Articles | Volume 7, issue 8
Atmos. Meas. Tech., 7, 2411–2420, 2014
https://doi.org/10.5194/amt-7-2411-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Special issue: Remote sensing of aerosols and clouds (EGU2012)
Research article 08 Aug 2014
Research article | 08 Aug 2014
Retrieval of aerosol optical depth over land surfaces from AVHRR data
L. L. Mei et al.
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Different approaches to retrieve the optical-equivalent snow grain size using satellite, airborne, and ground-based observations were evaluated and compared to modeled data. The study is focused on low Sun and partly rough surface conditions encountered North of Greenland in March/April 2018. We proposed an adjusted airborne retrieval method to reduce the retrieval uncertainty.
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This paper presents a new snow property retrieval algorithm from satellite observations. This is part 1 of the paper, which shows the method description and sensitivity study. The paper investigates the major impact factors, including the assumptions of snow optical properties and atmospheric conditions (cloud and aerosol) on snow properties retrievals from satellite observation.
Linlu Mei, Vladimir Rozanov, Evelyn Jäkel, Xiao Cheng, Marco Vountas, and John P. Burrows
The Cryosphere Discuss., https://doi.org/10.5194/tc-2020-270, https://doi.org/10.5194/tc-2020-270, 2020
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This paper presents a new snow property retrieval algorithm from satellite observations. This is part 2 of the paper, which shows the results and validation. The paper performs the new retrieval algorithm on the SLSTR instrument and compared the retrieved snow properties with ground-based measurements, aircraft measures, and other satellite products.
Soheila Jafariserajehlou, Linlu Mei, Marco Vountas, Vladimir Rozanov, John P. Burrows, and Rainer Hollmann
Atmos. Meas. Tech., 12, 1059–1076, https://doi.org/10.5194/amt-12-1059-2019, https://doi.org/10.5194/amt-12-1059-2019, 2019
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We developed a new algorithm for cloud identification over the Arctic. This algorithm called ASCIA, utilizes time-series measurements of Advanced Along-Track Scanning Radiometer (AATSR) on Envisat and Sea and Land Surface Temperature Radiometer (SLSTR) on Sentinel-3A and -3B.
The data product of ASCIA is compared with three satellite products: ASCIA shows an improved performance compared to them. We validated ASCIA by ground-based measurements and a promising agreement is achieved.
Linlu Mei, Vladimir Rozanov, Marco Vountas, John P. Burrows, and Andreas Richter
Atmos. Chem. Phys., 18, 2511–2523, https://doi.org/10.5194/acp-18-2511-2018, https://doi.org/10.5194/acp-18-2511-2018, 2018
Lily N. Zhang, Susan Solomon, Kane A. Stone, Jonathan D. Shanklin, Joshua D. Eveson, Steve Colwell, John P. Burrows, Mark Weber, Pieternel F. Levelt, Natalya A. Kramarova, and David P. Haffner
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-122, https://doi.org/10.5194/acp-2021-122, 2021
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In the 1980s, measurements at the British Antarctic Survey station in Halley, Antarctica led to the discovery of the ozone hole. The Halley total ozone record continues to be uniquely valuable for studies of long-term changes in Antarctic ozone. Environmental conditions in 2017 forced a temporary cessation of operations, leading to a gap in the historic record. We develop and test a method for filling in the Halley record using satellite data and find evidence to further support ozone recovery.
Jakob Borchardt, Konstantin Gerilowski, Sven Krautwurst, Heinrich Bovensmann, Andrew K. Thorpe, David R. Thompson, Christian Frankenberg, Charles E. Miller, Riley M. Duren, and John Philip Burrows
Atmos. Meas. Tech., 14, 1267–1291, https://doi.org/10.5194/amt-14-1267-2021, https://doi.org/10.5194/amt-14-1267-2021, 2021
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The AVIRIS-NG hyperspectral imager has been used successfully to identify and quantify anthropogenic methane sources utilizing different retrieval and inversion methods. Here, we examine the adaption and application of the WFM-DOAS algorithm to AVIRIS-NG measurements to retrieve local methane column enhancements, compare the results with other retrievals, and quantify the uncertainties resulting from the retrieval method. Additionally, we estimate emissions from five detected methane plumes.
Boming Liu, Jianping Guo, Wei Gong, Yong Zhang, Lijuan Shi, Yingying Ma, Jian Li, Xiaoran Guo, Ad Stoffelen, Gerrit de Leeuw, and Xiaofeng Xu
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-41, https://doi.org/10.5194/acp-2021-41, 2021
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Vertical wind profiles are crucial to a wide range of atmospheric disciplines. Aeolus is the first satellite mission to directly observe wind profile information on a global scale. However, Aeolus wind products over China were thus far not evaluated by in-situ comparison. This work is expected to let the public and science community better know the Aeolus wind products and to encourage use of these valuable data in future researches and applications.
Evelyn Jäkel, Tim Carlsen, André Ehrlich, Manfred Wendisch, Michael Schäfer, Sophie Rosenburg, Konstantina Nakoudi, Marco Zanatta, Gerit Birnbaum, Veit Helm, Andreas Herber, Larysa Istomina, Linlu Mei, and Anika Rohde
The Cryosphere Discuss., https://doi.org/10.5194/tc-2021-14, https://doi.org/10.5194/tc-2021-14, 2021
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Different approaches to retrieve the optical-equivalent snow grain size using satellite, airborne, and ground-based observations were evaluated and compared to modeled data. The study is focused on low Sun and partly rough surface conditions encountered North of Greenland in March/April 2018. We proposed an adjusted airborne retrieval method to reduce the retrieval uncertainty.
Yuqin Liu, Tao Lin, Juan Hong, Yonghong Wang, Lamei Shi, Yiyi Huang, Xian Wu, Hao Zhou, Jiahua Zhang, and Gerrit de Leeuw
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-1278, https://doi.org/10.5194/acp-2020-1278, 2021
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The 4-dimensional variation of aerosol properties over the BTH, YRD and PRD (east China) were investigated using satellite observations from 2007 to 2015. Distinct differences between the aerosol optical depth and the vertical distribution of the occurrence of aerosol types over these regions depend on season, aerosol loading and meteorological conditions. Day/night differences between the vertical distribution of aerosol types suggest effects of boundary layer dynamics and aerosol transport.
Soheila Jafariserajehlou, Vladimir V. Rozanov, Marco Vountas, Charles K. Gatebe, and John P. Burrows
Atmos. Meas. Tech., 14, 369–389, https://doi.org/10.5194/amt-14-369-2021, https://doi.org/10.5194/amt-14-369-2021, 2021
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In this work, we study retrieval of snow grain morphologies and their impact on the reflectance in a coupled snow–atmosphere system. We present a sensitivity study to highlight the importance of having adequate information about snow and atmosphere. A novel two-stage algorithm for retrieving the size and shape of snow grains is presented. The reflectance simulation results are compared to that of airborne measurements; high correlations of 0.98 at IR and 0.88–0.98 at VIS are achieved.
Maximilian Reuter, Heinrich Bovensmann, Michael Buchwitz, Jakob Borchardt, Sven Krautwurst, Konstantin Gerilowski, Matthias Lindauer, Dagmar Kubistin, and John P. Burrows
Atmos. Meas. Tech., 14, 153–172, https://doi.org/10.5194/amt-14-153-2021, https://doi.org/10.5194/amt-14-153-2021, 2021
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CO2 measurements from a small unmanned aircraft system (sUAS) can provide a cost-effective way to complement and validate satellite-based measurements of anthropogenic CO2 emissions. We introduce an sUAS which is capable of determining atmospheric CO2 mass fluxes from its own sensor data. We show results of validation flights at the ICOS atmospheric station in Steinkimmen and from demonstration flights downwind a CO2-emitting natural gas processing facility.
Sven Krautwurst, Konstantin Gerilowski, Jakob Borchardt, Norman Wildmann, Michal Galkowski, Justyna Swolkien, Julia Marshall, Alina Fiehn, Anke Roiger, Thomas Ruhtz, Christoph Gerbig, Jaroslaw Necki, John P. Burrows, Andreas Fix, and Heinrich Bovensmann
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-1014, https://doi.org/10.5194/acp-2020-1014, 2021
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The study reports on observations from the passive airborne remote sensing instrument MAMAP, from which atmospheric CH4 column anomalies are retrieved to investigate CH4 emissions from coal mine shafts in Poland.
Emissions from small groups of shafts have successfully been computed from the anomalies and compared to inventory data. The comparison revealed that caution is required if inventory data is only available on an annual basis and that an exact source assignment requires 2D instruments.
Daniel Zawada, Ghislain Franssens, Robert Loughman, Antti Mikkonen, Alexei Rozanov, Claudia Emde, Adam Bourassa, Seth Dueck, Hannakaisa Lindqvist, Didier Ramon, Vladimir Rozanov, Emmanuel Dekemper, Erkki Kyrölä, John P. Burrows, Didier Fussen, and Doug Degenstein
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-470, https://doi.org/10.5194/amt-2020-470, 2021
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Satellite measurements of atmospheric composition often rely on computer tools known as radiative transfer models to model the propagation of sunlight within the atmosphere. Here we have performed a detailed inter-comparison of seven different radiative transfer models in a variety of conditions. We have found that the models agree remarkably well, at a level better than previously reported. This result provides confidence in our understanding of atmospheric radiative transfer.
Stefan Noël, Maximilian Reuter, Michael Buchwitz, Jakob Borchardt, Michael Hilker, Heinrich Bovensmann, John P. Burrows, Antonio Di Noia, Hiroshi Suto, Yukio Yoshida, Matthias Buschmann, Nicholas M. Deutscher, Dietrich G. Feist, David W. T. Griffith, Frank Hase, Rigel Kivi, Isamu Morino, Justus Notholt, Hirofumi Ohyama, Christof Petri, James R. Podolske, David F. Pollard, Mahesh Kumar Sha, Kei Shiomi, Ralf Sussmann, Yao Té, Voltaire A. Velazco, and Thorsten Warneke
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-453, https://doi.org/10.5194/amt-2020-453, 2020
Preprint under review for AMT
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We present first GOSAT and GOSAT-2 XCO2 data derived with the FOCAL retrieval algorithm.
Comparisons of the GOSAT FOCAL product with other data reveal a long-term agreement within about 1 ppm over one decade, differences in seasonal variations of about 0.5 ppm and a mean regional bias to ground based TCCON data of 0.56 ppm with a mean scatter of 1.89 ppm.
GOSAT-2 FOCAL data are considered to be preliminary only, but first comparisons show that they compare well with the GOSAT FOCAL results.
Nick Schutgens, Oleg Dubovik, Otto Hasekamp, Omar Torres, Hiren Jethva, Peter J. T. Leonard, Pavel Litvinov, Jens Redemann, Yohei Shinozuka, Gerrit de Leeuw, Stefan Kinne, Thomas Popp, Michael Schulz, and Philip Stier
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-1207, https://doi.org/10.5194/acp-2020-1207, 2020
Revised manuscript under review for ACP
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Absorptive aerosol has a potentially large impact on climate change. We evaluate and intercompare four global satellite datasets of Absorptive Aerosol Optical Depth (AAOD) and Single Scattering Albedo (SSA). We show that these datasets show reasonable correlations with the AERONET reference although significant biases remain. In a follow-up paper we show that these observations nevertheless can be used for model evaluation.
Viktoria F. Sofieva, Monika Szelag, Johanna Tamminen, Erkki Kyrölä, Doug Degenstein, Chris Roth, Daniel Zawada, Alexei Rozanov, Carlo Arosio, John P. Burrows, Mark Weber, Alexandra Laeng, Gabriele Stiller, Thomas von Clarmann, Lucien Froidevaux, Nathaniel Livesey, Michel van Roozendael, and Christian Retscher
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-1117, https://doi.org/10.5194/acp-2020-1117, 2020
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The MErged GRIdded Dataset of Ozone Profiles is the long-term (2001–2018) stratospheric ozone profile climate data record with the resolved longitudinal structure, which combines the data from six limb satellite instruments. The dataset can be used various analyses, some of them are discussed in the paper. In particular, regional and vertically resolved ozone trends are evaluated, including the trends in polar regions.
Cheng Fan, Zhengqiang Li, Ying Li, Jiantao Dong, Ronald van der A, and Gerrit de Leeuw
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-1101, https://doi.org/10.5194/acp-2020-1101, 2020
Revised manuscript under review for ACP
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Emission control policy in China has resulted in the decrease of nitrogen dioxide concentrations, which however leveled off and stabilized in recent years, as shown from Satellite data. The effects of the further emission reduction during the COVID-19 lockdown in 2020 resulted in an initial improvement of air quality, which however was offset by chemical and meteorological effects. The study shows regional dependence over east China and results have wider application than China only.
Ying Zhang, Zhengqiang Li, Yu Chen, Gerrit de Leeuw, Chi Zhang, Yisong Xie, and Kaitao Li
Atmos. Chem. Phys., 20, 12795–12811, https://doi.org/10.5194/acp-20-12795-2020, https://doi.org/10.5194/acp-20-12795-2020, 2020
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Observation of atmospheric aerosol components plays an important role in reducing uncertainty in climate assessment. In this study, an improved remote sensing method which can better distinguish scattering components is developed, and the aerosol components in the atmospheric column over China are retrieved based on the Sun–sky radiometer Observation NETwork (SONET). The component distribution shows there could be a sea salt component in northwest China from a paleomarine source in desert land.
Nick Schutgens, Andrew M. Sayer, Andreas Heckel, Christina Hsu, Hiren Jethva, Gerrit de Leeuw, Peter J. T. Leonard, Robert C. Levy, Antti Lipponen, Alexei Lyapustin, Peter North, Thomas Popp, Caroline Poulsen, Virginia Sawyer, Larisa Sogacheva, Gareth Thomas, Omar Torres, Yujie Wang, Stefan Kinne, Michael Schulz, and Philip Stier
Atmos. Chem. Phys., 20, 12431–12457, https://doi.org/10.5194/acp-20-12431-2020, https://doi.org/10.5194/acp-20-12431-2020, 2020
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We intercompare 14 different datasets of satellite observations of aerosol. Such measurements are challenging but also provide the best opportunity to globally observe an atmospheric component strongly related to air pollution and climate change. Our study shows that most datasets perform similarly well on a global scale but that locally errors can be quite different. We develop a technique to estimate satellite errors everywhere, even in the absence of surface reference data.
Sora Seo, Andreas Richter, Anne-Marlene Blechschmidt, Ilias Bougoudis, and John Philip Burrows
Atmos. Chem. Phys., 20, 12285–12312, https://doi.org/10.5194/acp-20-12285-2020, https://doi.org/10.5194/acp-20-12285-2020, 2020
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In this study, we present spatial distributions of occurrence frequency of enhanced total BrO column and various meteorological parameters affecting it in the Arctic and Antarctic sea ice regions by using 10 years of GOME-2 measurements and meteorological model data. Statistical analysis using the long-term dataset shows clear differences in the meteorological conditions between the mean field and the situation of enhanced total BrO columns in both polar sea ice regions.
Ilias Bougoudis, Anne-Marlene Blechschmidt, Andreas Richter, Sora Seo, John Philip Burrows, Nicolas Theys, and Annette Rinke
Atmos. Chem. Phys., 20, 11869–11892, https://doi.org/10.5194/acp-20-11869-2020, https://doi.org/10.5194/acp-20-11869-2020, 2020
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A 22-year (1996 to 2017) consistent Arctic tropospheric BrO dataset derived from four satellite remote sensing instruments is presented. An increase in tropospheric BrO VCDs over this period, and especially during polar springs, can be seen. Comparisons of tropospheric BrO VCDs with first-year sea ice reveal a moderate spatial and temporal correlation between the two, suggesting that the increase in first-year sea ice in the Arctic has an impact on tropospheric BrO abundancies.
Stefan Noël, Klaus Bramstedt, Alexei Rozanov, Elizaveta Malinina, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 13, 5643–5666, https://doi.org/10.5194/amt-13-5643-2020, https://doi.org/10.5194/amt-13-5643-2020, 2020
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A new approach to derive stratospheric aerosol extinction profiles from SCIAMACHY solar occultation measurements based on an onion-peeling method is presented. The resulting extinctions at 452, 525 and 750 nm compare well with other limb and occultation data from, e.g. SAGE and SCIAMACHY, but show small oscillating features which vanish in monthly anomalies. Major volcanic eruptions, polar stratospheric clouds and influences of the quasi-biennial oscillation can be identified in the time series.
Michael Buchwitz, Maximilian Reuter, Stefan Noël, Klaus Bramstedt, Oliver Schneising, Michael Hilker, Blanca Fuentes Andrade, Heinrich Bovensmann, John P. Burrows, Antonio Di Noia, Hartmut Boesch, Lianghai Wu, Jochen Landgraf, Ilse Aben, Christian Retscher, Christopher W. O’Dell, and David Crisp
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-386, https://doi.org/10.5194/amt-2020-386, 2020
Revised manuscript accepted for AMT
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The COVID-19 pandemic resulted in reduced anthropogenic carbon dioxide (CO2) emissions during 2020 in large parts of the world. We have used a small emsemble of satellite retrievals of column-averaged CO2 (XCO2) to find out if a regional-scale reduction of atmospheric CO2 can be detected from space. We focus on East China and show that it is challenging to reliably detect and to accurately quantify the emission reduction, which only results in regional XCO2 reductions of about 0.1–0.2 ppm.
Linlu Mei, Vladimir Rozanov, Christine Pohl, Marco Vountas, and John P. Burrows
The Cryosphere Discuss., https://doi.org/10.5194/tc-2020-269, https://doi.org/10.5194/tc-2020-269, 2020
Preprint under review for TC
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This paper presents a new snow property retrieval algorithm from satellite observations. This is part 1 of the paper, which shows the method description and sensitivity study. The paper investigates the major impact factors, including the assumptions of snow optical properties and atmospheric conditions (cloud and aerosol) on snow properties retrievals from satellite observation.
Linlu Mei, Vladimir Rozanov, Evelyn Jäkel, Xiao Cheng, Marco Vountas, and John P. Burrows
The Cryosphere Discuss., https://doi.org/10.5194/tc-2020-270, https://doi.org/10.5194/tc-2020-270, 2020
Preprint under review for TC
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This paper presents a new snow property retrieval algorithm from satellite observations. This is part 2 of the paper, which shows the results and validation. The paper performs the new retrieval algorithm on the SLSTR instrument and compared the retrieved snow properties with ground-based measurements, aircraft measures, and other satellite products.
Hirofumi Ohyama, Isamu Morino, Voltaire A. Velazco, Theresa Klausner, Gerry Bagtasa, Matthäus Kiel, Matthias Frey, Akihiro Hori, Osamu Uchino, Tsuneo Matsunaga, Nicholas M. Deutscher, Joshua P. DiGangi, Yonghoon Choi, Glenn S. Diskin, Sally E. Pusede, Alina Fiehn, Anke Roiger, Michael Lichtenstern, Hans Schlager, Pao K. Wang, Charles C.-K. Chou, Maria Dolores Andrés-Hernández, and John P. Burrows
Atmos. Meas. Tech., 13, 5149–5163, https://doi.org/10.5194/amt-13-5149-2020, https://doi.org/10.5194/amt-13-5149-2020, 2020
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Column-averaged dry-air mole fractions of CO2 and CH4 measured by a solar viewing portable Fourier transform spectrometer (EM27/SUN) were validated with in situ profile data obtained during the transfer flights of two aircraft campaigns. Atmospheric dynamical properties based on ERA5 and WRF-Chem were used as criteria for selecting the best aircraft profiles for the validation. The resulting air-mass-independent correction factors for the EM27/SUN data were 0.9878 for CO2 and 0.9829 for CH4.
Jianping Guo, Boming Liu, Wei Gong, Lijuan Shi, Yong Zhang, Yingying Ma, Jian Zhang, Tianmeng Chen, Kaixu Bai, Ad Stoffelen, Gerrit de Leeuw, and Xiaofeng Xu
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-869, https://doi.org/10.5194/acp-2020-869, 2020
Revised manuscript accepted for ACP
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Vertical wind profiles are crucial to a wide range of atmospheric disciplines. Aeolus is the first satellite mission to directly observe wind profile information on a global scale. However, Aeolus wind products over China were thus far not evaluated by in-situ comparison. This work is expected to let the public and science community better know the Aeolus wind products and to encourage use of these valuable data in future researches and applications.
Elizaveta Malinina, Alexei Rozanov, Ulrike Niemeier, Sandra Peglow, Carlo Arosio, Felix Wrana, Claudia Timmreck, Christian von Savigny, and John P. Burrows
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-749, https://doi.org/10.5194/acp-2020-749, 2020
Preprint under review for ACP
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In the paper, changes in the stratospheric aerosol loading after the 2018 Ambae eruption were analyzed using OMPS-LP observations. The eruption was also simulated with MECHAM-HAM global climate model. Generally, the model and observations agree very well. We attribute good consistency of the results with precisely determined altitude and mass of the volcanic injection as well as with nudging of meteorological data. The radiative forcing from the eruption was estimated to be −0.13 W/m2.
Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Steffen Vanselow, Heinrich Bovensmann, and John P. Burrows
Atmos. Chem. Phys., 20, 9169–9182, https://doi.org/10.5194/acp-20-9169-2020, https://doi.org/10.5194/acp-20-9169-2020, 2020
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The switch from the use of coal to natural gas or oil for energy generation potentially reduces the impact on global warming due to lower CO2 emissions with the same energy content. However, this climate benefit is offset by fugitive methane emissions during the production and distribution process. We quantify emission and leakage rates relative to production for several large production regions based on satellite observations to evaluate the climate footprint of the gas and oil industry.
Tina Hilbig, Klaus Bramstedt, Mark Weber, John P. Burrows, and Matthijs Krijger
Atmos. Meas. Tech., 13, 3893–3907, https://doi.org/10.5194/amt-13-3893-2020, https://doi.org/10.5194/amt-13-3893-2020, 2020
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One of the main limitations for long-term space-based measurements is
instrument degradation. We present an optimisation of the
degradation correction approach (Krijger et al. 2014) for SCIAMACHY
on-board Envisat, focusing on the improvement of the solar spectral
irradiance data. The main achievement of this study is the
successful integration of SCIAMACHY’s internal white light source
(WLS) into the existing degradation model and the
characterisation of WLS ageing in space.
Steven Compernolle, Tijl Verhoelst, Gaia Pinardi, José Granville, Daan Hubert, Arno Keppens, Sander Niemeijer, Bruno Rino, Alkis Bais, Steffen Beirle, Folkert Boersma, John P. Burrows, Isabelle De Smedt, Henk Eskes, Florence Goutail, François Hendrick, Alba Lorente, Andrea Pazmino, Ankie Piters, Enno Peters, Jean-Pierre Pommereau, Julia Remmers, Andreas Richter, Jos van Geffen, Michel Van Roozendael, Thomas Wagner, and Jean-Christopher Lambert
Atmos. Chem. Phys., 20, 8017–8045, https://doi.org/10.5194/acp-20-8017-2020, https://doi.org/10.5194/acp-20-8017-2020, 2020
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Tropospheric and stratospheric NO2 columns from the OMI QA4ECV NO2 satellite product are validated by comparison with ground-based measurements at 11 sites. The OMI stratospheric column has a small negative bias, and the OMI tropospheric column has a stronger negative bias relative to the ground-based data. Discrepancies are attributed to comparison errors (e.g. difference in horizontal smoothing) and measurement errors (e.g. clouds, aerosols, vertical smoothing and a priori profile assumptions).
Margit Aun, Kaisa Lakkala, Ricardo Sanchez, Eija Asmi, Fernando Nollas, Outi Meinander, Larisa Sogacheva, Veerle De Bock, Antti Arola, Gerrit de Leeuw, Veijo Aaltonen, David Bolsée, Klara Cizkova, Alexander Mangold, Ladislav Metelka, Erko Jakobson, Tove Svendby, Didier Gillotay, and Bert Van Opstal
Atmos. Chem. Phys., 20, 6037–6054, https://doi.org/10.5194/acp-20-6037-2020, https://doi.org/10.5194/acp-20-6037-2020, 2020
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In 2017, new measurements of UV radiation started in Marambio, Antarctica, by the Finnish Meteorological Institute in collaboration with the Argentinian Servicio Meteorológico Nacional. The paper presents the results of UV irradiance measurements from March 2017 to March 2019, and it
compares them with those from 2000–2008 and also with UV measurements at other Antarctic stations. In 2017/2018, below average UV radiation levels were recorded due to favourable ozone and cloud conditions.
Midhun George, Maria Dolores Andrés Hernández, Vladyslav Nenakhov, Yangzhuoran Liu, and John Philip Burrows
Atmos. Meas. Tech., 13, 2577–2600, https://doi.org/10.5194/amt-13-2577-2020, https://doi.org/10.5194/amt-13-2577-2020, 2020
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The accurate measurement of peroxy radicals is essential for understanding the chemistry of air masses probed in the free troposphere. The PeRCEAS instrument has been designed, developed and thoroughly characterised for the measurement of the total sum of peroxy radicals (RO2*) aboard airborne platforms. Parameters expected to affect the precision and accuracy of the measurement have been investigated in detail.
Kaisa Lakkala, Margit Aun, Ricardo Sanchez, Germar Bernhard, Eija Asmi, Outi Meinander, Fernando Nollas, Gregor Hülsen, Tomi Karppinen, Veijo Aaltonen, Antti Arola, and Gerrit de Leeuw
Earth Syst. Sci. Data, 12, 947–960, https://doi.org/10.5194/essd-12-947-2020, https://doi.org/10.5194/essd-12-947-2020, 2020
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A GUV multi-filter radiometer was set up at Marambio, 64° S, 56° W, Antarctica, in 2017. The instrument continuously measures ultraviolet (UV) radiation, visible (VIS) radiation and photosynthetically active radiation (PAR). The measurements are designed for providing high-quality long-term time series that can be used to assess the impact of global climate change in the Antarctic region. The data from the last 5 d are plotted and updated daily.
Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Heinrich Bovensmann, and John P. Burrows
Atmos. Chem. Phys., 20, 3317–3332, https://doi.org/10.5194/acp-20-3317-2020, https://doi.org/10.5194/acp-20-3317-2020, 2020
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As a consequence of climate change, droughts in California are occurring more often, providing ample fuel for destructive wildfires. The associated smoke is reducing air quality as it contains pollutants considered harmful to public health and the environment such as carbon monoxide (CO). We analyse the statewide distribution of CO during the first days of two specific wildfires using satellite measurements and assess the corresponding air quality burden in major Californian cities.
Anne-Marlene Blechschmidt, Joaquim Arteta, Adriana Coman, Lyana Curier, Henk Eskes, Gilles Foret, Clio Gielen, Francois Hendrick, Virginie Marécal, Frédérik Meleux, Jonathan Parmentier, Enno Peters, Gaia Pinardi, Ankie J. M. Piters, Matthieu Plu, Andreas Richter, Arjo Segers, Mikhail Sofiev, Álvaro M. Valdebenito, Michel Van Roozendael, Julius Vira, Tim Vlemmix, and John P. Burrows
Atmos. Chem. Phys., 20, 2795–2823, https://doi.org/10.5194/acp-20-2795-2020, https://doi.org/10.5194/acp-20-2795-2020, 2020
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MAX-DOAS tropospheric NO2 vertical column retrievals from a set of European measurement stations are compared to regional air quality models which contribute to the operational Copernicus Atmosphere Monitoring Service (CAMS). Correlations are on the order of 35 %–75 %; large differences occur for individual pollution plumes. The results demonstrate that future model development needs to concentrate on improving representation of diurnal cycles and associated temporal scalings.
Leonardo M. A. Alvarado, Andreas Richter, Mihalis Vrekoussis, Andreas Hilboll, Anna B. Kalisz Hedegaard, Oliver Schneising, and John P. Burrows
Atmos. Chem. Phys., 20, 2057–2072, https://doi.org/10.5194/acp-20-2057-2020, https://doi.org/10.5194/acp-20-2057-2020, 2020
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We present CHOCHO and HCHO columns retrieved from measurements by TROPOMI. Elevated amounts of CHOCHO and HCHO are observed during the fire season in BC, Canada, where a large number of fires occurred in 2018. CHOCHO and HCHO plumes from individual fires are observed in air masses travelling over distances of up to 1500 km. Comparison with FLEXPART simulations with different lifetimes shows that effective lifetimes of 20 h and more are needed to explain the observations.
Larisa Sogacheva, Thomas Popp, Andrew M. Sayer, Oleg Dubovik, Michael J. Garay, Andreas Heckel, N. Christina Hsu, Hiren Jethva, Ralph A. Kahn, Pekka Kolmonen, Miriam Kosmale, Gerrit de Leeuw, Robert C. Levy, Pavel Litvinov, Alexei Lyapustin, Peter North, Omar Torres, and Antti Arola
Atmos. Chem. Phys., 20, 2031–2056, https://doi.org/10.5194/acp-20-2031-2020, https://doi.org/10.5194/acp-20-2031-2020, 2020
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The typical lifetime of a single satellite platform is on the order of 5–15 years; thus, for climate studies the usage of multiple satellite sensors should be considered.
Here we introduce and evaluate a monthly AOD merged product and AOD global and regional time series for the period 1995–2017 created from 12 individual satellite AOD products, which provide a long-term perspective on AOD changes over different regions of the globe.
Maximilian Reuter, Michael Buchwitz, Oliver Schneising, Stefan Noël, Heinrich Bovensmann, John P. Burrows, Hartmut Boesch, Antonio Di Noia, Jasdeep Anand, Robert J. Parker, Peter Somkuti, Lianghai Wu, Otto P. Hasekamp, Ilse Aben, Akihiko Kuze, Hiroshi Suto, Kei Shiomi, Yukio Yoshida, Isamu Morino, David Crisp, Christopher W. O'Dell, Justus Notholt, Christof Petri, Thorsten Warneke, Voltaire A. Velazco, Nicholas M. Deutscher, David W. T. Griffith, Rigel Kivi, David F. Pollard, Frank Hase, Ralf Sussmann, Yao V. Té, Kimberly Strong, Sébastien Roche, Mahesh K. Sha, Martine De Mazière, Dietrich G. Feist, Laura T. Iraci, Coleen M. Roehl, Christian Retscher, and Dinand Schepers
Atmos. Meas. Tech., 13, 789–819, https://doi.org/10.5194/amt-13-789-2020, https://doi.org/10.5194/amt-13-789-2020, 2020
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We present new satellite-derived data sets of atmospheric carbon dioxide (CO2) and methane (CH4). The data products are column-averaged dry-air mole fractions of CO2 and CH4, denoted XCO2 and XCH4. The products cover the years 2003–2018 and are merged Level 2 (satellite footprints) and merged Level 3 (gridded at monthly time and 5° x 5° spatial resolution) products obtained from combining several individual sensor products. We present the merging algorithms and product validation results.
Giulia Saponaro, Moa K. Sporre, David Neubauer, Harri Kokkola, Pekka Kolmonen, Larisa Sogacheva, Antti Arola, Gerrit de Leeuw, Inger H. H. Karset, Ari Laaksonen, and Ulrike Lohmann
Atmos. Chem. Phys., 20, 1607–1626, https://doi.org/10.5194/acp-20-1607-2020, https://doi.org/10.5194/acp-20-1607-2020, 2020
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The understanding of cloud processes is based on the quality of the representation of cloud properties. We compared cloud parameters from three models with satellite observations. We report on the performance of each data source, highlighting strengths and deficiencies, which should be considered when deriving the effect of aerosols on cloud properties.
Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Heinrich Bovensmann, John P. Burrows, Tobias Borsdorff, Nicholas M. Deutscher, Dietrich G. Feist, David W. T. Griffith, Frank Hase, Christian Hermans, Laura T. Iraci, Rigel Kivi, Jochen Landgraf, Isamu Morino, Justus Notholt, Christof Petri, David F. Pollard, Sébastien Roche, Kei Shiomi, Kimberly Strong, Ralf Sussmann, Voltaire A. Velazco, Thorsten Warneke, and Debra Wunch
Atmos. Meas. Tech., 12, 6771–6802, https://doi.org/10.5194/amt-12-6771-2019, https://doi.org/10.5194/amt-12-6771-2019, 2019
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We introduce an algorithm that is used to simultaneously derive the abundances of the important atmospheric constituents carbon monoxide and methane from the TROPOMI instrument onboard the Sentinel-5 Precursor satellite, which enables the determination of both gases with an unprecedented level of detail on a global scale. The quality of the resulting data sets is assessed and the first results are presented.
André Seyler, Andreas C. Meier, Folkard Wittrock, Lisa Kattner, Barbara Mathieu-Üffing, Enno Peters, Andreas Richter, Thomas Ruhtz, Anja Schönhardt, Stefan Schmolke, and John P. Burrows
Atmos. Meas. Tech., 12, 5959–5977, https://doi.org/10.5194/amt-12-5959-2019, https://doi.org/10.5194/amt-12-5959-2019, 2019
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This study describes a novel application of an
onion-peelingapproach to MAX-DOAS measurements of shipping emissions to study the inhomogeneous NO2 field above a shipping lane. It is shown how the method can be used to derive the approximate plume positions in the observed area, and, by using a simple Gaussian plume model, to calculate in-plume NO2 volume mixing ratios. For validation, a comparison to airborne imaging DOAS measurements during the NOSE campaign in July 2013 is included.
Lisa K. Behrens, Andreas Hilboll, Andreas Richter, Enno Peters, Leonardo M. A. Alvarado, Anna B. Kalisz Hedegaard, Folkard Wittrock, John P. Burrows, and Mihalis Vrekoussis
Atmos. Chem. Phys., 19, 10257–10278, https://doi.org/10.5194/acp-19-10257-2019, https://doi.org/10.5194/acp-19-10257-2019, 2019
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MAX-DOAS measurements were conducted on the research vessel Maria S. Merian during a cruise from the Azores to South Africa in October 2016. The measurements indicate enhanced levels of HCHO and CHOCHO over the remote Atlantic Ocean, which is unexpected due to their short lifetime. Precursors of these gases or gas–aerosol combinations might be transported. Model simulations indicate potential source regions over the African continent, probably related to biomass burning or biogenic emissions.
Enno Peters, Mareike Ostendorf, Tim Bösch, André Seyler, Anja Schönhardt, Stefan F. Schreier, Jeroen Sebastiaan Henzing, Folkard Wittrock, Andreas Richter, Mihalis Vrekoussis, and John P. Burrows
Atmos. Meas. Tech., 12, 4171–4190, https://doi.org/10.5194/amt-12-4171-2019, https://doi.org/10.5194/amt-12-4171-2019, 2019
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A novel imaging-DOAS instrument (IMPACT) is presented for measurements of nitrogen dioxide (NO2) in the atmosphere. The instrument combines full-azimuthal pointing (360°) with a large vertical coverage (40°). Complete panoramic scans and vertical NO2 profiles around the measurement site are acquired at a temporal resolution of 15 min. In addition, information about the aerosol phase function is retrieved from O4 slant columns along multiple almucantar scans measured simultaneously by IMPACT.
Yahui Che, Jie Guang, Gerrit de Leeuw, Yong Xue, Ling Sun, and Huizheng Che
Atmos. Meas. Tech., 12, 4091–4112, https://doi.org/10.5194/amt-12-4091-2019, https://doi.org/10.5194/amt-12-4091-2019, 2019
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The use of AOD data retrieved from ATSR-2, AATSR and AVHRR to produce a very long time series is investigated. The study is made over a small area in northern China with a large variation of AOD values. Sun photometer data from AERONET and CARSNET and radiance-derived AOD are used as reference. The results show that all data sets compare well. However, AVHRR underestimates high AOD (mainly occurring in summer) but performs better than (A)ATSR in winter.
Dan Weaver, Kimberly Strong, Kaley A. Walker, Chris Sioris, Matthias Schneider, C. Thomas McElroy, Holger Vömel, Michael Sommer, Katja Weigel, Alexei Rozanov, John P. Burrows, William G. Read, Evan Fishbein, and Gabriele Stiller
Atmos. Meas. Tech., 12, 4039–4063, https://doi.org/10.5194/amt-12-4039-2019, https://doi.org/10.5194/amt-12-4039-2019, 2019
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This work assesses water vapour profiles acquired by Atmospheric Chemistry Experiment (ACE) satellite instruments in the upper troposphere and lower stratosphere (UTLS) using comparisons to radiosondes and ground-based Fourier transform infrared spectrometer measurements acquired at a Canadian high Arctic measurement site in Eureka, Nunavut. Additional comparisons are made between these Eureka measurements and other water vapour satellite datasets for context, including AIRS, MLS, and others.
Maximilian Reuter, Michael Buchwitz, Oliver Schneising, Sven Krautwurst, Christopher W. O'Dell, Andreas Richter, Heinrich Bovensmann, and John P. Burrows
Atmos. Chem. Phys., 19, 9371–9383, https://doi.org/10.5194/acp-19-9371-2019, https://doi.org/10.5194/acp-19-9371-2019, 2019
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The quantification of anthropogenic emissions with current CO2 satellite sensors is difficult, but NO2 is co-emitted, making it a suitable tracer of recently emitted CO2. We analyze enhancements of CO2 and NO2 observed by OCO-2 and S5P and estimate the CO2 plume cross-sectional fluxes that we compare with emission databases. Our results demonstrate the usefulness of simultaneous satellite observations of CO2 and NO2 as envisaged for the European Copernicus anthropogenic CO2 monitoring mission
Hyeong-Ahn Kwon, Rokjin J. Park, Gonzalo González Abad, Kelly Chance, Thomas P. Kurosu, Jhoon Kim, Isabelle De Smedt, Michel Van Roozendael, Enno Peters, and John Burrows
Atmos. Meas. Tech., 12, 3551–3571, https://doi.org/10.5194/amt-12-3551-2019, https://doi.org/10.5194/amt-12-3551-2019, 2019
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The Geostationary Environment Monitoring Spectrometer (GEMS) will be launched by South Korea in 2019, and it will measure radiances ranging from 300 to 500 nm every hour with a fine spatial resolution of 7 km x 8 km over Seoul in South Korea to monitor column concentrations of air pollutants including O3, NO2, SO2, and HCHO, as well as aerosol optical properties. This paper describes a GEMS formaldehyde retrieval algorithm including a number of sensitivity tests for algorithm evaluation.
Elizaveta Malinina, Alexei Rozanov, Landon Rieger, Adam Bourassa, Heinrich Bovensmann, John P. Burrows, and Doug Degenstein
Atmos. Meas. Tech., 12, 3485–3502, https://doi.org/10.5194/amt-12-3485-2019, https://doi.org/10.5194/amt-12-3485-2019, 2019
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This paper covers the problems related to the derivation of aerosol extinction coefficients and Ångström exponents from space-borne instruments working in limb and occultation viewing geometries. Aerosol extinction coefficients and Ångström exponents were calculated from the SCIAMACHY aerosol particle size data set. The results were compared with the data from SAGE II and OSIRIS. The Ångström exponent in the tropical regions and its dependency on particle size parameters are discussed.
Sora Seo, Andreas Richter, Anne-Marlene Blechschmidt, Ilias Bougoudis, and John Philip Burrows
Atmos. Meas. Tech., 12, 2913–2932, https://doi.org/10.5194/amt-12-2913-2019, https://doi.org/10.5194/amt-12-2913-2019, 2019
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TROPOMI on board the Copernicus Sentinel-5 Precursor platform can measure various atmospheric compositions at high spatial resolution and improved spectral resolution compared to its predecessors. Bromine monoxide (BrO) is one of the gases that can be derived from the measured radiances of TROPOMI using the differential optical absorption spectroscopy method. In this paper, we present the first retrieval results of BrO column amounts from TROPOMI observations on global and regional scales.
Stefan Lossow, Farahnaz Khosrawi, Michael Kiefer, Kaley A. Walker, Jean-Loup Bertaux, Laurent Blanot, James M. Russell, Ellis E. Remsberg, John C. Gille, Takafumi Sugita, Christopher E. Sioris, Bianca M. Dinelli, Enzo Papandrea, Piera Raspollini, Maya García-Comas, Gabriele P. Stiller, Thomas von Clarmann, Anu Dudhia, William G. Read, Gerald E. Nedoluha, Robert P. Damadeo, Joseph M. Zawodny, Katja Weigel, Alexei Rozanov, Faiza Azam, Klaus Bramstedt, Stefan Noël, John P. Burrows, Hideo Sagawa, Yasuko Kasai, Joachim Urban, Patrick Eriksson, Donal P. Murtagh, Mark E. Hervig, Charlotta Högberg, Dale F. Hurst, and Karen H. Rosenlof
Atmos. Meas. Tech., 12, 2693–2732, https://doi.org/10.5194/amt-12-2693-2019, https://doi.org/10.5194/amt-12-2693-2019, 2019
Stefan F. Schreier, Andreas Richter, and John P. Burrows
Atmos. Chem. Phys., 19, 5853–5879, https://doi.org/10.5194/acp-19-5853-2019, https://doi.org/10.5194/acp-19-5853-2019, 2019
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In this case stuy, we have coupled ground-based remote-sensing measurements with surface in situ measurements to investigate NO2 distributions in the planetary boundary layer in the Viennese metropolitan area. We find that the application of a novel linear regression analysis for the conversion of tropospheric NO2 vertical columns into near-surface NO2 mixing ratios is promising and thus the method needs to be further explored and tested on satellite observations in future studies.
Carlo Arosio, Alexei Rozanov, Elizaveta Malinina, Mark Weber, and John P. Burrows
Atmos. Meas. Tech., 12, 2423–2444, https://doi.org/10.5194/amt-12-2423-2019, https://doi.org/10.5194/amt-12-2423-2019, 2019
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The aim of this study is the merging of stratospheric ozone profiles from three satellite data sets. The merged time series is used to compute long-term changes as a function of altitude, latitude and longitude to study the evolution of the ozone layer over 1985–2018. During the last 16 years we found positive trends in the upper stratosphere at mid latitudes, a large variability of the ozone changes as a function of longitude and a fluctuation in the tropical middle stratospheric trend.
