Articles | Volume 14, issue 6
https://doi.org/10.5194/amt-14-3989-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-14-3989-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
02 Jun 2021
Research article |
| 02 Jun 2021
| 02 Jun 2021
MICRU: an effective cloud fraction algorithm designed for UV–vis satellite instruments with large viewing angles
Max Planck Institute for Chemistry, Hahn-Meitner-Weg 1, Mainz, Germany
Steffen Beirle
Max Planck Institute for Chemistry, Hahn-Meitner-Weg 1, Mainz, Germany
Steffen Dörner
Max Planck Institute for Chemistry, Hahn-Meitner-Weg 1, Mainz, Germany
Marloes Gutenstein-Penning de Vries
Max Planck Institute for Chemistry, Hahn-Meitner-Weg 1, Mainz, Germany
now at: Faculty of Geo-Information Science and Earth Observation, University of Twente, Enschede, the Netherlands
Christoph Hörmann
Max Planck Institute for Chemistry, Hahn-Meitner-Weg 1, Mainz, Germany
now at: Volume Graphics GmbH, Heidelberg, Germany
Christian Borger
Max Planck Institute for Chemistry, Hahn-Meitner-Weg 1, Mainz, Germany
Simon Warnach
Max Planck Institute for Chemistry, Hahn-Meitner-Weg 1, Mainz, Germany
Thomas Wagner
Max Planck Institute for Chemistry, Hahn-Meitner-Weg 1, Mainz, Germany
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Ka Lok Chan, Pieter Valks, Klaus-Peter Heue, Ronny Lutz, Pascal Hedelt, Diego Loyola, Gaia Pinardi, Michel Van Roozendael, François Hendrick, Thomas Wagner, Vinod Kumar, Alkis Bais, Ankie Piters, Hitoshi Irie, Hisahiro Takashima, Yugo Kanaya, Yongjoo Choi, Kihong Park, Jihyo Chong, Alexander Cede, Udo Frieß, Andreas Richter, Jianzhong Ma, Nuria Benavent, Robert Holla, Oleg Postylyakov, Claudia Rivera Cárdenas, and Mark Wenig
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Thomas Wagner, Simon Warnach, Steffen Beirle, Nicole Bobrowski, Adrian Jost, Janis Puķīte, and Nicolas Theys
Atmos. Meas. Tech., 16, 1609–1662, https://doi.org/10.5194/amt-16-1609-2023, https://doi.org/10.5194/amt-16-1609-2023, 2023
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We investigate 3D effects of volcanic plumes on the retrieval results of satellite and ground-based UV–Vis observations. With its small ground pixels of 3.5 x 5.5 km², the TROPOMI instrument can detect much smaller volcanic plumes than previous instruments. At the same time, 3D effects become important. The effect of horizontal photon paths especially can lead to a strong underestimation of the derived plume contents of up to > 50 %, which can be further increased for strong absorbers like SO2.
Siyang Cheng, Xinghong Cheng, Jianzhong Ma, Xiangde Xu, Wenqian Zhang, Jinguang Lv, Gang Bai, Bing Chen, Siying Ma, Steffen Ziegler, Sebastian Donner, and Thomas Wagner
Atmos. Chem. Phys., 23, 3655–3677, https://doi.org/10.5194/acp-23-3655-2023, https://doi.org/10.5194/acp-23-3655-2023, 2023
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We made mobile MAX-DOAS measurements in the background atmosphere over the Tibetan Plateau in summer 2021. We retrieved the tropospheric NO2 and HCHO vertical column densities (VCDs) along extended driving routes and found a decreasing trend of the VCDs with altitude. Elevated NO2 VCDs along the driving routes could be attributed to enhanced traffic emissions from the towns crossed. The spatio-temporal distribution of the HCHO VCDs correlated strongly with the surface temperature.
Kezia Lange, Andreas Richter, Anja Schönhardt, Andreas C. Meier, Tim Bösch, André Seyler, Kai Krause, Lisa K. Behrens, Folkard Wittrock, Alexis Merlaud, Frederik Tack, Caroline Fayt, Martina M. Friedrich, Ermioni Dimitropoulou, Michel Van Roozendael, Vinod Kumar, Sebastian Donner, Steffen Dörner, Bianca Lauster, Maria Razi, Christian Borger, Katharina Uhlmannsiek, Thomas Wagner, Thomas Ruhtz, Henk Eskes, Birger Bohn, Daniel Santana Diaz, Nader Abuhassan, Dirk Schüttemeyer, and John P. Burrows
Atmos. Meas. Tech., 16, 1357–1389, https://doi.org/10.5194/amt-16-1357-2023, https://doi.org/10.5194/amt-16-1357-2023, 2023
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Bianca Lauster, Steffen Dörner, Carl-Fredrik Enell, Udo Frieß, Myojeong Gu, Janis Puķīte, Uwe Raffalski, and Thomas Wagner
Atmos. Chem. Phys., 22, 15925–15942, https://doi.org/10.5194/acp-22-15925-2022, https://doi.org/10.5194/acp-22-15925-2022, 2022
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Polar stratospheric clouds (PSCs) are an important component in ozone chemistry. Here, we use two differential optical absorption spectroscopy (DOAS) instruments in the Antarctic and Arctic to investigate the occurrence of PSCs based on the colour index, i.e. the colour of the zenith sky. Additionally using radiative transfer simulations, the variability and the seasonal cycle of PSC occurrence are analysed and an unexpectedly high signal during spring suggests the influence of volcanic aerosol.
Miriam Latsch, Andreas Richter, Henk Eskes, Maarten Sneep, Ping Wang, Pepijn Veefkind, Ronny Lutz, Diego Loyola, Athina Argyrouli, Pieter Valks, Thomas Wagner, Holger Sihler, Michel van Roozendael, Nicolas Theys, Huan Yu, Richard Siddans, and John P. Burrows
Atmos. Meas. Tech., 15, 6257–6283, https://doi.org/10.5194/amt-15-6257-2022, https://doi.org/10.5194/amt-15-6257-2022, 2022
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The article investigates different S5P TROPOMI cloud retrieval algorithms for tropospheric trace gas retrievals. The cloud products show differences primarily over snow and ice and for scenes under sun glint. Some issues regarding across-track dependence are found for the cloud fractions as well as for the cloud heights.
Maximilian Herrmann, Moritz Schöne, Christian Borger, Simon Warnach, Thomas Wagner, Ulrich Platt, and Eva Gutheil
Atmos. Chem. Phys., 22, 13495–13526, https://doi.org/10.5194/acp-22-13495-2022, https://doi.org/10.5194/acp-22-13495-2022, 2022
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Ozone depletion events (ODEs) are a common occurrence in the boundary layer during Arctic spring. Ozone is depleted by bromine species in an autocatalytic reaction cycle. Previous modeling studies assumed an infinite bromine source at the ground. An alternative emission scheme is presented in which a finite amount of bromide in the snow is tracked over time. The Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) is used to study ODEs in the Arctic from February to May 2019.
Christian Borger, Steffen Beirle, and Thomas Wagner
Atmos. Chem. Phys., 22, 10603–10621, https://doi.org/10.5194/acp-22-10603-2022, https://doi.org/10.5194/acp-22-10603-2022, 2022
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In this study, we analyse trends of total column water vapour (TCWV) using multiple years of satellite observations and find, on the global average, an increase in the TCWV amount by about 0.21 % per year. Further investigations of the hydrological cycle reveal that the assumption of temporally invariant relative humidity is not always fulfilled and that the response of the global water vapour turnover time to global warming is 2 to 3 times higher than previously reported values.
Gaia Pinardi, Michel Van Roozendael, François Hendrick, Andreas Richter, Pieter Valks, Ramina Alwarda, Kristof Bognar, Udo Frieß, José Granville, Myojeong Gu, Paul Johnston, Cristina Prados-Roman, Richard Querel, Kimberly Strong, Thomas Wagner, Folkard Wittrock, and Margarita Yela Gonzalez
Atmos. Meas. Tech., 15, 3439–3463, https://doi.org/10.5194/amt-15-3439-2022, https://doi.org/10.5194/amt-15-3439-2022, 2022
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We report on the GOME-2A and GOME-2B OClO dataset (2007 to 2016, from the EUMETSAT's AC SAF) validation using data from nine NDACC zenith-scattered-light DOAS (ZSL-DOAS) instruments distributed in both the Arctic and Antarctic. Specific sensitivity tests are performed on the ground-based data to estimate the impact of the different OClO DOAS analysis settings and their typical errors. Good agreement is found for both the inter-annual variability and the overall OClO seasonal behavior.
Gerrit Kuhlmann, Ka Lok Chan, Sebastian Donner, Ying Zhu, Marc Schwaerzel, Steffen Dörner, Jia Chen, Andreas Hueni, Duc Hai Nguyen, Alexander Damm, Annette Schütt, Florian Dietrich, Dominik Brunner, Cheng Liu, Brigitte Buchmann, Thomas Wagner, and Mark Wenig
Atmos. Meas. Tech., 15, 1609–1629, https://doi.org/10.5194/amt-15-1609-2022, https://doi.org/10.5194/amt-15-1609-2022, 2022
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Nitrogen dioxide (NO2) is an air pollutant whose concentration often exceeds air quality guideline values, especially in urban areas. To map the spatial distribution of NO2 in Munich, we conducted the Munich NO2 Imaging Campaign (MuNIC), where NO2 was measured with stationary, mobile, and airborne in situ and remote sensing instruments. The campaign provides a unique dataset that has been used to compare the different instruments and to study the spatial variability of NO2 and its sources.
