Articles | Volume 14, issue 7
https://doi.org/10.5194/amt-14-4915-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-14-4915-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
13 Jul 2021
Research article |
| 13 Jul 2021
| 13 Jul 2021
Total ozone column intercomparison of Brewers, Dobsons, and BTS-Solar at Hohenpeißenberg and Davos in 2019/2020
Ralf Zuber
CORRESPONDING AUTHOR
Gigahertz Optik GmbH, 82299 Türkenfeld, Germany
Deutscher Wetterdienst (DWD), 82383 Hohenpeißenberg, Germany
Luca Egli
CORRESPONDING AUTHOR
Physikalisch-Meteorologisches Observatorium Davos (PMOD/WRC), 7260
Davos Dorf, Switzerland
Mario Ribnitzky
Gigahertz Optik GmbH, 82299 Türkenfeld, Germany
Wolfgang Steinbrecht
Deutscher Wetterdienst (DWD), 82383 Hohenpeißenberg, Germany
Julian Gröbner
Physikalisch-Meteorologisches Observatorium Davos (PMOD/WRC), 7260
Davos Dorf, Switzerland
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Panagiotis G. Kosmopoulos, Stelios Kazadzis, Alois W. Schmalwieser, Panagiotis I. Raptis, Kyriakoula Papachristopoulou, Ilias Fountoulakis, Akriti Masoom, Alkiviadis F. Bais, Julia Bilbao, Mario Blumthaler, Axel Kreuter, Anna Maria Siani, Kostas Eleftheratos, Chrysanthi Topaloglou, Julian Gröbner, Bjørn Johnsen, Tove M. Svendby, Jose Manuel Vilaplana, Lionel Doppler, Ann R. Webb, Marina Khazova, Hugo De Backer, Anu Heikkilä, Kaisa Lakkala, Janusz Jaroslawski, Charikleia Meleti, Henri Diémoz, Gregor Hülsen, Barbara Klotz, John Rimmer, and Charalampos Kontoes
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Marek Šmíd, Geiland Porrovecchio, Jiří Tesař, Tim Burnitt, Luca Egli, Julian Grőbner, Petr Linduška, and Martin Staněk
Atmos. Meas. Tech., 14, 3573–3582, https://doi.org/10.5194/amt-14-3573-2021, https://doi.org/10.5194/amt-14-3573-2021, 2021
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We designed and developed a tuneable and portable radiation source (TuPS) to provide a reference wavelength scale, with a bandwidth of emitted radiation of 0.13 nm and uncertainty in wavelength of 0.02 nm. TuPS was successfully used for the in-field characterization of 14 Dobson spectrophotometers in campaigns in Europe. The line spread functions of Dobsons measured by TuPS in conjunction with the cross-sections from IUP improves the consistency between the Dobson and Brewer from 3 % to 1 %.
Julian Gröbner, Herbert Schill, Luca Egli, and René Stübi
Atmos. Meas. Tech., 14, 3319–3331, https://doi.org/10.5194/amt-14-3319-2021, https://doi.org/10.5194/amt-14-3319-2021, 2021
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Graeme Marlton, Andrew Charlton-Perez, Giles Harrison, Inna Polichtchouk, Alain Hauchecorne, Philippe Keckhut, Robin Wing, Thierry Leblanc, and Wolfgang Steinbrecht
Atmos. Chem. Phys., 21, 6079–6092, https://doi.org/10.5194/acp-21-6079-2021, https://doi.org/10.5194/acp-21-6079-2021, 2021
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Kaisa Lakkala, Jukka Kujanpää, Colette Brogniez, Nicolas Henriot, Antti Arola, Margit Aun, Frédérique Auriol, Alkiviadis F. Bais, Germar Bernhard, Veerle De Bock, Maxime Catalfamo, Christine Deroo, Henri Diémoz, Luca Egli, Jean-Baptiste Forestier, Ilias Fountoulakis, Katerina Garane, Rosa Delia Garcia, Julian Gröbner, Seppo Hassinen, Anu Heikkilä, Stuart Henderson, Gregor Hülsen, Bjørn Johnsen, Niilo Kalakoski, Angelos Karanikolas, Tomi Karppinen, Kevin Lamy, Sergio F. León-Luis, Anders V. Lindfors, Jean-Marc Metzger, Fanny Minvielle, Harel B. Muskatel, Thierry Portafaix, Alberto Redondas, Ricardo Sanchez, Anna Maria Siani, Tove Svendby, and Johanna Tamminen
Atmos. Meas. Tech., 13, 6999–7024, https://doi.org/10.5194/amt-13-6999-2020, https://doi.org/10.5194/amt-13-6999-2020, 2020
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The TROPOspheric Monitoring Instrument (TROPOMI) onboard the Sentinel-5 Precursor (S5P) satellite was launched on 13 October 2017 to provide the atmospheric composition for atmosphere and climate research. Ground-based data from 25 sites located in Arctic, subarctic, temperate, equatorial and Antarctic
areas were used for the validation of the TROPOMI surface ultraviolet (UV) radiation product. For most sites 60 %–80 % of TROPOMI data was within ± 20 % of ground-based data.
Ilias Fountoulakis, Henri Diémoz, Anna Maria Siani, Gregor Hülsen, and Julian Gröbner
Earth Syst. Sci. Data, 12, 2787–2810, https://doi.org/10.5194/essd-12-2787-2020, https://doi.org/10.5194/essd-12-2787-2020, 2020
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Robin Wing, Wolfgang Steinbrecht, Sophie Godin-Beekmann, Thomas J. McGee, John T. Sullivan, Grant Sumnicht, Gérard Ancellet, Alain Hauchecorne, Sergey Khaykin, and Philippe Keckhut
Atmos. Meas. Tech., 13, 5621–5642, https://doi.org/10.5194/amt-13-5621-2020, https://doi.org/10.5194/amt-13-5621-2020, 2020
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A lidar intercomparison campaign was conducted over a period of 28 nights at Observatoire de Haute-Provence (OHP) in 2017 and 2018. The objective is to validate the ozone and temperature profiles at OHP to ensure the quality of data submitted to the NDACC database remains high. A mobile reference lidar operated by NASA was transported to OHP and operated concurrently with the French lidars. Agreement for ozone was better than 5 % between 20 and 40 km, and temperatures were equal within 3 K.
M. Patrick McCormick, Liqiao Lei, Michael T. Hill, John Anderson, Richard Querel, and Wolfgang Steinbrecht
Atmos. Meas. Tech., 13, 1287–1297, https://doi.org/10.5194/amt-13-1287-2020, https://doi.org/10.5194/amt-13-1287-2020, 2020
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We present a validation of O3 data from the SAGE III-ISS instrument using ground-based lidars and ozonesondes from Hohenpeißenberg and Lauder as well as O3 data from the ACE-FTS instrument. Average differences in the O3 concentration between SAGE III-ISS and the lidar and sonde observations are < 10 % over much of the lower and middle stratosphere. The ACE comparisons are < 5 % from 20 to 45 km. These results provide confidence in the SAGE III measurements of global stratospheric O3 profiles.
Christine Aebi, Julian Gröbner, Stelios Kazadzis, Laurent Vuilleumier, Antonis Gkikas, and Niklaus Kämpfer
Atmos. Meas. Tech., 13, 907–923, https://doi.org/10.5194/amt-13-907-2020, https://doi.org/10.5194/amt-13-907-2020, 2020
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Clouds are one of the largest sources of uncertainties in climate models. The current study estimates the cloud optical thickness (COT), the effective droplet radius and the single scattering albedo of stratus–altostratus and cirrus–cirrostratus clouds in Payerne, Switzerland, by combining ground- and satellite-based measurements and radiative transfer models. The estimated values are thereafter compared with data retrieved from other methods. The mean COT is distinct for different seasons.
Stephan Nyeki, Stefan Wacker, Christine Aebi, Julian Gröbner, Giovanni Martucci, and Laurent Vuilleumier
Atmos. Chem. Phys., 19, 13227–13241, https://doi.org/10.5194/acp-19-13227-2019, https://doi.org/10.5194/acp-19-13227-2019, 2019
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The trends of meteorological parameters and surface downward shortwave radiation (DSR) and downward longwave radiation (DLR) were analysed at four stations (between 370 and 3580 m a. s. l.) in Switzerland for the 1996–2015 period. Trends in DSR and DLR were positive during cloudy as well as clear conditions. The trend due to the influence of clouds decreased in magnitude, which implies a reduction in cloud cover and/or a change towards a different cloud type over the four Swiss sites.
Emilio Cuevas, Pedro Miguel Romero-Campos, Natalia Kouremeti, Stelios Kazadzis, Petri Räisänen, Rosa Delia García, Africa Barreto, Carmen Guirado-Fuentes, Ramón Ramos, Carlos Toledano, Fernando Almansa, and Julian Gröbner
Atmos. Meas. Tech., 12, 4309–4337, https://doi.org/10.5194/amt-12-4309-2019, https://doi.org/10.5194/amt-12-4309-2019, 2019
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A comprehensive comparison of more than 70 000 synchronous 1 min aerosol optical depth (AOD) data from 3 Global Atmosphere Watch precision filter radiometers (GAW-PFR) and 15 Aerosol Robotic Network Cimel radiometers (AERONET-Cimel) was performed for the four
nearwavelengths (380, 440, 500 and 870 nm) in the period 2005–2015. The goal of this study is to assess whether their long term AOD data are comparable and consistent.
Leonie Bernet, Thomas von Clarmann, Sophie Godin-Beekmann, Gérard Ancellet, Eliane Maillard Barras, René Stübi, Wolfgang Steinbrecht, Niklaus Kämpfer, and Klemens Hocke
Atmos. Chem. Phys., 19, 4289–4309, https://doi.org/10.5194/acp-19-4289-2019, https://doi.org/10.5194/acp-19-4289-2019, 2019
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After severe ozone depletion, upper stratospheric ozone has started to recover in recent years. However, stratospheric ozone trends from various data sets still show differences. To partly explain such differences, we investigate how the trends are affected by different factors, for example, anomalies in the data. We show how trend estimates can be improved by considering such anomalies and present updated stratospheric ozone trends from ground data measured in central Europe.
Christine Aebi, Julian Gröbner, and Niklaus Kämpfer
Atmos. Meas. Tech., 11, 5549–5563, https://doi.org/10.5194/amt-11-5549-2018, https://doi.org/10.5194/amt-11-5549-2018, 2018
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A newly developed hemispherical thermal infrared cloud camera (IRCCAM) is presented. The IRCCAM allows automatic cloud detection during the day and at night-time. The cloud fraction determined from the IRCCAM is compared with the cloud fraction determined from other instruments over a time period of 2 years. The IRCCAM has an agreement of +/- 2 oktas cloud fraction in 90 % of the data compared to other instruments. There are no significant differences between seasons or different times of day.