Soheila Jafariserajehlou, Linlu Mei, Marco Vountas, Vladimir Rozanov, John P. Burrows, and Rainer Hollmann
Atmos. Meas. Tech., 12, 1059–1076, https://doi.org/10.5194/amt-12-1059-2019, https://doi.org/10.5194/amt-12-1059-2019, 2019
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We developed a new algorithm for cloud identification over the Arctic. This algorithm called ASCIA, utilizes time-series measurements of Advanced Along-Track Scanning Radiometer (AATSR) on Envisat and Sea and Land Surface Temperature Radiometer (SLSTR) on Sentinel-3A and -3B.
The data product of ASCIA is compared with three satellite products: ASCIA shows an improved performance compared to them. We validated ASCIA by ground-based measurements and a promising agreement is achieved.
Stefan Bender, Miriam Sinnhuber, Patrick J. Espy, and John P. Burrows
Atmos. Chem. Phys., 19, 2135–2147, https://doi.org/10.5194/acp-19-2135-2019, https://doi.org/10.5194/acp-19-2135-2019, 2019
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We present an empirical model for nitric oxide (NO) in the mesosphere (60–90 km) derived from SCIAMACHY limb scan data. Our model relates the daily (longitudinally) averaged NO number densities from SCIAMACHY as a function of geomagnetic latitude to the solar Lyman-alpha and the geomagnetic AE indices. We use a non-linear regression model, incorporating a finite and seasonally varying lifetime for the geomagnetically induced NO.
Michael Boy, Erik S. Thomson, Juan-C. Acosta Navarro, Olafur Arnalds, Ekaterina Batchvarova, Jaana Bäck, Frank Berninger, Merete Bilde, Zoé Brasseur, Pavla Dagsson-Waldhauserova, Dimitri Castarède, Maryam Dalirian, Gerrit de Leeuw, Monika Dragosics, Ella-Maria Duplissy, Jonathan Duplissy, Annica M. L. Ekman, Keyan Fang, Jean-Charles Gallet, Marianne Glasius, Sven-Erik Gryning, Henrik Grythe, Hans-Christen Hansson, Margareta Hansson, Elisabeth Isaksson, Trond Iversen, Ingibjorg Jonsdottir, Ville Kasurinen, Alf Kirkevåg, Atte Korhola, Radovan Krejci, Jon Egill Kristjansson, Hanna K. Lappalainen, Antti Lauri, Matti Leppäranta, Heikki Lihavainen, Risto Makkonen, Andreas Massling, Outi Meinander, E. Douglas Nilsson, Haraldur Olafsson, Jan B. C. Pettersson, Nønne L. Prisle, Ilona Riipinen, Pontus Roldin, Meri Ruppel, Matthew Salter, Maria Sand, Øyvind Seland, Heikki Seppä, Henrik Skov, Joana Soares, Andreas Stohl, Johan Ström, Jonas Svensson, Erik Swietlicki, Ksenia Tabakova, Throstur Thorsteinsson, Aki Virkkula, Gesa A. Weyhenmeyer, Yusheng Wu, Paul Zieger, and Markku Kulmala
Atmos. Chem. Phys., 19, 2015–2061, https://doi.org/10.5194/acp-19-2015-2019, https://doi.org/10.5194/acp-19-2015-2019, 2019
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The Nordic Centre of Excellence CRAICC (Cryosphere–Atmosphere Interactions in a Changing Arctic Climate), funded by NordForsk in the years 2011–2016, is the largest joint Nordic research and innovation initiative to date and aimed to strengthen research and innovation regarding climate change issues in the Nordic region. The paper presents an overview of the main scientific topics investigated and provides a state-of-the-art comprehensive summary of what has been achieved in CRAICC.
Evgenia Galytska, Alexey Rozanov, Martyn P. Chipperfield, Sandip. S. Dhomse, Mark Weber, Carlo Arosio, Wuhu Feng, and John P. Burrows
Atmos. Chem. Phys., 19, 767–783, https://doi.org/10.5194/acp-19-767-2019, https://doi.org/10.5194/acp-19-767-2019, 2019
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In this study we analysed ozone changes in the tropical mid-stratosphere as observed by the SCIAMACHY instrument during 2004–2012. We used simulations from TOMCAT model with different chemical and dynamical forcings to reveal primary causes of ozone changes. We also considered measured NO2 and modelled NOx, NOx, and N2O data. With modelled AoA data we identified seasonal changes in the upwelling speed and explained how those changes affect N2O chemistry which leads to observed ozone changes.
Yuqin Liu, Jiahua Zhang, Putian Zhou, Tao Lin, Juan Hong, Lamei Shi, Fengmei Yao, Jun Wu, Huadong Guo, and Gerrit de Leeuw
Atmos. Chem. Phys., 18, 18187–18202, https://doi.org/10.5194/acp-18-18187-2018, https://doi.org/10.5194/acp-18-18187-2018, 2018
Tim Bösch, Vladimir Rozanov, Andreas Richter, Enno Peters, Alexei Rozanov, Folkard Wittrock, Alexis Merlaud, Johannes Lampel, Stefan Schmitt, Marijn de Haij, Stijn Berkhout, Bas Henzing, Arnoud Apituley, Mirjam den Hoed, Jan Vonk, Martin Tiefengraber, Moritz Müller, and John Philip Burrows
Atmos. Meas. Tech., 11, 6833–6859, https://doi.org/10.5194/amt-11-6833-2018, https://doi.org/10.5194/amt-11-6833-2018, 2018
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A new MAX-DOAS profiling algorithm for aerosols and trace
gases was developed.
The performance of this novel algorithm was tested with the help of
synthetic data and measurements from the CINDI-2 campaign in Cabauw, the
Netherlands, in 2016.
Michael Buchwitz, Maximilian Reuter, Oliver Schneising, Stefan Noël, Bettina Gier, Heinrich Bovensmann, John P. Burrows, Hartmut Boesch, Jasdeep Anand, Robert J. Parker, Peter Somkuti, Rob G. Detmers, Otto P. Hasekamp, Ilse Aben, André Butz, Akihiko Kuze, Hiroshi Suto, Yukio Yoshida, David Crisp, and Christopher O'Dell
Atmos. Chem. Phys., 18, 17355–17370, https://doi.org/10.5194/acp-18-17355-2018, https://doi.org/10.5194/acp-18-17355-2018, 2018
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We present a new satellite data set of column-averaged mixing ratios of carbon dioxide (CO2), which covers the time period 2003 to 2016. We used this data set to compute annual mean atmospheric CO2 growth rates. We show that the growth rate is highest during 2015 and 2016 despite nearly constant CO2 emissions from fossil fuel burning in recent years. The high growth rates are attributed to year 2015-2016 El Nino episodes. We present correlations with fossil fuel emissions and ENSO indices.
Lu She, Yong Xue, Jie Guang, Yahui Che, Cheng Fan, Ying Li, and Yanqing Xie
Nat. Hazards Earth Syst. Sci., 18, 3187–3201, https://doi.org/10.5194/nhess-18-3187-2018, https://doi.org/10.5194/nhess-18-3187-2018, 2018
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Multi-satellite/sensor observations and ground-based measurements combined with the HYSPLIT model were used to analyse the dynamical processes of the origin and transport of a strong dust storm. The optical and microphysical properties of the dust particles were analysed using AERONET measurements. The combined observations revealed comprehensive information about the dynamic transport of dust and the dust-affected regions, and the effect of dust storms on the aerosol properties.
Larisa Sogacheva, Edith Rodriguez, Pekka Kolmonen, Timo H. Virtanen, Giulia Saponaro, Gerrit de Leeuw, Aristeidis K. Georgoulias, Georgia Alexandri, Konstantinos Kourtidis, and Ronald J. van der A
Atmos. Chem. Phys., 18, 16631–16652, https://doi.org/10.5194/acp-18-16631-2018, https://doi.org/10.5194/acp-18-16631-2018, 2018
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Understanding long-term trends in aerosol optical density (AOD) is essential for evaluating health and climate effects and the effectiveness of pollution control policies. A method to construct a combined AOD long time series (1995-2017) using ATSR and MODIS spaceborne instruments is introduced. The effect of changes in the emission regulation policy in China is seen in a gradual AOD decrease after 2011. The effect is more visible in highly populated and industrialized areas in southeast China.
Kaisa Lakkala, Alberto Redondas, Outi Meinander, Laura Thölix, Britta Hamari, Antonio Fernando Almansa, Virgilio Carreno, Rosa Delia García, Carlos Torres, Guillermo Deferrari, Hector Ochoa, Germar Bernhard, Ricardo Sanchez, and Gerrit de Leeuw
Atmos. Chem. Phys., 18, 16019–16031, https://doi.org/10.5194/acp-18-16019-2018, https://doi.org/10.5194/acp-18-16019-2018, 2018
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Solar UV irradiances were measured at Ushuaia (54° S) and Marambio (64° S) during 2000–2013. The measurements were part of the Antarctic NILU-UV network, which was maintained as a cooperation between Spain, Argentina and Finland. The time series of the network were analysed for the first time in this study. At both stations maximum UV indices and daily doses were measured when spring-time ozone loss episodes occurred. The maximum UV index was 13 and 12 in Ushuaia and Marambio, respectively.
Larisa Sogacheva, Gerrit de Leeuw, Edith Rodriguez, Pekka Kolmonen, Aristeidis K. Georgoulias, Georgia Alexandri, Konstantinos Kourtidis, Emmanouil Proestakis, Eleni Marinou, Vassilis Amiridis, Yong Xue, and Ronald J. van der A
Atmos. Chem. Phys., 18, 11389–11407, https://doi.org/10.5194/acp-18-11389-2018, https://doi.org/10.5194/acp-18-11389-2018, 2018
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Using AATSR ADV (1995–2011) and MODIS C6.1 (2000–2017) annual and seasonal aerosol optical depth (AOD) aggregates, we obtained information regarding the occurrence of aerosols and their spatial and temporal variation over China. We specifically focused on regional differences in annual and seasonal AOD behavior for selected regions. AOD dataset comparisons, validation results and AOD tendencies during the overlapping period (2000–2011) are discussed.
Farahnaz Khosrawi, Stefan Lossow, Gabriele P. Stiller, Karen H. Rosenlof, Joachim Urban, John P. Burrows, Robert P. Damadeo, Patrick Eriksson, Maya García-Comas, John C. Gille, Yasuko Kasai, Michael Kiefer, Gerald E. Nedoluha, Stefan Noël, Piera Raspollini, William G. Read, Alexei Rozanov, Christopher E. Sioris, Kaley A. Walker, and Katja Weigel
Atmos. Meas. Tech., 11, 4435–4463, https://doi.org/10.5194/amt-11-4435-2018, https://doi.org/10.5194/amt-11-4435-2018, 2018
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Time series of stratospheric and lower mesospheric water vapour using 33 data sets from 15 satellite instruments were compared in the framework of the second SPARC water vapour assessment. We find that most data sets can be considered in observational and modelling studies addressing, e.g. stratospheric and lower mesospheric water vapour variability and trends if data-set-specific characteristics (e.g. a drift) and restrictions (e.g. temporal and spatial coverage) are taken into account.
Alexander Kokhanovsky, Maxim Lamare, Biagio Di Mauro, Ghislain Picard, Laurent Arnaud, Marie Dumont, François Tuzet, Carsten Brockmann, and Jason E. Box
The Cryosphere, 12, 2371–2382, https://doi.org/10.5194/tc-12-2371-2018, https://doi.org/10.5194/tc-12-2371-2018, 2018
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This work presents a new technique with which to derive the snow microphysical and optical properties from snow spectral reflectance measurements. The technique is robust and easy to use, and it does not require the extraction of snow samples from a given snowpack. It can be used in processing satellite imagery over extended fresh dry, wet and polluted snowfields.
Landon A. Rieger, Elizaveta P. Malinina, Alexei V. Rozanov, John P. Burrows, Adam E. Bourassa, and Doug A. Degenstein
Atmos. Meas. Tech., 11, 3433–3445, https://doi.org/10.5194/amt-11-3433-2018, https://doi.org/10.5194/amt-11-3433-2018, 2018
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This paper compares aerosol extinction records from two limb scattering instruments, OSIRIS and SCIAMACHY, to that from the occultation instrument SAGE II. Differences are investigated through modelling and retrieval studies and important sources of systematic errors are quantified. It is found that the largest biases come from uncertainties in the aerosol size distribution and the aerosol particle concentration at altitudes above 30 km.
Stephen Broccardo, Klaus-Peter Heue, David Walter, Christian Meyer, Alexander Kokhanovsky, Ronald van der A, Stuart Piketh, Kristy Langerman, and Ulrich Platt
Atmos. Meas. Tech., 11, 2797–2819, https://doi.org/10.5194/amt-11-2797-2018, https://doi.org/10.5194/amt-11-2797-2018, 2018
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Measurements of nitrogen dioxide, known to originate from industrial and automotive combustion sources, have been made from space for two decades. Successive generations of instrument bring improvements in ground-pixel resolution; however features in the atmosphere are known to be smaller than what the satellites can resolve. Measurements of urban and industrial areas using a high-resolution airborne instrument allow the impact of the satellite's relatively low resolution to be evaluated.
Lisa K. Behrens, Andreas Hilboll, Andreas Richter, Enno Peters, Henk Eskes, and John P. Burrows
Atmos. Meas. Tech., 11, 2769–2795, https://doi.org/10.5194/amt-11-2769-2018, https://doi.org/10.5194/amt-11-2769-2018, 2018
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We developed a novel NO2 DOAS retrieval for the GOME-2A instrument in the UV spectral range, which is compared with a NO2 retrieval in the visible and model values. Regions representative for both anthropogenic and biomass burning NO2 pollution are investigated. Anthropogenic air pollution is mostly located in the boundary layer close to the surface. In contrast, biomass burning NO2 is often uplifted into elevated layers.
Carlo Arosio, Alexei Rozanov, Elizaveta Malinina, Kai-Uwe Eichmann, Thomas von Clarmann, and John P. Burrows
Atmos. Meas. Tech., 11, 2135–2149, https://doi.org/10.5194/amt-11-2135-2018, https://doi.org/10.5194/amt-11-2135-2018, 2018
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This paper describes the development of a retrieval algorithm at the University of Bremen which derives stratospheric ozone profiles from limb observations performed by the OMPS satellite instrument. Here we present the implementation of the algorithm and the validation of our results (1 year of data against independent satellite and ground-based measurements). Good agreement is generally found between 20 and 55 km, mostly within 10 % at all latitudes.
Evgenia Galytska, Vassyl Danylevsky, René Hommel, and John P. Burrows
Atmos. Meas. Tech., 11, 2101–2118, https://doi.org/10.5194/amt-11-2101-2018, https://doi.org/10.5194/amt-11-2101-2018, 2018
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This research assesses the influence of biomass burning during forest fires throughout summer 2010 on aerosol load over Ukraine, the European territory of Russia (ETR) and Eastern Europe. We apply and compare ground-based and satellite measurements to determine aerosol content, dynamics, and properties. With the application of modeling techniques (HYSPLIT), we show that the maximum AOD in August 2010 over Ukraine was caused by particle transport from the forest fires in the ETR.
Elizaveta Malinina, Alexei Rozanov, Vladimir Rozanov, Patricia Liebing, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 11, 2085–2100, https://doi.org/10.5194/amt-11-2085-2018, https://doi.org/10.5194/amt-11-2085-2018, 2018
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Stratospheric aerosols play an important role in climate change. This paper presents the retrieval algorithm of two aerosol particle size distribution parameters in the stratosphere from remote sensing instruments. A unique data set was created by implementing this algorithm on SCIAMACHY limb measurements. The general behaviour of the aerosol particle size parameters was revealed. Comparison of the retrieved parameters with another instrument showed good agreement.
Stefan Noël, Katja Weigel, Klaus Bramstedt, Alexei Rozanov, Mark Weber, Heinrich Bovensmann, and John P. Burrows
Atmos. Chem. Phys., 18, 4463–4476, https://doi.org/10.5194/acp-18-4463-2018, https://doi.org/10.5194/acp-18-4463-2018, 2018
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The combined analysis of stratospheric methane and water vapour data derived from SCIAMACHY solar occultation measurements shows the expected anti-correlation and a clear temporal variation related to waves in equatorial zonal winds. Above about 20 km most of the additional water vapour is attributed to the oxidation of methane. The SCIAMACHY data confirm that at lower altitudes water vapour and methane are transported from the tropics to higher latitudes.
Linlu Mei, Vladimir Rozanov, Marco Vountas, John P. Burrows, and Andreas Richter
Atmos. Chem. Phys., 18, 2511–2523, https://doi.org/10.5194/acp-18-2511-2018, https://doi.org/10.5194/acp-18-2511-2018, 2018
Timo H. Virtanen, Pekka Kolmonen, Larisa Sogacheva, Edith Rodríguez, Giulia Saponaro, and Gerrit de Leeuw
Atmos. Meas. Tech., 11, 925–938, https://doi.org/10.5194/amt-11-925-2018, https://doi.org/10.5194/amt-11-925-2018, 2018
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We study the collocation mismatch uncertainty related to validating coarse-resolution satellite-based aerosol data against point-like ground based measurements. We use the spatial variability in the satellite data to estimate the upper limit for the uncertainty and study the effect of sampling parameters in the validation. We find that accounting for the collocation mismatch uncertainty increases the fraction of consistent data in the validation.
Mark Weber, Melanie Coldewey-Egbers, Vitali E. Fioletov, Stacey M. Frith, Jeannette D. Wild, John P. Burrows, Craig S. Long, and Diego Loyola
Atmos. Chem. Phys., 18, 2097–2117, https://doi.org/10.5194/acp-18-2097-2018, https://doi.org/10.5194/acp-18-2097-2018, 2018
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This paper commemorates the 30-year anniversary of the initial signing of the Montreal Protocol (MP) on substances that deplete the ozone layer. The MP is so far successful in reducing ozone-depleting substances, and total ozone decline was successfully stopped by the late 1990s. Total ozone levels have been mostly stable since then. In some regions, barely significant upward trends are observed that suggest an emergence into the expected ozone recovery phase.
Thomas Krings, Bruno Neininger, Konstantin Gerilowski, Sven Krautwurst, Michael Buchwitz, John P. Burrows, Carsten Lindemann, Thomas Ruhtz, Dirk Schüttemeyer, and Heinrich Bovensmann
Atmos. Meas. Tech., 11, 721–739, https://doi.org/10.5194/amt-11-721-2018, https://doi.org/10.5194/amt-11-721-2018, 2018
Gerrit de Leeuw, Larisa Sogacheva, Edith Rodriguez, Konstantinos Kourtidis, Aristeidis K. Georgoulias, Georgia Alexandri, Vassilis Amiridis, Emmanouil Proestakis, Eleni Marinou, Yong Xue, and Ronald van der A
Atmos. Chem. Phys., 18, 1573–1592, https://doi.org/10.5194/acp-18-1573-2018, https://doi.org/10.5194/acp-18-1573-2018, 2018
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The complementary use of two sensors, ATSR and MODIS, to provide aerosol information over two decades (1995–2015) is described. To this end, the AOD retrieved from both instruments had to be compared, showing that ATSR slightly underestimates and MODIS overestimates by a similar amount. Results show the increase of aerosols over the years, with an indication of the onset of a decrease in recent years. The AOD spatial distribution shows seasonal variations across China.
Emmanouil Proestakis, Vassilis Amiridis, Eleni Marinou, Aristeidis K. Georgoulias, Stavros Solomos, Stelios Kazadzis, Julien Chimot, Huizheng Che, Georgia Alexandri, Ioannis Binietoglou, Vasiliki Daskalopoulou, Konstantinos A. Kourtidis, Gerrit de Leeuw, and Ronald J. van der A
Atmos. Chem. Phys., 18, 1337–1362, https://doi.org/10.5194/acp-18-1337-2018, https://doi.org/10.5194/acp-18-1337-2018, 2018
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We provide a 3-D climatology of desert dust aerosols over South and East Asia, based on 9 years of CALIPSO observations and an EARLINET methodology. The results provide the horizontal, vertical and seasonal distribution of dust aerosols over SE Asia along with the change in dust transport pathways. The dataset is unique for its potential applications, including evaluation and assimilation activities in atmospheric simulations and the estimation of the climatic impact of dust aerosols.
Amirmahdi Zarboo, Stefan Bender, John P. Burrows, Johannes Orphal, and Miriam Sinnhuber
Atmos. Meas. Tech., 11, 473–487, https://doi.org/10.5194/amt-11-473-2018, https://doi.org/10.5194/amt-11-473-2018, 2018
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We present the retrieved volume emission rates (VERs) from the airglow of both the daytime and twilight O2(1Σ) band and O2(1Δ) band emissions in the mesosphere and lower thermosphere (MLT). We have investigated the daily mean latitudinal distributions and the time series of the retrieved VER in the altitude range from 53 to 149 km. These observations provide information about the chemistry and dynamics and can be used to infer ozone, solar heating rates, and temperature in the MLT.