Leon Kuhn, Jonas Kuhn, Thomas Wagner, and Ulrich Platt
Atmos. Meas. Tech., 15, 1395–1414, https://doi.org/10.5194/amt-15-1395-2022, https://doi.org/10.5194/amt-15-1395-2022, 2022
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We present a novel instrument for imaging measurements of NO2 with high spatiotemporal resolution based on gas correlation spectroscopy, called the GCS NO2 camera. The instrument works by placing two gas cells (cuvettes) in front of two photosensor arrays, one filled with air and one filled with a high concentration of NO2, acting as a non-dispersive spectral filter. NO2 images are then generated on the basis of the signal ratio of the two channels in the spectral region of 430–445 nm.
Dimitris Karagkiozidis, Martina Michaela Friedrich, Steffen Beirle, Alkiviadis Bais, François Hendrick, Kalliopi Artemis Voudouri, Ilias Fountoulakis, Angelos Karanikolas, Paraskevi Tzoumaka, Michel Van Roozendael, Dimitris Balis, and Thomas Wagner
Atmos. Meas. Tech., 15, 1269–1301, https://doi.org/10.5194/amt-15-1269-2022, https://doi.org/10.5194/amt-15-1269-2022, 2022
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In this study we focus on the retrieval of aerosol, NO2, and HCHO vertical profiles from multi-axis differential optical absorption spectroscopy (MAX-DOAS) observations for the first time over Thessaloniki, Greece. We use two independent inversion algorithms for the profile retrievals. We evaluate their performance, we intercompare their results, and we validate their products with ancillary data, measured by other co-located reference instruments.
Steffen Beirle, Christian Borger, Steffen Dörner, Vinod Kumar, and Thomas Wagner
Atmos. Meas. Tech., 15, 987–1006, https://doi.org/10.5194/amt-15-987-2022, https://doi.org/10.5194/amt-15-987-2022, 2022
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We present a formalism that relates the vertical column density (VCD) of the oxygen collision complex O4 to surface values of temperature and pressure, based on physical laws. In addition, we propose an empirical modification which also accounts for surface relative humidity (RH). This allows for simple and quick but still accurate calculation of the O4 VCD without the need for constructing full vertical profiles, which is expected to be useful in particular for MAX-DOAS applications.
Fei Liu, Zhining Tao, Steffen Beirle, Joanna Joiner, Yasuko Yoshida, Steven J. Smith, K. Emma Knowland, and Thomas Wagner
Atmos. Chem. Phys., 22, 1333–1349, https://doi.org/10.5194/acp-22-1333-2022, https://doi.org/10.5194/acp-22-1333-2022, 2022
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In this work, we present a novel method to infer NOx emissions and lifetimes based on tropospheric NO2 observations together with reanalysis wind fields for cities located in polluted backgrounds. We evaluate the accuracy of the method using synthetic NO2 observations derived from a high-resolution model simulation. Our work provides an estimate for uncertainties in satellite-derived emissions inferred from chemical transport model (CTM)-independent approaches.
Tobias Küchler, Stefan Noël, Heinrich Bovensmann, John Philip Burrows, Thomas Wagner, Christian Borger, Tobias Borsdorff, and Andreas Schneider
Atmos. Meas. Tech., 15, 297–320, https://doi.org/10.5194/amt-15-297-2022, https://doi.org/10.5194/amt-15-297-2022, 2022
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We applied the air-mass-corrected differential optical absorption spectroscopy (AMC-DOAS) method to derive total column water vapour (TCWV) from Sentinel-5P measurements and compared it to independent data sets. The correlation coefficients of typically more than 0.9 and the small deviations up to 2.5 kg m−2 reveal good agreement between our data product and other TCWV data sets. In particular for the different Sentinel-5P water vapour products, the deviations are around 1 kg m−2.
Jānis Puķīte, Christian Borger, Steffen Dörner, Myojeong Gu, and Thomas Wagner
Atmos. Chem. Phys., 22, 245–272, https://doi.org/10.5194/acp-22-245-2022, https://doi.org/10.5194/acp-22-245-2022, 2022
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Chlorine dioxide (OClO) is an indicator for chlorine activation. New OClO data by TROPOMI (S5P) are interpreted in a meteorological context and related to CALIOP PSC observations. We report very high OClO levels for the northern hemispheric winter 2019/20 with an extraordinarily long period with a stable polar vortex. A minor stratospheric warming in the Southern Hemisphere was also observed in September 2019, where usual OClO values rapidly deactivated 1–2 weeks earlier.
Jonas Kuhn, Nicole Bobrowski, Thomas Wagner, and Ulrich Platt
Atmos. Meas. Tech., 14, 7873–7892, https://doi.org/10.5194/amt-14-7873-2021, https://doi.org/10.5194/amt-14-7873-2021, 2021
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We propose spectrograph implementations using Fabry–Pérot interferometers for atmospheric trace gas remote sensing. Compared with widely used grating spectrographs, we find substantial light throughput and mobility advantages for high resolving powers. Besides lowering detection limits and increasing the spatial and temporal resolution of many atmospheric trace gas measurements, this approach might enable remote sensing of further important gases such as tropospheric OH radicals.
Christophe Lerot, François Hendrick, Michel Van Roozendael, Leonardo M. A. Alvarado, Andreas Richter, Isabelle De Smedt, Nicolas Theys, Jonas Vlietinck, Huan Yu, Jeroen Van Gent, Trissevgeni Stavrakou, Jean-François Müller, Pieter Valks, Diego Loyola, Hitoshi Irie, Vinod Kumar, Thomas Wagner, Stefan F. Schreier, Vinayak Sinha, Ting Wang, Pucai Wang, and Christian Retscher
Atmos. Meas. Tech., 14, 7775–7807, https://doi.org/10.5194/amt-14-7775-2021, https://doi.org/10.5194/amt-14-7775-2021, 2021
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Global measurements of glyoxal tropospheric columns from the satellite instrument TROPOMI are presented. Such measurements can contribute to the estimation of atmospheric emissions of volatile organic compounds. This new glyoxal product has been fully characterized with a comprehensive error budget, with comparison with other satellite data sets as well as with validation based on independent ground-based remote sensing glyoxal observations.
Jānis Puķīte, Christian Borger, Steffen Dörner, Myojeong Gu, Udo Frieß, Andreas Carlos Meier, Carl-Fredrik Enell, Uwe Raffalski, Andreas Richter, and Thomas Wagner
Atmos. Meas. Tech., 14, 7595–7625, https://doi.org/10.5194/amt-14-7595-2021, https://doi.org/10.5194/amt-14-7595-2021, 2021
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Chlorine dioxide (OClO) is used as an indicator for chlorine activation. We present a new differential optical absorption spectroscopy retrieval algorithm for OClO from measurements of TROPOMI on the Sentinel-5P satellite. To achieve a substantially improved accuracy for the weak absorber OClO, we consider several additional fit parameters accounting for various higher-order spectral effects. The retrieved OClO slant column densities are compared with ground-based zenith sky measurements.
Song Liu, Pieter Valks, Gaia Pinardi, Jian Xu, Ka Lok Chan, Athina Argyrouli, Ronny Lutz, Steffen Beirle, Ehsan Khorsandi, Frank Baier, Vincent Huijnen, Alkiviadis Bais, Sebastian Donner, Steffen Dörner, Myrto Gratsea, François Hendrick, Dimitris Karagkiozidis, Kezia Lange, Ankie J. M. Piters, Julia Remmers, Andreas Richter, Michel Van Roozendael, Thomas Wagner, Mark Wenig, and Diego G. Loyola
Atmos. Meas. Tech., 14, 7297–7327, https://doi.org/10.5194/amt-14-7297-2021, https://doi.org/10.5194/amt-14-7297-2021, 2021
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In this work, an improved tropospheric NO2 retrieval algorithm from TROPOMI measurements over Europe is presented. The stratospheric estimation is implemented with correction for the dependency of the stratospheric NO2 on the viewing geometry. The AMF calculation is implemented using improved surface albedo, a priori NO2 profiles, and cloud correction. The improved tropospheric NO2 data show good correlations with ground-based MAX-DOAS measurements.
Nicolas Theys, Vitali Fioletov, Can Li, Isabelle De Smedt, Christophe Lerot, Chris McLinden, Nickolay Krotkov, Debora Griffin, Lieven Clarisse, Pascal Hedelt, Diego Loyola, Thomas Wagner, Vinod Kumar, Antje Innes, Roberto Ribas, François Hendrick, Jonas Vlietinck, Hugues Brenot, and Michel Van Roozendael
Atmos. Chem. Phys., 21, 16727–16744, https://doi.org/10.5194/acp-21-16727-2021, https://doi.org/10.5194/acp-21-16727-2021, 2021
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We present a new algorithm to retrieve sulfur dioxide from space UV measurements. We apply the technique to high-resolution TROPOMI measurements and demonstrate the high sensitivity of the approach to weak SO2 emissions worldwide with an unprecedented limit of detection of 8 kt yr−1. This result has broad implications for atmospheric science studies dealing with improving emission inventories and identifying and quantifying missing sources, in the context of air quality and climate.
