diffusers, spectral calibration and row anomaly are shown. The instrument shows overall degradation that is better than expected.
Sergey M. Khaykin, Sophie Godin-Beekmann, Philippe Keckhut, Alain Hauchecorne, Julien Jumelet, Jean-Paul Vernier, Adam Bourassa, Doug A. Degenstein, Landon A. Rieger, Christine Bingen, Filip Vanhellemont, Charles Robert, Matthew DeLand, and Pawan K. Bhartia
Atmos. Chem. Phys., 17, 1829–1845, https://doi.org/10.5194/acp-17-1829-2017, https://doi.org/10.5194/acp-17-1829-2017, 2017
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The article is devoted to the long-term evolution and variability of stratospheric aerosol, which plays an important role in climate change and the ozone layer. We use 22-year long continuous observations using laser radar soundings in southern France and satellite-based observations to distinguish between natural aerosol variability (caused by volcanic eruptions) and human-induced change in aerosol concentration. An influence of growing pollution above Asia on stratospheric aerosol is found.
Pawan Gupta, Joanna Joiner, Alexander Vasilkov, and Pawan K. Bhartia
Atmos. Meas. Tech., 9, 2813–2826, https://doi.org/10.5194/amt-9-2813-2016, https://doi.org/10.5194/amt-9-2813-2016, 2016
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The A-train constellation of satellites provides a unique opportunity to analyze near-simultaneous data from several of these sensors. In this paper, retrievals of cloud/aerosols parameters and total column ozone (TCO) from the Aura Ozone Monitoring Instrument (OMI) have been used to develop a variety of neural networks that estimate TOA SWF globally over ocean and land using only OMI data as inputs. Application of our method to other ultraviolet sensors may provide unique estimates of TOA SWF.
Daan Hubert, Jean-Christopher Lambert, Tijl Verhoelst, José Granville, Arno Keppens, Jean-Luc Baray, Adam E. Bourassa, Ugo Cortesi, Doug A. Degenstein, Lucien Froidevaux, Sophie Godin-Beekmann, Karl W. Hoppel, Bryan J. Johnson, Erkki Kyrölä, Thierry Leblanc, Günter Lichtenberg, Marion Marchand, C. Thomas McElroy, Donal Murtagh, Hideaki Nakane, Thierry Portafaix, Richard Querel, James M. Russell III, Jacobo Salvador, Herman G. J. Smit, Kerstin Stebel, Wolfgang Steinbrecht, Kevin B. Strawbridge, René Stübi, Daan P. J. Swart, Ghassan Taha, David W. Tarasick, Anne M. Thompson, Joachim Urban, Joanna A. E. van Gijsel, Roeland Van Malderen, Peter von der Gathen, Kaley A. Walker, Elian Wolfram, and Joseph M. Zawodny
Atmos. Meas. Tech., 9, 2497–2534, https://doi.org/10.5194/amt-9-2497-2016, https://doi.org/10.5194/amt-9-2497-2016, 2016
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A more detailed understanding of satellite O3 profile data records is vital for further progress in O3 research. To this end, we made a comprehensive assessment of 14 limb/occultation profilers using ground-based reference data. The mutual consistency of satellite O3 in terms of bias, short-term variability and decadal stability is generally good over most of the stratosphere. However, we identified some exceptions that impact the quality of recently merged data sets and ozone trend assessments.
Zhong Chen, Matthew DeLand, and Pawan K. Bhartia
Atmos. Meas. Tech., 9, 1239–1246, https://doi.org/10.5194/amt-9-1239-2016, https://doi.org/10.5194/amt-9-1239-2016, 2016
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U. Jeong, J. Kim, C. Ahn, O. Torres, X. Liu, P. K. Bhartia, R. J. D. Spurr, D. Haffner, K. Chance, and B. N. Holben
Atmos. Chem. Phys., 16, 177–193, https://doi.org/10.5194/acp-16-177-2016, https://doi.org/10.5194/acp-16-177-2016, 2016
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An aerosol retrieval and error analysis algorithm using OMI measurements based on an optimal-estimation method was developed in this study. The aerosol retrievals were validated using the DRAGON campaign products. The estimated errors of the retrievals represented the actual biases between retrieval and AERONET measurements well. The retrievals, with their estimated uncertainties, are expected to be valuable for relevant studies, such as trace gas retrieval and data assimilation.
N. R. P. Harris, B. Hassler, F. Tummon, G. E. Bodeker, D. Hubert, I. Petropavlovskikh, W. Steinbrecht, J. Anderson, P. K. Bhartia, C. D. Boone, A. Bourassa, S. M. Davis, D. Degenstein, A. Delcloo, S. M. Frith, L. Froidevaux, S. Godin-Beekmann, N. Jones, M. J. Kurylo, E. Kyrölä, M. Laine, S. T. Leblanc, J.-C. Lambert, B. Liley, E. Mahieu, A. Maycock, M. de Mazière, A. Parrish, R. Querel, K. H. Rosenlof, C. Roth, C. Sioris, J. Staehelin, R. S. Stolarski, R. Stübi, J. Tamminen, C. Vigouroux, K. A. Walker, H. J. Wang, J. Wild, and J. M. Zawodny
Atmos. Chem. Phys., 15, 9965–9982, https://doi.org/10.5194/acp-15-9965-2015, https://doi.org/10.5194/acp-15-9965-2015, 2015
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Trends in the vertical distribution of ozone are reported for new and recently revised data sets. The amount of ozone-depleting compounds in the stratosphere peaked in the second half of the 1990s. We examine the trends before and after that peak to see if any change in trend is discernible. The previously reported decreases are confirmed. Furthermore, the downward trend in upper stratospheric ozone has not continued. The possible significance of any increase is discussed in detail.
R. Loughman, D. Flittner, E. Nyaku, and P. K. Bhartia
Atmos. Chem. Phys., 15, 3007–3020, https://doi.org/10.5194/acp-15-3007-2015, https://doi.org/10.5194/acp-15-3007-2015, 2015
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The Gauss--Seidel limb scattering (GSLS) radiative transfer model simulates the transfer of solar radiation through the atmosphere. Several recent changes have been added that improve the accuracy and flexibility of the GSLS radiance calculations. The single-scattered radiance errors have been reduced from 4% in earlier studies to 0.3%, while total radiance errors generally decline from 10% to 1-3%. In all cases, the tangent height dependence of the GSLS radiance error is greatly reduced.