Patricia Liebing, Matthijs Krijger, Ralph Snel, Klaus Bramstedt, Stefan Noël, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 11, 265–289, https://doi.org/10.5194/amt-11-265-2018, https://doi.org/10.5194/amt-11-265-2018, 2018
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This article describes a method to determine the polarization sensitivity of SCIAMACHY, a spectrometer on Envisat, from in-orbit data. Polarization is a preference of a direction in which light oscillates, and many optical instruments suffer from a dependence of their measured signals on this. To measure and correct for this effect, a statistical analysis of in-flight data combined with a model of the atmosphere and the instrument was performed, showing that the instrument changed after launch.
Sven Krautwurst, Konstantin Gerilowski, Haflidi H. Jonsson, David R. Thompson, Richard W. Kolyer, Laura T. Iraci, Andrew K. Thorpe, Markus Horstjann, Michael Eastwood, Ira Leifer, Samuel A. Vigil, Thomas Krings, Jakob Borchardt, Michael Buchwitz, Matthew M. Fladeland, John P. Burrows, and Heinrich Bovensmann
Atmos. Meas. Tech., 10, 3429–3452, https://doi.org/10.5194/amt-10-3429-2017, https://doi.org/10.5194/amt-10-3429-2017, 2017
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This study investigates a subset of data collected during the CO2 and Methane EXperiment (COMEX) in 2014. It focuses on airborne measurements to quantify the emissions from landfills in the Los Angeles Basin. Airborne remote sensing data have been used to estimate the emission rate of one particular landfill on four different days. The results have been compared to airborne in situ measurements. Airborne imaging spectroscopy has been used to identify emission hotspots across the landfill.
André Seyler, Folkard Wittrock, Lisa Kattner, Barbara Mathieu-Üffing, Enno Peters, Andreas Richter, Stefan Schmolke, and John P. Burrows
Atmos. Chem. Phys., 17, 10997–11023, https://doi.org/10.5194/acp-17-10997-2017, https://doi.org/10.5194/acp-17-10997-2017, 2017
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Shipping accounts for a significant part of the emissions from the transportation sector. We have analyzed 3 years of MAX-DOAS measurements of NO2 and SO2 from a small island in the German Bight, showing that despite the vicinity to the shipping lane, the contribution of shipping sources to air pollution is only about 40 %. The implementation of stricter fuel sulfur limits led to a significant reduction in SO2-to-NO2 ratios in shipping emissions and ambient SO2 levels at the German coast.
Martin P. Langowski, Christian von Savigny, John P. Burrows, Didier Fussen, Erin C. M. Dawkins, Wuhu Feng, John M. C. Plane, and Daniel R. Marsh
Atmos. Meas. Tech., 10, 2989–3006, https://doi.org/10.5194/amt-10-2989-2017, https://doi.org/10.5194/amt-10-2989-2017, 2017
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Meteoric metals form metal layers in the upper atmosphere anandplay a role in the formation of middle-atmospheric clouds and aerosols. However, the total metal influx rate is not well known. Global Na datasets from measurements and a model are available, which had not been compared yet on a global scale until this paper. Overall the agreement is good, and many differences between measurements are also found in the model simulations. However, the modeled layer altitude is too low.
Christopher J. Merchant, Frank Paul, Thomas Popp, Michael Ablain, Sophie Bontemps, Pierre Defourny, Rainer Hollmann, Thomas Lavergne, Alexandra Laeng, Gerrit de Leeuw, Jonathan Mittaz, Caroline Poulsen, Adam C. Povey, Max Reuter, Shubha Sathyendranath, Stein Sandven, Viktoria F. Sofieva, and Wolfgang Wagner
Earth Syst. Sci. Data, 9, 511–527, https://doi.org/10.5194/essd-9-511-2017, https://doi.org/10.5194/essd-9-511-2017, 2017
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Climate data records (CDRs) contain data describing Earth's climate and should address uncertainty in the data to communicate what is known about climate variability or change and what range of doubt exists. This paper discusses good practice for including uncertainty information in CDRs for the essential climate variables (ECVs) derived from satellite data. Recommendations emerge from the shared experience of diverse ECV projects within the European Space Agency Climate Change Initiative.
Klaus Bramstedt, Thomas C. Stone, Manfred Gottwald, Stefan Noël, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 10, 2413–2423, https://doi.org/10.5194/amt-10-2413-2017, https://doi.org/10.5194/amt-10-2413-2017, 2017
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The satellite instrument SCIAMACHY on board the ESA's platform Envisat
(2002–2012) performed observations of the Earth's atmosphere. Using sun and moon observations of the instrument itself, we derived a set of correction
parameters for the determination of the viewing directions of the
instrument. From this work, all vertical profiles of atmospheric parameters
from SCIAMACHY's limb and occultation measurements will be improved by a more
accurate altitude information.
Andreas Carlos Meier, Anja Schönhardt, Tim Bösch, Andreas Richter, André Seyler, Thomas Ruhtz, Daniel-Eduard Constantin, Reza Shaiganfar, Thomas Wagner, Alexis Merlaud, Michel Van Roozendael, Livio Belegante, Doina Nicolae, Lucian Georgescu, and John Philip Burrows
Atmos. Meas. Tech., 10, 1831–1857, https://doi.org/10.5194/amt-10-1831-2017, https://doi.org/10.5194/amt-10-1831-2017, 2017
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We present airborne remote sensing measurements of NO2 in the urban area of Bucharest. NO2 is a harmful pollutant, which is emitted in combustion processes. The measurements presented here enable the creation of maps, showing the horizontal NO2 distribution across the whole city within a relatively short time window of 1.5 h. These data provide new insight into urban pollution levels and their spatial distribution.
Michael Buchwitz, Oliver Schneising, Maximilian Reuter, Jens Heymann, Sven Krautwurst, Heinrich Bovensmann, John P. Burrows, Hartmut Boesch, Robert J. Parker, Peter Somkuti, Rob G. Detmers, Otto P. Hasekamp, Ilse Aben, André Butz, Christian Frankenberg, and Alexander J. Turner
Atmos. Chem. Phys., 17, 5751–5774, https://doi.org/10.5194/acp-17-5751-2017, https://doi.org/10.5194/acp-17-5751-2017, 2017
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Methane is an important greenhouse gas and increasing atmospheric concentrations result in global warming. We present a simple method to derive annual methane emission estimates of methane hotspot areas from satellite data. We present results for four source areas. We found that our estimates are in good agreement with other studies/data sets for the Four Corners region in the USA and for Azerbaijan but we also found higher emissions for parts of California and Turkmenistan.
Yuqin Liu, Gerrit de Leeuw, Veli-Matti Kerminen, Jiahua Zhang, Putian Zhou, Wei Nie, Ximeng Qi, Juan Hong, Yonghong Wang, Aijun Ding, Huadong Guo, Olaf Krüger, Markku Kulmala, and Tuukka Petäjä
Atmos. Chem. Phys., 17, 5623–5641, https://doi.org/10.5194/acp-17-5623-2017, https://doi.org/10.5194/acp-17-5623-2017, 2017
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The aerosol effects on warm cloud parameters over the Yangtze River Delta are systematically examined using multi-sensor retrievals. This study shows that the COT–CDR and CWP–CDR relationships are not unique, but are affected by atmospheric aerosol loading. CDR and cloud fraction show different behaviours for low and high AOD. Aerosol–cloud interaction (ACI) is stronger for clouds mixed with smoke aerosol than for clouds mixed with dust. Meteorological conditions play an important role in ACI.
Jia Jia, Annette Ladstätter-Weißenmayer, Xuewei Hou, Alexei Rozanov, and John P. Burrows
Atmos. Chem. Phys., 17, 4915–4930, https://doi.org/10.5194/acp-17-4915-2017, https://doi.org/10.5194/acp-17-4915-2017, 2017
Anja Schönhardt, Andreas Richter, Nicolas Theys, and John P. Burrows
Atmos. Chem. Phys., 17, 4857–4870, https://doi.org/10.5194/acp-17-4857-2017, https://doi.org/10.5194/acp-17-4857-2017, 2017
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Iodine monoxide, IO, is observed in satellite measurements following the eruption of the Kasatochi volcano, Alaska, in August 2008. Large IO columns are detected by SCIAMACHY on ENVISAT and by GOME-2 on MetOp-A for several days. IO amounts are approximately 1 order of magnitude smaller than those of BrO. Details in the spatial distributions differ between IO, BrO and sulfur dioxide, SO2. The total mass of IO in the volcanic plume is determined to be on the order of 10 Mg.
Stefan Lossow, Farahnaz Khosrawi, Gerald E. Nedoluha, Faiza Azam, Klaus Bramstedt, John. P. Burrows, Bianca M. Dinelli, Patrick Eriksson, Patrick J. Espy, Maya García-Comas, John C. Gille, Michael Kiefer, Stefan Noël, Piera Raspollini, William G. Read, Karen H. Rosenlof, Alexei Rozanov, Christopher E. Sioris, Gabriele P. Stiller, Kaley A. Walker, and Katja Weigel
Atmos. Meas. Tech., 10, 1111–1137, https://doi.org/10.5194/amt-10-1111-2017, https://doi.org/10.5194/amt-10-1111-2017, 2017
Enno Peters, Gaia Pinardi, André Seyler, Andreas Richter, Folkard Wittrock, Tim Bösch, Michel Van Roozendael, François Hendrick, Theano Drosoglou, Alkiviadis F. Bais, Yugo Kanaya, Xiaoyi Zhao, Kimberly Strong, Johannes Lampel, Rainer Volkamer, Theodore Koenig, Ivan Ortega, Olga Puentedura, Mónica Navarro-Comas, Laura Gómez, Margarita Yela González, Ankie Piters, Julia Remmers, Yang Wang, Thomas Wagner, Shanshan Wang, Alfonso Saiz-Lopez, David García-Nieto, Carlos A. Cuevas, Nuria Benavent, Richard Querel, Paul Johnston, Oleg Postylyakov, Alexander Borovski, Alexander Elokhov, Ilya Bruchkouski, Haoran Liu, Cheng Liu, Qianqian Hong, Claudia Rivera, Michel Grutter, Wolfgang Stremme, M. Fahim Khokhar, Junaid Khayyam, and John P. Burrows
Atmos. Meas. Tech., 10, 955–978, https://doi.org/10.5194/amt-10-955-2017, https://doi.org/10.5194/amt-10-955-2017, 2017
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This work is about harmonization of differential optical absorption spectroscopy retrieval codes, which is a remote sensing technique widely used to derive atmospheric trace gas amounts. The study is based on ground-based measurements performed during the Multi-Axis DOAS Comparison campaign for Aerosols and Trace gases (MAD-CAT) in Mainz, Germany, in summer 2013. In total, 17 international groups working in the field of the DOAS technique participated in this study.
Andreas Hilboll, Andreas Richter, and John P. Burrows
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-101, https://doi.org/10.5194/acp-2017-101, 2017
Revised manuscript has not been submitted
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We investigate the temporal evolution of the important tropospheric air pollutant nitrogen dioxide (NO2) since the early 2000s, and correlate NO2 abundances with indicators of economic development. Until 2012, NO2 pollution and economic growth are strongly correlated, with annual increases of up to 4.4 %. Since then, tropospheric NO2 pollution has stabilized or is even declining, probably as a result of a slow-down in Indian economic growth combined with the implementation of cleaner technology.
Ruixiong Zhang, Yuhang Wang, Qiusheng He, Laiguo Chen, Yuzhong Zhang, Hang Qu, Charles Smeltzer, Jianfeng Li, Leonardo M. A. Alvarado, Mihalis Vrekoussis, Andreas Richter, Folkard Wittrock, and John P. Burrows
Atmos. Chem. Phys., 17, 3083–3095, https://doi.org/10.5194/acp-17-3083-2017, https://doi.org/10.5194/acp-17-3083-2017, 2017
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We use short-lived reactive aromatics as proxies to diagnose transport of pollutants to Tibet. In situ observations of short-lived reactive aromatics across the Tibetan Plateau are analyzed using a regional chemistry and transport model. Our results suggest that the cut-off low system is a major pathway for long-range transport of pollutants such as black carbon. The modeling analysis reveals that even the state-of-the-science reanalysis cannot simulate this cut-off system accurately.
Giulia Saponaro, Pekka Kolmonen, Larisa Sogacheva, Edith Rodriguez, Timo Virtanen, and Gerrit de Leeuw
Atmos. Chem. Phys., 17, 3133–3143, https://doi.org/10.5194/acp-17-3133-2017, https://doi.org/10.5194/acp-17-3133-2017, 2017
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The effect of aerosol upon cloud properties is studied over the Baltic Sea region, which presents a distinct contrast of aerosol loading between the clean Fennoscandia and the polluted area of central–eastern Europe. Statistically significant positive values are found over the Baltic Sea and Fennoscandia, while negative values are found over central–eastern Europe, contradicting the theory of aerosol indirect effect on clouds.
Larisa Sogacheva, Pekka Kolmonen, Timo H. Virtanen, Edith Rodriguez, Giulia Saponaro, and Gerrit de Leeuw
Atmos. Meas. Tech., 10, 491–505, https://doi.org/10.5194/amt-10-491-2017, https://doi.org/10.5194/amt-10-491-2017, 2017
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Clouds reflect solar light much more strongly than aerosol particles. Therefore, the retrieval of aerosol optical depth is usually only attempted over cloud-free areas. A very strict cloud detection scheme has to be applied to remove all cloudy pixels. However, often not all clouds are detected. To remove possibly cloud-contaminated pixels, a cloud post-processing algorithm has been designed, which effectively solves the problem and results in smoother AOD maps and improved validation results.
Stefan Bender, Miriam Sinnhuber, Martin Langowski, and John P. Burrows
Atmos. Meas. Tech., 10, 209–220, https://doi.org/10.5194/amt-10-209-2017, https://doi.org/10.5194/amt-10-209-2017, 2017
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We present the retrieval of NO number densities from 60 km to 85 km from measurements of SCIAMACHY/Envisat in its nominal limb mode (0–91 km). We derive the densities from the NO gamma bands (230–300 nm). Using prior input reduces the incorrect attribution of NO from the lower thermosphere. The SCIAMACHY nominal limb scans provide almost 10 years of daily NO data in this altitude range, a unique data record to constrain NO in the mesosphere for testing and validating chemistry climate models.
Patrick E. Sheese, Kaley A. Walker, Chris D. Boone, Chris A. McLinden, Peter F. Bernath, Adam E. Bourassa, John P. Burrows, Doug A. Degenstein, Bernd Funke, Didier Fussen, Gloria L. Manney, C. Thomas McElroy, Donal Murtagh, Cora E. Randall, Piera Raspollini, Alexei Rozanov, James M. Russell III, Makoto Suzuki, Masato Shiotani, Joachim Urban, Thomas von Clarmann, and Joseph M. Zawodny
Atmos. Meas. Tech., 9, 5781–5810, https://doi.org/10.5194/amt-9-5781-2016, https://doi.org/10.5194/amt-9-5781-2016, 2016
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This study validates version 3.5 of the ACE-FTS NOy species data sets by comparing diurnally scaled ACE-FTS data to correlative data from 11 other satellite limb sounders. For all five species examined (NO, NO2, HNO3, N2O5, and ClONO2), there is good agreement between ACE-FTS and the other data sets in various regions of the atmosphere. In these validated regions, these NOy data products can be used for further investigation into the composition, dynamics, and climate of the stratosphere.
Anu Heikkilä, Jakke Sakari Mäkelä, Kaisa Lakkala, Outi Meinander, Jussi Kaurola, Tapani Koskela, Juha Matti Karhu, Tomi Karppinen, Esko Kyrö, and Gerrit de Leeuw
Geosci. Instrum. Method. Data Syst., 5, 531–540, https://doi.org/10.5194/gi-5-531-2016, https://doi.org/10.5194/gi-5-531-2016, 2016
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Lamp measurements used for the UV irradiance calibration of two Brewer spectrophotometers operated for 20 years in Jokioinen and Sodankylä, Finland, were examined. Temporal development of the responsivity after fixing the irradiance measurements into a specific scale was studied. Both long-term gradual decrease and abrupt changes in responsiveness were detected. Frequent-enough measurements of working standard lamps were found necessary to detect the short-term variations in responsiveness.
Hanna K. Lappalainen, Veli-Matti Kerminen, Tuukka Petäjä, Theo Kurten, Aleksander Baklanov, Anatoly Shvidenko, Jaana Bäck, Timo Vihma, Pavel Alekseychik, Meinrat O. Andreae, Stephen R. Arnold, Mikhail Arshinov, Eija Asmi, Boris Belan, Leonid Bobylev, Sergey Chalov, Yafang Cheng, Natalia Chubarova, Gerrit de Leeuw, Aijun Ding, Sergey Dobrolyubov, Sergei Dubtsov, Egor Dyukarev, Nikolai Elansky, Kostas Eleftheriadis, Igor Esau, Nikolay Filatov, Mikhail Flint, Congbin Fu, Olga Glezer, Aleksander Gliko, Martin Heimann, Albert A. M. Holtslag, Urmas Hõrrak, Juha Janhunen, Sirkku Juhola, Leena Järvi, Heikki Järvinen, Anna Kanukhina, Pavel Konstantinov, Vladimir Kotlyakov, Antti-Jussi Kieloaho, Alexander S. Komarov, Joni Kujansuu, Ilmo Kukkonen, Ella-Maria Duplissy, Ari Laaksonen, Tuomas Laurila, Heikki Lihavainen, Alexander Lisitzin, Alexsander Mahura, Alexander Makshtas, Evgeny Mareev, Stephany Mazon, Dmitry Matishov, Vladimir Melnikov, Eugene Mikhailov, Dmitri Moisseev, Robert Nigmatulin, Steffen M. Noe, Anne Ojala, Mari Pihlatie, Olga Popovicheva, Jukka Pumpanen, Tatjana Regerand, Irina Repina, Aleksei Shcherbinin, Vladimir Shevchenko, Mikko Sipilä, Andrey Skorokhod, Dominick V. Spracklen, Hang Su, Dmitry A. Subetto, Junying Sun, Arkady Y. Terzhevik, Yuri Timofeyev, Yuliya Troitskaya, Veli-Pekka Tynkkynen, Viacheslav I. Kharuk, Nina Zaytseva, Jiahua Zhang, Yrjö Viisanen, Timo Vesala, Pertti Hari, Hans Christen Hansson, Gennady G. Matvienko, Nikolai S. Kasimov, Huadong Guo, Valery Bondur, Sergej Zilitinkevich, and Markku Kulmala
Atmos. Chem. Phys., 16, 14421–14461, https://doi.org/10.5194/acp-16-14421-2016, https://doi.org/10.5194/acp-16-14421-2016, 2016
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After kick off in 2012, the Pan-Eurasian Experiment (PEEX) program has expanded fast and today the multi-disciplinary research community covers ca. 80 institutes and a network of ca. 500 scientists from Europe, Russia, and China. Here we introduce scientific topics relevant in this context. This is one of the first multi-disciplinary overviews crossing scientific boundaries, from atmospheric sciences to socio-economics and social sciences.
Laura Riuttanen, Marja Bister, Veli-Matti Kerminen, Viju O. John, Anu-Maija Sundström, Miikka Dal Maso, Jouni Räisänen, Victoria A. Sinclair, Risto Makkonen, Filippo Xausa, Gerrit de Leeuw, and Markku Kulmala
Atmos. Chem. Phys., 16, 14331–14342, https://doi.org/10.5194/acp-16-14331-2016, https://doi.org/10.5194/acp-16-14331-2016, 2016
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Here we show observational evidence that aerosols increase upper tropospheric humidity (UTH) via changes in the microphysics of deep convection. Using remote sensing data over the ocean east of China in summer, we show that increased aerosol loads are associated with an UTH increase of 2.2 ± 1.5 in units of relative humidity. We show that humidification of aerosols or other meteorological covariation is very unlikely to be the cause for this result indicating relevance for the global climate.
Monique F. M. A. Albert, Magdalena D. Anguelova, Astrid M. M. Manders, Martijn Schaap, and Gerrit de Leeuw
Atmos. Chem. Phys., 16, 13725–13751, https://doi.org/10.5194/acp-16-13725-2016, https://doi.org/10.5194/acp-16-13725-2016, 2016
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Sea spray source functions (SSSFs) predict production of sea salt aerosol, important for climate. Sea spray originates from bubble bursting within whitecaps, mainly formed by wind speed (U). Using satellite-based whitecap fraction (W) data analyzed on global and regional scale and explicitly accounting for sea surface temperature (T) we derive a new W(U, T) parameterization. We use it to evaluate influence of secondary factors on a SSSF via W.
Dhanyalekshmi Pillai, Michael Buchwitz, Christoph Gerbig, Thomas Koch, Maximilian Reuter, Heinrich Bovensmann, Julia Marshall, and John P. Burrows
Atmos. Chem. Phys., 16, 9591–9610, https://doi.org/10.5194/acp-16-9591-2016, https://doi.org/10.5194/acp-16-9591-2016, 2016
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Approximately 70 % of total CO2 emissions arise from cities; however, there exist large uncertainties in quantifying urban emissions. The present study investigates the potential of a satellite mission like CarbonSat to retrieve the city emissions via inverse modelling techniques. The study makes a valid conclusion that an instrument like CarbonSat has high potential to provide important information on city emissions when exploiting the observations using a high-resolution modelling system.