Ulrich Platt, Thomas Wagner, Jonas Kuhn, and Thomas Leisner
Atmos. Meas. Tech., 14, 6867–6883, https://doi.org/10.5194/amt-14-6867-2021, https://doi.org/10.5194/amt-14-6867-2021, 2021
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Absorption spectroscopy of scattered sunlight is extremely useful for the analysis of atmospheric trace gas distributions. A central parameter for the achievable sensitivity of spectroscopic instruments is the light throughput, which can be enhanced in a number of ways. We present new ideas and considerations of how instruments could be optimized. Particular emphasis is on arrays of massively parallel instruments. Such arrays can reduce the size and weight of instruments by orders of magnitude.
Xin Tian, Yang Wang, Steffen Beirle, Pinhua Xie, Thomas Wagner, Jin Xu, Ang Li, Steffen Dörner, Bo Ren, and Xiaomei Li
Atmos. Chem. Phys., 21, 12867–12894, https://doi.org/10.5194/acp-21-12867-2021, https://doi.org/10.5194/acp-21-12867-2021, 2021
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The performances of two MAX-DOAS inversion algorithms were evaluated for various aerosol pollution scenarios. One inversion algorithm is based on optimal estimation; the other uses a parameterized approach. In this analysis, three types of profile shapes for aerosols and NO2 were considered: exponential, Boltzmann, and Gaussian. The evaluation results can effectively guide the application of the two inversion algorithms in the actual atmosphere and improve the accuracy of the actual inversion.
Bjorn Stevens, Sandrine Bony, David Farrell, Felix Ament, Alan Blyth, Christopher Fairall, Johannes Karstensen, Patricia K. Quinn, Sabrina Speich, Claudia Acquistapace, Franziska Aemisegger, Anna Lea Albright, Hugo Bellenger, Eberhard Bodenschatz, Kathy-Ann Caesar, Rebecca Chewitt-Lucas, Gijs de Boer, Julien Delanoë, Leif Denby, Florian Ewald, Benjamin Fildier, Marvin Forde, Geet George, Silke Gross, Martin Hagen, Andrea Hausold, Karen J. Heywood, Lutz Hirsch, Marek Jacob, Friedhelm Jansen, Stefan Kinne, Daniel Klocke, Tobias Kölling, Heike Konow, Marie Lothon, Wiebke Mohr, Ann Kristin Naumann, Louise Nuijens, Léa Olivier, Robert Pincus, Mira Pöhlker, Gilles Reverdin, Gregory Roberts, Sabrina Schnitt, Hauke Schulz, A. Pier Siebesma, Claudia Christine Stephan, Peter Sullivan, Ludovic Touzé-Peiffer, Jessica Vial, Raphaela Vogel, Paquita Zuidema, Nicola Alexander, Lyndon Alves, Sophian Arixi, Hamish Asmath, Gholamhossein Bagheri, Katharina Baier, Adriana Bailey, Dariusz Baranowski, Alexandre Baron, Sébastien Barrau, Paul A. Barrett, Frédéric Batier, Andreas Behrendt, Arne Bendinger, Florent Beucher, Sebastien Bigorre, Edmund Blades, Peter Blossey, Olivier Bock, Steven Böing, Pierre Bosser, Denis Bourras, Pascale Bouruet-Aubertot, Keith Bower, Pierre Branellec, Hubert Branger, Michal Brennek, Alan Brewer, Pierre-Etienne Brilouet, Björn Brügmann, Stefan A. Buehler, Elmo Burke, Ralph Burton, Radiance Calmer, Jean-Christophe Canonici, Xavier Carton, Gregory Cato Jr., Jude Andre Charles, Patrick Chazette, Yanxu Chen, Michal T. Chilinski, Thomas Choularton, Patrick Chuang, Shamal Clarke, Hugh Coe, Céline Cornet, Pierre Coutris, Fleur Couvreux, Susanne Crewell, Timothy Cronin, Zhiqiang Cui, Yannis Cuypers, Alton Daley, Gillian M. Damerell, Thibaut Dauhut, Hartwig Deneke, Jean-Philippe Desbios, Steffen Dörner, Sebastian Donner, Vincent Douet, Kyla Drushka, Marina Dütsch, André Ehrlich, Kerry Emanuel, Alexandros Emmanouilidis, Jean-Claude Etienne, Sheryl Etienne-Leblanc, Ghislain Faure, Graham Feingold, Luca Ferrero, Andreas Fix, Cyrille Flamant, Piotr Jacek Flatau, Gregory R. Foltz, Linda Forster, Iulian Furtuna, Alan Gadian, Joseph Galewsky, Martin Gallagher, Peter Gallimore, Cassandra Gaston, Chelle Gentemann, Nicolas Geyskens, Andreas Giez, John Gollop, Isabelle Gouirand, Christophe Gourbeyre, Dörte de Graaf, Geiske E. de Groot, Robert Grosz, Johannes Güttler, Manuel Gutleben, Kashawn Hall, George Harris, Kevin C. Helfer, Dean Henze, Calvert Herbert, Bruna Holanda, Antonio Ibanez-Landeta, Janet Intrieri, Suneil Iyer, Fabrice Julien, Heike Kalesse, Jan Kazil, Alexander Kellman, Abiel T. Kidane, Ulrike Kirchner, Marcus Klingebiel, Mareike Körner, Leslie Ann Kremper, Jan Kretzschmar, Ovid Krüger, Wojciech Kumala, Armin Kurz, Pierre L'Hégaret, Matthieu Labaste, Tom Lachlan-Cope, Arlene Laing, Peter Landschützer, Theresa Lang, Diego Lange, Ingo Lange, Clément Laplace, Gauke Lavik, Rémi Laxenaire, Caroline Le Bihan, Mason Leandro, Nathalie Lefevre, Marius Lena, Donald Lenschow, Qiang Li, Gary Lloyd, Sebastian Los, Niccolò Losi, Oscar Lovell, Christopher Luneau, Przemyslaw Makuch, Szymon Malinowski, Gaston Manta, Eleni Marinou, Nicholas Marsden, Sebastien Masson, Nicolas Maury, Bernhard Mayer, Margarette Mayers-Als, Christophe Mazel, Wayne McGeary, James C. McWilliams, Mario Mech, Melina Mehlmann, Agostino Niyonkuru Meroni, Theresa Mieslinger, Andreas Minikin, Peter Minnett, Gregor Möller, Yanmichel Morfa Avalos, Caroline Muller, Ionela Musat, Anna Napoli, Almuth Neuberger, Christophe Noisel, David Noone, Freja Nordsiek, Jakub L. Nowak, Lothar Oswald, Douglas J. Parker, Carolyn Peck, Renaud Person, Miriam Philippi, Albert Plueddemann, Christopher Pöhlker, Veronika Pörtge, Ulrich Pöschl, Lawrence Pologne, Michał Posyniak, Marc Prange, Estefanía Quiñones Meléndez, Jule Radtke, Karim Ramage, Jens Reimann, Lionel Renault, Klaus Reus, Ashford Reyes, Joachim Ribbe, Maximilian Ringel, Markus Ritschel, Cesar B. Rocha, Nicolas Rochetin, Johannes Röttenbacher, Callum Rollo, Haley Royer, Pauline Sadoulet, Leo Saffin, Sanola Sandiford, Irina Sandu, Michael Schäfer, Vera Schemann, Imke Schirmacher, Oliver Schlenczek, Jerome Schmidt, Marcel Schröder, Alfons Schwarzenboeck, Andrea Sealy, Christoph J. Senff, Ilya Serikov, Samkeyat Shohan, Elizabeth Siddle, Alexander Smirnov, Florian Späth, Branden Spooner, M. Katharina Stolla, Wojciech Szkółka, Simon P. de Szoeke, Stéphane Tarot, Eleni Tetoni, Elizabeth Thompson, Jim Thomson, Lorenzo Tomassini, Julien Totems, Alma Anna Ubele, Leonie Villiger, Jan von Arx, Thomas Wagner, Andi Walther, Ben Webber, Manfred Wendisch, Shanice Whitehall, Anton Wiltshire, Allison A. Wing, Martin Wirth, Jonathan Wiskandt, Kevin Wolf, Ludwig Worbes, Ethan Wright, Volker Wulfmeyer, Shanea Young, Chidong Zhang, Dongxiao Zhang, Florian Ziemen, Tobias Zinner, and Martin Zöger
Earth Syst. Sci. Data, 13, 4067–4119, https://doi.org/10.5194/essd-13-4067-2021, https://doi.org/10.5194/essd-13-4067-2021, 2021
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The EUREC4A field campaign, designed to test hypothesized mechanisms by which clouds respond to warming and benchmark next-generation Earth-system models, is presented. EUREC4A comprised roughly 5 weeks of measurements in the downstream winter trades of the North Atlantic – eastward and southeastward of Barbados. It was the first campaign that attempted to characterize the full range of processes and scales influencing trade wind clouds.