A. Parrish, I. S. Boyd, G. E. Nedoluha, P. K. Bhartia, S. M. Frith, N. A. Kramarova, B. J. Connor, G. E. Bodeker, L. Froidevaux, M. Shiotani, and T. Sakazaki
Atmos. Chem. Phys., 14, 7255–7272, https://doi.org/10.5194/acp-14-7255-2014, https://doi.org/10.5194/acp-14-7255-2014, 2014
E. W. Chiou, P. K. Bhartia, R. D. McPeters, D. G. Loyola, M. Coldewey-Egbers, V. E. Fioletov, M. Van Roozendael, R. Spurr, C. Lerot, and S. M. Frith
Atmos. Meas. Tech., 7, 1681–1692, https://doi.org/10.5194/amt-7-1681-2014, https://doi.org/10.5194/amt-7-1681-2014, 2014
B. Hassler, I. Petropavlovskikh, J. Staehelin, T. August, P. K. Bhartia, C. Clerbaux, D. Degenstein, M. De Mazière, B. M. Dinelli, A. Dudhia, G. Dufour, S. M. Frith, L. Froidevaux, S. Godin-Beekmann, J. Granville, N. R. P. Harris, K. Hoppel, D. Hubert, Y. Kasai, M. J. Kurylo, E. Kyrölä, J.-C. Lambert, P. F. Levelt, C. T. McElroy, R. D. McPeters, R. Munro, H. Nakajima, A. Parrish, P. Raspollini, E. E. Remsberg, K. H. Rosenlof, A. Rozanov, T. Sano, Y. Sasano, M. Shiotani, H. G. J. Smit, G. Stiller, J. Tamminen, D. W. Tarasick, J. Urban, R. J. van der A, J. P. Veefkind, C. Vigouroux, T. von Clarmann, C. von Savigny, K. A. Walker, M. Weber, J. Wild, and J. M. Zawodny
Atmos. Meas. Tech., 7, 1395–1427, https://doi.org/10.5194/amt-7-1395-2014, https://doi.org/10.5194/amt-7-1395-2014, 2014
N. A. Kramarova, E. R. Nash, P. A. Newman, P. K. Bhartia, R. D. McPeters, D. F. Rault, C. J. Seftor, P. Q. Xu, and G. J. Labow
Atmos. Chem. Phys., 14, 2353–2361, https://doi.org/10.5194/acp-14-2353-2014, https://doi.org/10.5194/acp-14-2353-2014, 2014
O. Torres, C. Ahn, and Z. Chen
Atmos. Meas. Tech., 6, 3257–3270, https://doi.org/10.5194/amt-6-3257-2013, https://doi.org/10.5194/amt-6-3257-2013, 2013
E. J. Bucsela, N. A. Krotkov, E. A. Celarier, L. N. Lamsal, W. H. Swartz, P. K. Bhartia, K. F. Boersma, J. P. Veefkind, J. F. Gleason, and K. E. Pickering
Atmos. Meas. Tech., 6, 2607–2626, https://doi.org/10.5194/amt-6-2607-2013, https://doi.org/10.5194/amt-6-2607-2013, 2013
P. K. Bhartia, R. D. McPeters, L. E. Flynn, S. Taylor, N. A. Kramarova, S. Frith, B. Fisher, and M. DeLand
Atmos. Meas. Tech., 6, 2533–2548, https://doi.org/10.5194/amt-6-2533-2013, https://doi.org/10.5194/amt-6-2533-2013, 2013
N. A. Kramarova, P. K. Bhartia, S. M. Frith, R. D. McPeters, and R. S. Stolarski
Atmos. Meas. Tech., 6, 2089–2099, https://doi.org/10.5194/amt-6-2089-2013, https://doi.org/10.5194/amt-6-2089-2013, 2013
N. A. Kramarova, S. M. Frith, P. K. Bhartia, R. D. McPeters, S. L. Taylor, B. L. Fisher, G. J. Labow, and M. T. DeLand
Atmos. Chem. Phys., 13, 6887–6905, https://doi.org/10.5194/acp-13-6887-2013, https://doi.org/10.5194/acp-13-6887-2013, 2013
Related subject area
Subject: Gases | Technique: Remote Sensing | Topic: Validation and Intercomparisons
Intercomparison of long-term ground-based measurements of total, tropospheric, and stratospheric ozone at Lauder, New Zealand
First evaluation of the GEMS glyoxal products against TROPOMI and ground-based measurements
Validation of GEMS tropospheric NO2 columns and their diurnal variation with ground-based DOAS measurements
Using open-path dual-comb spectroscopy to monitor methane emissions from simulated grazing cattle
Greenhouse gas column observations from a portable spectrometer in Uganda
Independent validation of IASI/MetOp-A LMD and RAL CH4 products using CAMS model, in situ profiles, and ground-based FTIR measurements
Joint spectral retrievals of ozone with Suomi NPP CrIS augmented by S5P/TROPOMI
An evaluation of atmospheric absorption models at millimetre and sub-millimetre wavelengths using airborne observations
Validation of the version 4.5 MAESTRO ozone and NO2 measurements
Applicability of the inverse dispersion method to measure emissions from animal housings
Validation of ACE-FTS version 5.2 ozone data with ozonesonde measurements
5 years of Sentinel-5P TROPOMI operational ozone profiling and geophysical validation using ozonesonde and lidar ground-based networks
Using a portable FTIR spectrometer to evaluate the consistency of Total Carbon Column Observing Network (TCCON) measurements on a global scale: the Collaborative Carbon Column Observing Network (COCCON) travel standard
Comparison of the H2O, HDO and δD stratospheric climatologies between the MIPAS-ESA V8, MIPAS-IMK V5 and ACE-FTS V4.1/4.2 satellite datasets
TROPESS-CrIS CO single-pixel vertical profiles: intercomparisons with MOPITT and model simulations for 2020 western US wildfires
TOLNet validation of satellite ozone profiles in the troposphere: impact of retrieval wavelengths
An uncertainty methodology for solar occultation flux measurements: ammonia emissions from livestock production
Validation of Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) chlorodifluoromethane (HCFC-22) in the upper troposphere and lower stratosphere
First validation of high-resolution satellite-derived methane emissions from an active gas leak in the UK
Diurnal variations of NO2 tropospheric vertical column density over the Seoul Metropolitan Area from the Geostationary Environment Monitoring Spectrometer (GEMS): seasonal differences and impacts of varying a priori NO2 profile data
Ship- and aircraft-based XCH4 over oceans as a new tool for satellite validation
Validation of 12 years (2008–2019) of IASI-CO with IAGOS aircraft observations
Single-blind test of nine methane-sensing satellite systems from three continents
Water vapor measurements inside clouds and storms using a differential absorption radar
Evaluation of the first year of Pandora NO2 measurements over Beijing and application to satellite validation
Validation of MUSES NH3 observations from AIRS and CrIS against aircraft measurements from DISCOVER-AQ and a surface network in the Magic Valley
Benchmarking data-driven inversion methods for the estimation of local CO2 emissions from XCO2 and NO2 satellite images
Performance and sensitivity of column-wise and pixel-wise methane retrievals for imaging spectrometers
Methane point source quantification using MethaneAIR: a new airborne imaging spectrometer
Evaluation of total ozone measurements from Geostationary Environmental Monitoring Spectrometer (GEMS)
To new heights by flying low: comparison of aircraft vertical NO2 profiles to model simulations and implications for TROPOMI NO2 retrievals
Local comparisons of tropospheric ozone: vertical soundings at two neighbouring stations in southern Bavaria
Ground-based Multi-AXis Differential Optical Absorption Spectroscopy (MAX-DOAS) observations of NO2 and H2CO at Kinshasa and comparisons with TROPOMI observations
Total column ozone trends from the NASA Merged Ozone time series 1979 to 2021 showing latitude-dependent ozone recovery dates (1994 to 1998)
The SPARC water vapour assessment II: biases and drifts of water vapour satellite data records with respect to frost point hygrometer records
Vicarious calibration of the Tropospheric Monitoring Instrument (TROPOMI) short-wave infrared (SWIR) module over the Railroad Valley Playa
First-time comparison between NO2 vertical columns from Geostationary Environmental Monitoring Spectrometer (GEMS) and Pandora measurements