Yahui Che, Yong Xue, Linlu Mei, Jie Guang, Lu She, Jianping Guo, Yincui Hu, Hui Xu, Xingwei He, Aojie Di, and Cheng Fan
Atmos. Chem. Phys., 16, 9655–9674, https://doi.org/10.5194/acp-16-9655-2016, https://doi.org/10.5194/acp-16-9655-2016, 2016
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Remotely sensed data could provide continuous spatial coverage of aerosol property over the pan-Eurasian area for PEEX program. The AATSR data can be used to retrieve aerosol optical depth (AOD). The Aerosol_cci project provides users with three AOD retrieval algorithms for AATSR data. Because China is vast in territory and has great differences in terms of land surfaces, the combination of the AERONET and CARSNET data can validate the Level 2 AOD products from AATSR data more comprehensively.
Elpida Leventidou, Kai-Uwe Eichmann, Mark Weber, and John P. Burrows
Atmos. Meas. Tech., 9, 3407–3427, https://doi.org/10.5194/amt-9-3407-2016, https://doi.org/10.5194/amt-9-3407-2016, 2016
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Here, we present a 17 years tropical tropospheric ozone columns dataset (1996–2012) using GOME, SCIAMACHY, and GOME-2 data, developed as part of the verification algorithm for TROPOMI on S5p mission.The uncertainty is less than 2 DU. Validation with SHADOZ ozonesonde data showed biases within 5 DU and RMS errors less than 10 DU. Comparisons with tropospheric ozone columns derived from limb–nadir matching showed that the bias and RMS are within the range of the CCD_IUP comparison with the sondes.
U. Frieß, H. Klein Baltink, S. Beirle, K. Clémer, F. Hendrick, B. Henzing, H. Irie, G. de Leeuw, A. Li, M. M. Moerman, M. van Roozendael, R. Shaiganfar, T. Wagner, Y. Wang, P. Xie, S. Yilmaz, and P. Zieger
Atmos. Meas. Tech., 9, 3205–3222, https://doi.org/10.5194/amt-9-3205-2016, https://doi.org/10.5194/amt-9-3205-2016, 2016
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This article describes the first direct comparison of aerosol extinction profiles from Multi-Axis DOAS measurements of the oxygen collision complex using five different retrieval algorithms. A comparison of the retrieved profiles with co-located aerosol measurements shows good agreement with respect to profile shape and aerosol optical thickness. This study shows that MAX-DOAS is a simple, versatile and cost-effective method for the measurement of aerosol properties in the lower troposphere.
Tero Mielonen, Anca Hienola, Thomas Kühn, Joonas Merikanto, Antti Lipponen, Tommi Bergman, Hannele Korhonen, Pekka Kolmonen, Larisa Sogacheva, Darren Ghent, Antti Arola, Gerrit de Leeuw, and Harri Kokkola
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-625, https://doi.org/10.5194/acp-2016-625, 2016
Revised manuscript not accepted
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We studied the temperature dependence of AOD and its radiative effects over the southeastern US. We used spaceborne observations of AOD, LST and tropospheric NO2 with simulations of ECHAM-HAMMOZ. The level of AOD in this region is governed by anthropogenic emissions but the temperature dependency is most likely caused by BVOC emissions. According to the observations and simulations, the regional clear-sky DRE for biogenic aerosols is −0.43 ± 0.88 W/m2/K and −0.86 ± 0.06 W/m2/K, respectively.
Jakke Sakari Mäkelä, Kaisa Lakkala, Tapani Koskela, Tomi Karppinen, Juha Matti Karhu, Vladimir Savastiouk, Hanne Suokanerva, Jussi Kaurola, Antti Arola, Anders Vilhelm Lindfors, Outi Meinander, Gerrit de Leeuw, and Anu Heikkilä
Geosci. Instrum. Method. Data Syst., 5, 193–203, https://doi.org/10.5194/gi-5-193-2016, https://doi.org/10.5194/gi-5-193-2016, 2016
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We describe the steps that are used at the Finnish Meteorological Institute (FMI) to process spectral ultraviolet (UV) radiation measurements made with its three Brewer spectrophotometers, located in Sodankylä (67° N) and Jokioinen (61° N). Multiple corrections are made to the data in near-real time and quality control is also performed automatically. Several data products are produced, including the near-real-time UV index and various daily dosages, and submitted to databases.
Stefan Noël, Klaus Bramstedt, Michael Hilker, Patricia Liebing, Johannes Plieninger, Max Reuter, Alexei Rozanov, Christopher E. Sioris, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 9, 1485–1503, https://doi.org/10.5194/amt-9-1485-2016, https://doi.org/10.5194/amt-9-1485-2016, 2016
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Stratospheric methane (CH4) and carbon dioxide (CO2) profiles have been derived from solar occultation measurements of the SCIAMACHY satellite instrument. The accuracy of these profiles is estimated to be about 5–10 % for CH4 and 2–3 % for CO2, mainly limited by unexpected vertical oscillations. Results are available for August 2002 to April 2012 and latitudes between about 50 and 70° N. From these, time series trends have been estimated, which are in reasonable agreement with total column trends.
Rosemary Munro, Rüdiger Lang, Dieter Klaes, Gabriele Poli, Christian Retscher, Rasmus Lindstrot, Roger Huckle, Antoine Lacan, Michael Grzegorski, Andriy Holdak, Alexander Kokhanovsky, Jakob Livschitz, and Michael Eisinger
Atmos. Meas. Tech., 9, 1279–1301, https://doi.org/10.5194/amt-9-1279-2016, https://doi.org/10.5194/amt-9-1279-2016, 2016
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The Global Ozone Monitoring Experiment-2 (GOME-2) flies on the Metop series of satellites. In this paper we will provide an overview of the instrument design, the on-ground calibration and characterization activities, in-flight calibration, and level 0 to 1 data processing. The information contained in this paper summarizes a large number of technical reports and related documents containing information that is not currently available in the published literature.
Stefan F. Schreier, Andreas Richter, Folkard Wittrock, and John P. Burrows
Atmos. Chem. Phys., 16, 2803–2817, https://doi.org/10.5194/acp-16-2803-2016, https://doi.org/10.5194/acp-16-2803-2016, 2016
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Mixing ratios of NO2 and HCHO in the free troposphere are obtained from MAX-DOAS measurements at two mountain stations at midlatitudes and in the tropics using a modified geometrical approach. The method is applied in the UV wavelength range and, thus, allows the detection of HCHO mixing ratios, in addition to NO2. We find that mixing ratios of both species are increased in the tropical free troposphere due to biomass burning.
Kai-Uwe Eichmann, Luca Lelli, Christian von Savigny, Harjinder Sembhi, and John P. Burrows
Atmos. Meas. Tech., 9, 793–815, https://doi.org/10.5194/amt-9-793-2016, https://doi.org/10.5194/amt-9-793-2016, 2016
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Height-resolved limb radiance spectra of the satellite instrument SCIAMACHY are used to retrieve cloud top heights with a colour index method. Clouds are detectable from the lower to the uppermost troposphere. These cloud heights help to improve the trace gas retrieval for the upper troposphere and lower stratosphere. Comparisons with other data sets have shown good agreement. As clouds and aerosols are not distinguishable, lower stratospheric volcanic aerosol clouds are detected in some years.
A.-M. Blechschmidt, A. Richter, J. P. Burrows, L. Kaleschke, K. Strong, N. Theys, M. Weber, X. Zhao, and A. Zien
Atmos. Chem. Phys., 16, 1773–1788, https://doi.org/10.5194/acp-16-1773-2016, https://doi.org/10.5194/acp-16-1773-2016, 2016
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A comprehensive case study of a comma-shaped bromine monoxide plume in the Arctic, which was transported by a polar cyclone and was observed by the GOME-2 satellite sensor over several days, is presented. By making combined use of different kinds of satellite data and numerical models, we demonstrate the important role of the frontal weather system in favouring the bromine activation cycle and blowing snow production, which may have acted as a bromine source during the bromine explosion event.
Sébastien Massart, Anna Agustí-Panareda, Jens Heymann, Michael Buchwitz, Frédéric Chevallier, Maximilian Reuter, Michael Hilker, John P. Burrows, Nicholas M. Deutscher, Dietrich G. Feist, Frank Hase, Ralf Sussmann, Filip Desmet, Manvendra K. Dubey, David W. T. Griffith, Rigel Kivi, Christof Petri, Matthias Schneider, and Voltaire A. Velazco
Atmos. Chem. Phys., 16, 1653–1671, https://doi.org/10.5194/acp-16-1653-2016, https://doi.org/10.5194/acp-16-1653-2016, 2016
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This study presents the European Centre for Medium-Range Weather Forecasts (ECMWF) monitoring of atmospheric CO2 using measurements from the Greenhouse gases Observing Satellite (GOSAT). We show that the modelled CO2 has a better precision than standard CO2 satellite products compared to ground-based measurements. We also present the CO2 forecast based on our best knowledge of the atmospheric CO2 distribution. We show that it has skill to forecast the largest scale CO2 patterns up to day 5.
M. P. Langowski, C. von Savigny, J. P. Burrows, V. V. Rozanov, T. Dunker, U.-P. Hoppe, M. Sinnhuber, and A. C. Aikin
Atmos. Meas. Tech., 9, 295–311, https://doi.org/10.5194/amt-9-295-2016, https://doi.org/10.5194/amt-9-295-2016, 2016
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An algorithm has been developed for the retrieval of sodium atom (Na) number density on a latitude and altitude grid from SCIAMACHY limb measurements of the Na resonance fluorescence (multiannual means 2008–2012). The Na layer peaks at 90 to 93 km altitude and has a FWHM of 5 to 15 km. A summer minimum in peak density and width is observed at high latitudes. At low latitudes, a semiannual oscillation is found. The results are compared with other measurements and models and agree well with these.
F. Ebojie, J. P. Burrows, C. Gebhardt, A. Ladstätter-Weißenmayer, C. von Savigny, A. Rozanov, M. Weber, and H. Bovensmann
Atmos. Chem. Phys., 16, 417–436, https://doi.org/10.5194/acp-16-417-2016, https://doi.org/10.5194/acp-16-417-2016, 2016
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The goal of this study is to determine the global and zonal changes in the tropospheric ozone data product derived from SCIAMACHY limb-nadir-matching (LNM) observations during the period 2003–2011.
Tropospheric O3 shows statistically significant increases over some regions of South Asia, the South American continent, Alaska, around Congo in Africa and over some continental outflows. Significant decrease in TOC is observed over some continents and oceans.
K. Weigel, A. Rozanov, F. Azam, K. Bramstedt, R. Damadeo, K.-U. Eichmann, C. Gebhardt, D. Hurst, M. Kraemer, S. Lossow, W. Read, N. Spelten, G. P. Stiller, K. A. Walker, M. Weber, H. Bovensmann, and J. P. Burrows
Atmos. Meas. Tech., 9, 133–158, https://doi.org/10.5194/amt-9-133-2016, https://doi.org/10.5194/amt-9-133-2016, 2016
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The SCanning Imaging Absorption spectroMeter for Atmospheric CHartographY (SCIAMACHY) aboard the Envisat satellite provided measurements between 2002 and 2012 with different viewing geometries. The limb viewing geometry allows the retrieval of water vapour profiles in the UTLS (upper troposphere and lower stratosphere) from the near-infrared spectral range (1353–1410 nm). Here, we present data version 3.01 and compare it to other water vapour data.
F. Khosrawi, J. Urban, S. Lossow, G. Stiller, K. Weigel, P. Braesicke, M. C. Pitts, A. Rozanov, J. P. Burrows, and D. Murtagh
Atmos. Chem. Phys., 16, 101–121, https://doi.org/10.5194/acp-16-101-2016, https://doi.org/10.5194/acp-16-101-2016, 2016
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Our sensitivity studies based on air parcel trajectories confirm that Polar stratospheric cloud (PSC) formation is quite sensitive to water vapour and temperature changes. Considering water vapour time series from satellite measurements we do not find a consistent, significant trend in water vapour in the lower stratosphere during the past 15 years (2000–2014). Thus, the severe dentrification observed in 2010/2011 cannot be directly related to increases in stratospheric water vapour.
C. von Savigny, F. Ernst, A. Rozanov, R. Hommel, K.-U. Eichmann, V. Rozanov, J. P. Burrows, and L. W. Thomason
Atmos. Meas. Tech., 8, 5223–5235, https://doi.org/10.5194/amt-8-5223-2015, https://doi.org/10.5194/amt-8-5223-2015, 2015
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This article presents validation results for stratospheric aerosol extinction profiles retrieved from limb-scatter measurements with the SCIAMACHY instrument on the Envisat satellite. The SCIAMACHY retrievals are compared to co-located measurements with the SAGE II instrument. Very good agreement to within about 15% is found in a global average sense at altitudes above 15 km. The article also presents sample results on the global morphology of the stratospheric aerosol layer from 2003 to 2011.
J. I. Peltoniemi, M. Gritsevich, T. Hakala, P. Dagsson-Waldhauserová, Ó. Arnalds, K. Anttila, H.-R. Hannula, N. Kivekäs, H. Lihavainen, O. Meinander, J. Svensson, A. Virkkula, and G. de Leeuw
The Cryosphere, 9, 2323–2337, https://doi.org/10.5194/tc-9-2323-2015, https://doi.org/10.5194/tc-9-2323-2015, 2015
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Light-absorbing impurities change the reflectance of snow in different ways. Some particles are heated by the Sun and they sink out of sight. During the process, snow may look darker than pure snow when observed by nadir, but at larger view zenith angles the snow may look as white as clean snow. Thus an observer on the ground may overestimate the albedo, while a satellite underestimates the albedo. Climate studies need to examine how the contaminants behave in snow, not only their total amounts.
A. Schönhardt, P. Altube, K. Gerilowski, S. Krautwurst, J. Hartmann, A. C. Meier, A. Richter, and J. P. Burrows
Atmos. Meas. Tech., 8, 5113–5131, https://doi.org/10.5194/amt-8-5113-2015, https://doi.org/10.5194/amt-8-5113-2015, 2015
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The study reports on the application of an aircraft-based instrument (AirMAP) measuring atmospheric nitrogen dioxide. Two-dimensional maps are produced at a spatial resolution of 28m x 30m and with wide spatial coverage. The instrument characteristics are explained and the detailed mapping of a power plant emission plume is demonstrated. Small-scale enhanced amounts of nitrogen dioxide from traffic are observed above a motorway.
N. Rahpoe, M. Weber, A. V. Rozanov, K. Weigel, H. Bovensmann, J. P. Burrows, A. Laeng, G. Stiller, T. von Clarmann, E. Kyrölä, V. F. Sofieva, J. Tamminen, K. Walker, D. Degenstein, A. E. Bourassa, R. Hargreaves, P. Bernath, J. Urban, and D. P. Murtagh
Atmos. Meas. Tech., 8, 4369–4381, https://doi.org/10.5194/amt-8-4369-2015, https://doi.org/10.5194/amt-8-4369-2015, 2015
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The analyses among six satellite instruments measuring ozone reveals that the relative drift between the sensors is not significant in the stratosphere and we conclude that merging of data from these instruments is possible. The merged ozone profiles can then be ingested in global climate models for long-term forecasts of ozone and climate change in the atmosphere. The added drift uncertainty is estimated at about 3% per decade (1 sigma) and should be applied in the calculation of ozone trends.
S. Bender, M. Sinnhuber, T. von Clarmann, G. Stiller, B. Funke, M. López-Puertas, J. Urban, K. Pérot, K. A. Walker, and J. P. Burrows
Atmos. Meas. Tech., 8, 4171–4195, https://doi.org/10.5194/amt-8-4171-2015, https://doi.org/10.5194/amt-8-4171-2015, 2015
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We compare the nitric oxide (NO) daily zonal mean number density data sets in the mesosphere and lower thermosphere (MLT, 60km to 150km) from four instruments: ACE-FTS (2004--2010), MIPAS (2005--2012), SCIAMACHY (2008--2012), and SMR (2003--2012). We find that these data sets from different instruments consistently constrain NO in the MLT. Thus, they offer reliable forcing inputs for climate and chemistry climate models as an initial step to include solar and geomagnetic activity.
K. Atlaskina, F. Berninger, and G. de Leeuw
The Cryosphere, 9, 1879–1893, https://doi.org/10.5194/tc-9-1879-2015, https://doi.org/10.5194/tc-9-1879-2015, 2015
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Snow cover explained most of the spring surface albedo changes in the Northern Hemisphere in the years 2000−2012. However, there are vast areas where albedo changed up to ±0.2 under full snow-covered conditions. We found that if in these areas, the mean monthly air temperature exceeds a value between -15°C and -10°C, depending on the region, albedo decreases with an increase of the temperature. The complexity of processes involved in surface albedo changes is discussed.
L. Kattner, B. Mathieu-Üffing, J. P. Burrows, A. Richter, S. Schmolke, A. Seyler, and F. Wittrock
Atmos. Chem. Phys., 15, 10087–10092, https://doi.org/10.5194/acp-15-10087-2015, https://doi.org/10.5194/acp-15-10087-2015, 2015
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On 1 January 2015, the International Maritime Organisation tightened the regulations for sulfur content of shipping fuels in Sulfur Emission Control Areas. Here we present data from a station near Hamburg harbour in the North Sea SECA, which uses in situ measurements of atmospheric trace gases to deduce the sulphur fuel content of passing ships. We compare data from 2014 before the regulation change and from January 2015 and show how this method can be used for compliance monitoring.
J. Jia, A. Rozanov, A. Ladstätter-Weißenmayer, and J. P. Burrows
Atmos. Meas. Tech., 8, 3369–3383, https://doi.org/10.5194/amt-8-3369-2015, https://doi.org/10.5194/amt-8-3369-2015, 2015
E. Rodríguez, P. Kolmonen, T. H. Virtanen, L. Sogacheva, A.-M. Sundström, and G. de Leeuw
Atmos. Meas. Tech., 8, 3075–3085, https://doi.org/10.5194/amt-8-3075-2015, https://doi.org/10.5194/amt-8-3075-2015, 2015
J. Heymann, M. Reuter, M. Hilker, M. Buchwitz, O. Schneising, H. Bovensmann, J. P. Burrows, A. Kuze, H. Suto, N. M. Deutscher, M. K. Dubey, D. W. T. Griffith, F. Hase, S. Kawakami, R. Kivi, I. Morino, C. Petri, C. Roehl, M. Schneider, V. Sherlock, R. Sussmann, V. A. Velazco, T. Warneke, and D. Wunch
Atmos. Meas. Tech., 8, 2961–2980, https://doi.org/10.5194/amt-8-2961-2015, https://doi.org/10.5194/amt-8-2961-2015, 2015
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Long-term data sets of global atmospheric carbon dioxide concentrations based on observations from different satellite instruments may suffer from inconsistencies originating from the use of different retrieval algorithms. This issue has been addressed by applying the Bremen Optimal Estimation DOAS retrieval algorithm to SCIAMACHY and TANSO-FTS observations. Detailed comparisons with TCCON and CarbonTracker show good consistency between the SCIAMACHY and TANSO-FTS data sets.
P. Zieger, P. P. Aalto, V. Aaltonen, M. Äijälä, J. Backman, J. Hong, M. Komppula, R. Krejci, M. Laborde, J. Lampilahti, G. de Leeuw, A. Pfüller, B. Rosati, M. Tesche, P. Tunved, R. Väänänen, and T. Petäjä
Atmos. Chem. Phys., 15, 7247–7267, https://doi.org/10.5194/acp-15-7247-2015, https://doi.org/10.5194/acp-15-7247-2015, 2015
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The effect of water uptake (hygroscopicity) on aerosol light scattering properties is generally lower for boreal aerosol due to the dominance of organic substances. A columnar optical closure study using ground-based and airborne measurements of aerosol optical, chemical and microphysical properties was conducted and the implications and limitations are discussed.
P. Räisänen, A. Kokhanovsky, G. Guyot, O. Jourdan, and T. Nousiainen
The Cryosphere, 9, 1277–1301, https://doi.org/10.5194/tc-9-1277-2015, https://doi.org/10.5194/tc-9-1277-2015, 2015
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While snow grains are distinctly non-spherical, spheres are often assumed in radiative transfer calculations. Here, angular scattering measurements for blowing snow are used to select an optically equivalent snow grain shape model. Parameterizations are then developed for the asymmetry parameter, single-scattering co-albedo and phase function of snow. The parameterizations will help to improve the treatment of snow in radiative transfer applications, including remote sensing and climate models.