Carlos Toledano, Ramiro González, David Fuertes, Emilio Cuevas, Thomas F. Eck, Stelios Kazadzis, Natalia Kouremeti, Julian Gröbner, Philippe Goloub, Luc Blarel, Roberto Román, África Barreto, Alberto Berjón, Brent N. Holben, and Victoria E. Cachorro
Atmos. Chem. Phys., 18, 14555–14567, https://doi.org/10.5194/acp-18-14555-2018, https://doi.org/10.5194/acp-18-14555-2018, 2018
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Most of the ground-based radiometric networks have their reference instruments and/or calibrate them at Mauna Loa or Izaña. The suitability of these high-mountain stations for absolute radiometric calibrations is investigated with the support of 20 years of first-class Sun photometer data from the AERONET and GAW-PFR networks. We analyze the number of calibration days at each site in a climatological sense and investigate the uncertainty of the calibrations based on long-term statistics.
Kaisa Lakkala, Antti Arola, Julian Gröbner, Sergio Fabian León-Luis, Alberto Redondas, Stelios Kazadzis, Tomi Karppinen, Juha Matti Karhu, Luca Egli, Anu Heikkilä, Tapani Koskela, Antonio Serrano, and José Manuel Vilaplana
Atmos. Meas. Tech., 11, 5167–5180, https://doi.org/10.5194/amt-11-5167-2018, https://doi.org/10.5194/amt-11-5167-2018, 2018
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The performance of the cosine error correction method for correcting spectral UV measurements of the Brewer spectroradiometer was studied. The correction depends on the sky radiation distribution, which can change during one spectral scan. The results showed that the correction varied between 4 and 14 %, and that the relative differences between the reference and the Brewer diminished by 10 %. The method is applicable to other instruments as long as the required input parameters are available.
Alberto Redondas, Virgilio Carreño, Sergio F. León-Luis, Bentorey Hernández-Cruz, Javier López-Solano, Juan J. Rodriguez-Franco, José M. Vilaplana, Julian Gröbner, John Rimmer, Alkiviadis F. Bais, Vladimir Savastiouk, Juan R. Moreta, Lamine Boulkelia, Nis Jepsen, Keith M. Wilson, Vadim Shirotov, and Tomi Karppinen
Atmos. Chem. Phys., 18, 9441–9455, https://doi.org/10.5194/acp-18-9441-2018, https://doi.org/10.5194/acp-18-9441-2018, 2018
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This work shows an overview of the total ozone comparison of the Brewer instrument during the 10th RBCC-E campaign in a joint effort with the EUBREWNET COST 1207 action. The status of the network after 2 years of calibration shows 16 out of the 21 participating Brewer instruments (76 %) agreed within better than ±1 %, and 10 instruments (50 %) agreed within better than ±0.5 %. After applying the final calibration and the stray light correction all working instruments agreed at the ±0.5 % level.
Anna Vaskuri, Petri Kärhä, Luca Egli, Julian Gröbner, and Erkki Ikonen
Atmos. Meas. Tech., 11, 3595–3610, https://doi.org/10.5194/amt-11-3595-2018, https://doi.org/10.5194/amt-11-3595-2018, 2018
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In this work, we introduce a Monte Carlo uncertainty analysis that takes into account possible systematic spectral deviations in the atmospheric full spectrum ozone retrieval method. Accounting for possible systematic spectral deviations in the spectral data is important since they produce larger total ozone column uncertainties than uncorrelated noise-like variations that traditional uncertainty estimations predict.
Rosa Delia García, Africa Barreto, Emilio Cuevas, Julian Gröbner, Omaira Elena García, Angel Gómez-Peláez, Pedro Miguel Romero-Campos, Alberto Redondas, Victoria Eugenia Cachorro, and Ramon Ramos
Geosci. Model Dev., 11, 2139–2152, https://doi.org/10.5194/gmd-11-2139-2018, https://doi.org/10.5194/gmd-11-2139-2018, 2018
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A 7-year comparison study between measured and simulated longwave
downward radiation under cloud-free conditions has been performed at BSRN Izaña. Results show an excellent agreement with a mean bias (simulated–measured) less than 1.1 % and RMSE less than 1 %, which are within the instrumental error (2 %).
Christos Zerefos, John Kapsomenakis, Kostas Eleftheratos, Kleareti Tourpali, Irina Petropavlovskikh, Daan Hubert, Sophie Godin-Beekmann, Wolfgang Steinbrecht, Stacey Frith, Viktoria Sofieva, and Birgit Hassler
Atmos. Chem. Phys., 18, 6427–6440, https://doi.org/10.5194/acp-18-6427-2018, https://doi.org/10.5194/acp-18-6427-2018, 2018
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We point out the representativeness of single lidar stations for zonally averaged ozone profile variations in the middle/upper stratosphere. We examine the contribution of chemistry and natural proxies to ozone profile trends. Above 10 hPa an “inflection point” between 1997–99 marks the end of significant negative ozone trends, followed by a recent period of positive ozone change in 1998–2015. Below 15 hPa the pre-1998 negative ozone trends tend to become insignificant as we move to 2015.
Ralf Zuber, Peter Sperfeld, Stefan Riechelmann, Saulius Nevas, Meelis Sildoja, and Gunther Seckmeyer
Atmos. Meas. Tech., 11, 2477–2484, https://doi.org/10.5194/amt-11-2477-2018, https://doi.org/10.5194/amt-11-2477-2018, 2018
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A compact array spectroradiometer technology that enables precise and robust measurements of UV spectral irradiance is presented. We show that this instrument can retrieve total ozone column (TOC) accurately. The internal stray light, which is often the limiting factor for measurements in the UV spectral range, is physically reduced so that no other stray-light reduction methods are needed.
During an international total ozone measurement intercomparison, the high quality was verified.
Martine De Mazière, Anne M. Thompson, Michael J. Kurylo, Jeannette D. Wild, Germar Bernhard, Thomas Blumenstock, Geir O. Braathen, James W. Hannigan, Jean-Christopher Lambert, Thierry Leblanc, Thomas J. McGee, Gerald Nedoluha, Irina Petropavlovskikh, Gunther Seckmeyer, Paul C. Simon, Wolfgang Steinbrecht, and Susan E. Strahan
Atmos. Chem. Phys., 18, 4935–4964, https://doi.org/10.5194/acp-18-4935-2018, https://doi.org/10.5194/acp-18-4935-2018, 2018
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This paper serves as an introduction to the special issue "Twenty-five years of operations of the Network for the Detection of Atmospheric Composition Change (NDACC)". It describes the origins of the network, its actual status, and some perspectives for its future evolution in the context of atmospheric sciences.
Ulf Köhler, Saulius Nevas, Glen McConville, Robert Evans, Marek Smid, Martin Stanek, Alberto Redondas, and Fritz Schönenborn
Atmos. Meas. Tech., 11, 1989–1999, https://doi.org/10.5194/amt-11-1989-2018, https://doi.org/10.5194/amt-11-1989-2018, 2018
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Laboratory investigations of optical characteristics of three standard Dobsons provide real wavelength settings and slit functions. These parameters were compared with the original values given in the manuals. The differences between real and nominal values are not too large, but their application will in any case improve the quality of the total ozone column measurements in the global
network. This improvement was the main objective of the ATMOZ project funding these activities.
Daniela Meloni, Alcide di Sarra, Gérard Brogniez, Cyrielle Denjean, Lorenzo De Silvestri, Tatiana Di Iorio, Paola Formenti, José L. Gómez-Amo, Julian Gröbner, Natalia Kouremeti, Giuliano Liuzzi, Marc Mallet, Giandomenico Pace, and Damiano M. Sferlazzo
Atmos. Chem. Phys., 18, 4377–4401, https://doi.org/10.5194/acp-18-4377-2018, https://doi.org/10.5194/acp-18-4377-2018, 2018
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This study examines how different aerosol optical properties determine the dust longwave radiative effects at the surface, in the atmosphere and at the top of the atmosphere, based on the combination of remote sensing and in situ observations from the ground, from airborne sensors, and from space, by means of radiative transfer modelling. The closure experiment is based on longwave irradiances and spectral brightness temperatures measured during the 2013 ChArMEx–ADRIMED campaign at Lampedusa.
Christof Janssen, Hadj Elandaloussi, and Julian Gröbner
Atmos. Meas. Tech., 11, 1707–1723, https://doi.org/10.5194/amt-11-1707-2018, https://doi.org/10.5194/amt-11-1707-2018, 2018
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Monitoring ozone layer recovery at a rate of few percent per decade requires dedicated instrumentation and spectroscopic data of the highest quality. Highly accurate absorption cross sections of ozone are rare, especially in the important UV region between 300 and 340 nm. Our measurement provides the first reference point with permil level of accuracy in this range. Interestingly, our value is lower than currently used data. This might resolve an inconsistency between UV and IR measurements.
Javier López-Solano, Alberto Redondas, Thomas Carlund, Juan J. Rodriguez-Franco, Henri Diémoz, Sergio F. León-Luis, Bentorey Hernández-Cruz, Carmen Guirado-Fuentes, Natalia Kouremeti, Julian Gröbner, Stelios Kazadzis, Virgilio Carreño, Alberto Berjón, Daniel Santana-Díaz, Manuel Rodríguez-Valido, Veerle De Bock, Juan R. Moreta, John Rimmer, Andrew R. D. Smedley, Lamine Boulkelia, Nis Jepsen, Paul Eriksen, Alkiviadis F. Bais, Vadim Shirotov, José M. Vilaplana, Keith M. Wilson, and Tomi Karppinen
Atmos. Chem. Phys., 18, 3885–3902, https://doi.org/10.5194/acp-18-3885-2018, https://doi.org/10.5194/acp-18-3885-2018, 2018
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The European Brewer Network (EUBREWNET, COST Action ES1207) is comprised of close to 50 instruments and currently provides near-real-time ozone and UV data. Aerosols also play key role in the Earth–atmosphere system and introduce a large uncertainty into our understanding of climate change. In this work we describe and validate a method to incorporate the measurement of aerosols in EUBREWNET. We find that this Brewer network can provide reliable aerosol data across Europe in the UV range.
Stelios Kazadzis, Natalia Kouremeti, Henri Diémoz, Julian Gröbner, Bruce W. Forgan, Monica Campanelli, Victor Estellés, Kathleen Lantz, Joseph Michalsky, Thomas Carlund, Emilio Cuevas, Carlos Toledano, Ralf Becker, Stephan Nyeki, Panagiotis G. Kosmopoulos, Viktar Tatsiankou, Laurent Vuilleumier, Frederick M. Denn, Nozomu Ohkawara, Osamu Ijima, Philippe Goloub, Panagiotis I. Raptis, Michael Milner, Klaus Behrens, Africa Barreto, Giovanni Martucci, Emiel Hall, James Wendell, Bryan E. Fabbri, and Christoph Wehrli
Atmos. Chem. Phys., 18, 3185–3201, https://doi.org/10.5194/acp-18-3185-2018, https://doi.org/10.5194/acp-18-3185-2018, 2018
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Aerosol optical depth measured from ground-based sun photometers is the most important parameter for studying the changes in the Earth's radiation balance due to aerosols. Representatives for various sun photometer types belonging to individual institutions or international aerosol networks gather every 5 years, for 3 weeks, in Davos, Switzerland, in order to compare their aeorosol optical depth retrievals. This work presents the results of the latest (fourth) filter radiometer intercomparison.