A blended TROPOMI+GOSAT satellite data product for atmospheric methane using machine learning to correct retrieval biases
Evaluating the consistency between OCO-2 and OCO-3 XCO2 estimates derived from the NASA ACOS version 10 retrieval algorithm
OLCI-A/B tandem phase: evaluation of FLuorescence EXplorer (FLEX)-like radiances and estimation of systematic differences between OLCI-A and OLCI-FLEX
Multi-parameter dynamical diagnostics for upper tropospheric and lower stratospheric studies
An approach to track instrument calibration and produce consistent products with the version-8 total column ozone algorithm (V8TOZ)
Satellite remote-sensing capability to assess tropospheric-column ratios of formaldehyde and nitrogen dioxide: case study during the Long Island Sound Tropospheric Ozone Study 2018 (LISTOS 2018) field campaign
Validation of Sentinel-5P TROPOMI tropospheric NO2 products by comparison with NO2 measurements from airborne imaging DOAS, ground-based stationary DOAS, and mobile car DOAS measurements during the S5P-VAL-DE-Ruhr campaign
Evaluation of open- and closed-path sampling systems for the determination of emission rates of NH3 and CH4 with inverse dispersion modeling
Performance of AIRS ozone retrieval over the central Himalayas: use of ozonesonde and other satellite datasets
Solar occultation measurement of mesospheric ozone by SAGE III/ISS: impact of variations along the line of sight caused by photochemistry
Understanding the potential of Sentinel-2 for monitoring methane point emissions
TROPOMI/S5P Total Column Water Vapor validation against AERONET ground-based measurements
Assessing the consistency of satellite-derived upper tropospheric humidity measurements
Robin Björklund, Corinne Vigouroux, Peter Effertz, Omaira E. García, Alex Geddes, James Hannigan, Koji Miyagawa, Michael Kotkamp, Bavo Langerock, Gerald Nedoluha, Ivan Ortega, Irina Petropavlovskikh, Deniz Poyraz, Richard Querel, John Robinson, Hisako Shiona, Dan Smale, Penny Smale, Roeland Van Malderen, and Martine De Mazière
Atmos. Meas. Tech., 17, 6819–6849, https://doi.org/10.5194/amt-17-6819-2024, https://doi.org/10.5194/amt-17-6819-2024, 2024
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Different ground-based ozone measurements from the last 2 decades at Lauder are compared to each other. We want to know why different trends have been observed in the stratosphere. Also, the quality and relevance of tropospheric datasets need to be evaluated. While remaining drifts are still present, our study explains roughly half of the differences in observed trends in previous studies and shows the necessity for continuous review and improvement of the measurements.
Eunjo S. Ha, Rokjin J. Park, Hyeong-Ahn Kwon, Gitaek T. Lee, Sieun D. Lee, Seunga Shin, Dong-Won Lee, Hyunkee Hong, Christophe Lerot, Isabelle De Smedt, Thomas Danckaert, Francois Hendrick, and Hitoshi Irie
Atmos. Meas. Tech., 17, 6369–6384, https://doi.org/10.5194/amt-17-6369-2024, https://doi.org/10.5194/amt-17-6369-2024, 2024
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In this study, we evaluated the GEMS glyoxal products by comparing them with TROPOMI and MAX-DOAS measurements. GEMS and TROPOMI VCDs present similar spatial distributions. Monthly variations in GEMS VCDs and TROPOMI and MAX-DOAS VCDs differ in northeastern Asia, which we attributed to a polluted reference spectrum and high NO2 concentrations. GEMS glyoxal products with unparalleled temporal resolution would enrich our understanding of VOC emissions and diurnal variation.
Kezia Lange, Andreas Richter, Tim Bösch, Bianca Zilker, Miriam Latsch, Lisa K. Behrens, Chisom M. Okafor, Hartmut Bösch, John P. Burrows, Alexis Merlaud, Gaia Pinardi, Caroline Fayt, Martina M. Friedrich, Ermioni Dimitropoulou, Michel Van Roozendael, Steffen Ziegler, Simona Ripperger-Lukosiunaite, Leon Kuhn, Bianca Lauster, Thomas Wagner, Hyunkee Hong, Donghee Kim, Lim-Seok Chang, Kangho Bae, Chang-Keun Song, Jong-Uk Park, and Hanlim Lee
Atmos. Meas. Tech., 17, 6315–6344, https://doi.org/10.5194/amt-17-6315-2024, https://doi.org/10.5194/amt-17-6315-2024, 2024
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Instruments for air quality observations on geostationary satellites provide multiple observations per day and allow for the analysis of the diurnal variation of important air pollutants such as nitrogen dioxide (NO2) over large areas. The South Korean instrument GEMS, launched in February 2020, is the first instrument in geostationary orbit and covers a large part of Asia. Our investigations show the observed diurnal evolution of NO2 at different measurement sites.
Chinthaka Weerasekara, Lindsay C. Morris, Nathan A. Malarich, Fabrizio R. Giorgetta, Daniel I. Herman, Kevin C. Cossel, Nathan R. Newbury, Clenton E. Owensby, Stephen M. Welch, Cosmin Blaga, Brett D. DePaola, Ian Coddington, Brian R. Washburn, and Eduardo A. Santos
Atmos. Meas. Tech., 17, 6107–6117, https://doi.org/10.5194/amt-17-6107-2024, https://doi.org/10.5194/amt-17-6107-2024, 2024
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Most methane emissions during the life cycle of beef cattle occur during the grazing phase. Measuring methane in grazing systems is difficult due to the high mobility and low density of animals. This work investigates if dual-comb spectroscopy can measure methane emissions from small cattle herds. An enhancement of 10 nmol mol-1 methane above the atmospheric background was measured, equivalent to 20 head located 60 m away. The calculated methane flux was within 5 % of the actual release rate.
Neil Humpage, Hartmut Boesch, William Okello, Jia Chen, Florian Dietrich, Mark F. Lunt, Liang Feng, Paul I. Palmer, and Frank Hase
Atmos. Meas. Tech., 17, 5679–5707, https://doi.org/10.5194/amt-17-5679-2024, https://doi.org/10.5194/amt-17-5679-2024, 2024
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We used a Bruker EM27/SUN spectrometer within an automated weatherproof enclosure to measure greenhouse gas column concentrations over a 3-month period in Jinja, Uganda. The portability of the EM27/SUN allows us to evaluate satellite and model data in locations not covered by traditional validation networks. This is of particular value in tropical Africa, where extensive terrestrial ecosystems are a significant store of carbon and play a key role in the atmospheric budgets of CO2 and CH4.
Bart Dils, Minqiang Zhou, Claude Camy-Peyret, Martine De Mazière, Yannick Kangah, Bavo Langerock, Pascal Prunet, Carmine Serio, Richard Siddans, and Brian Kerridge
Atmos. Meas. Tech., 17, 5491–5524, https://doi.org/10.5194/amt-17-5491-2024, https://doi.org/10.5194/amt-17-5491-2024, 2024
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The paper discusses two very distinct methane products from the IASI instrument aboard the MetOp-A satellite. One (referred to as LMD NLISv8.3) uses a machine-learning approach, while the other (RALv2.0) uses a more conventional optimal estimation approach. We used a variety of model and independent reference measurement data to assess both products' overall quality, their differences, and specific aspects of each product that would benefit from further analysis by the product development teams.