T. Dinter, V. V. Rozanov, J. P. Burrows, and A. Bracher
Ocean Sci., 11, 373–389, https://doi.org/10.5194/os-11-373-2015, https://doi.org/10.5194/os-11-373-2015, 2015
A.-M. Sundström, A. Nikandrova, K. Atlaskina, T. Nieminen, V. Vakkari, L. Laakso, J. P. Beukes, A. Arola, P. G. van Zyl, M. Josipovic, A. D. Venter, K. Jaars, J. J. Pienaar, S. Piketh, A. Wiedensohler, E. K. Chiloane, G. de Leeuw, and M. Kulmala
Atmos. Chem. Phys., 15, 4983–4996, https://doi.org/10.5194/acp-15-4983-2015, https://doi.org/10.5194/acp-15-4983-2015, 2015
J. Svensson, A. Virkkula, O. Meinander, N. Kivekäs, H.-R. Hannula, O. Järvinen, J. I. Peltoniemi, M. Gritsevich, A. Heikkilä, A. Kontu, A.-P. Hyvärinen, K. Neitola, D. Brus, P. Dagsson-Waldhauserova, K. Anttila, T. Hakala, H. Kaartinen, M. Vehkamäki, G. de Leeuw, and H. Lihavainen
The Cryosphere Discuss., https://doi.org/10.5194/tcd-9-1227-2015, https://doi.org/10.5194/tcd-9-1227-2015, 2015
Revised manuscript not accepted
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Soot's (including black carbon and organics) negative effect on a natural snow pack is experimentally addressed in this paper through a series of experiments. Soot concentrations in the snow in the range of 200-200 000 ppb verify the negative effects on the albedo, the physical snow characteristics, as well as increasing the melt rate of the snow pack. Our experimental data generally agrees when compared with the Snow, Ice and Aerosol Radiation model.
L. Sogacheva, P. Kolmonen, T. H. Virtanen, E. Rodriguez, A.-M. Sundström, and G. de Leeuw
Atmos. Meas. Tech., 8, 891–906, https://doi.org/10.5194/amt-8-891-2015, https://doi.org/10.5194/amt-8-891-2015, 2015
A.-M. Sundström, A. Arola, P. Kolmonen, Y. Xue, G. de Leeuw, and M. Kulmala
Atmos. Chem. Phys., 15, 505–518, https://doi.org/10.5194/acp-15-505-2015, https://doi.org/10.5194/acp-15-505-2015, 2015
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In this work, a satellite-based approach to derive the aerosol direct shortwave (SW) radiative effect (ADRE) is studied. The method is based on using coincident satellite observations of SW fluxes and aerosol optical depths (AODs). The key findings of this study are that using normalized values of observed fluxes improves the estimates of ADRE and aerosol-free TOA fluxes as compared to a model. The method was applied over eastern China where the satellite-based mean ADRE of -5Wm-2 was obtained.
M. P. Langowski, C. von Savigny, J. P. Burrows, W. Feng, J. M. C. Plane, D. R. Marsh, D. Janches, M. Sinnhuber, A. C. Aikin, and P. Liebing
Atmos. Chem. Phys., 15, 273–295, https://doi.org/10.5194/acp-15-273-2015, https://doi.org/10.5194/acp-15-273-2015, 2015
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Global concentration fields of Mg and Mg+ in the Earth's upper mesosphere and lower thermosphere (70-150km) are presented. These are retrieved from SCIAMACHY/Envisat satellite grating spectrometer measurements in limb viewing geometry between 2008 and 2012.
These were compared with WACCM-Mg model results and a large fraction of the available measurement results for these species, and an interpretation of the results is done. The variation of these species during NLC presence is discussed.
M. Reuter, M. Buchwitz, M. Hilker, J. Heymann, O. Schneising, D. Pillai, H. Bovensmann, J. P. Burrows, H. Bösch, R. Parker, A. Butz, O. Hasekamp, C. W. O'Dell, Y. Yoshida, C. Gerbig, T. Nehrkorn, N. M. Deutscher, T. Warneke, J. Notholt, F. Hase, R. Kivi, R. Sussmann, T. Machida, H. Matsueda, and Y. Sawa
Atmos. Chem. Phys., 14, 13739–13753, https://doi.org/10.5194/acp-14-13739-2014, https://doi.org/10.5194/acp-14-13739-2014, 2014
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Current knowledge about the European terrestrial biospheric carbon sink relies upon bottom-up and global surface flux inverse model estimates using in situ measurements. Our analysis of five satellite data sets comprises a regional inversion designed to be insensitive to potential retrieval biases and transport errors. We show that the satellite-derived sink is larger (1.0±0.3GtC/a) than previous estimates (0.4±0.4GtC/a).
G. D. Hayman, F. M. O'Connor, M. Dalvi, D. B. Clark, N. Gedney, C. Huntingford, C. Prigent, M. Buchwitz, O. Schneising, J. P. Burrows, C. Wilson, N. Richards, and M. Chipperfield
Atmos. Chem. Phys., 14, 13257–13280, https://doi.org/10.5194/acp-14-13257-2014, https://doi.org/10.5194/acp-14-13257-2014, 2014
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Globally, wetlands are a major source of methane, which is the second most important greenhouse gas. We find the JULES wetland methane scheme to perform well in general, although there is a tendency for it to overpredict emissions in the tropics and underpredict them in northern latitudes. Our study highlights novel uses of satellite data as a major tool to constrain land-atmosphere methane flux models in a warming world.
J. Aschmann, J. P. Burrows, C. Gebhardt, A. Rozanov, R. Hommel, M. Weber, and A. M. Thompson
Atmos. Chem. Phys., 14, 12803–12814, https://doi.org/10.5194/acp-14-12803-2014, https://doi.org/10.5194/acp-14-12803-2014, 2014
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This study compares observations and simulation results of ozone in the lower tropical stratosphere. It shows that ozone in this region decreased from 1985 up to about 2002, which is consistent with an increase in tropical upwelling predicted by climate models. However, the decrease effectively stops after 2002, indicating that significant changes in tropical upwelling have occurred. The most important factor appears to be that the vertical ascent in the tropics is no longer accelerating.
E. Peters, F. Wittrock, A. Richter, L. M. A. Alvarado, V. V. Rozanov, and J. P. Burrows
Atmos. Meas. Tech., 7, 4203–4221, https://doi.org/10.5194/amt-7-4203-2014, https://doi.org/10.5194/amt-7-4203-2014, 2014
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In this study, a correction spectrum accounting for insufficiencies in commonly used liquid water absorption spectra in DOAS applications is retrieved from ship-borne field measurements. The correction spectrum compensates at the same time for broadband parts of vibrational Raman scattering. With this, an entire compensation of liquid water spectral effects in DOAS applications was achieved.
L. M. A. Alvarado, A. Richter, M. Vrekoussis, F. Wittrock, A. Hilboll, S. F. Schreier, and J. P. Burrows
Atmos. Meas. Tech., 7, 4133–4150, https://doi.org/10.5194/amt-7-4133-2014, https://doi.org/10.5194/amt-7-4133-2014, 2014
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An improved glyoxal retrieval for OMI measurements using the DOAS method has been developed. The retrieval is based on sensitivity tests for the selection of most appropriate retrieval parameters. Also, corrections for reduction of interferences with other species have been applied. In addition, the link between pyrogenic emissions and glyoxal over regions with large wildfires have been investigated, and showed that fires are an important source of glyoxal.
A.-I. Partanen, E. M. Dunne, T. Bergman, A. Laakso, H. Kokkola, J. Ovadnevaite, L. Sogacheva, D. Baisnée, J. Sciare, A. Manders, C. O'Dowd, G. de Leeuw, and H. Korhonen
Atmos. Chem. Phys., 14, 11731–11752, https://doi.org/10.5194/acp-14-11731-2014, https://doi.org/10.5194/acp-14-11731-2014, 2014
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New parameterizations for the sea spray aerosol source flux and its organic fraction were incorporated into a global aerosol-climate model. The emissions of sea salt were considerably less than previous estimates. This study demonstrates that sea spray aerosol may actually decrease the number of cloud droplets, which has a warming effect on climate. Overall, sea spray aerosol was predicted to have a global cooling effect due to the scattering of solar radiation from sea spray aerosol particles.
J. Strandgren, L. Mei, M. Vountas, J. P. Burrows, A. Lyapustin, and Y. Wang
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-14-25869-2014, https://doi.org/10.5194/acpd-14-25869-2014, 2014
Revised manuscript not accepted
K. Noguchi, A. Richter, V. Rozanov, A. Rozanov, J. P. Burrows, H. Irie, and K. Kita
Atmos. Meas. Tech., 7, 3497–3508, https://doi.org/10.5194/amt-7-3497-2014, https://doi.org/10.5194/amt-7-3497-2014, 2014
A. Spolaor, P. Vallelonga, J. Gabrieli, T. Martma, M. P. Björkman, E. Isaksson, G. Cozzi, C. Turetta, H. A. Kjær, M. A. J. Curran, A. D. Moy, A. Schönhardt, A.-M. Blechschmidt, J. P. Burrows, J. M. C. Plane, and C. Barbante
Atmos. Chem. Phys., 14, 9613–9622, https://doi.org/10.5194/acp-14-9613-2014, https://doi.org/10.5194/acp-14-9613-2014, 2014
T. H. Virtanen, P. Kolmonen, E. Rodríguez, L. Sogacheva, A.-M. Sundström, and G. de Leeuw
Atmos. Meas. Tech., 7, 2437–2456, https://doi.org/10.5194/amt-7-2437-2014, https://doi.org/10.5194/amt-7-2437-2014, 2014
A. W. Zien, A. Richter, A. Hilboll, A.-M. Blechschmidt, and J. P. Burrows
Atmos. Chem. Phys., 14, 7367–7396, https://doi.org/10.5194/acp-14-7367-2014, https://doi.org/10.5194/acp-14-7367-2014, 2014
W. Chehade, M. Weber, and J. P. Burrows
Atmos. Chem. Phys., 14, 7059–7074, https://doi.org/10.5194/acp-14-7059-2014, https://doi.org/10.5194/acp-14-7059-2014, 2014
F. Ebojie, C. von Savigny, A. Ladstätter-Weißenmayer, A. Rozanov, M. Weber, K.-U. Eichmann, S. Bötel, N. Rahpoe, H. Bovensmann, and J. P. Burrows
Atmos. Meas. Tech., 7, 2073–2096, https://doi.org/10.5194/amt-7-2073-2014, https://doi.org/10.5194/amt-7-2073-2014, 2014
J. Yoon, J. P. Burrows, M. Vountas, W. von Hoyningen-Huene, D. Y. Chang, A. Richter, and A. Hilboll
Atmos. Chem. Phys., 14, 6881–6902, https://doi.org/10.5194/acp-14-6881-2014, https://doi.org/10.5194/acp-14-6881-2014, 2014
B. Dils, M. Buchwitz, M. Reuter, O. Schneising, H. Boesch, R. Parker, S. Guerlet, I. Aben, T. Blumenstock, J. P. Burrows, A. Butz, N. M. Deutscher, C. Frankenberg, F. Hase, O. P. Hasekamp, J. Heymann, M. De Mazière, J. Notholt, R. Sussmann, T. Warneke, D. Griffith, V. Sherlock, and D. Wunch
Atmos. Meas. Tech., 7, 1723–1744, https://doi.org/10.5194/amt-7-1723-2014, https://doi.org/10.5194/amt-7-1723-2014, 2014
L. Lelli, A. A. Kokhanovsky, V. V. Rozanov, M. Vountas, and J. P. Burrows
Atmos. Chem. Phys., 14, 5679–5692, https://doi.org/10.5194/acp-14-5679-2014, https://doi.org/10.5194/acp-14-5679-2014, 2014
O. Meinander, A. Kontu, A. Virkkula, A. Arola, L. Backman, P. Dagsson-Waldhauserová, O. Järvinen, T. Manninen, J. Svensson, G. de Leeuw, and M. Leppäranta
The Cryosphere, 8, 991–995, https://doi.org/10.5194/tc-8-991-2014, https://doi.org/10.5194/tc-8-991-2014, 2014
M. Horstjann, M. D. Andrés Hernández, V. Nenakhov, A. Chrobry, and J. P. Burrows
Atmos. Meas. Tech., 7, 1245–1257, https://doi.org/10.5194/amt-7-1245-2014, https://doi.org/10.5194/amt-7-1245-2014, 2014
A. Virkkula, J. Levula, T. Pohja, P. P. Aalto, P. Keronen, S. Schobesberger, C. B. Clements, L. Pirjola, A.-J. Kieloaho, L. Kulmala, H. Aaltonen, J. Patokoski, J. Pumpanen, J. Rinne, T. Ruuskanen, M. Pihlatie, H. E. Manninen, V. Aaltonen, H. Junninen, T. Petäjä, J. Backman, M. Dal Maso, T. Nieminen, T. Olsson, T. Grönholm, J. Aalto, T. H. Virtanen, M. Kajos, V.-M. Kerminen, D. M. Schultz, J. Kukkonen, M. Sofiev, G. De Leeuw, J. Bäck, P. Hari, and M. Kulmala
Atmos. Chem. Phys., 14, 4473–4502, https://doi.org/10.5194/acp-14-4473-2014, https://doi.org/10.5194/acp-14-4473-2014, 2014
D. C. S. Beddows, M. Dall'Osto, R. M. Harrison, M. Kulmala, A. Asmi, A. Wiedensohler, P. Laj, A.M. Fjaeraa, K. Sellegri, W. Birmili, N. Bukowiecki, E. Weingartner, U. Baltensperger, V. Zdimal, N. Zikova, J.-P. Putaud, A. Marinoni, P. Tunved, H.-C. Hansson, M. Fiebig, N. Kivekäs, E. Swietlicki, H. Lihavainen, E. Asmi, V. Ulevicius, P. P. Aalto, N. Mihalopoulos, N. Kalivitis, I. Kalapov, G. Kiss, G. de Leeuw, B. Henzing, C. O'Dowd, S. G. Jennings, H. Flentje, F. Meinhardt, L. Ries, H. A. C. Denier van der Gon, and A. J. H. Visschedijk
Atmos. Chem. Phys., 14, 4327–4348, https://doi.org/10.5194/acp-14-4327-2014, https://doi.org/10.5194/acp-14-4327-2014, 2014
R. Hommel, K.-U. Eichmann, J. Aschmann, K. Bramstedt, M. Weber, C. von Savigny, A. Richter, A. Rozanov, F. Wittrock, F. Khosrawi, R. Bauer, and J. P. Burrows
Atmos. Chem. Phys., 14, 3247–3276, https://doi.org/10.5194/acp-14-3247-2014, https://doi.org/10.5194/acp-14-3247-2014, 2014
M. Tjernström, C. Leck, C. E. Birch, J. W. Bottenheim, B. J. Brooks, I. M. Brooks, L. Bäcklin, R. Y.-W. Chang, G. de Leeuw, L. Di Liberto, S. de la Rosa, E. Granath, M. Graus, A. Hansel, J. Heintzenberg, A. Held, A. Hind, P. Johnston, J. Knulst, M. Martin, P. A. Matrai, T. Mauritsen, M. Müller, S. J. Norris, M. V. Orellana, D. A. Orsini, J. Paatero, P. O. G. Persson, Q. Gao, C. Rauschenberg, Z. Ristovski, J. Sedlar, M. D. Shupe, B. Sierau, A. Sirevaag, S. Sjogren, O. Stetzer, E. Swietlicki, M. Szczodrak, P. Vaattovaara, N. Wahlberg, M. Westberg, and C. R. Wheeler
Atmos. Chem. Phys., 14, 2823–2869, https://doi.org/10.5194/acp-14-2823-2014, https://doi.org/10.5194/acp-14-2823-2014, 2014
S. F. Schreier, A. Richter, J. W. Kaiser, and J. P. Burrows
Atmos. Chem. Phys., 14, 2447–2466, https://doi.org/10.5194/acp-14-2447-2014, https://doi.org/10.5194/acp-14-2447-2014, 2014
V. Gorshelev, A. Serdyuchenko, M. Weber, W. Chehade, and J. P. Burrows
Atmos. Meas. Tech., 7, 609–624, https://doi.org/10.5194/amt-7-609-2014, https://doi.org/10.5194/amt-7-609-2014, 2014
A. Serdyuchenko, V. Gorshelev, M. Weber, W. Chehade, and J. P. Burrows
Atmos. Meas. Tech., 7, 625–636, https://doi.org/10.5194/amt-7-625-2014, https://doi.org/10.5194/amt-7-625-2014, 2014
J. Ovadnevaite, A. Manders, G. de Leeuw, D. Ceburnis, C. Monahan, A.-I. Partanen, H. Korhonen, and C. D. O'Dowd
Atmos. Chem. Phys., 14, 1837–1852, https://doi.org/10.5194/acp-14-1837-2014, https://doi.org/10.5194/acp-14-1837-2014, 2014
C. Gebhardt, A. Rozanov, R. Hommel, M. Weber, H. Bovensmann, J. P. Burrows, D. Degenstein, L. Froidevaux, and A. M. Thompson
Atmos. Chem. Phys., 14, 831–846, https://doi.org/10.5194/acp-14-831-2014, https://doi.org/10.5194/acp-14-831-2014, 2014
M. Langowski, M. Sinnhuber, A. C. Aikin, C. von Savigny, and J. P. Burrows
Atmos. Meas. Tech., 7, 29–48, https://doi.org/10.5194/amt-7-29-2014, https://doi.org/10.5194/amt-7-29-2014, 2014
O. Schneising, M. Reuter, M. Buchwitz, J. Heymann, H. Bovensmann, and J. P. Burrows
Atmos. Chem. Phys., 14, 133–141, https://doi.org/10.5194/acp-14-133-2014, https://doi.org/10.5194/acp-14-133-2014, 2014
M. Buchwitz, M. Reuter, H. Bovensmann, D. Pillai, J. Heymann, O. Schneising, V. Rozanov, T. Krings, J. P. Burrows, H. Boesch, C. Gerbig, Y. Meijer, and A. Löscher
Atmos. Meas. Tech., 6, 3477–3500, https://doi.org/10.5194/amt-6-3477-2013, https://doi.org/10.5194/amt-6-3477-2013, 2013
W. Chehade, V. Gorshelev, A. Serdyuchenko, J. P. Burrows, and M. Weber
Atmos. Meas. Tech., 6, 3055–3065, https://doi.org/10.5194/amt-6-3055-2013, https://doi.org/10.5194/amt-6-3055-2013, 2013
N. Rahpoe, C. von Savigny, M. Weber, A.V. Rozanov, H. Bovensmann, and J. P. Burrows
Atmos. Meas. Tech., 6, 2825–2837, https://doi.org/10.5194/amt-6-2825-2013, https://doi.org/10.5194/amt-6-2825-2013, 2013
S. Bender, M. Sinnhuber, J. P. Burrows, M. Langowski, B. Funke, and M. López-Puertas
Atmos. Meas. Tech., 6, 2521–2531, https://doi.org/10.5194/amt-6-2521-2013, https://doi.org/10.5194/amt-6-2521-2013, 2013
G. Saponaro, P. Kolmonen, J. Karhunen, J. Tamminen, and G. de Leeuw
Atmos. Meas. Tech., 6, 2301–2309, https://doi.org/10.5194/amt-6-2301-2013, https://doi.org/10.5194/amt-6-2301-2013, 2013
T. Holzer-Popp, G. de Leeuw, J. Griesfeller, D. Martynenko, L. Klüser, S. Bevan, W. Davies, F. Ducos, J. L. Deuzé, R. G. Graigner, A. Heckel, W. von Hoyningen-Hüne, P. Kolmonen, P. Litvinov, P. North, C. A. Poulsen, D. Ramon, R. Siddans, L. Sogacheva, D. Tanre, G. E. Thomas, M. Vountas, J. Descloitres, J. Griesfeller, S. Kinne, M. Schulz, and S. Pinnock
Atmos. Meas. Tech., 6, 1919–1957, https://doi.org/10.5194/amt-6-1919-2013, https://doi.org/10.5194/amt-6-1919-2013, 2013
W. Chehade, B. Gür, P. Spietz, V. Gorshelev, A. Serdyuchenko, J. P. Burrows, and M. Weber
Atmos. Meas. Tech., 6, 1623–1632, https://doi.org/10.5194/amt-6-1623-2013, https://doi.org/10.5194/amt-6-1623-2013, 2013
M. D. Andrés-Hernández, D. Kartal, J. N. Crowley, V. Sinha, E. Regelin, M. Martínez-Harder, V. Nenakhov, J. Williams, H. Harder, H. Bozem, W. Song, J. Thieser, M. J. Tang, Z. Hosaynali Beigi, and J. P. Burrows
Atmos. Chem. Phys., 13, 5731–5749, https://doi.org/10.5194/acp-13-5731-2013, https://doi.org/10.5194/acp-13-5731-2013, 2013
P. Kolmonen, A.-M. Sundström, L. Sogacheva, E. Rodriguez, T. Virtanen, and G. de Leeuw
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amtd-6-4039-2013, https://doi.org/10.5194/amtd-6-4039-2013, 2013
Revised manuscript has not been submitted
A. Hilboll, A. Richter, and J. P. Burrows
Atmos. Chem. Phys., 13, 4145–4169, https://doi.org/10.5194/acp-13-4145-2013, https://doi.org/10.5194/acp-13-4145-2013, 2013
O. Schneising, J. Heymann, M. Buchwitz, M. Reuter, H. Bovensmann, and J. P. Burrows
Atmos. Chem. Phys., 13, 2445–2454, https://doi.org/10.5194/acp-13-2445-2013, https://doi.org/10.5194/acp-13-2445-2013, 2013
A. Hilboll, A. Richter, A. Rozanov, Ø. Hodnebrog, A. Heckel, S. Solberg, F. Stordal, and J. P. Burrows
Atmos. Meas. Tech., 6, 565–584, https://doi.org/10.5194/amt-6-565-2013, https://doi.org/10.5194/amt-6-565-2013, 2013
S. J. Norris, I. M. Brooks, B. I. Moat, M. J. Yelland, G. de Leeuw, R. W. Pascal, and B. Brooks
Ocean Sci., 9, 133–145, https://doi.org/10.5194/os-9-133-2013, https://doi.org/10.5194/os-9-133-2013, 2013
M. Reuter, H. Bösch, H. Bovensmann, A. Bril, M. Buchwitz, A. Butz, J. P. Burrows, C. W. O'Dell, S. Guerlet, O. Hasekamp, J. Heymann, N. Kikuchi, S. Oshchepkov, R. Parker, S. Pfeifer, O. Schneising, T. Yokota, and Y. Yoshida
Atmos. Chem. Phys., 13, 1771–1780, https://doi.org/10.5194/acp-13-1771-2013, https://doi.org/10.5194/acp-13-1771-2013, 2013
L. Riuttanen, M. Dal Maso, G. de Leeuw, I. Riipinen, L. Sogacheva, V. Vakkari, L. Laakso, and M. Kulmala
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-13-4289-2013, https://doi.org/10.5194/acpd-13-4289-2013, 2013
Revised manuscript has not been submitted
T. Krings, K. Gerilowski, M. Buchwitz, J. Hartmann, T. Sachs, J. Erzinger, J. P. Burrows, and H. Bovensmann
Atmos. Meas. Tech., 6, 151–166, https://doi.org/10.5194/amt-6-151-2013, https://doi.org/10.5194/amt-6-151-2013, 2013
Related subject area
Subject: Aerosols | Technique: Remote Sensing | Topic: Data Processing and Information Retrieval
OMPS LP Version 2.0 multi-wavelength aerosol extinction coefficient retrieval algorithm
Simulated reflectance above snow constrained by airborne measurements of solar radiation: implications for the snow grain morphology in the Arctic
ModIs Dust AeroSol (MIDAS): a global fine-resolution dust optical depth data set
Integrated System for Atmospheric Boundary Layer Height Estimation (ISABLE) using a ceilometer and microwave radiometer
Effects of clouds on the UV Absorbing Aerosol Index from TROPOMI
Correction of a lunar-irradiance model for aerosol optical depth retrieval and comparison with a star photometer
Improving GOES Advanced Baseline Imager (ABI) aerosol optical depth (AOD) retrievals using an empirical bias correction algorithm
Relative sky radiance from multi-exposure all-sky camera images
Stratospheric aerosol extinction profiles from SCIAMACHY solar occultation