Isabelle De Smedt, Gaia Pinardi, Corinne Vigouroux, Steven Compernolle, Alkis Bais, Nuria Benavent, Folkert Boersma, Ka-Lok Chan, Sebastian Donner, Kai-Uwe Eichmann, Pascal Hedelt, François Hendrick, Hitoshi Irie, Vinod Kumar, Jean-Christopher Lambert, Bavo Langerock, Christophe Lerot, Cheng Liu, Diego Loyola, Ankie Piters, Andreas Richter, Claudia Rivera Cárdenas, Fabian Romahn, Robert George Ryan, Vinayak Sinha, Nicolas Theys, Jonas Vlietinck, Thomas Wagner, Ting Wang, Huan Yu, and Michel Van Roozendael
Atmos. Chem. Phys., 21, 12561–12593, https://doi.org/10.5194/acp-21-12561-2021, https://doi.org/10.5194/acp-21-12561-2021, 2021
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This paper assess the performances of the TROPOMI formaldehyde observations compared to its predecessor OMI at different spatial and temporal scales. We also use a global network of MAX-DOAS instruments to validate both satellite datasets for a large range of HCHO columns. The precision obtained with daily TROPOMI observations is comparable to monthly OMI observations. We present clear detection of weak HCHO column enhancements related to shipping emissions in the Indian Ocean.
Anoop S. Mahajan, Mriganka S. Biswas, Steffen Beirle, Thomas Wagner, Anja Schönhardt, Nuria Benavent, and Alfonso Saiz-Lopez
Atmos. Chem. Phys., 21, 11829–11842, https://doi.org/10.5194/acp-21-11829-2021, https://doi.org/10.5194/acp-21-11829-2021, 2021
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Iodine plays a vital role in oxidation chemistry over Antarctica, with past observations showing highly elevated levels of iodine oxide (IO) leading to severe depletion of boundary layer ozone. We present IO observations over three summers (2015–2017) at the Indian Antarctic bases of Bharati and Maitri. IO was observed during all campaigns with mixing ratios below 2 pptv, which is lower than the peak levels observed in West Antarctica, showing the differences in regional chemistry and emissions.
Vinod Kumar, Julia Remmers, Steffen Beirle, Joachim Fallmann, Astrid Kerkweg, Jos Lelieveld, Mariano Mertens, Andrea Pozzer, Benedikt Steil, Marc Barra, Holger Tost, and Thomas Wagner
Atmos. Meas. Tech., 14, 5241–5269, https://doi.org/10.5194/amt-14-5241-2021, https://doi.org/10.5194/amt-14-5241-2021, 2021
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We present high-resolution regional atmospheric chemistry model simulations focused around Germany. We highlight the importance of spatial resolution of the model itself as well as the input emissions inventory and short-scale temporal variability of emissions for simulations. We propose a consistent approach for evaluating the simulated vertical distribution of NO2 using MAX-DOAS measurements while also considering its spatial sensitivity volume and change in sensitivity within this volume.
Steffen Beirle, Christian Borger, Steffen Dörner, Henk Eskes, Vinod Kumar, Adrianus de Laat, and Thomas Wagner
Earth Syst. Sci. Data, 13, 2995–3012, https://doi.org/10.5194/essd-13-2995-2021, https://doi.org/10.5194/essd-13-2995-2021, 2021
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A catalog of point sources of nitrogen oxides was created using satellite observations of NO2. Key for the identification of point sources was the divergence, i.e., the difference between upwind and downwind levels of NO2.
The catalog lists 451 locations, of which 242 could be automatically matched to power plants. Other point sources are metal smelters, cement plants, or industrial areas. The catalog thus allows checking and improving of existing emission inventories.
Florian Dinger, Timo Kleinbek, Steffen Dörner, Nicole Bobrowski, Ulrich Platt, Thomas Wagner, Martha Ibarra, and Eveling Espinoza
Atmos. Chem. Phys., 21, 9367–9404, https://doi.org/10.5194/acp-21-9367-2021, https://doi.org/10.5194/acp-21-9367-2021, 2021
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Monitoring magnitude or chemical composition of volcanic gas emissions can help to forecast volcanic eruptions and provides empirical data on the impact of volcanoes on the chemistry in the local and global atmosphere. This study reports and discusses continuous time series of the sulfur and bromine emission fluxes of Masaya from 2014 to 2020. We observed an annual cyclicity in the BrO / SO2 molar ratio, possibly caused by the annual variability in the atmospheric humidity.
Thomas Wagner, Steffen Dörner, Steffen Beirle, Sebastian Donner, and Stefan Kinne
Atmos. Meas. Tech., 14, 3871–3893, https://doi.org/10.5194/amt-14-3871-2021, https://doi.org/10.5194/amt-14-3871-2021, 2021
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We compare measured and simulated O4 absorptions for conditions of extremely low aerosol optical depth, for which the uncertainties related to imperfect knowledge of aerosol properties do not significantly affect the comparison results. The simulations underestimate the measurements by 15 % to 20 %. Even if no aerosols are considered, the simulated O4 absorptions are systematically lower than the measurements. Our results indicate a fundamental inconsistency between simulations and measurements.
Maximilian Herrmann, Holger Sihler, Udo Frieß, Thomas Wagner, Ulrich Platt, and Eva Gutheil
Atmos. Chem. Phys., 21, 7611–7638, https://doi.org/10.5194/acp-21-7611-2021, https://doi.org/10.5194/acp-21-7611-2021, 2021
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Time-dependent 3D numerical simulations of tropospheric bromine release and ozone depletion events (ODEs) in the Arctic polar spring of 2009 are compared to observations. Simulation results agree well with the observations at both Utqiaġvik, Alaska, and at Summit, Greenland. In a parameter study, different settings for the bromine release mechanism are evaluated. An enhancement of the bromine release mechanism improves the agreement regarding the occurrence of ODEs with the observations.
Thomas Wagner, Steffen Beirle, Steffen Dörner, Christian Borger, and Roeland Van Malderen
Atmos. Chem. Phys., 21, 5315–5353, https://doi.org/10.5194/acp-21-5315-2021, https://doi.org/10.5194/acp-21-5315-2021, 2021
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A global long-term (1995–2015) data set of total column water vapour (TCWV) derived from satellite observations is used to quantify the influence of teleconnections. Based on a newly developed empirical method more than 40 teleconnection indices are significantly detected in our global TCWV data set. After orthogonalisation, only 20 indices are left significant. The global distribution of the cumulative influence of teleconnection indices is strongest in the tropics and high latitudes.
Bianca Lauster, Steffen Dörner, Steffen Beirle, Sebastian Donner, Sergey Gromov, Katharina Uhlmannsiek, and Thomas Wagner
Atmos. Meas. Tech., 14, 769–783, https://doi.org/10.5194/amt-14-769-2021, https://doi.org/10.5194/amt-14-769-2021, 2021
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In urban areas, road traffic is a dominant source of nitrogen oxides. In this study, two multi-axis differential optical absorption spectroscopy (MAX-DOAS) instruments on opposite sides of a motorway were used to measure the nitrogen dioxide absorption near Mainz, Germany. Total nitrogen oxide emissions are estimated for the occurring traffic flux. We show that the measured emissions systematically exceed the maximum expected emissions calculated from the European emission standards.
Tijl Verhoelst, Steven Compernolle, Gaia Pinardi, Jean-Christopher Lambert, Henk J. Eskes, Kai-Uwe Eichmann, Ann Mari Fjæraa, José Granville, Sander Niemeijer, Alexander Cede, Martin Tiefengraber, François Hendrick, Andrea Pazmiño, Alkiviadis Bais, Ariane Bazureau, K. Folkert Boersma, Kristof Bognar, Angelika Dehn, Sebastian Donner, Aleksandr Elokhov, Manuel Gebetsberger, Florence Goutail, Michel Grutter de la Mora, Aleksandr Gruzdev, Myrto Gratsea, Georg H. Hansen, Hitoshi Irie, Nis Jepsen, Yugo Kanaya, Dimitris Karagkiozidis, Rigel Kivi, Karin Kreher, Pieternel F. Levelt, Cheng Liu, Moritz Müller, Monica Navarro Comas, Ankie J. M. Piters, Jean-Pierre Pommereau, Thierry Portafaix, Cristina Prados-Roman, Olga Puentedura, Richard Querel, Julia Remmers, Andreas Richter, John Rimmer, Claudia Rivera Cárdenas, Lidia Saavedra de Miguel, Valery P. Sinyakov, Wolfgang Stremme, Kimberly Strong, Michel Van Roozendael, J. Pepijn Veefkind, Thomas Wagner, Folkard Wittrock, Margarita Yela González, and Claus Zehner
Atmos. Meas. Tech., 14, 481–510, https://doi.org/10.5194/amt-14-481-2021, https://doi.org/10.5194/amt-14-481-2021, 2021
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This paper reports on the ground-based validation of the NO2 data produced operationally by the TROPOMI instrument on board the Sentinel-5 Precursor satellite. Tropospheric, stratospheric, and total NO2 columns are compared to measurements collected from MAX-DOAS, ZSL-DOAS, and PGN/Pandora instruments respectively. The products are found to satisfy mission requirements in general, though negative mean differences are found at sites with high pollution levels. Potential causes are discussed.