Panagiotis-Ioannis Raptis, Stelios Kazadzis, Julian Gröbner, Natalia Kouremeti, Lionel Doppler, Ralf Becker, and Constantinos Helmis
Atmos. Meas. Tech., 11, 1143–1157, https://doi.org/10.5194/amt-11-1143-2018, https://doi.org/10.5194/amt-11-1143-2018, 2018
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The purpose of this work is to retrieve integrated water vapour using spectral measurements from Precision Solar Spectroradiometer (PSR). Two different approaches were developed one using single-channel direct sun irradiance measurements, and the second one integrating at a certain spectral region. The results of the spectral approach are closer to the retrievals of non-photometric techniques (GPS, microwave radiometer and radiosondes), suggesting this method provide more accurate IWV product.
Stelios Kazadzis, Natalia Kouremeti, Stephan Nyeki, Julian Gröbner, and Christoph Wehrli
Geosci. Instrum. Method. Data Syst., 7, 39–53, https://doi.org/10.5194/gi-7-39-2018, https://doi.org/10.5194/gi-7-39-2018, 2018
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The World Optical Depth Research Calibration Center (WORCC) has been established after the recommendations of WMO for calibration of aerosol optical depth (AOD) -related sun photometers. WORCC is mandated to initiate homogenization activities among different AOD networks and to run a network (GAW-PFR) of sun photometers. To calibrate such instruments aiming at low measurement uncertainties the quality assurance, quality control and a basic hierarchy have to be defined and followed.
Christine Aebi, Julian Gröbner, Niklaus Kämpfer, and Laurent Vuilleumier
Atmos. Meas. Tech., 10, 4587–4600, https://doi.org/10.5194/amt-10-4587-2017, https://doi.org/10.5194/amt-10-4587-2017, 2017
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The current study analyses the cloud radiative effect during the daytime depending on cloud fraction and cloud type at two stations in Switzerland over a time period of 3–5 years. Information about fractional cloud coverage and cloud type is retrieved from images taken by visible all-sky cameras. Cloud cover, cloud type and other atmospheric parameters have an influence on the magnitude of the longwave cloud effect as well as on the shortwave.
Francisco Navas-Guzmán, Niklaus Kämpfer, Franziska Schranz, Wolfgang Steinbrecht, and Alexander Haefele
Atmos. Chem. Phys., 17, 14085–14104, https://doi.org/10.5194/acp-17-14085-2017, https://doi.org/10.5194/acp-17-14085-2017, 2017
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The paper presents assessment of the stratospheric measurements of a relatively new temperature radiometer (TEMPERA) at 60 GHz. The temperature profiles from TEMPERA have been compared with measurements from different techniques such as radiosondes, MLS satellite and Rayleigh lidar and with the temperature outputs from the SD-WACCM model. The results showed absolute biases and standard deviations lower than 2 K for most of the altitudes and comparisons, proving the good performance of TEMPERA.
René Stübi, Herbert Schill, Jörg Klausen, Laurent Vuilleumier, Julian Gröbner, Luca Egli, and Dominique Ruffieux
Atmos. Meas. Tech., 10, 4479–4490, https://doi.org/10.5194/amt-10-4479-2017, https://doi.org/10.5194/amt-10-4479-2017, 2017
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Long-term measurement series are the pillars of all climate change analysis. The Arosa total ozone series is the world's longest record, starting in 1926. To secure the future of these measurements, it is foreseen to move the instruments in Davos. To ascertain that the series will not be affected by this change, a multiyear campaign of parallel measurements on both sites has been done. The analysis of these data is presented and it is concluded that no discernible difference can be identified.
Julian Gröbner, Ingo Kröger, Luca Egli, Gregor Hülsen, Stefan Riechelmann, and Peter Sperfeld
Atmos. Meas. Tech., 10, 3375–3383, https://doi.org/10.5194/amt-10-3375-2017, https://doi.org/10.5194/amt-10-3375-2017, 2017
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We have produced a benchmark high-resolution solar extraterrestrial spectrum from ground-based measurements of direct solar irradiance in the wavelength range 300 to 500 nm. This spectrum can be used for model calculations and for validating solar spectra measured in space. The metrological traceability of this solar spectrum to the International System of Units (SI) is assured by an unbroken chain of calibrations traceable to the primary spectral irradiance standard of PTB.
Wolfgang Steinbrecht, Lucien Froidevaux, Ryan Fuller, Ray Wang, John Anderson, Chris Roth, Adam Bourassa, Doug Degenstein, Robert Damadeo, Joe Zawodny, Stacey Frith, Richard McPeters, Pawan Bhartia, Jeannette Wild, Craig Long, Sean Davis, Karen Rosenlof, Viktoria Sofieva, Kaley Walker, Nabiz Rahpoe, Alexei Rozanov, Mark Weber, Alexandra Laeng, Thomas von Clarmann, Gabriele Stiller, Natalya Kramarova, Sophie Godin-Beekmann, Thierry Leblanc, Richard Querel, Daan Swart, Ian Boyd, Klemens Hocke, Niklaus Kämpfer, Eliane Maillard Barras, Lorena Moreira, Gerald Nedoluha, Corinne Vigouroux, Thomas Blumenstock, Matthias Schneider, Omaira García, Nicholas Jones, Emmanuel Mahieu, Dan Smale, Michael Kotkamp, John Robinson, Irina Petropavlovskikh, Neil Harris, Birgit Hassler, Daan Hubert, and Fiona Tummon
Atmos. Chem. Phys., 17, 10675–10690, https://doi.org/10.5194/acp-17-10675-2017, https://doi.org/10.5194/acp-17-10675-2017, 2017
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Thanks to the 1987 Montreal Protocol and its amendments, ozone-depleting chlorine (and bromine) in the stratosphere has declined slowly since the late 1990s. Improved and extended long-term ozone profile observations from satellites and ground-based stations confirm that ozone is responding as expected and has increased by about 2 % per decade since 2000 in the upper stratosphere, around 40 km altitude. At lower altitudes, however, ozone has not changed significantly since 2000.
Stephan Nyeki, Stefan Wacker, Julian Gröbner, Wolfgang Finsterle, and Martin Wild
Atmos. Meas. Tech., 10, 3057–3071, https://doi.org/10.5194/amt-10-3057-2017, https://doi.org/10.5194/amt-10-3057-2017, 2017
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A large number of radiometers used to measure solar and terrestrial broadband radiation are traceable to World Standard Groups at PMOD/WRC in Davos, Switzerland. A small correction of each group may be required in the future, and this study examines the methods and implications of this on data sets collected at four remote baseline stations since the 1990s. The goal is to develop a better estimate of the solar and terrestrial radiation budget at the Earth's surface.
Thomas Carlund, Natalia Kouremeti, Stelios Kazadzis, and Julian Gröbner
Atmos. Meas. Tech., 10, 905–923, https://doi.org/10.5194/amt-10-905-2017, https://doi.org/10.5194/amt-10-905-2017, 2017
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Aerosols play an important role in atmospheric processes. Aerosol optical depth is the most common measure of columnar aerosol load. We present a sunphotometer called UVPFR that is able to measure aerosol optical depth in the ultraviolet range, including the calibration, characterization and validation of the instrument/measurements. The instrument will serve as a reference on the intercalibration of Brewer spectrophotometers that are also able to measure aerosol optical depth in the UV region.
Christos S. Zerefos, Kostas Eleftheratos, John Kapsomenakis, Stavros Solomos, Antje Inness, Dimitris Balis, Alberto Redondas, Henk Eskes, Marc Allaart, Vassilis Amiridis, Arne Dahlback, Veerle De Bock, Henri Diémoz, Ronny Engelmann, Paul Eriksen, Vitali Fioletov, Julian Gröbner, Anu Heikkilä, Irina Petropavlovskikh, Janusz Jarosławski, Weine Josefsson, Tomi Karppinen, Ulf Köhler, Charoula Meleti, Christos Repapis, John Rimmer, Vladimir Savinykh, Vadim Shirotov, Anna Maria Siani, Andrew R. D. Smedley, Martin Stanek, and René Stübi
Atmos. Chem. Phys., 17, 551–574, https://doi.org/10.5194/acp-17-551-2017, https://doi.org/10.5194/acp-17-551-2017, 2017
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The paper makes a convincing case that the Brewer network is capable of detecting enhanced SO2 columns, as observed, e.g., after volcanic eruptions. For this reason, large volcanic eruptions of the past decade have been used to detect and forecast SO2 plumes of volcanic origin using the Brewer and other ground-based networks, aided by satellite, trajectory analysis calculations and modelling.
Christoph Kalicinsky, Peter Knieling, Ralf Koppmann, Dirk Offermann, Wolfgang Steinbrecht, and Johannes Wintel
Atmos. Chem. Phys., 16, 15033–15047, https://doi.org/10.5194/acp-16-15033-2016, https://doi.org/10.5194/acp-16-15033-2016, 2016
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The analysis of temperatures in the mesopause region between 1988 to 2015 shows, besides the known correlation with the 11-year solar activity cycle, a trend reversal in 2008 that can be described by a long-term oscillation. Understanding such long periodic oscillations in the atmosphere is of prime importance for climate modelling and predictions of future trends.
Daan Hubert, Jean-Christopher Lambert, Tijl Verhoelst, José Granville, Arno Keppens, Jean-Luc Baray, Adam E. Bourassa, Ugo Cortesi, Doug A. Degenstein, Lucien Froidevaux, Sophie Godin-Beekmann, Karl W. Hoppel, Bryan J. Johnson, Erkki Kyrölä, Thierry Leblanc, Günter Lichtenberg, Marion Marchand, C. Thomas McElroy, Donal Murtagh, Hideaki Nakane, Thierry Portafaix, Richard Querel, James M. Russell III, Jacobo Salvador, Herman G. J. Smit, Kerstin Stebel, Wolfgang Steinbrecht, Kevin B. Strawbridge, René Stübi, Daan P. J. Swart, Ghassan Taha, David W. Tarasick, Anne M. Thompson, Joachim Urban, Joanna A. E. van Gijsel, Roeland Van Malderen, Peter von der Gathen, Kaley A. Walker, Elian Wolfram, and Joseph M. Zawodny
Atmos. Meas. Tech., 9, 2497–2534, https://doi.org/10.5194/amt-9-2497-2016, https://doi.org/10.5194/amt-9-2497-2016, 2016
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A more detailed understanding of satellite O3 profile data records is vital for further progress in O3 research. To this end, we made a comprehensive assessment of 14 limb/occultation profilers using ground-based reference data. The mutual consistency of satellite O3 in terms of bias, short-term variability and decadal stability is generally good over most of the stratosphere. However, we identified some exceptions that impact the quality of recently merged data sets and ozone trend assessments.