A feasibility study to use machine learning as an inversion algorithm for aerosol profile and property retrieval from multi-axis differential absorption spectroscopy measurements
Leveraging spatial textures, through machine learning, to identify aerosols and distinct cloud types from multispectral observations
Retrieval of aerosol properties from Airborne Hyper-Angular Rainbow Polarimeter (AirHARP) observations during ACEPOL 2017
Reducing cloud contamination in AOD measurements
Retrieval of stratospheric aerosol size distribution parameters using SAGE-III/ISS extinction measurements at three wavelengths
An uncertainty-based protocol for the setup and measurement of soot/black carbon emissions from gas flares using sky-LOSA
Aerosol optical properties as observed from an ultralight aircraft over the Strait of Gibraltar
Evaluation of a method for converting Stratospheric Aerosol and Gas Experiment (SAGE) extinction coefficients to backscatter coefficients for intercomparison with lidar observations
Inversion of multiangular polarimetric measurements from the ACEPOL campaign: an application of improving aerosol property and hyperspectral ocean color retrievals
A new measurement approach for validating satellite-based above cloud aerosol optical depth
Improved water vapour retrieval from AMSU-B and MHS in the Arctic
The AERONET Version 3 aerosol retrieval algorithm, associated uncertainties and comparisons to Version 2
Issues related to the retrieval of stratospheric-aerosol particle size information based on optical measurements
A new lidar inversion method using a surface reference target applied to the backscattering coefficient and lidar ratio retrievals of a fog-oil plume at short range
A multi-axis differential optical absorption spectroscopy aerosol profile retrieval algorithm for high-altitude measurements: application to measurements at Schneefernerhaus (UFS), Germany
The potential of elastic and polarization lidars to retrieve extinction profiles
Introducing the 4.4 km spatial resolution Multi-Angle Imaging SpectroRadiometer (MISR) aerosol product
Retrieval of gridded aerosol direct radiative forcing based on multiplatform datasets
Assessing the stability of surface lights for use in retrievals of nocturnal atmospheric parameters
A neural network radiative transfer model approach applied to the Tropospheric Monitoring Instrument aerosol height algorithm
Applying the Dark Target aerosol algorithm with Advanced Himawari Imager observations during the KORUS-AQ field campaign
Above-cloud aerosol radiative effects based on ORACLES 2016 and ORACLES 2017 aircraft experiments
The role of aerosol layer height in quantifying aerosol absorption from ultraviolet satellite observations
Cloud-Aerosol Transport System (CATS) 1064 nm calibration and validation
CALIPSO level 3 stratospheric aerosol profile product: version 1.00 algorithm description and initial assessment
Neural network for aerosol retrieval from hyperspectral imagery
Unified quantitative observation of coexisting volcanic sulfur dioxide and sulfate aerosols using ground-based Fourier transform infrared spectroscopy
Aerosol direct radiative effect over clouds from a synergy of Ozone Monitoring Instrument (OMI) and Moderate Resolution Imaging Spectroradiometer (MODIS) reflectances
A Tale of Two Dust Storms: analysis of a complex dust event in the Middle East
Dust mass, cloud condensation nuclei, and ice-nucleating particle profiling with polarization lidar: updated POLIPHON conversion factors from global AERONET analysis
3+2 + X: what is the most useful depolarization input for retrieving microphysical properties of non-spherical particles from lidar measurements using the spheroid model of Dubovik et al. (2006)?
Analyzing the atmospheric boundary layer using high-order moments obtained from multiwavelength lidar data: impact of wavelength choice
Year-round stratospheric aerosol backscatter ratios calculated from lidar measurements above northern Norway
Inversion of multiangular polarimetric measurements over open and coastal ocean waters: a joint retrieval algorithm for aerosol and water-leaving radiance properties
An adaptation of the CO2 slicing technique for the Infrared Atmospheric Sounding Interferometer to obtain the height of tropospheric volcanic ash clouds
Method to retrieve cloud condensation nuclei number concentrations using lidar measurements
Aerosol-type classification based on AERONET version 3 inversion products
The Mineral Aerosol Profiling from Infrared Radiances (MAPIR) algorithm: version 4.1 description and evaluation
Two decades observing smoke above clouds in the south-eastern Atlantic Ocean: Deep Blue algorithm updates and validation with ORACLES field campaign data
Detecting layer height of smoke aerosols over vegetated land and water surfaces via oxygen absorption bands: hourly results from EPIC/DSCOVR in deep space
A new method to determine the aerosol optical properties from multiple-wavelength O4 absorptions by MAX-DOAS observation
Ghassan Taha, Robert Loughman, Tong Zhu, Larry Thomason, Jayanta Kar, Landon Rieger, and Adam Bourassa
Atmos. Meas. Tech., 14, 1015–1036, https://doi.org/10.5194/amt-14-1015-2021, https://doi.org/10.5194/amt-14-1015-2021, 2021
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This work describes the newly released OMPS LP aerosol extinction profile multi-wavelength Version 2.0 algorithm and dataset. It is shown that the V2.0 aerosols exhibit significant improvements in OMPS LP retrieval performance in the Southern Hemisphere and at lower altitudes. The new product is compared to the SAGE III/ISS, OSIRIS and CALIPSO missions and shown to be of good quality and suitable for scientific studies.
Soheila Jafariserajehlou, Vladimir V. Rozanov, Marco Vountas, Charles K. Gatebe, and John P. Burrows
Atmos. Meas. Tech., 14, 369–389, https://doi.org/10.5194/amt-14-369-2021, https://doi.org/10.5194/amt-14-369-2021, 2021
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In this work, we study retrieval of snow grain morphologies and their impact on the reflectance in a coupled snow–atmosphere system. We present a sensitivity study to highlight the importance of having adequate information about snow and atmosphere. A novel two-stage algorithm for retrieving the size and shape of snow grains is presented. The reflectance simulation results are compared to that of airborne measurements; high correlations of 0.98 at IR and 0.88–0.98 at VIS are achieved.
Antonis Gkikas, Emmanouil Proestakis, Vassilis Amiridis, Stelios Kazadzis, Enza Di Tomaso, Alexandra Tsekeri, Eleni Marinou, Nikos Hatzianastassiou, and Carlos Pérez García-Pando
Atmos. Meas. Tech., 14, 309–334, https://doi.org/10.5194/amt-14-309-2021, https://doi.org/10.5194/amt-14-309-2021, 2021
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We present the development of the MIDAS (ModIs Dust AeroSol) data set, providing daily dust optical depth (DOD; 550 nm) at a global scale and fine spatial resolution (0.1° x 0.1°) over a 15-year period (2003–2017). It has been developed via the synergy of MODIS-Aqua and MERRA-2 data, while CALIOP and AERONET retrievals are used for its assessment. MIDAS upgrades existing dust observational capabilities, and it is suitable for dust climatological studies, model evaluation, and data assimilation.
Jae-Sik Min, Moon-Soo Park, Jung-Hoon Chae, and Minsoo Kang
Atmos. Meas. Tech., 13, 6965–6987, https://doi.org/10.5194/amt-13-6965-2020, https://doi.org/10.5194/amt-13-6965-2020, 2020
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An algorithm for an integrated system for ABLH estimation (ISABLE) was developed and applied to the vertical profile data obtained by a ceilometer and a microwave radiometer in Seoul city, Korea. The ISABLE algorithm finds an optimal ABLH through the post-processing including k-means clustering and density-based spatial clustering of applications with noise (DBSCAN) techniques. The ISABLE ABLH exhibited better performance than those obtained by most conventional methods.
Maurits L. Kooreman, Piet Stammes, Victor Trees, Maarten Sneep, L. Gijsbert Tilstra, Martin de Graaf, Deborah C. Stein Zweers, Ping Wang, Olaf N. E. Tuinder, and J. Pepijn Veefkind
Atmos. Meas. Tech., 13, 6407–6426, https://doi.org/10.5194/amt-13-6407-2020, https://doi.org/10.5194/amt-13-6407-2020, 2020
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We investigated the influence of clouds on the Absorbing Aerosol Index (AAI), an indicator of the presence of small particles in the atmosphere. Clouds produce artifacts in AAI calculations on the individual measurement (7 km) scale, which was not seen with previous instruments, as well as on large (1000+ km) scales. To reduce these artefacts, we used three different AAI calculation techniques of varying complexity. We find that the AAI artifacts are reduced when using more complex techniques.
Roberto Román, Ramiro González, Carlos Toledano, África Barreto, Daniel Pérez-Ramírez, Jose A. Benavent-Oltra, Francisco J. Olmo, Victoria E. Cachorro, Lucas Alados-Arboledas, and Ángel M. de Frutos
Atmos. Meas. Tech., 13, 6293–6310, https://doi.org/10.5194/amt-13-6293-2020, https://doi.org/10.5194/amt-13-6293-2020, 2020
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Atmospheric-aerosol and gaseous properties can be derived at night-time if the lunar irradiance at the ground is measured. To this end, the knowledge of lunar irradiance at the top of the atmosphere is necessary. This extraterrestrial lunar irradiance is usually calculated by models since it varies with several geometric factors mainly depending on time and location. This paper proposes a correction to the most used lunar-irradiance model to be applied for atmospheric-aerosol characterization.
Hai Zhang, Shobha Kondragunta, Istvan Laszlo, and Mi Zhou
Atmos. Meas. Tech., 13, 5955–5975, https://doi.org/10.5194/amt-13-5955-2020, https://doi.org/10.5194/amt-13-5955-2020, 2020
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Geostationary Operational Environmental Satellites (GOES) retrieve high temporal resolution aerosol optical depth, which is a measure of the aerosol quantity within the atmospheric column. This work introduces an algorithm that improves the accuracy of the aerosol optical depth retrievals from GOES. The resulting data product can be used in monitoring the air quality and climate change research.
Juan C. Antuña-Sánchez, Roberto Román, Victoria E. Cachorro, Carlos Toledano, César López, Ramiro González, David Mateos, Abel Calle, and Ángel M. de Frutos
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-421, https://doi.org/10.5194/amt-2020-421, 2020
Revised manuscript accepted for AMT
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This paper presents a new technique to exploit the potential of all sky cameras. The sky radiance at three effective wavelengths are calculated and compared with alternative measurements and simulated data. The proposed method will be useful for the retrieval of aerosols and clouds properties.
Stefan Noël, Klaus Bramstedt, Alexei Rozanov, Elizaveta Malinina, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 13, 5643–5666, https://doi.org/10.5194/amt-13-5643-2020, https://doi.org/10.5194/amt-13-5643-2020, 2020
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A new approach to derive stratospheric aerosol extinction profiles from SCIAMACHY solar occultation measurements based on an onion-peeling method is presented. The resulting extinctions at 452, 525 and 750 nm compare well with other limb and occultation data from, e.g. SAGE and SCIAMACHY, but show small oscillating features which vanish in monthly anomalies. Major volcanic eruptions, polar stratospheric clouds and influences of the quasi-biennial oscillation can be identified in the time series.
Yun Dong, Elena Spinei, and Anuj Karpatne
Atmos. Meas. Tech., 13, 5537–5550, https://doi.org/10.5194/amt-13-5537-2020, https://doi.org/10.5194/amt-13-5537-2020, 2020
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This paper is about a feasibility study of applying a machine learning technique to derive aerosol properties from a single MAX-DOAS sky scan, which detects sky-scattered UV–visible photons at multiple elevation angles. Evaluation of retrieved aerosol properties shows good performance of the ML algorithm, suggesting several advantages of a ML-based inversion algorithm such as fast data inversion, simple implementation and the ability to extract information not available using other algorithms.
Willem J. Marais, Robert E. Holz, Jeffrey S. Reid, and Rebecca M. Willett
Atmos. Meas. Tech., 13, 5459–5480, https://doi.org/10.5194/amt-13-5459-2020, https://doi.org/10.5194/amt-13-5459-2020, 2020
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Space agencies use moderate-resolution satellite imagery to study how smoke, dust, pollution (aerosols) and cloud types impact the Earth's climate; these space agencies include NASA, ESA and the China Meteorological Administration. We demonstrate in this paper that an algorithm with convolutional neural networks can greatly enhance the automated detection of aerosols and cloud types from satellite imagery. Our algorithm is an improvement on current aerosol and cloud detection algorithms.
Anin Puthukkudy, J. Vanderlei Martins, Lorraine A. Remer, Xiaoguang Xu, Oleg Dubovik, Pavel Litvinov, Brent McBride, Sharon Burton, and Henrique M. J. Barbosa
Atmos. Meas. Tech., 13, 5207–5236, https://doi.org/10.5194/amt-13-5207-2020, https://doi.org/10.5194/amt-13-5207-2020, 2020
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In this work, we report the demonstration and validation of the aerosol properties retrieved using AirHARP and GRASP for data from the NASA ACEPOL campaign 2017. These results serve as a proxy for the scale and detail of aerosol retrievals that are anticipated from future space mission data, as HARP CubeSat (mission begins 2020) and HARP2 (aboard the NASA PACE mission with the launch in 2023) are near duplicates of AirHARP and are expected to provide the same level of aerosol characterization.
Verena Schenzinger and Axel Kreuter
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-368, https://doi.org/10.5194/amt-2020-368, 2020
Revised manuscript accepted for AMT
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When measuring the aerosol optical depth of the atmosphere, clouds in front of the sun lead to erroneously high values. Therefore, measurements that are potentially affected by clouds need to be removed from the dataset by an automatic process. As the currently used algorithm cannot reliably identify thin clouds, we developed a new one based on a method borrowed from machine learning. Tests with 10 years of data show improved performance of the new routine and therefore higher data quality.
Felix Wrana, Christian von Savigny, Jacob Zalach, and Larry W. Thomason
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-277, https://doi.org/10.5194/amt-2020-277, 2020
Revised manuscript accepted for AMT
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In this paper we describe a new method to calculate the size of naturally occurring droplets (aerosols) made mostly of sulfuric acid and water, that can be found roughly in 20 km altitude in the atmosphere. For this we use data from the instrument SAGE III/ISS that is mounted on the International Space Station. We show that our method works well and that the size parameters we calculate are reasonable and can be a valuable addition to better understand the aerosols and their effect on climate.
Bradley M. Conrad and Matthew R. Johnson
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-255, https://doi.org/10.5194/amt-2020-255, 2020
Revised manuscript accepted for AMT
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A general uncertainty analysis (GUA) is performed for the sky-LOSA technique used to remotely measure soot emissions from gas flares. GUA data are compiled in an open-source software tool to help sky-LOSA users select critical setup and acquisition parameters while giving quantitative visual feedback on anticipated uncertainties for a specific measurement. The software tool enables easy acquisition of optimal measurement data, significantly increasing the accessibility of the sky-LOSA technique.
Patrick Chazette
Atmos. Meas. Tech., 13, 4461–4477, https://doi.org/10.5194/amt-13-4461-2020, https://doi.org/10.5194/amt-13-4461-2020, 2020
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By coupling lidar on board a ULA and ground-based lidar measurements, this paper highlights aerosol transport over the Strait of Gibraltar. It shows that the lidar-derived aerosol optical properties can be different from what is commonly accepted. It presents unprecedented vertical profiles over this region and relates them to the origin of air masses. The results are based on ground, airborne, and spaceborne observations, as well as multiple retro-trajectory analyses.
Travis N. Knepp, Larry Thomason, Marilee Roell, Robert Damadeo, Kevin Leavor, Thierry Leblanc, Fernando Chouza, Sergey Khaykin, Sophie Godin-Beekmann, and David Flittner
Atmos. Meas. Tech., 13, 4261–4276, https://doi.org/10.5194/amt-13-4261-2020, https://doi.org/10.5194/amt-13-4261-2020, 2020
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Two common measurements that represent atmospheric aerosol loading are the backscatter and extinction coefficients. Measuring backscatter and extinction coefficients requires different viewing geometries and fundamentally different instrument systems. Further, these coefficients are not directly comparable. We present an algorithm to convert SAGE-observed extinction coefficients to backscatter coefficients for intercomparison with lidar backscatter products, followed by evaluation of the method.
Meng Gao, Peng-Wang Zhai, Bryan A. Franz, Kirk Knobelspiesse, Amir Ibrahim, Brian Cairns, Susanne E. Craig, Guangliang Fu, Otto Hasekamp, Yongxiang Hu, and P. Jeremy Werdell
Atmos. Meas. Tech., 13, 3939–3956, https://doi.org/10.5194/amt-13-3939-2020, https://doi.org/10.5194/amt-13-3939-2020, 2020
Charles K. Gatebe, Hiren Jethva, Ritesh Gautam, Rajesh Poudyal, and Tamas Várnai
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-246, https://doi.org/10.5194/amt-2020-246, 2020
Revised manuscript accepted for AMT
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The retrieval of aerosol parameters from passive satellite instruments in cloudy scenes is challenging, partly because clouds and cloud-related processes may significantly modify the aerosol properties and partly because of the 3D radiative effects. This study shows demonstrate a novel airborne measurement approach for assessing satellite retrievals of aerosols above clouds using SAFARI 2000 field data over ocean, thereby filling a major gap that exists in the global aerosol observations.
Arantxa M. Triana-Gómez, Georg Heygster, Christian Melsheimer, Gunnar Spreen, Monia Negusini, and Boyan H. Petkov
Atmos. Meas. Tech., 13, 3697–3715, https://doi.org/10.5194/amt-13-3697-2020, https://doi.org/10.5194/amt-13-3697-2020, 2020
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In the Arctic, in situ measurements are sparse and standard remote sensing retrieval methods have problems. We present advances in a retrieval algorithm for vertically integrated water vapour tuned for polar regions. In addition to the initial sensor used (AMSU-B), we can now also use data from the successor instrument (MHS). Additionally, certain artefacts are now filtered out. Comparison with radiosondes shows the overall good performance of the updated algorithm.