Marloes Gutenstein, Karsten Fennig, Marc Schröder, Tim Trent, Stephan Bakan, J. Brent Roberts, and Franklin R. Robertson
Hydrol. Earth Syst. Sci., 25, 121–146, https://doi.org/10.5194/hess-25-121-2021, https://doi.org/10.5194/hess-25-121-2021, 2021
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The net exchange of water between the surface and atmosphere is mainly determined by the freshwater flux: the difference between evaporation (E) and precipitation (P), or E−P. Although there is consensus among modelers that with a warming climate E−P will increase, evidence from satellite data is still not conclusive, mainly due to sensor calibration issues. We here investigate the degree of correspondence among six recent
satellite-based climate data records and ERA5 reanalysis E−P data.
Jan-Lukas Tirpitz, Udo Frieß, François Hendrick, Carlos Alberti, Marc Allaart, Arnoud Apituley, Alkis Bais, Steffen Beirle, Stijn Berkhout, Kristof Bognar, Tim Bösch, Ilya Bruchkouski, Alexander Cede, Ka Lok Chan, Mirjam den Hoed, Sebastian Donner, Theano Drosoglou, Caroline Fayt, Martina M. Friedrich, Arnoud Frumau, Lou Gast, Clio Gielen, Laura Gomez-Martín, Nan Hao, Arjan Hensen, Bas Henzing, Christian Hermans, Junli Jin, Karin Kreher, Jonas Kuhn, Johannes Lampel, Ang Li, Cheng Liu, Haoran Liu, Jianzhong Ma, Alexis Merlaud, Enno Peters, Gaia Pinardi, Ankie Piters, Ulrich Platt, Olga Puentedura, Andreas Richter, Stefan Schmitt, Elena Spinei, Deborah Stein Zweers, Kimberly Strong, Daan Swart, Frederik Tack, Martin Tiefengraber, René van der Hoff, Michel van Roozendael, Tim Vlemmix, Jan Vonk, Thomas Wagner, Yang Wang, Zhuoru Wang, Mark Wenig, Matthias Wiegner, Folkard Wittrock, Pinhua Xie, Chengzhi Xing, Jin Xu, Margarita Yela, Chengxin Zhang, and Xiaoyi Zhao
Atmos. Meas. Tech., 14, 1–35, https://doi.org/10.5194/amt-14-1-2021, https://doi.org/10.5194/amt-14-1-2021, 2021
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Multi-axis differential optical absorption spectroscopy (MAX-DOAS) is a ground-based remote sensing measurement technique that derives atmospheric aerosol and trace gas vertical profiles from skylight spectra. In this study, consistency and reliability of MAX-DOAS profiles are assessed by applying nine different evaluation algorithms to spectral data recorded during an intercomparison campaign in the Netherlands and by comparing the results to colocated supporting observations.
Vinod Kumar, Steffen Beirle, Steffen Dörner, Abhishek Kumar Mishra, Sebastian Donner, Yang Wang, Vinayak Sinha, and Thomas Wagner
Atmos. Chem. Phys., 20, 14183–14235, https://doi.org/10.5194/acp-20-14183-2020, https://doi.org/10.5194/acp-20-14183-2020, 2020
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We present the first long-term MAX-DOAS measurements of aerosols, nitrogen dioxide and formaldehyde tropospheric columns, vertical distributions, and temporal variation from Mohali in the Indo-Gangetic Plain. We investigate the effect of various emission sources and meteorological conditions on the measured pollutants and how they control ozone formation. These measurements are also used to validate the corresponding satellite observations and are also compared against in situ observations.
Gaia Pinardi, Michel Van Roozendael, François Hendrick, Nicolas Theys, Nader Abuhassan, Alkiviadis Bais, Folkert Boersma, Alexander Cede, Jihyo Chong, Sebastian Donner, Theano Drosoglou, Anatoly Dzhola, Henk Eskes, Udo Frieß, José Granville, Jay R. Herman, Robert Holla, Jari Hovila, Hitoshi Irie, Yugo Kanaya, Dimitris Karagkiozidis, Natalia Kouremeti, Jean-Christopher Lambert, Jianzhong Ma, Enno Peters, Ankie Piters, Oleg Postylyakov, Andreas Richter, Julia Remmers, Hisahiro Takashima, Martin Tiefengraber, Pieter Valks, Tim Vlemmix, Thomas Wagner, and Folkard Wittrock
Atmos. Meas. Tech., 13, 6141–6174, https://doi.org/10.5194/amt-13-6141-2020, https://doi.org/10.5194/amt-13-6141-2020, 2020
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We validate several GOME-2 and OMI tropospheric NO2 products with 23 MAX-DOAS and 16 direct sun instruments distributed worldwide, highlighting large horizontal inhomogeneities at several sites affecting the validation results. We propose a method for quantification and correction. We show the application of such correction reduces the satellite underestimation in almost all heterogeneous cases, but a negative bias remains over the MAX-DOAS and direct sun network ensemble for both satellites.
Yeyuan Huang, Ang Li, Thomas Wagner, Yang Wang, Zhaokun Hu, Pinhua Xie, Jin Xu, Hongmei Ren, Julia Remmers, Xiaoyi Fang, and Bing Dang
Atmos. Meas. Tech., 13, 6025–6051, https://doi.org/10.5194/amt-13-6025-2020, https://doi.org/10.5194/amt-13-6025-2020, 2020
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Mobile DOAS has become an important tool for the quantification of emission sources. In this study, we focused on the error budget of mobile DOAS measurements from NOx and SO2 point sources based on the model simulations, and we also offered recommendations for the optimum settings of such measurements.
Alexis Merlaud, Livio Belegante, Daniel-Eduard Constantin, Mirjam Den Hoed, Andreas Carlos Meier, Marc Allaart, Magdalena Ardelean, Maxim Arseni, Tim Bösch, Hugues Brenot, Andreea Calcan, Emmanuel Dekemper, Sebastian Donner, Steffen Dörner, Mariana Carmelia Balanica Dragomir, Lucian Georgescu, Anca Nemuc, Doina Nicolae, Gaia Pinardi, Andreas Richter, Adrian Rosu, Thomas Ruhtz, Anja Schönhardt, Dirk Schuettemeyer, Reza Shaiganfar, Kerstin Stebel, Frederik Tack, Sorin Nicolae Vâjâiac, Jeni Vasilescu, Jurgen Vanhamel, Thomas Wagner, and Michel Van Roozendael
Atmos. Meas. Tech., 13, 5513–5535, https://doi.org/10.5194/amt-13-5513-2020, https://doi.org/10.5194/amt-13-5513-2020, 2020
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Short summary
The AROMAT campaigns took place in Romania in 2014 and 2015. They aimed to test airborne observation systems dedicated to air quality studies and to verify the concept of such campaigns in support of the validation of space-borne atmospheric missions. We show that airborne measurements of NO2 can be valuable for the validation of air quality satellites. For H2CO and SO2, the validation should involve ground-based measurement systems at key locations that the AROMAT measurements help identify.
Yang Wang, Arnoud Apituley, Alkiviadis Bais, Steffen Beirle, Nuria Benavent, Alexander Borovski, Ilya Bruchkouski, Ka Lok Chan, Sebastian Donner, Theano Drosoglou, Henning Finkenzeller, Martina M. Friedrich, Udo Frieß, David Garcia-Nieto, Laura Gómez-Martín, François Hendrick, Andreas Hilboll, Junli Jin, Paul Johnston, Theodore K. Koenig, Karin Kreher, Vinod Kumar, Aleksandra Kyuberis, Johannes Lampel, Cheng Liu, Haoran Liu, Jianzhong Ma, Oleg L. Polyansky, Oleg Postylyakov, Richard Querel, Alfonso Saiz-Lopez, Stefan Schmitt, Xin Tian, Jan-Lukas Tirpitz, Michel Van Roozendael, Rainer Volkamer, Zhuoru Wang, Pinhua Xie, Chengzhi Xing, Jin Xu, Margarita Yela, Chengxin Zhang, and Thomas Wagner
Atmos. Meas. Tech., 13, 5087–5116, https://doi.org/10.5194/amt-13-5087-2020, https://doi.org/10.5194/amt-13-5087-2020, 2020
Cited articles
AC SAF: GOME-2A Absorbing Aerosol Index MSC (R1) – Metop, EUMETSAT SAF on Atmospheric Composition Monitoring, https://doi.org/10.15770/EUM_SAF_O3M_0003, 2017a. a
AC SAF: GOME-2A Absorbing Aerosol Index PMD (R1) – Metop, EUMETSAT SAF on Atmospheric Composition Monitoring, https://doi.org/10.15770/EUM_SAF_O3M_0004, 2017b. a
Ahmad, Z., Bhartia, P. K., and Krotkov, N.: Spectral properties of
backscattered UV radiation in cloudy atmospheres, J. Geophys. Res., 109,
D01201, https://doi.org/10.1029/2003JD003395, 2004. a
Barkley, M. P., Kurosu, T. P., Chance, K., De Smedt, I., Van Roozendael,
M., Arneth, A., Hagberg, D., and Guenther, A.: Assessing sources of
uncertainty in formaldehyde air mass factors over tropical South America:
Implications for top-down isoprene emission estimates, J. Geophys. Res., 117,
2156–2202, https://doi.org/10.1029/2011JD016827, 2012. a
Blum, M., Rozanov, V. V., Burrows, J. P., and Bracher, A.: Coupled
ocean-atmosphere radiative transfer model in the framework of software
package SCIATRAN: Selected comparisons to model and satellite data, Adv.