Luca Egli, Julian Gröbner, Gregor Hülsen, Luciano Bachmann, Mario Blumthaler, Jimmy Dubard, Marina Khazova, Richard Kift, Kees Hoogendijk, Antonio Serrano, Andrew Smedley, and José-Manuel Vilaplana
Atmos. Meas. Tech., 9, 1553–1567, https://doi.org/10.5194/amt-9-1553-2016, https://doi.org/10.5194/amt-9-1553-2016, 2016
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Array spectroradiometers are small, light, robust and cost-effective instruments, and are increasingly used for atmospheric measurements. The quality of array spectroradiometers is assessed for the reliable quantification of ultraviolet radiation (UV) in order to monitor the exposure of UV radiation to human health. The study shows that reliable UV measurements with these instruments are limited for observations around noon and show large biases in the morning and evening.
África Barreto, Emilio Cuevas, María-José Granados-Muñoz, Lucas Alados-Arboledas, Pedro M. Romero, Julian Gröbner, Natalia Kouremeti, Antonio F. Almansa, Tom Stone, Carlos Toledano, Roberto Román, Mikhail Sorokin, Brent Holben, Marius Canini, and Margarita Yela
Atmos. Meas. Tech., 9, 631–654, https://doi.org/10.5194/amt-9-631-2016, https://doi.org/10.5194/amt-9-631-2016, 2016
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This paper presents the new photometer CE318-T, able to perform daytime and
night-time photometric measurements using the sun and the moon as light
sources. This new device permits a complete cycle of diurnal aerosol and water vapour measurements to be extracted, valuable to enhance atmospheric monitoring. We have also highlighted the ability of this new device to capture short-term atmospheric variations, critical for climate studies.
S. Hassinen, D. Balis, H. Bauer, M. Begoin, A. Delcloo, K. Eleftheratos, S. Gimeno Garcia, J. Granville, M. Grossi, N. Hao, P. Hedelt, F. Hendrick, M. Hess, K.-P. Heue, J. Hovila, H. Jønch-Sørensen, N. Kalakoski, A. Kauppi, S. Kiemle, L. Kins, M. E. Koukouli, J. Kujanpää, J.-C. Lambert, R. Lang, C. Lerot, D. Loyola, M. Pedergnana, G. Pinardi, F. Romahn, M. van Roozendael, R. Lutz, I. De Smedt, P. Stammes, W. Steinbrecht, J. Tamminen, N. Theys, L. G. Tilstra, O. N. E. Tuinder, P. Valks, C. Zerefos, W. Zimmer, and I. Zyrichidou
Atmos. Meas. Tech., 9, 383–407, https://doi.org/10.5194/amt-9-383-2016, https://doi.org/10.5194/amt-9-383-2016, 2016
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The three GOME-2 instruments will provide unique and long data sets for atmospheric research and applications. The complete time period will be 2007–2022, including the period of ozone depletion as well as the beginning of ozone layer recovery. The GOME-2 products (ozone, trace gases, aerosols and UV radiation) are important for ozone chemistry, air quality studies, climate modeling, policy monitoring and hazard warnings. The processing and dissemination is done by EUMETSAT O3M SAF project.
T. Verhoelst, J. Granville, F. Hendrick, U. Köhler, C. Lerot, J.-P. Pommereau, A. Redondas, M. Van Roozendael, and J.-C. Lambert
Atmos. Meas. Tech., 8, 5039–5062, https://doi.org/10.5194/amt-8-5039-2015, https://doi.org/10.5194/amt-8-5039-2015, 2015
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Comparisons between satellite and ground-based measurements of the
atmosphere are inevitably affected by natural variability due to
mismatches in spatial and temporal co-location. These
additional terms in the comparison error budget are quantified here
for total ozone column comparisons using an Observing System Simulation
Experiment. Even when using tight co-location criteria, atmospheric
variability is found to impact the comparisons significantly.
N. R. P. Harris, B. Hassler, F. Tummon, G. E. Bodeker, D. Hubert, I. Petropavlovskikh, W. Steinbrecht, J. Anderson, P. K. Bhartia, C. D. Boone, A. Bourassa, S. M. Davis, D. Degenstein, A. Delcloo, S. M. Frith, L. Froidevaux, S. Godin-Beekmann, N. Jones, M. J. Kurylo, E. Kyrölä, M. Laine, S. T. Leblanc, J.-C. Lambert, B. Liley, E. Mahieu, A. Maycock, M. de Mazière, A. Parrish, R. Querel, K. H. Rosenlof, C. Roth, C. Sioris, J. Staehelin, R. S. Stolarski, R. Stübi, J. Tamminen, C. Vigouroux, K. A. Walker, H. J. Wang, J. Wild, and J. M. Zawodny
Atmos. Chem. Phys., 15, 9965–9982, https://doi.org/10.5194/acp-15-9965-2015, https://doi.org/10.5194/acp-15-9965-2015, 2015
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Trends in the vertical distribution of ozone are reported for new and recently revised data sets. The amount of ozone-depleting compounds in the stratosphere peaked in the second half of the 1990s. We examine the trends before and after that peak to see if any change in trend is discernible. The previously reported decreases are confirmed. Furthermore, the downward trend in upper stratospheric ozone has not continued. The possible significance of any increase is discussed in detail.
J. A. E. van Gijsel, R. Zurita-Milla, P. Stammes, S. Godin-Beekmann, T. Leblanc, M. Marchand, I. S. McDermid, K. Stebel, W. Steinbrecht, and D. P. J. Swart
Atmos. Meas. Tech., 8, 1951–1963, https://doi.org/10.5194/amt-8-1951-2015, https://doi.org/10.5194/amt-8-1951-2015, 2015
F. Tummon, B. Hassler, N. R. P. Harris, J. Staehelin, W. Steinbrecht, J. Anderson, G. E. Bodeker, A. Bourassa, S. M. Davis, D. Degenstein, S. M. Frith, L. Froidevaux, E. Kyrölä, M. Laine, C. Long, A. A. Penckwitt, C. E. Sioris, K. H. Rosenlof, C. Roth, H.-J. Wang, and J. Wild
Atmos. Chem. Phys., 15, 3021–3043, https://doi.org/10.5194/acp-15-3021-2015, https://doi.org/10.5194/acp-15-3021-2015, 2015
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Understanding ozone trends in the vertical is vital in terms of assessing the success of the Montreal Protocol. This paper compares and analyses the long-term trends in stratospheric ozone from seven new merged satellite data sets. The data sets largely agree well with each other, particularly for the negative trends seen in the early period 1984-1997. For the 1998-2011 period there is less agreement, but a clear shift from negative to mostly positive trends.
Y. Bühler, M. Marty, L. Egli, J. Veitinger, T. Jonas, P. Thee, and C. Ginzler
The Cryosphere, 9, 229–243, https://doi.org/10.5194/tc-9-229-2015, https://doi.org/10.5194/tc-9-229-2015, 2015
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We are able to map snow depth over large areas ( > 100km2) using airborne digital photogrammetry. Digital photogrammetry is more economical than airborne Laser Scanning but slightly less accurate. Comparisons to independent snow depth measurements reveal an accuracy of about 30cm. Spatial continuous mapping of snow depth is a major step forward compared to point measurements usually applied today. Limitations are steep slopes (> 50°) and areas covered by trees and scrubs.