Alexander Sinyuk, Brent N. Holben, Thomas F. Eck, David M. Giles, Ilya Slutsker, Sergey Korkin, Joel S. Schafer, Alexander Smirnov, Mikhail Sorokin, and Alexei Lyapustin
Atmos. Meas. Tech., 13, 3375–3411, https://doi.org/10.5194/amt-13-3375-2020, https://doi.org/10.5194/amt-13-3375-2020, 2020
Christian von Savigny and Christoph G. Hoffmann
Atmos. Meas. Tech., 13, 1909–1920, https://doi.org/10.5194/amt-13-1909-2020, https://doi.org/10.5194/amt-13-1909-2020, 2020
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Stratospheric sulfate aerosols increase the Earth's planetary albedo and can lead to significant surface cooling, for example in the aftermath of volcanic eruptions. Their particle size distribution, important for physical and chemical effects of these aerosols, is still not fully understood. The present paper proposes an explanation for systematic differences in aerosol particle size retrieved from measurements made in different measurement geometries and reported in earlier studies.
Florian Gaudfrin, Olivier Pujol, Romain Ceolato, Guillaume Huss, and Nicolas Riviere
Atmos. Meas. Tech., 13, 1921–1935, https://doi.org/10.5194/amt-13-1921-2020, https://doi.org/10.5194/amt-13-1921-2020, 2020
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A new elastic lidar inversion equation is presented. It is based on the backscattering signal from a surface reference target rather than that from a volumetric layer of reference as is usually done. The method presented can be used in the case of airborne elastic lidar measurements or when the lidar–target line is horizontal. Also, a new algorithm is described to retrieve the lidar ratio and the backscattering coefficient of an aerosol plume without any a priori assumptions about the plume.
Zhuoru Wang, Ka Lok Chan, Klaus-Peter Heue, Adrian Doicu, Thomas Wagner, Robert Holla, and Matthias Wiegner
Atmos. Meas. Tech., 13, 1835–1866, https://doi.org/10.5194/amt-13-1835-2020, https://doi.org/10.5194/amt-13-1835-2020, 2020
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We present a new aerosol profile retrieval algorithm for MAX-DOAS measurements at high-altitude sites and applied to the MAX-DOAS measurements at UFS. The retrieval algorithm is based on a O4 DSCD lookup table which is dedicated to high-altitude MAX-DOAS measurements. The comparison of retrieved aerosol optical depths (AODs) to sun photometer observations shows good agreement with a correlation coefficient (R) of 0.733 and 0.798 at 360 and 477 nm, respectively.
Elina Giannakaki, Panos Kokkalis, Eleni Marinou, Nikolaos S. Bartsotas, Vassilis Amiridis, Albert Ansmann, and Mika Komppula
Atmos. Meas. Tech., 13, 893–905, https://doi.org/10.5194/amt-13-893-2020, https://doi.org/10.5194/amt-13-893-2020, 2020
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A new method, called ElEx, is proposed for the estimation of extinction coefficient lidar profiles using only the information provided by the elastic and polarization channels of a lidar system. The method is applicable to lidar measurements both during daytime and nighttime under well-defined aerosol mixtures. Comparisons with both Raman lidar profiles during nightime and sun photometer daytime aerosol optical depth observations demonstrate the potential of the ElEx methodology.
Michael J. Garay, Marcin L. Witek, Ralph A. Kahn, Felix C. Seidel, James A. Limbacher, Michael A. Bull, David J. Diner, Earl G. Hansen, Olga V. Kalashnikova, Huikyo Lee, Abigail M. Nastan, and Yan Yu
Atmos. Meas. Tech., 13, 593–628, https://doi.org/10.5194/amt-13-593-2020, https://doi.org/10.5194/amt-13-593-2020, 2020
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The Multi-angle Imaging SpectroRadiometer (MISR) instrument has been operational since early 2000, creating an extensive data set of global Earth observations. Here we introduce the latest version (V23) of the MISR aerosol products, which is reported on a 4.4 km spatial grid and contains retrieved aerosol optical depth and aerosol particle property information derived over both land and water. The changes implemented in V23 have significant impacts on the data product and its interpretation.
Yanyu Wang, Rui Lyu, Xin Xie, Ze Meng, Meijin Huang, Junshi Wu, Haizhen Mu, Qiu-Run Yu, Qianshan He, and Tiantao Cheng
Atmos. Meas. Tech., 13, 575–592, https://doi.org/10.5194/amt-13-575-2020, https://doi.org/10.5194/amt-13-575-2020, 2020
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A satellite-based method for clear-sky aerosol direct radiative forcing (ADRF) retrieval and spatiotemporal characteristics of ADRF in eastern China were displayed during 2000–2016. Our analysis shows aerosols have a strong cooling effect at the surface, and the changes of ADRF are closely related to the changes of AOD with the development of economic growth and rapid urbanization in eastern China.
Jeremy E. Solbrig, Steven D. Miller, Jianglong Zhang, Lewis Grasso, and Anton Kliewer
Atmos. Meas. Tech., 13, 165–190, https://doi.org/10.5194/amt-13-165-2020, https://doi.org/10.5194/amt-13-165-2020, 2020
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New satellite sensors are able to view visible light, such as that emitted by cities, at night. It may be possible to use the light from cities to assess the amount of particulate matter in the atmosphere and the thickness of clouds. To do this we must understand how light emitted from the Earth's surface changes with time and viewing conditions. This study takes a step towards understanding the characteristics of light emitted by cities and its stability in time.
Swadhin Nanda, Martin de Graaf, J. Pepijn Veefkind, Mark ter Linden, Maarten Sneep, Johan de Haan, and Pieternel F. Levelt
Atmos. Meas. Tech., 12, 6619–6634, https://doi.org/10.5194/amt-12-6619-2019, https://doi.org/10.5194/amt-12-6619-2019, 2019
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This paper discusses a neural network forward model used by the operational aerosol layer height (ALH) retrieval algorithm for the TROPOspheric Monitoring Instrument (TROPOMI) on board the European Sentinel-5 Precursor satellite mission. This model replaces online radiative transfer calculations within the oxygen A-band, improving the speed of the algorithm by 3 orders of magnitude. With this advancement in the algorithm's speed, TROPOMI is set to deliver the ALH product operationally.
Pawan Gupta, Robert C. Levy, Shana Mattoo, Lorraine A. Remer, Robert E. Holz, and Andrew K. Heidinger
Atmos. Meas. Tech., 12, 6557–6577, https://doi.org/10.5194/amt-12-6557-2019, https://doi.org/10.5194/amt-12-6557-2019, 2019
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Aerosol optical depth (AOD) from a geostationary satellite has been retrieved, and validated and diurnal cycles of aerosols are discussed over the eastern hemisphere and a 2-month period of May–June 2016. The new AOD product matches well with AERONET as well as with the standard MODIS product. Future work to make this algorithm operational will need to re-examine masking including snow masks, re-evaluate assumed aerosol models for geosynchronous geometry and address the surface characterization.
Sabrina P. Cochrane, K. Sebastian Schmidt, Hong Chen, Peter Pilewskie, Scott Kittelman, Jens Redemann, Samuel LeBlanc, Kristina Pistone, Meloë Kacenelenbogen, Michal Segal Rozenhaimer, Yohei Shinozuka, Connor Flynn, Steven Platnick, Kerry Meyer, Rich Ferrare, Sharon Burton, Chris Hostetler, Steven Howell, Steffen Freitag, Amie Dobracki, and Sarah Doherty
Atmos. Meas. Tech., 12, 6505–6528, https://doi.org/10.5194/amt-12-6505-2019, https://doi.org/10.5194/amt-12-6505-2019, 2019
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For two cases from the NASA ORACLES experiments, we retrieve aerosol and cloud properties and calculate a direct aerosol radiative effect (DARE). We investigate the relationship between DARE and the cloud albedo by specifying the albedo for which DARE transitions from a cooling to warming radiative effect. Our new aerosol retrieval algorithm is successful despite complexities associated with scenes that contain aerosols above clouds and decreases the uncertainty on retrieved aerosol parameters.
Jiyunting Sun, Pepijn Veefkind, Swadhin Nanda, Peter van Velthoven, and Pieternel Levelt
Atmos. Meas. Tech., 12, 6319–6340, https://doi.org/10.5194/amt-12-6319-2019, https://doi.org/10.5194/amt-12-6319-2019, 2019
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Single scattering albedo (SSA) is critical for reducing uncertainties in radiative forcing assessment. This paper presents two methods to retrieve SSA from satellite observations of the near-UV absorbing aerosol index (UVAI). The first is physically based radiative transfer simulations; the second is a statistically based machine learning algorithm. The result of the latter is encouraging. Both methods show that the ALH is necessary to quantitatively interpret aerosol absorption from UVAI.
Rebecca M. Pauly, John E. Yorks, Dennis L. Hlavka, Matthew J. McGill, Vassilis Amiridis, Stephen P. Palm, Sharon D. Rodier, Mark A. Vaughan, Patrick A. Selmer, Andrew W. Kupchock, Holger Baars, and Anna Gialitaki
Atmos. Meas. Tech., 12, 6241–6258, https://doi.org/10.5194/amt-12-6241-2019, https://doi.org/10.5194/amt-12-6241-2019, 2019
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The Cloud Aerosol Transport System (CATS) demonstrated that direct calibration of 1064 nm lidar data from a spaceborne platform is possible. By normalizing the CATS signal to a modeled molecular backscatter profile the CATS data were calibrated, enabling the derivation of optical properties of clouds and aerosols. Comparisons of the calibrated signal with airborne lidar, ground-based lidar, and spaceborne lidar all show agreement within the estimated error bars of the respective instruments.
Jayanta Kar, Kam-Pui Lee, Mark A. Vaughan, Jason L. Tackett, Charles R. Trepte, David M. Winker, Patricia L. Lucker, and Brian J. Getzewich
Atmos. Meas. Tech., 12, 6173–6191, https://doi.org/10.5194/amt-12-6173-2019, https://doi.org/10.5194/amt-12-6173-2019, 2019
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This work describes the science algorithm for the recently released CALIPSO level 3 stratospheric aerosol product. It is shown that the retrieved extinction profiles capture the major stratospheric perturbations over the last decade resulting from volcanic eruptions, pyroCb smoke events, and signatures of stratospheric dynamics. An initial assessment is also provided by intercomparison with the latest aerosol retrievals from the SAGE III instrument aboard the International Space Station.
Steffen Mauceri, Bruce Kindel, Steven Massie, and Peter Pilewskie
Atmos. Meas. Tech., 12, 6017–6036, https://doi.org/10.5194/amt-12-6017-2019, https://doi.org/10.5194/amt-12-6017-2019, 2019
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Aerosols are fine particles that are suspended in Earth’s atmosphere. A better understanding of aerosols is important to lower uncertainties in climate predictions. We propose measuring aerosols from satellites and airplanes equipped with hyperspectral cameras using an artificial neural network, a form of machine learning. We applied our neural network to hyperspectral observations from a recent airplane flight over India and find general agreement with independent aerosol measurements.
Pasquale Sellitto, Henda Guermazi, Elisa Carboni, Richard Siddans, and Mike Burton
Atmos. Meas. Tech., 12, 5381–5389, https://doi.org/10.5194/amt-12-5381-2019, https://doi.org/10.5194/amt-12-5381-2019, 2019
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Volcanoes release complex plumes of gas and particles. Volcanic gases, like SO2, can additionally condense, once released, to form particles, sulphate aerosol (SA). Observing simultaneously SO2+SA is important: their proportion provides information on the internal state of volcanoes, and can be used to predict plumes' atmospheric evolution and their environmental and climatic impacts. We developed a new method to observe simultaneously, for the first time, SO2+SA using infrared remote sensing.
Martin de Graaf, L. Gijsbert Tilstra, and Piet Stammes
Atmos. Meas. Tech., 12, 5119–5135, https://doi.org/10.5194/amt-12-5119-2019, https://doi.org/10.5194/amt-12-5119-2019, 2019
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A new algorithm is described, which was used to derive direct radiative effects of aerosols above clouds. These effects are among the largest uncertainties in global climate model simulations, and observations are needed to constrain these simulations. A recently developed method was applied to a combination of satellite reflectance measurements to cover the entire shortwave (solar) spectrum. Radiative effects of aerosols over the south-east Atlantic are presented, where the effects are largest.
Steven D. Miller, Louie D. Grasso, Qijing Bian, Sonia M. Kreidenweis, Jack F. Dostalek, Jeremy E. Solbrig, Jennifer Bukowski, Susan C. van den Heever, Yi Wang, Xiaoguang Xu, Jun Wang, Annette L. Walker, Ting-Chi Wu, Milija Zupanski, Christine Chiu, and Jeffrey S. Reid
Atmos. Meas. Tech., 12, 5101–5118, https://doi.org/10.5194/amt-12-5101-2019, https://doi.org/10.5194/amt-12-5101-2019, 2019
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Satellite–based detection of lofted mineral via infrared–window channels, well established in the literature, faces significant challenges in the presence of atmospheric moisture. Here, we consider a case featuring the juxtaposition of two dust plumes embedded within dry and moist air masses. The case is considered from the vantage points of numerical modeling, multi–sensor observations, and radiative transfer theory arriving at a new method for mitigating the water vapor masking effect.
Albert Ansmann, Rodanthi-Elisavet Mamouri, Julian Hofer, Holger Baars, Dietrich Althausen, and Sabur F. Abdullaev
Atmos. Meas. Tech., 12, 4849–4865, https://doi.org/10.5194/amt-12-4849-2019, https://doi.org/10.5194/amt-12-4849-2019, 2019
Matthias Tesche, Alexei Kolgotin, Moritz Haarig, Sharon P. Burton, Richard A. Ferrare, Chris A. Hostetler, and Detlef Müller
Atmos. Meas. Tech., 12, 4421–4437, https://doi.org/10.5194/amt-12-4421-2019, https://doi.org/10.5194/amt-12-4421-2019, 2019
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Today, few lidar are capable of triple-wavelength particle linear depolarization ratio (PLDR) measurements. This study is the first systematic investigation of the effect of different choices of PLDR input on the inversion of lidar measurements of mineral dust and dusty mixtures using light scattering by randomly oriented spheroids. We provide recommendations of the most suitable input parameters for use with the applied methodology, based on a relational assessment of the inversion output.
Gregori de Arruda Moreira, Fábio Juliano da Silva Lopes, Juan Luis Guerrero-Rascado, Jonatan João da Silva, Antonio Arleques Gomes, Eduardo Landulfo, and Lucas Alados-Arboledas
Atmos. Meas. Tech., 12, 4261–4276, https://doi.org/10.5194/amt-12-4261-2019, https://doi.org/10.5194/amt-12-4261-2019, 2019
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In this paper, we present a comparative analysis of the use of lidar-backscattered signals at three wavelengths (355, 532 and 1064 nm) to study the ABL by investigating high-order moments, which gives us information about the ABL height (derived using the variance method), aerosol layer movements (skewness) and mixing conditions (kurtosis) at several heights.
Arvid Langenbach, Gerd Baumgarten, Jens Fiedler, Franz-Josef Lübken, Christian von Savigny, and Jacob Zalach
Atmos. Meas. Tech., 12, 4065–4076, https://doi.org/10.5194/amt-12-4065-2019, https://doi.org/10.5194/amt-12-4065-2019, 2019
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Stratospheric aerosol backscatter ratios in the Arctic using Rayleigh, Mie and Raman backscattered signals were calculated. A backscatter ratio calculation during daytime was performed for the first time. Sharp aerosol layers thinner than 1 km over several days were observed. The seasonal cycle of stratospheric background aerosol in high latitudes including the summer months was calculated for the first time. Top altitude of the aerosol layer was found to reach up to 34 km, especially in summer.
Meng Gao, Peng-Wang Zhai, Bryan A. Franz, Yongxiang Hu, Kirk Knobelspiesse, P. Jeremy Werdell, Amir Ibrahim, Brian Cairns, and Alison Chase
Atmos. Meas. Tech., 12, 3921–3941, https://doi.org/10.5194/amt-12-3921-2019, https://doi.org/10.5194/amt-12-3921-2019, 2019
Isabelle A. Taylor, Elisa Carboni, Lucy J. Ventress, Tamsin A. Mather, and Roy G. Grainger
Atmos. Meas. Tech., 12, 3853–3883, https://doi.org/10.5194/amt-12-3853-2019, https://doi.org/10.5194/amt-12-3853-2019, 2019
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Volcanic ash is a hazard associated with volcanoes. Knowing an ash cloud’s location is essential for minimising the hazard. This includes knowing the height. This study adapted a well-known technique for obtaining the height of meteorological clouds, known as CO2 slicing, for volcanic ash. Modelled data were used to refine the method and then demonstrate that the technique could work for volcanic ash. It was then successfully applied to data from the Eyjafjallajökull and Grímsvötn eruptions.
Wangshu Tan, Gang Zhao, Yingli Yu, Chengcai Li, Jian Li, Ling Kang, Tong Zhu, and Chunsheng Zhao
Atmos. Meas. Tech., 12, 3825–3839, https://doi.org/10.5194/amt-12-3825-2019, https://doi.org/10.5194/amt-12-3825-2019, 2019
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A new method to retrieve CCN number concentrations using multiwavelength Raman lidars is proposed. The method implements hygroscopic enhancements of backscatter and extinction with relative humidity to represent particle hygroscopicity. The retrieved CCN number concentrations are in good agreement with theoretical calculated values. Sensitivity tests indicate that retrieval error in CCN arises mostly from uncertainties in extinction coefficients and RH profiles.
Sung-Kyun Shin, Matthias Tesche, Youngmin Noh, and Detlef Müller
Atmos. Meas. Tech., 12, 3789–3803, https://doi.org/10.5194/amt-12-3789-2019, https://doi.org/10.5194/amt-12-3789-2019, 2019
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This study proposes an aerosol-type classification based on parameters from the AErosol RObotic NETwork (AERONET) version 3 level 2.0 inversion product that describe light depolarization and absorption properties of atmospheric particles.
We compare our classification with an earlier method and find that the new approach allows for a refined classification of mineral dust that occurs as a mixture with other absorbing aerosols.
Sieglinde Callewaert, Sophie Vandenbussche, Nicolas Kumps, Arve Kylling, Xiaoxia Shang, Mika Komppula, Philippe Goloub, and Martine De Mazière
Atmos. Meas. Tech., 12, 3673–3698, https://doi.org/10.5194/amt-12-3673-2019, https://doi.org/10.5194/amt-12-3673-2019, 2019
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This article presents the updated MAPIR algorithm, which uses infrared satellite data to obtain the global 3-D distribution of mineral aerosols. A description of the method together with its technical improvements is given. Additionally, a 10-year data set was generated and used to evaluate this new algorithm against AERONET, CALIOP, CATS and two ground-based lidar stations. We have shown that the new MAPIR algorithm provides reliable aerosol optical depth and dust layer mean altitude profiles.
Andrew M. Sayer, N. Christina Hsu, Jaehwa Lee, Woogyung V. Kim, Sharon Burton, Marta A. Fenn, Richard A. Ferrare, Meloë Kacenelenbogen, Samuel LeBlanc, Kristina Pistone, Jens Redemann, Michal Segal-Rozenhaimer, Yohei Shinozuka, and Si-Chee Tsay
Atmos. Meas. Tech., 12, 3595–3627, https://doi.org/10.5194/amt-12-3595-2019, https://doi.org/10.5194/amt-12-3595-2019, 2019
Short summary
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Aerosols are small particles in the atmosphere such as dust or smoke. They are routinely monitored by satellites due to their importance for climate and air quality. However aerosols above clouds are more difficult to monitor. This study describes an improvement to a technique to monitor light-absorbing aerosols above clouds from four Earth-orbiting satellite instruments. The improved method is evaluated using data from the ORACLES field campaign, which measured these aerosols from aircraft.
Xiaoguang Xu, Jun Wang, Yi Wang, Jing Zeng, Omar Torres, Jeffrey S. Reid, Steven D. Miller, J. Vanderlei Martins, and Lorraine A. Remer
Atmos. Meas. Tech., 12, 3269–3288, https://doi.org/10.5194/amt-12-3269-2019, https://doi.org/10.5194/amt-12-3269-2019, 2019
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Detecting aerosol layer height from space is challenging. The traditional method relies on active sensors such as lidar that provide the detailed vertical structure of the aerosol profile but is costly with limited spatial coverage (more than 1 year is needed for global coverage). Here we developed a passive remote sensing technique that uses backscattered sunlight to retrieve smoke aerosol layer height over both water and vegetated surfaces from a sensor 1.5 million kilometers from the Earth.
Chengzhi Xing, Cheng Liu, Shanshan Wang, Qihou Hu, Haoran Liu, Wei Tan, Wenqiang Zhang, Bo Li, and Jianguo Liu
Atmos. Meas. Tech., 12, 3289–3302, https://doi.org/10.5194/amt-12-3289-2019, https://doi.org/10.5194/amt-12-3289-2019, 2019
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Ground-based MAX-DOAS has been utilized for the remote sensing of aerosol and trace gases for more than 10 years. Here we developed a new method to determine the aerosol optical properties, including scattering and absorption, from multiple-wavelength O4 absorptions from ground-based MAX-DOAS observations, which were validated well by other independent instruments at low elevations. It is beneficial to obtain the vertical profiles of aerosol properties using multiple elevations.
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