Space Res., 49, 1728–1742, https://doi.org/10.1016/j.asr.2012.02.012, 2012. a
Boersma, K. F., Eskes, H. J., and Brinksma, E. J.: Error analysis for
tropospheric NO2 retrieval from space, J. Geophys. Res., 109, D04311,
https://doi.org/10.1029/2003JD003962, 2004. a
Bovensmann, H., Burrows, J. P., Buchwitz, M., Frerick, J., Noël, S.,
Rozanov, V. V., Chance, K. V., and Goede, A. P. H.: SCIAMACHY: mission
objectives and measurement modes, J. Atmos. Sci., 56, 127–150,
https://doi.org/10.1175/1520-0469(1999)056<0127:SMOAMM>2.0.CO;2, 1999. a
Burrows, J. P., Weber, M., Buchwitz, M., Rozanov, V., Ladstätter-Weißenmayer,
A., Richter, A., DeBeek, R., Hoogen, R., Bramstedt, K., Eichmann, K.-U.,
Eisinger, M., and Perner, D.: The Global Ozone Monitoring Experiment (GOME):
Mission concept and first scientific results, J. Atmos. Sci., 56, 151–175,
https://doi.org/10.1175/1520-0469(1999)056<0151:TGOMEG>2.0.CO;2, 1999. a
Callies, J., Corpaccioli, E., Eisinger, M., Hahne, A., and Lefebvre, A.: GOME-2
– MetOp's Second-Generation Sensor for Operational Ozone Monitoring, ESA
Bull.-Eur. Space, 102, 28–36, 2000. a
Cantrell, C. A.: Technical Note: Review of methods for linear least-squares fitting of data and application to atmospheric chemistry problems, Atmos. Chem. Phys., 8, 5477–5487, https://doi.org/10.5194/acp-8-5477-2008, 2008. a
Cavalieri, D. J., Parkinson, C. L., Gloersen, P., and Zwally, H. J.: Sea Ice
Concentrations from Nimbus-7 SMMR and DMSP SSM/I-SSMIS Passive Microwave
Data, Version 1, NSIDC-0051, 2007–2013, NASA National Snow and Ice Data
Center Distributed Active Archive Center, Boulder, Colorado USA,
https://doi.org/10.5067/8GQ8LZQVL0VL, 1996. a, b, c
Coleman, T. F. and Li, Y.: On the Convergence of Reflective Newton Methods for
Large-Scale Nonlinear Minimization Subject to Bounds, Math. Program., 67,
189–224, https://doi.org/10.1007/BF01582221, 1994. a
Coleman, T. F. and Li, Y.: An Interior, Trust Region Approach for Nonlinear
Minimization Subject to Bounds, SIAM J. Optimiz., 6, 418–445,
https://doi.org/10.1137/0806023, 1996. a
Cox, C. and Munk, W. H.: Statistics of the sea surface derived from sun
glitter, J. Mar. Res., 13, 198–227,
1954b. a
Cracknell, A.: The Advanced Very High Resolution Radiometer, Taylor and
Francis, London, UK, ISBN 9780748402090, 1997. a
Dee, D. P., Uppala, S. M., Simmons, A. J., Berrisford, P., Poli, P., Kobayashi,
S., Andrae, U., Balmaseda, M. A., Balsamo, G., Bauer, P., Bechtold, P.,
Beljaars, A. C. M., van de Berg, L., Bidlot, J., Bormann, N., Delsol, C.,
Dragani, R., Fuentes, M., Geer, A. J., Haimberger, L., Healy, S. B.,
Hersbach, H., Hólm, E. V., Isaksen, L., Kållberg, P., Köhler, M.,
Matricardi, M., McNally, A. P., Monge-Sanz, B. M., Morcrette, J.-J., Park,
B.-K., Peubey, C., de Rosnay, P., Tavolato, C., Thépaut, J.-N., and Vitart,
F.: The ERA-Interim reanalysis: configuration and performance of the data
assimilation system, Q. J. Roy. Meteor. Soc., 137, 553–597,
https://doi.org/10.1002/qj.828, 2011. a, b
de Graaf, M., Sihler, H., Tilstra, L. G., and Stammes, P.: How big is an OMI pixel?, Atmos. Meas. Tech., 9, 3607–3618, https://doi.org/10.5194/amt-9-3607-2016, 2016. a, b
De Smedt, I., Müller, J.-F., Stavrakou, T., van der A, R., Eskes, H., and Van Roozendael, M.: Twelve years of global observations of formaldehyde in the troposphere using GOME and SCIAMACHY sensors, Atmos. Chem. Phys., 8, 4947–4963, https://doi.org/10.5194/acp-8-4947-2008, 2008. a
Desmons, M., Wang, P., Stammes, P., and Tilstra, L. G.: FRESCO-B: a fast cloud retrieval algorithm using oxygen B-band measurements from GOME-2, Atmos. Meas. Tech., 12, 2485–2498, https://doi.org/10.5194/amt-12-2485-2019, 2019. a
Deutschmann, T., Beirle, S., Frieß, U., Grzegorski, M., Kern, C., Kritten, L.,
Platt, U., Prados-Román, C., Pukite, J., Wagner, T., Werner, B., and
Pfeilsticker, K.: The Monte Carlo atmospheric radiative transfer model
McArtim: Introduction and validation of Jacobians and 3D features, J.
Quant. Spectrosc. Ra., 112, 1119–1137, https://doi.org/10.1016/j.jqsrt.2010.12.009,
2011. a
Ebuchi, N. and Kizu, S.: Probability Distribution of Surface Wave Slope Derived
Using Sun Glitter Images from Geostationary Meteorological Satellite and
Surface Vector Winds from Scatterometers, J. Oceanogr., 58, 477–486,
https://doi.org/10.1023/A:1021213331788, 2002. a, b
EUMETSAT: GOME-2/Metop-A instrument, PPF and auxiliary-data change history,
available at: http://oiswww.eumetsat.org/epsreports/html/history/MetopAGOME2PPFhist.pdf
(last access: 22 May 2019), 2014. a
Fasnacht, Z., Vasilkov, A., Haffner, D., Qin, W., Joiner, J., Krotkov, N., Sayer, A. M., and Spurr, R.: A geometry-dependent surface Lambertian-equivalent reflectivity product for UV–Vis retrievals – Part 2: Evaluation over open ocean, Atmos. Meas. Tech., 12, 6749–6769, https://doi.org/10.5194/amt-12-6749-2019, 2019. a
Fournier, N., Stammes, P., de Graaf, M., van der A, R., Piters, A., Grzegorski, M., and Kokhanovsky, A.: Improving cloud information over deserts from SCIAMACHY Oxygen A-band measurements, Atmos. Chem. Phys., 6, 163–172, https://doi.org/10.5194/acp-6-163-2006, 2006. a
Grainger, J. F. and Ring, J.: Anomalous Fraunhofer Line Profiles, Nature, 193, 762, https://doi.org/10.1038/193762a0, 1962. a
Grzegorski, M.: Cloud retrieval from UV/VIS satellite instruments (SCIAMACHY
and GOME), Dissertation, University of Heidelberg,
https://doi.org/10.11588/heidok.00010423, 2009. a
Hall, D. K. and Riggs, G. A.: MODIS/Terra Snow Cover 8-Day L3 Global 0.05Deg
CMG, Version 6, 2007–2013, NASA National Snow and Ice Data Center
Distributed Active Archive Center, Boulder, Colorado USA,
https://doi.org/10.5067/MODIS/MOD10C2.006, 2016. a, b, c
Harmel, T. and Chami, M.: Estimation of the sunglint radiance field from
optical satellite imagery over open ocean: multidirectional approach and
polarization aspects, J. Geophys. Res.-Oceans, 118, 76–90,
https://doi.org/10.1029/2012JC008221, 2013. a
Herman, J. R. and Celarier, E. A.: Earth surface reflectivity climatology at
340–380 nm from TOMS data, J. Geophys. Res., 102, 28003–28012,
https://doi.org/10.1029/97JD02074, 1997. a
IFE-Bremen: User's Guide for the Software Package SCIATRAN (Radiative
Transfer Model and Retrieval Algorithm) – Version 3.8, Internet, Institute
of Remote Sensing (IFE), University of Bremen, Germany, available at:
http://www.iup.uni-bremen.de/sciatran/free_downloads/users_guide_sciatran.pdf
(last access: 14 February 2019), 2018. a
Justice, C., Vermote, E., Townshend, J., Defries, R., Roy, D., Hall, D.,
Salomonson, V., Privette, J., Riggs, G., Strahler, A., Lucht, W., Myneni, R.,
Knyazikhin, Y., Running, S., Nemani, R., Wan, Z., Huete, A., van Leeuwen,
W., Wolfe, R., Giglio, L., Muller, J., Lewis, P., and Barnsley, M.: The
Moderate Resolution Imaging Spectroradiometer (MODIS): land remote sensing
for global change research, IEEE T. Geosci. Remote., 36, 1228–1249,
https://doi.org/10.1109/36.701075, 1998. a
Kleipool, Q. L., Dobber, M. R., de Haan, J. F., and Levelt, P. F.: Earth
surface reflectance climatology from 3 years of OMI data, J. Geophys.