Edward Malina, Kevin W. Bowman, Valentin Kantchev, Le Kuai, Thomas P. Kurosu, Kazuyuki Miyazaki, Vijay Natraj, Gregory B. Osterman, Fabiano Oyafuso, and Matthew D. Thill
Atmos. Meas. Tech., 17, 5341–5371, https://doi.org/10.5194/amt-17-5341-2024, https://doi.org/10.5194/amt-17-5341-2024, 2024
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Characterizing the distribution of ozone in the atmosphere is a challenging problem, with current Earth observation satellites using either thermal infrared (TIR) or ultraviolet (UV) instruments, sensitive to different portions of the atmosphere, making it difficult to gain a full picture. In this work, we combine measurements from the TIR and UV instruments Suomi NPP CrIS and Sentinel-5P/TROPOMI to improve sensitivity through the whole atmosphere and improve knowledge of ozone distribution.
Stuart Fox, Vinia Mattioli, Emma Turner, Alan Vance, Domenico Cimini, and Donatello Gallucci
Atmos. Meas. Tech., 17, 4957–4978, https://doi.org/10.5194/amt-17-4957-2024, https://doi.org/10.5194/amt-17-4957-2024, 2024
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Airborne observations are used to evaluate two models for absorption and emission by atmospheric gases, including water vapour and oxygen, at microwave and sub-millimetre wavelengths. These models are needed for the Ice Cloud Imager (ICI) on the next generation of European polar-orbiting weather satellites, which measures at frequencies up to 664 GHz. Both models can provide a good match to measurements from airborne radiometers and are sufficiently accurate for use with ICI.
Paul S. Jeffery, James R. Drummond, C. Thomas McElroy, Kaley A. Walker, and Jiansheng Zou
EGUsphere, https://doi.org/10.5194/egusphere-2024-2115, https://doi.org/10.5194/egusphere-2024-2115, 2024
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The MAESTRO instrument has been monitoring ozone and NO2 since February 2004. A new version of these data products has recently been released; however, these new products must be validated against other datasets to ensure their validity. This study presents such an assessment, using measurements from eleven satellite instruments to characterize the new MAESTRO products. In the stratosphere, good agreement is found for ozone and acceptable agreement is found for NO2 with these other datasets.
Marcel Bühler, Christoph Häni, Albrecht Neftel, Patrice Bühler, Christof Ammann, and Thomas Kupper
Atmos. Meas. Tech., 17, 4649–4658, https://doi.org/10.5194/amt-17-4649-2024, https://doi.org/10.5194/amt-17-4649-2024, 2024
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Methane was released from an artificial source inside a barn to test the applicability of the inverse dispersion method (IDM). Multiple open-path concentration devices and ultrasonic anemometers were used at the site. It is concluded that, for the present study case, the effect of a building and a tree in the main wind axis led to a systematic underestimation of the IDM-derived emission rate probably due to deviations in the wind field and turbulent dispersion from the ideal assumptions.
Jiansheng Zou, Kaley A. Walker, Patrick E. Sheese, Chris D. Boone, Ryan M. Stauffer, Anne M. Thompson, and David W. Tarasick
EGUsphere, https://doi.org/10.5194/egusphere-2024-1916, https://doi.org/10.5194/egusphere-2024-1916, 2024
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Ozone measurements from the ACE-FTS satellite instrument have been compared to worldwide balloon-borne ozonesonde profiles using pairs of closely-spaced profiles and monthly averaged profiles. ACE-FTS typically measures more ozone in the stratosphere by up to 10 %. The long-term stability of the ACE-FTS ozone data is good exhibiting small (but not significant) drifts of less than 3 % per decade in the stratosphere. Lower in the profiles, the calculated drifts are larger (up to 10 % per decade).
Arno Keppens, Serena Di Pede, Daan Hubert, Jean-Christopher Lambert, Pepijn Veefkind, Maarten Sneep, Johan De Haan, Mark ter Linden, Thierry Leblanc, Steven Compernolle, Tijl Verhoelst, José Granville, Oindrila Nath, Ann Mari Fjæraa, Ian Boyd, Sander Niemeijer, Roeland Van Malderen, Herman G. J. Smit, Valentin Duflot, Sophie Godin-Beekmann, Bryan J. Johnson, Wolfgang Steinbrecht, David W. Tarasick, Debra E. Kollonige, Ryan M. Stauffer, Anne M. Thompson, Angelika Dehn, and Claus Zehner
Atmos. Meas. Tech., 17, 3969–3993, https://doi.org/10.5194/amt-17-3969-2024, https://doi.org/10.5194/amt-17-3969-2024, 2024
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The Sentinel-5P satellite operated by the European Space Agency has carried the TROPOspheric Monitoring Instrument (TROPOMI) around the Earth since October 2017. This mission also produces atmospheric ozone profile data which are described in detail for May 2018 to April 2023. Independent validation using ground-based reference measurements demonstrates that the operational ozone profile product mostly fully and at least partially complies with all mission requirements.
Benedikt Herkommer, Carlos Alberti, Paolo Castracane, Jia Chen, Angelika Dehn, Florian Dietrich, Nicholas M. Deutscher, Matthias Max Frey, Jochen Groß, Lawson Gillespie, Frank Hase, Isamu Morino, Nasrin Mostafavi Pak, Brittany Walker, and Debra Wunch
Atmos. Meas. Tech., 17, 3467–3494, https://doi.org/10.5194/amt-17-3467-2024, https://doi.org/10.5194/amt-17-3467-2024, 2024
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The Total Carbon Column Observing Network is a network of ground-based Fourier transform infrared (FTIR) spectrometers used mainly for satellite validation. To ensure the highest-quality validation data, the network needs to be highly consistent. This is a major challenge, which so far is solved by site comparisons with airborne in situ measurements. In this work, we describe the use of a portable FTIR spectrometer as a travel standard for evaluating the consistency of TCCON sites.
Karen De Los Ríos, Paulina Ordoñez, Gabriele P. Stiller, Piera Raspollini, Marco Gai, Kaley A. Walker, Cristina Peña-Ortiz, and Luis Acosta
Atmos. Meas. Tech., 17, 3401–3418, https://doi.org/10.5194/amt-17-3401-2024, https://doi.org/10.5194/amt-17-3401-2024, 2024
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This study examines newer versions of H2O and HDO retrievals from Envisat/MIPAS and SCISAT/ACE-FTS. Results reveal a better agreement in stratospheric H2O profiles than in HDO profiles. The H2O tape recorder signal is consistent across databases, but δD tape recorder composites show differences that impact the interpretation of water vapour transport. These findings enhance the need for intercomparisons to refine our insights.
Ming Luo, Helen M. Worden, Robert D. Field, Kostas Tsigaridis, and Gregory S. Elsaesser
Atmos. Meas. Tech., 17, 2611–2624, https://doi.org/10.5194/amt-17-2611-2024, https://doi.org/10.5194/amt-17-2611-2024, 2024
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The TROPESS CrIS single-pixel CO profile retrievals are compared to the MOPITT CO products in steps of adjusting them to the common a priori assumptions. The two data sets are found to agree within 5 %. We also demonstrated and analyzed the proper steps in evaluating GISS ModelE CO simulations using satellite CO retrieval products for the western US wildfire events in September 2020.
Matthew S. Johnson, Alexei Rozanov, Mark Weber, Nora Mettig, John Sullivan, Michael J. Newchurch, Shi Kuang, Thierry Leblanc, Fernando Chouza, Timothy A. Berkoff, Guillaume Gronoff, Kevin B. Strawbridge, Raul J. Alvarez, Andrew O. Langford, Christoph J. Senff, Guillaume Kirgis, Brandi McCarty, and Larry Twigg
Atmos. Meas. Tech., 17, 2559–2582, https://doi.org/10.5194/amt-17-2559-2024, https://doi.org/10.5194/amt-17-2559-2024, 2024
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Monitoring tropospheric ozone (O3), a harmful pollutant negatively impacting human health, is primarily done using ground-based measurements and ozonesondes. However, these observation types lack the coverage to fully understand tropospheric O3. Satellites can retrieve tropospheric ozone with near-daily global coverage; however, they are known to have biases and errors. This study uses ground-based lidars to validate multiple satellites' ability to observe tropospheric O3.