M. Lothon, F. Lohou, D. Pino, F. Couvreux, E. R. Pardyjak, J. Reuder, J. Vilà-Guerau de Arellano, P Durand, O. Hartogensis, D. Legain, P. Augustin, B. Gioli, D. H. Lenschow, I. Faloona, C. Yagüe, D. C. Alexander, W. M. Angevine, E Bargain, J. Barrié, E. Bazile, Y. Bezombes, E. Blay-Carreras, A. van de Boer, J. L. Boichard, A. Bourdon, A. Butet, B. Campistron, O. de Coster, J. Cuxart, A. Dabas, C. Darbieu, K. Deboudt, H. Delbarre, S. Derrien, P. Flament, M. Fourmentin, A. Garai, F. Gibert, A. Graf, J. Groebner, F. Guichard, M. A. Jiménez, M. Jonassen, A. van den Kroonenberg, V. Magliulo, S. Martin, D. Martinez, L. Mastrorillo, A. F. Moene, F. Molinos, E. Moulin, H. P. Pietersen, B. Piguet, E. Pique, C. Román-Cascón, C. Rufin-Soler, F. Saïd, M. Sastre-Marugán, Y. Seity, G. J. Steeneveld, P. Toscano, O. Traullé, D. Tzanos, S. Wacker, N. Wildmann, and A. Zaldei
Atmos. Chem. Phys., 14, 10931–10960, https://doi.org/10.5194/acp-14-10931-2014, https://doi.org/10.5194/acp-14-10931-2014, 2014
S. Kazadzis, I. Veselovskii, V. Amiridis, J. Gröbner, A. Suvorina, S. Nyeki, E. Gerasopoulos, N. Kouremeti, M. Taylor, A. Tsekeri, and C. Wehrli
Atmos. Meas. Tech., 7, 2013–2025, https://doi.org/10.5194/amt-7-2013-2014, https://doi.org/10.5194/amt-7-2013-2014, 2014
E. Eckert, T. von Clarmann, M. Kiefer, G. P. Stiller, S. Lossow, N. Glatthor, D. A. Degenstein, L. Froidevaux, S. Godin-Beekmann, T. Leblanc, S. McDermid, M. Pastel, W. Steinbrecht, D. P. J. Swart, K. A. Walker, and P. F. Bernath
Atmos. Chem. Phys., 14, 2571–2589, https://doi.org/10.5194/acp-14-2571-2014, https://doi.org/10.5194/acp-14-2571-2014, 2014
A. Redondas, R. Evans, R. Stuebi, U. Köhler, and M. Weber
Atmos. Chem. Phys., 14, 1635–1648, https://doi.org/10.5194/acp-14-1635-2014, https://doi.org/10.5194/acp-14-1635-2014, 2014
A. Stenke, C. R. Hoyle, B. Luo, E. Rozanov, J. Gröbner, L. Maag, S. Brönnimann, and T. Peter
Atmos. Chem. Phys., 13, 9713–9729, https://doi.org/10.5194/acp-13-9713-2013, https://doi.org/10.5194/acp-13-9713-2013, 2013
T. Egorova, E. Rozanov, J. Gröbner, M. Hauser, and W. Schmutz
Atmos. Chem. Phys., 13, 3811–3823, https://doi.org/10.5194/acp-13-3811-2013, https://doi.org/10.5194/acp-13-3811-2013, 2013
Related subject area
Subject: Gases | Technique: Remote Sensing | Topic: Validation and Intercomparisons
An evaluation of atmospheric absorption models at millimetre and sub-millimetre wavelengths using airborne observations
Applicability of the inverse dispersion method to measure emissions from animal housings
5 years of Sentinel-5P TROPOMI operational ozone profiling and geophysical validation using ozonesonde and lidar ground-based networks
Using a portable FTIR spectrometer to evaluate the consistency of Total Carbon Column Observing Network (TCCON) measurements on a global scale: the Collaborative Carbon Column Observing Network (COCCON) travel standard
Comparison of the H2O, HDO and δD stratospheric climatologies between the MIPAS-ESA V8, MIPAS-IMK V5 and ACE-FTS V4.1/4.2 satellite datasets
Using Open-Path Dual-Comb Spectroscopy to Monitor Methane Emissions from Simulated Grazing Cattle
TROPESS-CrIS CO single-pixel vertical profiles: intercomparisons with MOPITT and model simulations for 2020 western US wildfires
TOLNet validation of satellite ozone profiles in the troposphere: impact of retrieval wavelengths
An uncertainty methodology for solar occultation flux measurements: ammonia emissions from livestock production
Validation of Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) chlorodifluoromethane (HCFC-22) in the upper troposphere and lower stratosphere
Validation of GEMS tropospheric NO2 columns and their diurnal variation with ground-based DOAS measurements
First validation of high-resolution satellite-derived methane emissions from an active gas leak in the UK
First evaluation of the GEMS glyoxal products against TROPOMI and ground-based measurements
Ship- and aircraft-based XCH4 over oceans as a new tool for satellite validation
Single-blind test of nine methane-sensing satellite systems from three continents
Water vapor measurements inside clouds and storms using a differential absorption radar
Evaluation of the first year of Pandora NO2 measurements over Beijing and application to satellite validation
Validation of MUSES NH3 observations from AIRS and CrIS against aircraft measurements from DISCOVER-AQ and a surface network in the Magic Valley
Performance and sensitivity of column-wise and pixel-wise methane retrievals for imaging spectrometers
Methane point source quantification using MethaneAIR: a new airborne imaging spectrometer
Greenhouse gas column observations from a portable spectrometer in Uganda
Independent validation of IASI/METOP-A LMD and RAL CH4 products using CAMS model, in situ profiles and ground-based FTIR measurements
Evaluation of total ozone measurements from Geostationary Environmental Monitoring Spectrometer (GEMS)
To new heights by flying low: comparison of aircraft vertical NO2 profiles to model simulations and implications for TROPOMI NO2 retrievals
Local comparisons of tropospheric ozone: vertical soundings at two neighbouring stations in southern Bavaria
Ground-based Multi-AXis Differential Optical Absorption Spectroscopy (MAX-DOAS) observations of NO2 and H2CO at Kinshasa and comparisons with TROPOMI observations
Total column ozone trends from the NASA Merged Ozone time series 1979 to 2021 showing latitude-dependent ozone recovery dates (1994 to 1998)
The SPARC water vapour assessment II: biases and drifts of water vapour satellite data records with respect to frost point hygrometer records
Vicarious calibration of the Tropospheric Monitoring Instrument (TROPOMI) short-wave infrared (SWIR) module over the Railroad Valley Playa
First-time comparison between NO2 vertical columns from Geostationary Environmental Monitoring Spectrometer (GEMS) and Pandora measurements
A blended TROPOMI+GOSAT satellite data product for atmospheric methane using machine learning to correct retrieval biases
Evaluating the consistency between OCO-2 and OCO-3 XCO2 estimates derived from the NASA ACOS version 10 retrieval algorithm
OLCI-A/B tandem phase: evaluation of FLuorescence EXplorer (FLEX)-like radiances and estimation of systematic differences between OLCI-A and OLCI-FLEX
Multi-parameter dynamical diagnostics for upper tropospheric and lower stratospheric studies
An approach to track instrument calibration and produce consistent products with the version-8 total column ozone algorithm (V8TOZ)
Satellite remote-sensing capability to assess tropospheric-column ratios of formaldehyde and nitrogen dioxide: case study during the Long Island Sound Tropospheric Ozone Study 2018 (LISTOS 2018) field campaign
Validation of Sentinel-5P TROPOMI tropospheric NO2 products by comparison with NO2 measurements from airborne imaging DOAS, ground-based stationary DOAS, and mobile car DOAS measurements during the S5P-VAL-DE-Ruhr campaign
Evaluation of open- and closed-path sampling systems for the determination of emission rates of NH3 and CH4 with inverse dispersion modeling
Performance of AIRS ozone retrieval over the central Himalayas: use of ozonesonde and other satellite datasets
Solar occultation measurement of mesospheric ozone by SAGE III/ISS: impact of variations along the line of sight caused by photochemistry
Understanding the potential of Sentinel-2 for monitoring methane point emissions
TROPOMI/S5P Total Column Water Vapor validation against AERONET ground-based measurements
Assessing the consistency of satellite-derived upper tropospheric humidity measurements
A comparison of carbon monoxide retrievals between the MOPITT satellite and Canadian high-Arctic ground-based NDACC and TCCON FTIR measurements
Long-term validation of MIPAS ESA operational products using MIPAS-B measurements
Comparison of OCO-2 target observations to MUCCnet – is it possible to capture urban XCO2 gradients from space?
SAGE III/ISS ozone and NO2 validation using diurnal scaling factors
An improved OSIRIS NO2 profile retrieval in the upper troposphere–lower stratosphere and intercomparison with ACE-FTS and SAGE III/ISS
Joint spectral retrievals of ozone with Suomi NPP CrIS augmented by S5P/TROPOMI
TROPESS/CrIS carbon monoxide profile validation with NOAA GML and ATom in situ aircraft observations
Stuart Fox, Vinia Mattioli, Emma Turner, Alan Vance, Domenico Cimini, and Donatello Gallucci
Atmos. Meas. Tech., 17, 4957–4978, https://doi.org/10.5194/amt-17-4957-2024, https://doi.org/10.5194/amt-17-4957-2024, 2024
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Airborne observations are used to evaluate two models for absorption and emission by atmospheric gases, including water vapour and oxygen, at microwave and sub-millimetre wavelengths. These models are needed for the Ice Cloud Imager (ICI) on the next generation of European polar-orbiting weather satellites, which measures at frequencies up to 664 GHz. Both models can provide a good match to measurements from airborne radiometers and are sufficiently accurate for use with ICI.
Marcel Bühler, Christoph Häni, Albrecht Neftel, Patrice Bühler, Christof Ammann, and Thomas Kupper
Atmos. Meas. Tech., 17, 4649–4658, https://doi.org/10.5194/amt-17-4649-2024, https://doi.org/10.5194/amt-17-4649-2024, 2024
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Methane was released from an artificial source inside a barn to test the applicability of the inverse dispersion method (IDM). Multiple open-path concentration devices and ultrasonic anemometers were used at the site. It is concluded that, for the present study case, the effect of a building and a tree in the main wind axis led to a systematic underestimation of the IDM-derived emission rate probably due to deviations in the wind field and turbulent dispersion from the ideal assumptions.
Arno Keppens, Serena Di Pede, Daan Hubert, Jean-Christopher Lambert, Pepijn Veefkind, Maarten Sneep, Johan De Haan, Mark ter Linden, Thierry Leblanc, Steven Compernolle, Tijl Verhoelst, José Granville, Oindrila Nath, Ann Mari Fjæraa, Ian Boyd, Sander Niemeijer, Roeland Van Malderen, Herman G. J. Smit, Valentin Duflot, Sophie Godin-Beekmann, Bryan J. Johnson, Wolfgang Steinbrecht, David W. Tarasick, Debra E. Kollonige, Ryan M. Stauffer, Anne M. Thompson, Angelika Dehn, and Claus Zehner
Atmos. Meas. Tech., 17, 3969–3993, https://doi.org/10.5194/amt-17-3969-2024, https://doi.org/10.5194/amt-17-3969-2024, 2024
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The Sentinel-5P satellite operated by the European Space Agency has carried the TROPOspheric Monitoring Instrument (TROPOMI) around the Earth since October 2017. This mission also produces atmospheric ozone profile data which are described in detail for May 2018 to April 2023. Independent validation using ground-based reference measurements demonstrates that the operational ozone profile product mostly fully and at least partially complies with all mission requirements.
Benedikt Herkommer, Carlos Alberti, Paolo Castracane, Jia Chen, Angelika Dehn, Florian Dietrich, Nicholas M. Deutscher, Matthias Max Frey, Jochen Groß, Lawson Gillespie, Frank Hase, Isamu Morino, Nasrin Mostafavi Pak, Brittany Walker, and Debra Wunch
Atmos. Meas. Tech., 17, 3467–3494, https://doi.org/10.5194/amt-17-3467-2024, https://doi.org/10.5194/amt-17-3467-2024, 2024
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The Total Carbon Column Observing Network is a network of ground-based Fourier transform infrared (FTIR) spectrometers used mainly for satellite validation. To ensure the highest-quality validation data, the network needs to be highly consistent. This is a major challenge, which so far is solved by site comparisons with airborne in situ measurements. In this work, we describe the use of a portable FTIR spectrometer as a travel standard for evaluating the consistency of TCCON sites.
Karen De Los Ríos, Paulina Ordoñez, Gabriele P. Stiller, Piera Raspollini, Marco Gai, Kaley A. Walker, Cristina Peña-Ortiz, and Luis Acosta
Atmos. Meas. Tech., 17, 3401–3418, https://doi.org/10.5194/amt-17-3401-2024, https://doi.org/10.5194/amt-17-3401-2024, 2024
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This study examines newer versions of H2O and HDO retrievals from Envisat/MIPAS and SCISAT/ACE-FTS. Results reveal a better agreement in stratospheric H2O profiles than in HDO profiles. The H2O tape recorder signal is consistent across databases, but δD tape recorder composites show differences that impact the interpretation of water vapour transport. These findings enhance the need for intercomparisons to refine our insights.
Chinthaka Weerasekara, Lindsay Morris, Nathan Malarich, Fabrizio Giorgetta, Daniel Herman, Kevin Cossel, Nathan Newbury, Clenton Owensby, Stephen Welch, Cosmin Blaga, Brett DePaola, Ian Coddington, Eduardo Santos, and Brian Washburn
EGUsphere, https://doi.org/10.5194/egusphere-2024-1181, https://doi.org/10.5194/egusphere-2024-1181, 2024
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Most methane emissions during the life cycle of beef cattle occur during the grazing phase. Measuring methane in grazing systems is difficult due to the high mobility and low density of animals. This work investigates if dual-comb spectroscopy can measure methane emissions from small cattle herds. An enhancement of 10 nmol mol-1 methane above the atmospheric background was measured, equivalent to 20 head located 60 m away. The calculated methane flux was within 5 % of the actual release rate.