Res.-Atmos., 113, D18308, https://doi.org/10.1029/2008JD010290, 2008. a
KNMI: OMI Instrument Characteristics, available at:
https://projects.knmi.nl/omi/research/instrument/characteristics.php
(last access: 4 February 2015), 2019. a
Koelemeijer, R. B. A., Stammes, P., Hovenier, J. W., and de Haan, J. F.: A
fast method for retrieval of cloud parameters using oxygen A-band
measurements from Global Ozone Monitoring Experiment, J. Geophys. Res., 106,
3475–3490, https://doi.org/10.1029/2000JD900657, 2001. a, b, c
Koelemeijer, R. B. A., de Haan, J. F., and Stammes, P.: A database of
spectral surface reflectivity in the range 335–772 nm derived from 5.5
years of GOME observations, J. Geophys. Res., 108, 4070,
https://doi.org/10.1029/2002JD002429, 2003. a, b
Kokhanovsky, A. A., von Hoyningen-Huene, W., and Burrows, J. P.:
Determination of the cloud fraction in the SCIAMACHY ground scene using MERIS
spectral measurements,, Int. J. Remote Sens., 30, 6151–6167,
https://doi.org/10.1080/01431160902842326, 2009. a
Krijger, J. M., van Weele, M., Aben, I., and Frey, R.: Technical Note: The effect of sensor resolution on the number of cloud-free observations from space, Atmos. Chem. Phys., 7, 2881–2891, https://doi.org/10.5194/acp-7-2881-2007, 2007. a, b
Kuze, A. and Chance, K. V.: Analysis of cloud top height and cloud coverage
from satellites using the O2 A and B bands, J. Geophys. Res., 99,
14481–14491, https://doi.org/10.1029/94JD01152, 1994. a
Levelt, P. F., van den Oord, G. H. J., Dobber, M. R., Malkki, A., Visser, H.,
de Vries, J., Stammes, P., Lundell, J. O. V., and Saari, H.: The Ozone
Monitoring Instrument, IEEE T. Geosci. Remote, 44, 1093–1101,
https://doi.org/10.1109/TGRS.2006.872333, 2006. a
Li, X. and Strahler, A. H.: Geometric-optical bidirectional reflectance
modeling of the discrete crown vegetation canopy: effect of crown shape and
mutual shadowing, IEEE T. Geosci. Remote, 30, 276–292,
https://doi.org/10.1109/36.134078, 1992. a
Liu, C., Beirle, S., Butler, T., Liu, J., Hoor, P., Jöckel, P., Penning de Vries, M., Pozzer, A., Frankenberg, C., Lawrence, M. G., Lelieveld, J., Platt, U., and Wagner, T.: Application of SCIAMACHY and MOPITT CO total column measurements to evaluate model results over biomass burning regions and Eastern China, Atmos. Chem. Phys., 11, 6083–6114, https://doi.org/10.5194/acp-11-6083-2011, 2011. a
Lorente, A., Folkert Boersma, K., Yu, H., Dörner, S., Hilboll, A., Richter, A., Liu, M., Lamsal, L. N., Barkley, M., De Smedt, I., Van Roozendael, M., Wang, Y., Wagner, T., Beirle, S., Lin, J.-T., Krotkov, N., Stammes, P., Wang, P., Eskes, H. J., and Krol, M.: Structural uncertainty in air mass factor calculation for NO2 and HCHO satellite retrievals, Atmos. Meas. Tech., 10, 759–782, https://doi.org/10.5194/amt-10-759-2017, 2017. a, b
Lorente, A., Boersma, K. F., Stammes, P., Tilstra, L. G., Richter, A., Yu, H., Kharbouche, S., and Muller, J.-P.: The importance of surface reflectance anisotropy for cloud and NO2 retrievals from GOME-2 and OMI, Atmos. Meas. Tech., 11, 4509–4529, https://doi.org/10.5194/amt-11-4509-2018, 2018. a, b, c, d, e, f
Loyola, D.: A new cloud recognition algorithm for optical sensors, in: IGARSS
'98. Sensing and Managing the Environment. 1998 IEEE International Geoscience
and Remote Sensing. Symposium Proceedings (Cat. No.98CH36174), 6–10 July 1998, Seattle, USA, 97-80873,
IEEE, 572–574, https://doi.org/10.1109/IGARSS.1998.699514, 1998. a
Loyola, D., Thomas, W., Livschitz, Y., Ruppert, T., Albert, P., and Hollmann,
R.: Cloud Properties Derived From GOME/ERS-2 Backscatter Data for Trace Gas
Retrieval, IEEE T. Geosci. Remote, 45, 2747–2758,
https://doi.org/10.1109/TGRS.2007.901043, 2007. a, b
Loyola, D., Koukouli, M., Valks, P., Balis, D., Hao, N., Van Roozendael, M., Spurr, R., Zimmer, W., Kiemle, S., Lerot, C., and Lambert, J.-C.: The GOME-2 Total Column Ozone Product: Retrieval Algorithm and Ground-Based Validation,
J. Geophys. Res, 116, D07302, https://doi.org/10.1029/2010JD014675, 2011. a
Loyola, D. G., Gimeno García, S., Lutz, R., Argyrouli, A., Romahn, F., Spurr, R. J. D., Pedergnana, M., Doicu, A., Molina García, V., and Schüssler, O.: The operational cloud retrieval algorithms from TROPOMI on board Sentinel-5 Precursor, Atmos. Meas. Tech., 11, 409–427, https://doi.org/10.5194/amt-11-409-2018, 2018. a, b, c, d
Loyola, D. G., Xu, J., Heue, K.-P., and Zimmer, W.: Applying FP_ILM to the retrieval of geometry-dependent effective Lambertian equivalent reflectivity (GE_LER) daily maps from UVN satellite measurements, Atmos. Meas. Tech., 13, 985–999, https://doi.org/10.5194/amt-13-985-2020, 2020. a
Martin, J., Eugenio, F., Marcello, J., and Medina, A.: Automatic Sun Glint
Removal of Multispectral High-Resolution Worldview-2 Imagery for Retrieving
Coastal Shallow Water Parameters, Remote Sens., 8, 37, https://doi.org/10.3390/rs8010037,
2016. a
Martin, R. V., Chance, K., Jacob, D., Kurosu, T. P., Spurr, R. J. D., Bucsela,
E., Gleason, J. F., Palmer, P. I., Bey, I., Fiore, A. M., Li, Q., Yantosca,
R. M., and Koelemeijer, R. B. A.: An improved retrieval of tropospheric
nitrogen dioxide from GOME, J. Geophys. Res., 107, 4437,
https://doi.org/10.1029/2001JD001027, 2002. a
McKenzie, R. L., Johnston, P. V., McElroy, C. T., Kerr, J. B., and Solomon, S.: Altitude distributions of stratospheric constituents from ground‐based
measurements at twilight, J. Geophys. Res.-Atmos., 96, 15499–15511,
https://doi.org/10.1029/91JD01361, 1991. a
McPeters, R., Bhartia, P. K., Krueger, A. J., Herman, J. R., Schlesinger,
B. M., Wellemeyer, C. G., Seftor, C. J., Jaross, G., Taylor, S. L., Swissler,
T., Torres, O., Labow, G., Byerly, W., and Cebula, R. P.: Nimbus-7 Total
Ozone Mapping Spectrometer (TOMS) Data Products User’s Guide, Nasa
reference publication 138, NASA, available at:
https://ozoneaq.gsfc.nasa.gov/media/docs/epusrguide.pdf (last
access: 17 November 2020), 1996. a, b
Munro, R., Eisinger, M., Anderson, C., Callies, J., Corpaccioli, E., Lang, R.,
Lefebvre, A., Livschitz, Y., and Albiñana, A. P.: GOME-2 on MetOp, in:
Proc. of The 2006 EUMETSAT Meteorological Satellite Conference, 12–16 June 2006, Helsinki, Finland, EUMETSAT, p. 48, 2006. a
Munro, R., Lang, R., Klaes, D., Poli, G., Retscher, C., Lindstrot, R., Huckle, R., Lacan, A., Grzegorski, M., Holdak, A., Kokhanovsky, A., Livschitz, J., and Eisinger, M.: The GOME-2 instrument on the Metop series of satellites: instrument design, calibration, and level 1 data processing – an overview, Atmos. Meas. Tech., 9, 1279–1301, https://doi.org/10.5194/amt-9-1279-2016, 2016. a, b, c, d, e, f
NOAA: Advanced Very High Resolution Radiometer – AVHRR, available at:
https://www.avl.class.noaa.gov/release/data_available/avhrr/index.htm, last access: 11 April 2021. a
Noguchi, K., Richter, A., Rozanov, V., Rozanov, A., Burrows, J. P., Irie, H., and Kita, K.: Effect of surface BRDF of various land cover types on geostationary observations of tropospheric NO2, Atmos. Meas. Tech., 7, 3497–3508, https://doi.org/10.5194/amt-7-3497-2014, 2014. a
Noxon, J. F., Whipple, E. C., and Hyde, R. S.: Stratospheric NO2 – 1.