Johan Mellqvist, Nathalia T. Vechi, Charlotte Scheutz, Marc Durif, Francois Gautier, John Johansson, Jerker Samuelsson, Brian Offerle, and Samuel Brohede
Atmos. Meas. Tech., 17, 2465–2479, https://doi.org/10.5194/amt-17-2465-2024, https://doi.org/10.5194/amt-17-2465-2024, 2024
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The solar occultation flux method retrieves ammonia gas columns from the solar spectrum. Emissions are obtained by multiplying the integrated plume concentration by the wind speed profile. The methodology for uncertainty estimation was established considering an error budget with systematic and random components, resulting in an expanded uncertainty in the range of 20 % to 30 %. The method was validated in a controlled release, and its application was demonstrated in different farms.
Felicia Kolonjari, Patrick E. Sheese, Kaley A. Walker, Chris D. Boone, David A. Plummer, Andreas Engel, Stephen A. Montzka, David E. Oram, Tanja Schuck, Gabriele P. Stiller, and Geoffrey C. Toon
Atmos. Meas. Tech., 17, 2429–2449, https://doi.org/10.5194/amt-17-2429-2024, https://doi.org/10.5194/amt-17-2429-2024, 2024
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The Canadian Atmospheric Chemistry Experiment Fourier transform spectrometer (ACE-FTS) satellite instrument is currently providing the only vertically resolved chlorodifluoromethane (HCFC-22) measurements from space. This study assesses the most current ACE-FTS HCFC-22 data product in the upper troposphere and lower stratosphere, as well as modelled HCFC-22 from a 39-year run of the Canadian Middle Atmosphere Model (CMAM39) in the same region.
Emily Dowd, Alistair J. Manning, Bryn Orth-Lashley, Marianne Girard, James France, Rebecca E. Fisher, Dave Lowry, Mathias Lanoisellé, Joseph R. Pitt, Kieran M. Stanley, Simon O'Doherty, Dickon Young, Glen Thistlethwaite, Martyn P. Chipperfield, Emanuel Gloor, and Chris Wilson
Atmos. Meas. Tech., 17, 1599–1615, https://doi.org/10.5194/amt-17-1599-2024, https://doi.org/10.5194/amt-17-1599-2024, 2024
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We provide the first validation of the satellite-derived emission estimates using surface-based mobile greenhouse gas surveys of an active gas leak detected near Cheltenham, UK. GHGSat’s emission estimates broadly agree with the surface-based mobile survey and steps were taken to fix the leak, highlighting the importance of satellite data in identifying emissions and helping to reduce our human impact on climate change.
Seunghwan Seo, Si-Wan Kim, Kyoung-Min Kim, Andreas Richter, Kezia Lange, John Philip Burrows, Junsung Park, Hyunkee Hong, Hanlim Lee, Ukkyo Jeong, and Jhoon Kim
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2024-33, https://doi.org/10.5194/amt-2024-33, 2024
Revised manuscript accepted for AMT
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Over the Seoul Metropolitan Area, GEMS tropospheric NO2 vertical column densities (NO2 TropVCD) show distinct seasonal characteristics, including the absolute values and diurnal patterns. Also, varying a priori data have the substantial impacts on the GEMS NO2 TropVCD. The a priori data from different CTMs resulted in differences of up to 19.2 %. Notably, diurnal patterns of VCDs are similar for all datasets, although theri a priori data exhibit contrasting diurnal patterns.
Astrid Müller, Hiroshi Tanimoto, Takafumi Sugita, Prabir K. Patra, Shin-ichiro Nakaoka, Toshinobu Machida, Isamu Morino, André Butz, and Kei Shiomi
Atmos. Meas. Tech., 17, 1297–1316, https://doi.org/10.5194/amt-17-1297-2024, https://doi.org/10.5194/amt-17-1297-2024, 2024
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Satellite CH4 observations with high accuracy are needed to understand changes in atmospheric CH4 concentrations. But over oceans, reference data are limited. We combine various ship and aircraft observations with the help of atmospheric chemistry models to derive observation-based column-averaged mixing ratios of CH4 (obs. XCH4). We discuss three different approaches and demonstrate the applicability of the new reference dataset for carbon cycle studies and satellite evaluation.
Brice Barret, Pierre Loicq, Eric Le Flochmoën, Yasmine Bennouna, Juliette Hadji-Lazaro, Daniel Hurtmans, and Bastien Sauvage
EGUsphere, https://doi.org/10.5194/egusphere-2024-30, https://doi.org/10.5194/egusphere-2024-30, 2024
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Atmospheric profiles of carbon monoxide (CO) retrieved from the IASI spaceborne sensor with the SOFRID and FORLI algorithms are validated against airborne data from the IAGOS Infrastructure for 2008–2020. 8500 daily observations at 33 airports allow a comprehensive spatio-temporal evaluation of the IASI-CO products. They are globally underestimating IAGOS-CO with stronger bias in the mid-upper troposphere south of Bangkok for SOFRID and in the lower troposphere north of Philadelphia for FORLI.
Evan D. Sherwin, Sahar H. El Abbadi, Philippine M. Burdeau, Zhan Zhang, Zhenlin Chen, Jeffrey S. Rutherford, Yuanlei Chen, and Adam R. Brandt
Atmos. Meas. Tech., 17, 765–782, https://doi.org/10.5194/amt-17-765-2024, https://doi.org/10.5194/amt-17-765-2024, 2024
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Countries and companies increasingly rely on a growing fleet of satellites to find large emissions of climate-warming methane, particularly from oil and natural gas systems across the globe. We independently assessed the performance of nine such systems by releasing controlled, undisclosed amounts of methane as satellites passed overhead. The tested systems produced reliable detection and quantification results, including the smallest-ever emission detected from space in such a test.
Luis F. Millán, Matthew D. Lebsock, Ken B. Cooper, Jose V. Siles, Robert Dengler, Raquel Rodriguez Monje, Amin Nehrir, Rory A. Barton-Grimley, James E. Collins, Claire E. Robinson, Kenneth L. Thornhill, and Holger Vömel
Atmos. Meas. Tech., 17, 539–559, https://doi.org/10.5194/amt-17-539-2024, https://doi.org/10.5194/amt-17-539-2024, 2024
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In this study, we describe and validate a new technique in which three radar tones are used to estimate the water vapor inside clouds and precipitation. This instrument flew on board NASA's P-3 aircraft during the Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Snowstorms (IMPACTS) campaign and the Synergies Of Active optical and Active microwave Remote Sensing Experiment (SOA2RSE) campaign.
Ouyang Liu, Zhengqiang Li, Yangyan Lin, Cheng Fan, Ying Zhang, Kaitao Li, Peng Zhang, Yuanyuan Wei, Tianzeng Chen, Jiantao Dong, and Gerrit de Leeuw
Atmos. Meas. Tech., 17, 377–395, https://doi.org/10.5194/amt-17-377-2024, https://doi.org/10.5194/amt-17-377-2024, 2024
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Nitrogen dioxide (NO2) is a trace gas which is important for atmospheric chemistry and may affect human health. To understand processes leading to harmful concentrations, it is important to monitor NO2 concentrations near the surface and higher up. To this end, a Pandora instrument has been installed in Beijing. An overview of the first year of data shows the large variability on diurnal to seasonal timescales and how this is affected by wind speed and direction and chemistry.