Ming Luo, Helen M. Worden, Robert D. Field, Kostas Tsigaridis, and Gregory S. Elsaesser
Atmos. Meas. Tech., 17, 2611–2624, https://doi.org/10.5194/amt-17-2611-2024, https://doi.org/10.5194/amt-17-2611-2024, 2024
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The TROPESS CrIS single-pixel CO profile retrievals are compared to the MOPITT CO products in steps of adjusting them to the common a priori assumptions. The two data sets are found to agree within 5 %. We also demonstrated and analyzed the proper steps in evaluating GISS ModelE CO simulations using satellite CO retrieval products for the western US wildfire events in September 2020.
Matthew S. Johnson, Alexei Rozanov, Mark Weber, Nora Mettig, John Sullivan, Michael J. Newchurch, Shi Kuang, Thierry Leblanc, Fernando Chouza, Timothy A. Berkoff, Guillaume Gronoff, Kevin B. Strawbridge, Raul J. Alvarez, Andrew O. Langford, Christoph J. Senff, Guillaume Kirgis, Brandi McCarty, and Larry Twigg
Atmos. Meas. Tech., 17, 2559–2582, https://doi.org/10.5194/amt-17-2559-2024, https://doi.org/10.5194/amt-17-2559-2024, 2024
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Monitoring tropospheric ozone (O3), a harmful pollutant negatively impacting human health, is primarily done using ground-based measurements and ozonesondes. However, these observation types lack the coverage to fully understand tropospheric O3. Satellites can retrieve tropospheric ozone with near-daily global coverage; however, they are known to have biases and errors. This study uses ground-based lidars to validate multiple satellites' ability to observe tropospheric O3.
Johan Mellqvist, Nathalia T. Vechi, Charlotte Scheutz, Marc Durif, Francois Gautier, John Johansson, Jerker Samuelsson, Brian Offerle, and Samuel Brohede
Atmos. Meas. Tech., 17, 2465–2479, https://doi.org/10.5194/amt-17-2465-2024, https://doi.org/10.5194/amt-17-2465-2024, 2024
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The solar occultation flux method retrieves ammonia gas columns from the solar spectrum. Emissions are obtained by multiplying the integrated plume concentration by the wind speed profile. The methodology for uncertainty estimation was established considering an error budget with systematic and random components, resulting in an expanded uncertainty in the range of 20 % to 30 %. The method was validated in a controlled release, and its application was demonstrated in different farms.
Felicia Kolonjari, Patrick E. Sheese, Kaley A. Walker, Chris D. Boone, David A. Plummer, Andreas Engel, Stephen A. Montzka, David E. Oram, Tanja Schuck, Gabriele P. Stiller, and Geoffrey C. Toon
Atmos. Meas. Tech., 17, 2429–2449, https://doi.org/10.5194/amt-17-2429-2024, https://doi.org/10.5194/amt-17-2429-2024, 2024
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The Canadian Atmospheric Chemistry Experiment Fourier transform spectrometer (ACE-FTS) satellite instrument is currently providing the only vertically resolved chlorodifluoromethane (HCFC-22) measurements from space. This study assesses the most current ACE-FTS HCFC-22 data product in the upper troposphere and lower stratosphere, as well as modelled HCFC-22 from a 39-year run of the Canadian Middle Atmosphere Model (CMAM39) in the same region.
Kezia Lange, Andreas Richter, Tim Bösch, Bianca Zilker, Miriam Latsch, Lisa K. Behrens, Chisom M. Okafor, Hartmut Bösch, John P. Burrows, Alexis Merlaud, Gaia Pinardi, Caroline Fayt, Martina M. Friedrich, Ermioni Dimitropoulou, Michel Van Roozendael, Steffen Ziegler, Simona Ripperger-Lukosiunaite, Leon Kuhn, Bianca Lauster, Thomas Wagner, Hyunkee Hong, Donghee Kim, Lim-Seok Chang, Kangho Bae, Chang-Keun Song, and Hanlim Lee
EGUsphere, https://doi.org/10.5194/egusphere-2024-617, https://doi.org/10.5194/egusphere-2024-617, 2024
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Instruments for air quality observations on geostationary satellites provide multiple observations per day and allow for the analysis of the diurnal variation of important air pollutants such as nitrogen dioxide (NO2) over large areas. The South Korean instrument GEMS, launched in February 2020, is the first instrument in geostationary orbit and covers a large part of Asia. Our investigations show the observed diurnal evolution of NO2 at different measurement sites.
Emily Dowd, Alistair J. Manning, Bryn Orth-Lashley, Marianne Girard, James France, Rebecca E. Fisher, Dave Lowry, Mathias Lanoisellé, Joseph R. Pitt, Kieran M. Stanley, Simon O'Doherty, Dickon Young, Glen Thistlethwaite, Martyn P. Chipperfield, Emanuel Gloor, and Chris Wilson
Atmos. Meas. Tech., 17, 1599–1615, https://doi.org/10.5194/amt-17-1599-2024, https://doi.org/10.5194/amt-17-1599-2024, 2024
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We provide the first validation of the satellite-derived emission estimates using surface-based mobile greenhouse gas surveys of an active gas leak detected near Cheltenham, UK. GHGSat’s emission estimates broadly agree with the surface-based mobile survey and steps were taken to fix the leak, highlighting the importance of satellite data in identifying emissions and helping to reduce our human impact on climate change.
Eunjo S. Ha, Rokjin J. Park, Hyeong-Ahn Kwon, Gitaek T. Lee, Sieun D. Lee, Seunga Shin, Dong-Won Lee, Hyunkee Hong, Christophe Lerot, Isabelle De Smedt, Francois Hendrick, and Hitoshi Irie
EGUsphere, https://doi.org/10.5194/egusphere-2024-589, https://doi.org/10.5194/egusphere-2024-589, 2024
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In this study, we evaluated the GEMS glyoxal products by comparing them with TROPOMI and MAX-DOAS measurements. GEMS and TROPOMI VCDs present similar spatial distributions. Monthly variations of GEMS VCDs with those of TROPOMI and MAX-DOAS VCDs differ in Northeast Asia, which we attributed to a polluted reference spectrum and high NO2 concentrations. GEMS glyoxal products with unparalleled temporal resolution would enrich our understanding of VOC emissions and diurnal variation.
Astrid Müller, Hiroshi Tanimoto, Takafumi Sugita, Prabir K. Patra, Shin-ichiro Nakaoka, Toshinobu Machida, Isamu Morino, André Butz, and Kei Shiomi
Atmos. Meas. Tech., 17, 1297–1316, https://doi.org/10.5194/amt-17-1297-2024, https://doi.org/10.5194/amt-17-1297-2024, 2024
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Satellite CH4 observations with high accuracy are needed to understand changes in atmospheric CH4 concentrations. But over oceans, reference data are limited. We combine various ship and aircraft observations with the help of atmospheric chemistry models to derive observation-based column-averaged mixing ratios of CH4 (obs. XCH4). We discuss three different approaches and demonstrate the applicability of the new reference dataset for carbon cycle studies and satellite evaluation.
Evan D. Sherwin, Sahar H. El Abbadi, Philippine M. Burdeau, Zhan Zhang, Zhenlin Chen, Jeffrey S. Rutherford, Yuanlei Chen, and Adam R. Brandt
Atmos. Meas. Tech., 17, 765–782, https://doi.org/10.5194/amt-17-765-2024, https://doi.org/10.5194/amt-17-765-2024, 2024
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Countries and companies increasingly rely on a growing fleet of satellites to find large emissions of climate-warming methane, particularly from oil and natural gas systems across the globe. We independently assessed the performance of nine such systems by releasing controlled, undisclosed amounts of methane as satellites passed overhead. The tested systems produced reliable detection and quantification results, including the smallest-ever emission detected from space in such a test.
Luis F. Millán, Matthew D. Lebsock, Ken B. Cooper, Jose V. Siles, Robert Dengler, Raquel Rodriguez Monje, Amin Nehrir, Rory A. Barton-Grimley, James E. Collins, Claire E. Robinson, Kenneth L. Thornhill, and Holger Vömel
Atmos. Meas. Tech., 17, 539–559, https://doi.org/10.5194/amt-17-539-2024, https://doi.org/10.5194/amt-17-539-2024, 2024
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In this study, we describe and validate a new technique in which three radar tones are used to estimate the water vapor inside clouds and precipitation. This instrument flew on board NASA's P-3 aircraft during the Investigation of Microphysics and Precipitation for Atlantic Coast-Threatening Snowstorms (IMPACTS) campaign and the Synergies Of Active optical and Active microwave Remote Sensing Experiment (SOA2RSE) campaign.
Ouyang Liu, Zhengqiang Li, Yangyan Lin, Cheng Fan, Ying Zhang, Kaitao Li, Peng Zhang, Yuanyuan Wei, Tianzeng Chen, Jiantao Dong, and Gerrit de Leeuw
Atmos. Meas. Tech., 17, 377–395, https://doi.org/10.5194/amt-17-377-2024, https://doi.org/10.5194/amt-17-377-2024, 2024
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Nitrogen dioxide (NO2) is a trace gas which is important for atmospheric chemistry and may affect human health. To understand processes leading to harmful concentrations, it is important to monitor NO2 concentrations near the surface and higher up. To this end, a Pandora instrument has been installed in Beijing. An overview of the first year of data shows the large variability on diurnal to seasonal timescales and how this is affected by wind speed and direction and chemistry.
Karen E. Cady-Pereira, Xuehui Guo, Rui Wang, April B. Leytem, Chase Calkins, Elizabeth Berry, Kang Sun, Markus Müller, Armin Wisthaler, Vivienne H. Payne, Mark W. Shephard, Mark A. Zondlo, and Valentin Kantchev
Atmos. Meas. Tech., 17, 15–36, https://doi.org/10.5194/amt-17-15-2024, https://doi.org/10.5194/amt-17-15-2024, 2024
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Ammonia is a significant precursor of PM2.5 particles and thus contributes to poor air quality in many regions. Furthermore, ammonia concentrations are rising due to the increase of large-scale, intensive agricultural activities. Here we evaluate satellite measurements of ammonia against aircraft and surface network data, and show that there are differences in magnitude, but the satellite data are spatially and temporally well correlated with the in situ data.