Observational method and behaviour at mid-latitude, J. Geophys. Res., 84,
5047–5076, https://doi.org/10.1029/JC084iC08p05047, 1979. a
Perliski, L. and Solomon, S.: On the evaluation of air mass factors for
atmospheric near-ultraviolet and visible absorption spectroscopy, J. Geophys.
Res., 98, 10363–10374, https://doi.org/10.1029/93JD00465, 1993. a
Popp, C., Wang, P., Brunner, D., Stammes, P., Zhou, Y., and Grzegorski, M.: MERIS albedo climatology for FRESCO+ O2 A-band cloud retrieval, Atmos. Meas. Tech., 4, 463–483, https://doi.org/10.5194/amt-4-463-2011, 2011. a, b
Rozanov, V. V. and Rozanov, A. V.: Differential optical absorption spectroscopy (DOAS) and air mass factor concept for a multiply scattering vertically inhomogeneous medium: theoretical consideration, Atmos. Meas. Tech., 3, 751–780, https://doi.org/10.5194/amt-3-751-2010, 2010. a
Rozanov, V. V., Rozanov, A. V., Kokhanovsky, A. A., and Burrows, J. P.:
Radiative transferthrough terrestrial atmosphere and ocean: Software package
SCIATRAN, J. Quant. Spectrosc. Ra., 113, 13–71,
https://doi.org/10.1016/j.jqsrt.2013.07.004, 2014. a
Sarkissian, A., Roscoe, H. K., and Fish, D. J.: Ozone measurementsby zenith-sky
spectrometers: an evaluation of errors in air-massfactors calculated by
radiative transfer model, J. Quant. Spectrosc. Ra., 54, 471–480,
https://doi.org/10.1016/0022-4073(95)00085-Y, 1995. a
Schueler, C. F., Clement, J. E., Ardanuy, P. E., Welsch, C., DeLuccia, F., and Swenson, H.: NPOESS VIIRS sensor design overview, Proc. SPIE 4483, in: Earth
Observing Systems VI, https://doi.org/10.1117/12.453451, 2002. a
Sihler, H. and Wagner, T.: MICRU effective cloud fractions from GOME-2A, Max Planck Digital Library, https://doi.org/10.17617/3.59, 2020. a
Sihler, H., Lübcke, P., Lang, R., Beirle, S., de Graaf, M., Hörmann, C., Lampel, J., Penning de Vries, M., Remmers, J., Trollope, E., Wang, Y., and Wagner, T.: In-operation field-of-view retrieval (IFR) for satellite and ground-based DOAS-type instruments applying coincident high-resolution imager data, Atmos. Meas. Tech., 10, 881–903, https://doi.org/10.5194/amt-10-881-2017, 2017. a, b, c, d
Solomon, S., Schmeltekopf, A. L., and Sanders, R. W.: On the interpretation of zenith sky absorption measurements, J. Geophys. Res.-Atmos., 92, 8311–8319,
https://doi.org/10.1029/JD092iD07p08311, 1987. a, b
Stammes, P., Sneep, M., de Haan, J. F., Veefkind, J. P., Wang, P., and
Levelt, P. F.: Effective cloud fractions from the Ozone Monitoring
Instrument: Theoretical framework and validation, J. Geophys. Res.-Atmos.,
113, D16S38, https://doi.org/10.1029/2007JD008820, 2008. a, b, c
Tilstra, L. G., De Graaf, M., Aben, I., and Stammes, P.: In‐flight
degradation correction of SCIAMACHY UV reflectances and Absorbing Aerosol
Index, J. Geophys. Res.-Atmos., 117, D06209, https://doi.org/10.1029/2011JD016957,
2012. a
Tilstra, L. G., Tuinder, O. N. E., and Stammes, P.: Algorithm theoretical basis document – GOME-2 surface LER product, available at:
https://acsaf.org/docs/atbd/Algorithm_Theoretical_Basis_Document_LER_Mar_2019.pdf
(last access: 15 May 2021), 2017a. a
Tilstra, L. G., Tuinder, O. N. E., Wang, P., and Stammes, P.: Surface
reflectivity climatologies from UV to NIR determined from Earth observations
by GOME-2 and SCIAMACHY, J. Geophys. Res.-Atmos., 122, 4084–4111,
https://doi.org/10.1002/2016JD025940, 2017b. a, b, c, d
Tuinder, O. N. E., de Winter-Sorkina, R., and Builtjes, P. J. H.: Retrieval methods of effective cloud cover from the GOME instrument: an intercomparison, Atmos. Chem. Phys., 4, 255–273, https://doi.org/10.5194/acp-4-255-2004, 2004. a
Tuinder, O., de Graaf, M., Tilstra, G., Penning de Vries, M., and Kooreman, M.: Algorithm theoretical basis document – ATBD for the Absorbing Aerosol Index product, available at:
https://acsaf.org/docs/atbd/Algorithm_Theoretical_Basis_Document_NAR_NAP_ARS_ARP_Sep_2019.pdf,
last access: 28 November 2020. a, b
USGS: Global 30 Arc-Second Elevation (GTOPO30), Internet, USGS EROS Archive,
https://doi.org/10.5066/F7DF6PQS, 2018. a, b, c
Várnai, T. and Marshak, A.: View angle dependence of cloud optical
thicknesses retrieved by Moderate Resolution Imaging
Spectroradiometer (MODIS), J. Geophys. Res., 112, D06203,
https://doi.org/10.1029/2005JD006912, 2007. a
Vasilkov, A., Qin, W., Krotkov, N., Lamsal, L., Spurr, R., Haffner, D., Joiner, J., Yang, E.-S., and Marchenko, S.: Accounting for the effects of surface BRDF on satellite cloud and trace-gas retrievals: a new approach based on geometry-dependent Lambertian equivalent reflectivity applied to OMI algorithms, Atmos. Meas. Tech., 10, 333–349, https://doi.org/10.5194/amt-10-333-2017, 2017. a, b, c, d, e
Vasilkov, A., Yang, E.-S., Marchenko, S., Qin, W., Lamsal, L., Joiner, J., Krotkov, N., Haffner, D., Bhartia, P. K., and Spurr, R.: A cloud algorithm based on the O2-O2 477 nm absorption band featuring an advanced spectral fitting method and the use of surface geometry-dependent Lambertian-equivalent reflectivity, Atmos. Meas. Tech., 11, 4093–4107, https://doi.org/10.5194/amt-11-4093-2018, 2018. a, b
Veefkind, J. P., Aben, I., McMullan, K., Förster, H., de Vries, J., Otter, G.,
Claas, J., Eskes, H. J., de Haan, J. F., Kleipool, Q., van Weele, M.,
Hasekamp, O., Hoogeveen, R., Landgraf, J., Snel, R., Tol, P., Ingmann, P.,
Voors, R., Kruizinga, B., Vink, R., Visser, H., and Levelt, P. F.: TROPOMI
on the ESA Sentinel-5 Precursor: A GMES mission for global
observations of the atmospheric composition for climate, air quality and
ozone layer applications, Remote Sens. Environ., 120, 70–83,
https://doi.org/10.1016/j.rse.2011.09.027, 2012. a, b
Veefkind, J. P., de Haan, J. F., Sneep, M., and Levelt, P. F.: Improvements to the OMI O2–O2 operational cloud algorithm and comparisons with ground-based radar–lidar observations, Atmos. Meas. Tech., 9, 6035–6049, https://doi.org/10.5194/amt-9-6035-2016, 2016. a, b
Wagner, T., Heland, J., Zöger, M., and Platt, U.: A fast H2O total column density product from GOME – Validation with in-situ aircraft measurements, Atmos. Chem. Phys., 3, 651–663, https://doi.org/10.5194/acp-3-651-2003, 2003. a
Wang, P., Tuinder, O., and Stammes, P.: FRESCO+ version 2 for GOME-2
Metop-C processing, available at:
http://www.temis.nl/fresco/frescopv2_metopc_WP1_report_20181026.pdf
(last access: 25 May 2021), 2018. a
Wanner, W., Li, X., and Strahler, A. H.: On the derivation of kernels for
kernel-driven models of bidirectional reflectance, J. Geophys. Res., 100,
21077–21089, https://doi.org/10.1029/95JD02371, 1995.
a, b
Zhang, H. and Wang, M.: Evaluation of sun glint models using MODIS
measurements, J. Quant. Spectrosc. Ra., 111, 492–506,
https://doi.org/10.1016/j.jqsrt.2009.10.001, 2010. a, b
Short summary
MICRU is an algorithm for the retrieval of effective cloud fractions (CFs) from satellite measurements. CFs describe the amount of clouds, which have a significant impact on the vertical sensitivity profile of trace gases like NO2 and HCHO. MICRU retrieves small CFs with an accuracy of 0.04 over the entire satellite swath. It features an empirical surface reflectivity model accounting for physical anisotropy (BRDF, sun glitter) and instrumental effects. MICRU is also applicable to imager data.
MICRU is an algorithm for the retrieval of effective cloud fractions (CFs) from satellite...