Karen E. Cady-Pereira, Xuehui Guo, Rui Wang, April B. Leytem, Chase Calkins, Elizabeth Berry, Kang Sun, Markus Müller, Armin Wisthaler, Vivienne H. Payne, Mark W. Shephard, Mark A. Zondlo, and Valentin Kantchev
Atmos. Meas. Tech., 17, 15–36, https://doi.org/10.5194/amt-17-15-2024, https://doi.org/10.5194/amt-17-15-2024, 2024
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Ammonia is a significant precursor of PM2.5 particles and thus contributes to poor air quality in many regions. Furthermore, ammonia concentrations are rising due to the increase of large-scale, intensive agricultural activities. Here we evaluate satellite measurements of ammonia against aircraft and surface network data, and show that there are differences in magnitude, but the satellite data are spatially and temporally well correlated with the in situ data.
Diego Santaren, Janne Hakkarainen, Gerrit Kuhlmann, Erik Koene, Frédéric Chevallier, Iolanda Ialongo, Hannakaisa Lindqvist, Janne Nurmela, Johanna Tamminen, Laia Amoros, Dominik Brunner, and Grégoire Broquet
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-241, https://doi.org/10.5194/amt-2023-241, 2024
Revised manuscript accepted for AMT
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This study evaluates data-driven inversion methods for the estimate of CO2 emissions from local sources such as power plants and cities based on meteorological data and XCO2 and NO2 satellite images without atmospheric transport modeling. We assess and compare the performance of five different methods with simulations of one year of images from the future CO2M satellite mission over 15 power plants and the city of Berlin in Eastern Germany.
Alana K. Ayasse, Daniel Cusworth, Kelly O'Neill, Justin Fisk, Andrew K. Thorpe, and Riley Duren
Atmos. Meas. Tech., 16, 6065–6074, https://doi.org/10.5194/amt-16-6065-2023, https://doi.org/10.5194/amt-16-6065-2023, 2023
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Methane is a powerful greenhouse gas, and a significant portion of methane comes from large individual plumes. Recently, airplane-mounted infrared technologies have proven very good at detecting and quantifying these plumes. In order to extract the methane signal from the infrared image, there are two widely used approaches. In this study, we assess the performance of both approaches using controlled-release experiments. We also examine the minimum detection limit of the infrared technology.
Apisada Chulakadabba, Maryann Sargent, Thomas Lauvaux, Joshua S. Benmergui, Jonathan E. Franklin, Christopher Chan Miller, Jonas S. Wilzewski, Sébastien Roche, Eamon Conway, Amir H. Souri, Kang Sun, Bingkun Luo, Jacob Hawthrone, Jenna Samra, Bruce C. Daube, Xiong Liu, Kelly Chance, Yang Li, Ritesh Gautam, Mark Omara, Jeff S. Rutherford, Evan D. Sherwin, Adam Brandt, and Steven C. Wofsy
Atmos. Meas. Tech., 16, 5771–5785, https://doi.org/10.5194/amt-16-5771-2023, https://doi.org/10.5194/amt-16-5771-2023, 2023
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We show that MethaneAIR, a precursor to the MethaneSAT satellite, demonstrates accurate point source quantification during controlled release experiments and regional observations in 2021 and 2022. Results from our two independent quantification methods suggest the accuracy of our sensor and algorithms is better than 25 % for sources emitting 200 kg h−1 or more. Insights from these measurements help establish the capabilities of MethaneSAT and MethaneAIR.
Kanghyun Baek, Jae Hwan Kim, Juseon Bak, David P. Haffner, Mina Kang, and Hyunkee Hong
Atmos. Meas. Tech., 16, 5461–5478, https://doi.org/10.5194/amt-16-5461-2023, https://doi.org/10.5194/amt-16-5461-2023, 2023
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The GEMS mission was the first mission of the geostationary satellite constellation for hourly atmospheric composition monitoring. The GEMS ozone measurements were cross-compared to those of Pandora, OMPS, and TROPOMI satellite sensors and excellent agreement was found. GEMS has proven to be a powerful new instrument for monitoring and assessing the diurnal variation in atmospheric ozone. This experience can be used to advance research with future geostationary environmental satellite missions.
Tobias Christoph Valentin Werner Riess, Klaas Folkert Boersma, Ward Van Roy, Jos de Laat, Enrico Dammers, and Jasper van Vliet
Atmos. Meas. Tech., 16, 5287–5304, https://doi.org/10.5194/amt-16-5287-2023, https://doi.org/10.5194/amt-16-5287-2023, 2023
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Satellite retrievals of trace gases require prior knowledge of the vertical distribution of the pollutant, which is usually obtained from models. Using aircraft-measured vertical NO2 profiles over the North Sea in summer 2021, we evaluate the Transport Model 5 profiles used in the TROPOMI NO2 retrieval. We conclude that driven by the low horizontal resolution and the overestimated vertical mixing, resulting NO2 columns are 20 % too low. This has important implications for emission estimates.
Thomas Trickl, Martin Adelwart, Dina Khordakova, Ludwig Ries, Christian Rolf, Michael Sprenger, Wolfgang Steinbrecht, and Hannes Vogelmann
Atmos. Meas. Tech., 16, 5145–5165, https://doi.org/10.5194/amt-16-5145-2023, https://doi.org/10.5194/amt-16-5145-2023, 2023
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Tropospheric ozone have been measured for more than a century. Highly quantitative ozone measurements have been made at monitoring stations. However, deficits have been reported for vertical sounding systems. Here, we report a thorough intercomparison effort between a differential-absorption lidar system and two types of balloon-borne ozone sondes, also using ozone sensors at nearby mountain sites as references. The sondes agree very well with the lidar after offset corrections.
Rodriguez Yombo Phaka, Alexis Merlaud, Gaia Pinardi, Martina M. Friedrich, Michel Van Roozendael, Jean-François Müller, Trissevgeni Stavrakou, Isabelle De Smedt, François Hendrick, Ermioni Dimitropoulou, Richard Bopili Mbotia Lepiba, Edmond Phuku Phuati, Buenimio Lomami Djibi, Lars Jacobs, Caroline Fayt, Jean-Pierre Mbungu Tsumbu, and Emmanuel Mahieu
Atmos. Meas. Tech., 16, 5029–5050, https://doi.org/10.5194/amt-16-5029-2023, https://doi.org/10.5194/amt-16-5029-2023, 2023
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We present air quality measurements in Kinshasa, Democratic Republic of the Congo, performed with a newly developed instrument which was installed on a roof of the University of Kinshasa in November 2019. The instrument records spectra of the scattered sunlight, from which we derive the abundances of nitrogen dioxide and formaldehyde, two important pollutants. We compare our ground-based measurements with those of the TROPOspheric Monitoring Instrument (TROPOMI).
Jay Herman, Jerald Ziemke, and Richard McPeters
Atmos. Meas. Tech., 16, 4693–4707, https://doi.org/10.5194/amt-16-4693-2023, https://doi.org/10.5194/amt-16-4693-2023, 2023
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Fourier series multivariate linear regression trends (% per decade) in ozone were estimated from the Merged Ozone Data Set (MOD) from 1979 to 2021 in two different regimes, from 1979 to TA (the date when ozone stopped decreasing) and TA to 2021. The derived TA is a latitude-dependent date, ranging from 1994 to 1998. TA(θ) is a marker for photochemistry dynamics models attempting to represent ozone change over the past 42 years.