Alana K. Ayasse, Daniel Cusworth, Kelly O'Neill, Justin Fisk, Andrew K. Thorpe, and Riley Duren
Atmos. Meas. Tech., 16, 6065–6074, https://doi.org/10.5194/amt-16-6065-2023, https://doi.org/10.5194/amt-16-6065-2023, 2023
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Methane is a powerful greenhouse gas, and a significant portion of methane comes from large individual plumes. Recently, airplane-mounted infrared technologies have proven very good at detecting and quantifying these plumes. In order to extract the methane signal from the infrared image, there are two widely used approaches. In this study, we assess the performance of both approaches using controlled-release experiments. We also examine the minimum detection limit of the infrared technology.
Apisada Chulakadabba, Maryann Sargent, Thomas Lauvaux, Joshua S. Benmergui, Jonathan E. Franklin, Christopher Chan Miller, Jonas S. Wilzewski, Sébastien Roche, Eamon Conway, Amir H. Souri, Kang Sun, Bingkun Luo, Jacob Hawthrone, Jenna Samra, Bruce C. Daube, Xiong Liu, Kelly Chance, Yang Li, Ritesh Gautam, Mark Omara, Jeff S. Rutherford, Evan D. Sherwin, Adam Brandt, and Steven C. Wofsy
Atmos. Meas. Tech., 16, 5771–5785, https://doi.org/10.5194/amt-16-5771-2023, https://doi.org/10.5194/amt-16-5771-2023, 2023
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We show that MethaneAIR, a precursor to the MethaneSAT satellite, demonstrates accurate point source quantification during controlled release experiments and regional observations in 2021 and 2022. Results from our two independent quantification methods suggest the accuracy of our sensor and algorithms is better than 25 % for sources emitting 200 kg h−1 or more. Insights from these measurements help establish the capabilities of MethaneSAT and MethaneAIR.
Neil Humpage, Hartmut Boesch, William Okello, Jia Chen, Florian Dietrich, Mark F. Lunt, Liang Feng, Paul I. Palmer, and Frank Hase
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-234, https://doi.org/10.5194/amt-2023-234, 2023
Revised manuscript accepted for AMT
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We used a Bruker EM27/SUN spectrometer within an automated weatherproof enclosure to measure greenhouse gas column concentrations over a three-month period in Jinja, Uganda. The portability of the EM27/SUN allows us to evaluate satellite and model data in locations not covered by traditional validation networks. This is of particular value in tropical Africa, where extensive terrestrial ecosystems are a significant store of carbon and play a key role in the atmospheric budgets of CO2 and CH4.
Bart Dils, Minqiang Zhou, Claude Camy-Peyret, Martine De Mazière, Yannick Kangah, Bavo Langerock, Pascal Prunet, Carmine Serio, Richard Siddans, and Brian Kerridge
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-237, https://doi.org/10.5194/amt-2023-237, 2023
Revised manuscript accepted for AMT
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Here we looked at two very distinct methane products from the IASI instrument onboard the MetOp-A satellite. One (referred to as LMD NLISv8.3) uses a machine learning approach while the other (RALv2.0) uses a more conventional optimal estimation approach. We used a variety of model and independent reference measurement data to assess both product’s overall quality, their differences, and specific aspects of each product that would benefit from further analysis by the product development teams.
Kanghyun Baek, Jae Hwan Kim, Juseon Bak, David P. Haffner, Mina Kang, and Hyunkee Hong
Atmos. Meas. Tech., 16, 5461–5478, https://doi.org/10.5194/amt-16-5461-2023, https://doi.org/10.5194/amt-16-5461-2023, 2023
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The GEMS mission was the first mission of the geostationary satellite constellation for hourly atmospheric composition monitoring. The GEMS ozone measurements were cross-compared to those of Pandora, OMPS, and TROPOMI satellite sensors and excellent agreement was found. GEMS has proven to be a powerful new instrument for monitoring and assessing the diurnal variation in atmospheric ozone. This experience can be used to advance research with future geostationary environmental satellite missions.
Tobias Christoph Valentin Werner Riess, Klaas Folkert Boersma, Ward Van Roy, Jos de Laat, Enrico Dammers, and Jasper van Vliet
Atmos. Meas. Tech., 16, 5287–5304, https://doi.org/10.5194/amt-16-5287-2023, https://doi.org/10.5194/amt-16-5287-2023, 2023
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Satellite retrievals of trace gases require prior knowledge of the vertical distribution of the pollutant, which is usually obtained from models. Using aircraft-measured vertical NO2 profiles over the North Sea in summer 2021, we evaluate the Transport Model 5 profiles used in the TROPOMI NO2 retrieval. We conclude that driven by the low horizontal resolution and the overestimated vertical mixing, resulting NO2 columns are 20 % too low. This has important implications for emission estimates.
Thomas Trickl, Martin Adelwart, Dina Khordakova, Ludwig Ries, Christian Rolf, Michael Sprenger, Wolfgang Steinbrecht, and Hannes Vogelmann
Atmos. Meas. Tech., 16, 5145–5165, https://doi.org/10.5194/amt-16-5145-2023, https://doi.org/10.5194/amt-16-5145-2023, 2023
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Tropospheric ozone have been measured for more than a century. Highly quantitative ozone measurements have been made at monitoring stations. However, deficits have been reported for vertical sounding systems. Here, we report a thorough intercomparison effort between a differential-absorption lidar system and two types of balloon-borne ozone sondes, also using ozone sensors at nearby mountain sites as references. The sondes agree very well with the lidar after offset corrections.
Rodriguez Yombo Phaka, Alexis Merlaud, Gaia Pinardi, Martina M. Friedrich, Michel Van Roozendael, Jean-François Müller, Trissevgeni Stavrakou, Isabelle De Smedt, François Hendrick, Ermioni Dimitropoulou, Richard Bopili Mbotia Lepiba, Edmond Phuku Phuati, Buenimio Lomami Djibi, Lars Jacobs, Caroline Fayt, Jean-Pierre Mbungu Tsumbu, and Emmanuel Mahieu
Atmos. Meas. Tech., 16, 5029–5050, https://doi.org/10.5194/amt-16-5029-2023, https://doi.org/10.5194/amt-16-5029-2023, 2023
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We present air quality measurements in Kinshasa, Democratic Republic of the Congo, performed with a newly developed instrument which was installed on a roof of the University of Kinshasa in November 2019. The instrument records spectra of the scattered sunlight, from which we derive the abundances of nitrogen dioxide and formaldehyde, two important pollutants. We compare our ground-based measurements with those of the TROPOspheric Monitoring Instrument (TROPOMI).
Jay Herman, Jerald Ziemke, and Richard McPeters
Atmos. Meas. Tech., 16, 4693–4707, https://doi.org/10.5194/amt-16-4693-2023, https://doi.org/10.5194/amt-16-4693-2023, 2023
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Fourier series multivariate linear regression trends (% per decade) in ozone were estimated from the Merged Ozone Data Set (MOD) from 1979 to 2021 in two different regimes, from 1979 to TA (the date when ozone stopped decreasing) and TA to 2021. The derived TA is a latitude-dependent date, ranging from 1994 to 1998. TA(θ) is a marker for photochemistry dynamics models attempting to represent ozone change over the past 42 years.
Michael Kiefer, Dale F. Hurst, Gabriele P. Stiller, Stefan Lossow, Holger Vömel, John Anderson, Faiza Azam, Jean-Loup Bertaux, Laurent Blanot, Klaus Bramstedt, John P. Burrows, Robert Damadeo, Bianca Maria Dinelli, Patrick Eriksson, Maya García-Comas, John C. Gille, Mark Hervig, Yasuko Kasai, Farahnaz Khosrawi, Donal Murtagh, Gerald E. Nedoluha, Stefan Noël, Piera Raspollini, William G. Read, Karen H. Rosenlof, Alexei Rozanov, Christopher E. Sioris, Takafumi Sugita, Thomas von Clarmann, Kaley A. Walker, and Katja Weigel
Atmos. Meas. Tech., 16, 4589–4642, https://doi.org/10.5194/amt-16-4589-2023, https://doi.org/10.5194/amt-16-4589-2023, 2023
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We quantify biases and drifts (and their uncertainties) between the stratospheric water vapor measurement records of 15 satellite-based instruments (SATs, with 31 different retrievals) and balloon-borne frost point hygrometers (FPs) launched at 27 globally distributed stations. These comparisons of measurements during the period 2000–2016 are made using robust, consistent statistical methods. With some exceptions, the biases and drifts determined for most SAT–FP pairs are < 10 % and < 1 % yr−1.
Tim A. van Kempen, Tim J. Rotmans, Richard M. van Hees, Carol Bruegge, Dejian Fu, Ruud Hoogeveen, Thomas J. Pongetti, Robert Rosenberg, and Ilse Aben
Atmos. Meas. Tech., 16, 4507–4527, https://doi.org/10.5194/amt-16-4507-2023, https://doi.org/10.5194/amt-16-4507-2023, 2023
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Validation of satellite measurements is essential for providing reliable and consistent products. In this paper, a validation method for TROPOMI-SWIR (Tropospheric Measurement Instrument in the short-wavelength infrared) is explored. TROPOMI-SWIR has been shown to be exceptionally stable, a necessity to explore the methodology. Railroad Valley, Nevada, is a prime location to perform the necessary measurements to validate the satellite measurements of TROPOMI-SWIR.
Serin Kim, Daewon Kim, Hyunkee Hong, Lim-Seok Chang, Hanlim Lee, Deok-Rae Kim, Donghee Kim, Jeong-Ah Yu, Dongwon Lee, Ukkyo Jeong, Chang-Kuen Song, Sang-Woo Kim, Sang Seo Park, Jhoon Kim, Thomas F. Hanisco, Junsung Park, Wonei Choi, and Kwangyul Lee
Atmos. Meas. Tech., 16, 3959–3972, https://doi.org/10.5194/amt-16-3959-2023, https://doi.org/10.5194/amt-16-3959-2023, 2023
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A first evaluation of the Geostationary Environmental Monitoring Spectrometer (GEMS) NO2 was carried out via comparison with the NO2 data obtained from the ground-based Pandora direct-sun measurements at four sites in Seosan, Republic of Korea. Comparisons between GEMS NO2 and Pandora NO2 were performed according to GEMS cloud fraction. GEMS NO2 showed good agreement with that of Pandora NO2 under less cloudy conditions.
Nicholas Balasus, Daniel J. Jacob, Alba Lorente, Joannes D. Maasakkers, Robert J. Parker, Hartmut Boesch, Zichong Chen, Makoto M. Kelp, Hannah Nesser, and Daniel J. Varon
Atmos. Meas. Tech., 16, 3787–3807, https://doi.org/10.5194/amt-16-3787-2023, https://doi.org/10.5194/amt-16-3787-2023, 2023
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We use machine learning to remove biases in TROPOMI satellite observations of atmospheric methane, with GOSAT observations serving as a reference. We find that the TROPOMI biases relative to GOSAT are related to the presence of aerosols and clouds, the surface brightness, and the specific detector that makes the observation aboard TROPOMI. The resulting blended TROPOMI+GOSAT product is more reliable for quantifying methane emissions.