Michael Kiefer, Dale F. Hurst, Gabriele P. Stiller, Stefan Lossow, Holger Vömel, John Anderson, Faiza Azam, Jean-Loup Bertaux, Laurent Blanot, Klaus Bramstedt, John P. Burrows, Robert Damadeo, Bianca Maria Dinelli, Patrick Eriksson, Maya García-Comas, John C. Gille, Mark Hervig, Yasuko Kasai, Farahnaz Khosrawi, Donal Murtagh, Gerald E. Nedoluha, Stefan Noël, Piera Raspollini, William G. Read, Karen H. Rosenlof, Alexei Rozanov, Christopher E. Sioris, Takafumi Sugita, Thomas von Clarmann, Kaley A. Walker, and Katja Weigel
Atmos. Meas. Tech., 16, 4589–4642, https://doi.org/10.5194/amt-16-4589-2023, https://doi.org/10.5194/amt-16-4589-2023, 2023
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We quantify biases and drifts (and their uncertainties) between the stratospheric water vapor measurement records of 15 satellite-based instruments (SATs, with 31 different retrievals) and balloon-borne frost point hygrometers (FPs) launched at 27 globally distributed stations. These comparisons of measurements during the period 2000–2016 are made using robust, consistent statistical methods. With some exceptions, the biases and drifts determined for most SAT–FP pairs are < 10 % and < 1 % yr−1.
Tim A. van Kempen, Tim J. Rotmans, Richard M. van Hees, Carol Bruegge, Dejian Fu, Ruud Hoogeveen, Thomas J. Pongetti, Robert Rosenberg, and Ilse Aben
Atmos. Meas. Tech., 16, 4507–4527, https://doi.org/10.5194/amt-16-4507-2023, https://doi.org/10.5194/amt-16-4507-2023, 2023
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Validation of satellite measurements is essential for providing reliable and consistent products. In this paper, a validation method for TROPOMI-SWIR (Tropospheric Measurement Instrument in the short-wavelength infrared) is explored. TROPOMI-SWIR has been shown to be exceptionally stable, a necessity to explore the methodology. Railroad Valley, Nevada, is a prime location to perform the necessary measurements to validate the satellite measurements of TROPOMI-SWIR.
Serin Kim, Daewon Kim, Hyunkee Hong, Lim-Seok Chang, Hanlim Lee, Deok-Rae Kim, Donghee Kim, Jeong-Ah Yu, Dongwon Lee, Ukkyo Jeong, Chang-Kuen Song, Sang-Woo Kim, Sang Seo Park, Jhoon Kim, Thomas F. Hanisco, Junsung Park, Wonei Choi, and Kwangyul Lee
Atmos. Meas. Tech., 16, 3959–3972, https://doi.org/10.5194/amt-16-3959-2023, https://doi.org/10.5194/amt-16-3959-2023, 2023
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A first evaluation of the Geostationary Environmental Monitoring Spectrometer (GEMS) NO2 was carried out via comparison with the NO2 data obtained from the ground-based Pandora direct-sun measurements at four sites in Seosan, Republic of Korea. Comparisons between GEMS NO2 and Pandora NO2 were performed according to GEMS cloud fraction. GEMS NO2 showed good agreement with that of Pandora NO2 under less cloudy conditions.
Nicholas Balasus, Daniel J. Jacob, Alba Lorente, Joannes D. Maasakkers, Robert J. Parker, Hartmut Boesch, Zichong Chen, Makoto M. Kelp, Hannah Nesser, and Daniel J. Varon
Atmos. Meas. Tech., 16, 3787–3807, https://doi.org/10.5194/amt-16-3787-2023, https://doi.org/10.5194/amt-16-3787-2023, 2023
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We use machine learning to remove biases in TROPOMI satellite observations of atmospheric methane, with GOSAT observations serving as a reference. We find that the TROPOMI biases relative to GOSAT are related to the presence of aerosols and clouds, the surface brightness, and the specific detector that makes the observation aboard TROPOMI. The resulting blended TROPOMI+GOSAT product is more reliable for quantifying methane emissions.
Thomas E. Taylor, Christopher W. O'Dell, David Baker, Carol Bruegge, Albert Chang, Lars Chapsky, Abhishek Chatterjee, Cecilia Cheng, Frédéric Chevallier, David Crisp, Lan Dang, Brian Drouin, Annmarie Eldering, Liang Feng, Brendan Fisher, Dejian Fu, Michael Gunson, Vance Haemmerle, Graziela R. Keller, Matthäus Kiel, Le Kuai, Thomas Kurosu, Alyn Lambert, Joshua Laughner, Richard Lee, Junjie Liu, Lucas Mandrake, Yuliya Marchetti, Gregory McGarragh, Aronne Merrelli, Robert R. Nelson, Greg Osterman, Fabiano Oyafuso, Paul I. Palmer, Vivienne H. Payne, Robert Rosenberg, Peter Somkuti, Gary Spiers, Cathy To, Brad Weir, Paul O. Wennberg, Shanshan Yu, and Jia Zong
Atmos. Meas. Tech., 16, 3173–3209, https://doi.org/10.5194/amt-16-3173-2023, https://doi.org/10.5194/amt-16-3173-2023, 2023
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NASA's Orbiting Carbon Observatory 2 and 3 (OCO-2 and OCO-3, respectively) provide complementary spatiotemporal coverage from a sun-synchronous and precession orbit, respectively. Estimates of total column carbon dioxide (XCO2) derived from the two sensors using the same retrieval algorithm show broad consistency over a 2.5-year overlapping time record. This suggests that data from the two satellites may be used together for scientific analysis.
Lena Katharina Jänicke, Rene Preusker, Marco Celesti, Marin Tudoroiu, Jürgen Fischer, Dirk Schüttemeyer, and Matthias Drusch
Atmos. Meas. Tech., 16, 3101–3121, https://doi.org/10.5194/amt-16-3101-2023, https://doi.org/10.5194/amt-16-3101-2023, 2023
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To compare two top-of-atmosphere radiances measured by instruments with different spectral characteristics, a transfer function has been developed. It is applied to a tandem data set of Sentinel-3A and B, for which OLCI-B mimicked the ESA’s eighth Earth Explorer FLEX. We found that OLCI-A measured radiances about 2 % brighter than OLCI-FLEX. Only at larger wavelengths were OLCI-A measurements about 5 % darker. The method is thus successful, being sensitive to calibration and processing issues.
Luis F. Millán, Gloria L. Manney, Harald Boenisch, Michaela I. Hegglin, Peter Hoor, Daniel Kunkel, Thierry Leblanc, Irina Petropavlovskikh, Kaley Walker, Krzysztof Wargan, and Andreas Zahn
Atmos. Meas. Tech., 16, 2957–2988, https://doi.org/10.5194/amt-16-2957-2023, https://doi.org/10.5194/amt-16-2957-2023, 2023
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The determination of atmospheric composition trends in the upper troposphere and lower stratosphere (UTLS) is still highly uncertain. We present the creation of dynamical diagnostics to map several ozone datasets (ozonesondes, lidars, aircraft, and satellite measurements) in geophysically based coordinate systems. The diagnostics can also be used to analyze other greenhouse gases relevant to surface climate and UTLS chemistry.
Zhihua Zhang, Jianguo Niu, Lawrence E. Flynn, Eric Beach, and Trevor Beck
Atmos. Meas. Tech., 16, 2919–2941, https://doi.org/10.5194/amt-16-2919-2023, https://doi.org/10.5194/amt-16-2919-2023, 2023
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This study mainly focused on addressing stability and improvement when using a broadband approach, establishing soft-calibration adjustments for both OMPS S-NPP and N20, analyzing error biases based on multi-sensor bias correction, and comparing total column ozone and aerosol index retrievals from NOAA OMPS with those from other products.
Matthew S. Johnson, Amir H. Souri, Sajeev Philip, Rajesh Kumar, Aaron Naeger, Jeffrey Geddes, Laura Judd, Scott Janz, Heesung Chong, and John Sullivan
Atmos. Meas. Tech., 16, 2431–2454, https://doi.org/10.5194/amt-16-2431-2023, https://doi.org/10.5194/amt-16-2431-2023, 2023
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Satellites provide vital information for studying the processes controlling ozone formation. Based on the abundance of particular gases in the atmosphere, ozone formation is sensitive to specific human-induced and natural emission sources. However, errors and biases in satellite retrievals hinder this data source’s application for studying ozone formation sensitivity. We conducted a thorough statistical evaluation of two commonly applied satellites for investigating ozone formation sensitivity.
Kezia Lange, Andreas Richter, Anja Schönhardt, Andreas C. Meier, Tim Bösch, André Seyler, Kai Krause, Lisa K. Behrens, Folkard Wittrock, Alexis Merlaud, Frederik Tack, Caroline Fayt, Martina M. Friedrich, Ermioni Dimitropoulou, Michel Van Roozendael, Vinod Kumar, Sebastian Donner, Steffen Dörner, Bianca Lauster, Maria Razi, Christian Borger, Katharina Uhlmannsiek, Thomas Wagner, Thomas Ruhtz, Henk Eskes, Birger Bohn, Daniel Santana Diaz, Nader Abuhassan, Dirk Schüttemeyer, and John P. Burrows
Atmos. Meas. Tech., 16, 1357–1389, https://doi.org/10.5194/amt-16-1357-2023, https://doi.org/10.5194/amt-16-1357-2023, 2023
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We present airborne imaging DOAS and ground-based stationary and car DOAS measurements conducted during the S5P-VAL-DE-Ruhr campaign in the Rhine-Ruhr region. The measurements are used to validate spaceborne NO2 data products from the Sentinel-5 Precursor TROPOspheric Monitoring Instrument (TROPOMI). Auxiliary data of the TROPOMI NO2 retrieval, such as spatially higher resolved a priori NO2 vertical profiles, surface reflectivity, and cloud treatment are investigated to evaluate their impact.
Yolanda Maria Lemes, Christoph Häni, Jesper Nørlem Kamp, and Anders Feilberg
Atmos. Meas. Tech., 16, 1295–1309, https://doi.org/10.5194/amt-16-1295-2023, https://doi.org/10.5194/amt-16-1295-2023, 2023
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The implementation of a new method, line-averaged concentration measurement with a closed-path analyzer, will enable the measurement of fluxes of multiple gases from different types of sources and will evaluate the effects of mitigation strategies on emissions. In addition, this method allows for continuous online measurements that resolve temporal variation in ammonia emissions and the peak emissions of methane.
Prajjwal Rawat, Manish Naja, Evan Fishbein, Pradeep K. Thapliyal, Rajesh Kumar, Piyush Bhardwaj, Aditya Jaiswal, Sugriva N. Tiwari, Sethuraman Venkataramani, and Shyam Lal
Atmos. Meas. Tech., 16, 889–909, https://doi.org/10.5194/amt-16-889-2023, https://doi.org/10.5194/amt-16-889-2023, 2023
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Satellite-based ozone observations have gained importance due to their global coverage. However, satellite-retrieved products are indirect and need to be validated, particularly over mountains. Ozonesondes launched from a Himalayan site are used to assess the Atmospheric Infrared Sounder (AIRS) ozone retrieval. AIRS is shown to overestimate ozone in the upper troposphere and lower stratosphere, while the differences from ozonesondes are more minor in the middle troposphere and stratosphere.
Murali Natarajan, Robert Damadeo, and David Flittner
Atmos. Meas. Tech., 16, 75–87, https://doi.org/10.5194/amt-16-75-2023, https://doi.org/10.5194/amt-16-75-2023, 2023
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Photochemically induced changes in mesospheric O3 concentration at twilight can cause asymmetry in the distribution along the line of sight of solar occultation observations that must be considered in the retrieval algorithm. Correction factors developed from diurnal photochemical model simulations were used to modify the archived SAGE III/ISS mesospheric O3 concentrations. For June 2021 the bias caused by the neglect of diurnal variations is over 30% at 64 km altitude and low latitudes.
Javier Gorroño, Daniel J. Varon, Itziar Irakulis-Loitxate, and Luis Guanter
Atmos. Meas. Tech., 16, 89–107, https://doi.org/10.5194/amt-16-89-2023, https://doi.org/10.5194/amt-16-89-2023, 2023
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We present a methane flux rate retrieval methodology using the Sentinel-2 mission, validating the algorithm for different scenes and plumes. The detection limit is 1000–2000 kg h−1 for homogeneous scenes and temporally invariant surfaces and above 5000 kg h−1 for heterogeneous ones. Dominant quantification errors are wind-related or plume mask-related. For heterogeneous scenes, the surface structure underlying the methane plume can become a dominant source of uncertainty.
Katerina Garane, Ka Lok Chan, Maria-Elissavet Koukouli, Diego Loyola, and Dimitris Balis
Atmos. Meas. Tech., 16, 57–74, https://doi.org/10.5194/amt-16-57-2023, https://doi.org/10.5194/amt-16-57-2023, 2023
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In this work, 2.5 years of TROPOMI/S5P Total Column Water Vapor (TCWV) observations retrieved from the blue wavelength band are validated against co-located precipitable water measurements from NASA AERONET, which uses Cimel Sun photometers globally. Overall, the TCWV product agrees well on a global scale with the ground-based dataset (Pearson correl. coefficient 0.909) and has a mean relative bias of −2.7 ± 4.9 % with respect to the AERONET observations for moderate albedo and cloudiness.
Lei Shi, Carl J. Schreck III, Viju O. John, Eui-Seok Chung, Theresa Lang, Stefan A. Buehler, and Brian J. Soden
Atmos. Meas. Tech., 15, 6949–6963, https://doi.org/10.5194/amt-15-6949-2022, https://doi.org/10.5194/amt-15-6949-2022, 2022
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Four upper tropospheric humidity (UTH) datasets derived from satellite microwave and infrared sounders are evaluated to assess their consistency as part of the activities for the Global Energy and Water Exchanges (GEWEX) water vapor assessment project. The study shows that the four datasets are consistent in the interannual temporal and spatial variability of the tropics. However, differences are found in the magnitudes of the anomalies and in the changing rates during the common period.
Cited articles
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Short summary
UV backscatter limb sounding sensors have difficulty determining altitude registration to the accuracy needed for long-term ozone monitoring. We describe two methods to achieve this by comparing radiance measurements to models. Wavelengths and altitudes chosen minimize errors from aerosol interference, calibration errors, and ozone assumptions. The techniques are inexpensive, more comprehensive than external sources of attitude information, and track drifts in our altitude to better than 100 m.
UV backscatter limb sounding sensors have difficulty determining altitude registration to the...