Thomas E. Taylor, Christopher W. O'Dell, David Baker, Carol Bruegge, Albert Chang, Lars Chapsky, Abhishek Chatterjee, Cecilia Cheng, Frédéric Chevallier, David Crisp, Lan Dang, Brian Drouin, Annmarie Eldering, Liang Feng, Brendan Fisher, Dejian Fu, Michael Gunson, Vance Haemmerle, Graziela R. Keller, Matthäus Kiel, Le Kuai, Thomas Kurosu, Alyn Lambert, Joshua Laughner, Richard Lee, Junjie Liu, Lucas Mandrake, Yuliya Marchetti, Gregory McGarragh, Aronne Merrelli, Robert R. Nelson, Greg Osterman, Fabiano Oyafuso, Paul I. Palmer, Vivienne H. Payne, Robert Rosenberg, Peter Somkuti, Gary Spiers, Cathy To, Brad Weir, Paul O. Wennberg, Shanshan Yu, and Jia Zong
Atmos. Meas. Tech., 16, 3173–3209, https://doi.org/10.5194/amt-16-3173-2023, https://doi.org/10.5194/amt-16-3173-2023, 2023
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NASA's Orbiting Carbon Observatory 2 and 3 (OCO-2 and OCO-3, respectively) provide complementary spatiotemporal coverage from a sun-synchronous and precession orbit, respectively. Estimates of total column carbon dioxide (XCO2) derived from the two sensors using the same retrieval algorithm show broad consistency over a 2.5-year overlapping time record. This suggests that data from the two satellites may be used together for scientific analysis.
Lena Katharina Jänicke, Rene Preusker, Marco Celesti, Marin Tudoroiu, Jürgen Fischer, Dirk Schüttemeyer, and Matthias Drusch
Atmos. Meas. Tech., 16, 3101–3121, https://doi.org/10.5194/amt-16-3101-2023, https://doi.org/10.5194/amt-16-3101-2023, 2023
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To compare two top-of-atmosphere radiances measured by instruments with different spectral characteristics, a transfer function has been developed. It is applied to a tandem data set of Sentinel-3A and B, for which OLCI-B mimicked the ESA’s eighth Earth Explorer FLEX. We found that OLCI-A measured radiances about 2 % brighter than OLCI-FLEX. Only at larger wavelengths were OLCI-A measurements about 5 % darker. The method is thus successful, being sensitive to calibration and processing issues.
Luis F. Millán, Gloria L. Manney, Harald Boenisch, Michaela I. Hegglin, Peter Hoor, Daniel Kunkel, Thierry Leblanc, Irina Petropavlovskikh, Kaley Walker, Krzysztof Wargan, and Andreas Zahn
Atmos. Meas. Tech., 16, 2957–2988, https://doi.org/10.5194/amt-16-2957-2023, https://doi.org/10.5194/amt-16-2957-2023, 2023
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The determination of atmospheric composition trends in the upper troposphere and lower stratosphere (UTLS) is still highly uncertain. We present the creation of dynamical diagnostics to map several ozone datasets (ozonesondes, lidars, aircraft, and satellite measurements) in geophysically based coordinate systems. The diagnostics can also be used to analyze other greenhouse gases relevant to surface climate and UTLS chemistry.
Zhihua Zhang, Jianguo Niu, Lawrence E. Flynn, Eric Beach, and Trevor Beck
Atmos. Meas. Tech., 16, 2919–2941, https://doi.org/10.5194/amt-16-2919-2023, https://doi.org/10.5194/amt-16-2919-2023, 2023
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This study mainly focused on addressing stability and improvement when using a broadband approach, establishing soft-calibration adjustments for both OMPS S-NPP and N20, analyzing error biases based on multi-sensor bias correction, and comparing total column ozone and aerosol index retrievals from NOAA OMPS with those from other products.
Matthew S. Johnson, Amir H. Souri, Sajeev Philip, Rajesh Kumar, Aaron Naeger, Jeffrey Geddes, Laura Judd, Scott Janz, Heesung Chong, and John Sullivan
Atmos. Meas. Tech., 16, 2431–2454, https://doi.org/10.5194/amt-16-2431-2023, https://doi.org/10.5194/amt-16-2431-2023, 2023
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Satellites provide vital information for studying the processes controlling ozone formation. Based on the abundance of particular gases in the atmosphere, ozone formation is sensitive to specific human-induced and natural emission sources. However, errors and biases in satellite retrievals hinder this data source’s application for studying ozone formation sensitivity. We conducted a thorough statistical evaluation of two commonly applied satellites for investigating ozone formation sensitivity.
Kezia Lange, Andreas Richter, Anja Schönhardt, Andreas C. Meier, Tim Bösch, André Seyler, Kai Krause, Lisa K. Behrens, Folkard Wittrock, Alexis Merlaud, Frederik Tack, Caroline Fayt, Martina M. Friedrich, Ermioni Dimitropoulou, Michel Van Roozendael, Vinod Kumar, Sebastian Donner, Steffen Dörner, Bianca Lauster, Maria Razi, Christian Borger, Katharina Uhlmannsiek, Thomas Wagner, Thomas Ruhtz, Henk Eskes, Birger Bohn, Daniel Santana Diaz, Nader Abuhassan, Dirk Schüttemeyer, and John P. Burrows
Atmos. Meas. Tech., 16, 1357–1389, https://doi.org/10.5194/amt-16-1357-2023, https://doi.org/10.5194/amt-16-1357-2023, 2023
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We present airborne imaging DOAS and ground-based stationary and car DOAS measurements conducted during the S5P-VAL-DE-Ruhr campaign in the Rhine-Ruhr region. The measurements are used to validate spaceborne NO2 data products from the Sentinel-5 Precursor TROPOspheric Monitoring Instrument (TROPOMI). Auxiliary data of the TROPOMI NO2 retrieval, such as spatially higher resolved a priori NO2 vertical profiles, surface reflectivity, and cloud treatment are investigated to evaluate their impact.
Yolanda Maria Lemes, Christoph Häni, Jesper Nørlem Kamp, and Anders Feilberg
Atmos. Meas. Tech., 16, 1295–1309, https://doi.org/10.5194/amt-16-1295-2023, https://doi.org/10.5194/amt-16-1295-2023, 2023
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The implementation of a new method, line-averaged concentration measurement with a closed-path analyzer, will enable the measurement of fluxes of multiple gases from different types of sources and will evaluate the effects of mitigation strategies on emissions. In addition, this method allows for continuous online measurements that resolve temporal variation in ammonia emissions and the peak emissions of methane.
Prajjwal Rawat, Manish Naja, Evan Fishbein, Pradeep K. Thapliyal, Rajesh Kumar, Piyush Bhardwaj, Aditya Jaiswal, Sugriva N. Tiwari, Sethuraman Venkataramani, and Shyam Lal
Atmos. Meas. Tech., 16, 889–909, https://doi.org/10.5194/amt-16-889-2023, https://doi.org/10.5194/amt-16-889-2023, 2023
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Satellite-based ozone observations have gained importance due to their global coverage. However, satellite-retrieved products are indirect and need to be validated, particularly over mountains. Ozonesondes launched from a Himalayan site are used to assess the Atmospheric Infrared Sounder (AIRS) ozone retrieval. AIRS is shown to overestimate ozone in the upper troposphere and lower stratosphere, while the differences from ozonesondes are more minor in the middle troposphere and stratosphere.
Murali Natarajan, Robert Damadeo, and David Flittner
Atmos. Meas. Tech., 16, 75–87, https://doi.org/10.5194/amt-16-75-2023, https://doi.org/10.5194/amt-16-75-2023, 2023
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Photochemically induced changes in mesospheric O3 concentration at twilight can cause asymmetry in the distribution along the line of sight of solar occultation observations that must be considered in the retrieval algorithm. Correction factors developed from diurnal photochemical model simulations were used to modify the archived SAGE III/ISS mesospheric O3 concentrations. For June 2021 the bias caused by the neglect of diurnal variations is over 30% at 64 km altitude and low latitudes.
Javier Gorroño, Daniel J. Varon, Itziar Irakulis-Loitxate, and Luis Guanter
Atmos. Meas. Tech., 16, 89–107, https://doi.org/10.5194/amt-16-89-2023, https://doi.org/10.5194/amt-16-89-2023, 2023
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We present a methane flux rate retrieval methodology using the Sentinel-2 mission, validating the algorithm for different scenes and plumes. The detection limit is 1000–2000 kg h−1 for homogeneous scenes and temporally invariant surfaces and above 5000 kg h−1 for heterogeneous ones. Dominant quantification errors are wind-related or plume mask-related. For heterogeneous scenes, the surface structure underlying the methane plume can become a dominant source of uncertainty.
Katerina Garane, Ka Lok Chan, Maria-Elissavet Koukouli, Diego Loyola, and Dimitris Balis
Atmos. Meas. Tech., 16, 57–74, https://doi.org/10.5194/amt-16-57-2023, https://doi.org/10.5194/amt-16-57-2023, 2023
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In this work, 2.5 years of TROPOMI/S5P Total Column Water Vapor (TCWV) observations retrieved from the blue wavelength band are validated against co-located precipitable water measurements from NASA AERONET, which uses Cimel Sun photometers globally. Overall, the TCWV product agrees well on a global scale with the ground-based dataset (Pearson correl. coefficient 0.909) and has a mean relative bias of −2.7 ± 4.9 % with respect to the AERONET observations for moderate albedo and cloudiness.
Lei Shi, Carl J. Schreck III, Viju O. John, Eui-Seok Chung, Theresa Lang, Stefan A. Buehler, and Brian J. Soden
Atmos. Meas. Tech., 15, 6949–6963, https://doi.org/10.5194/amt-15-6949-2022, https://doi.org/10.5194/amt-15-6949-2022, 2022
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Four upper tropospheric humidity (UTH) datasets derived from satellite microwave and infrared sounders are evaluated to assess their consistency as part of the activities for the Global Energy and Water Exchanges (GEWEX) water vapor assessment project. The study shows that the four datasets are consistent in the interannual temporal and spatial variability of the tropics. However, differences are found in the magnitudes of the anomalies and in the changing rates during the common period.
Ali Jalali, Kaley A. Walker, Kimberly Strong, Rebecca R. Buchholz, Merritt N. Deeter, Debra Wunch, Sébastien Roche, Tyler Wizenberg, Erik Lutsch, Erin McGee, Helen M. Worden, Pierre Fogal, and James R. Drummond
Atmos. Meas. Tech., 15, 6837–6863, https://doi.org/10.5194/amt-15-6837-2022, https://doi.org/10.5194/amt-15-6837-2022, 2022
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This study validates MOPITT version 8 carbon monoxide measurements over the Canadian high Arctic for the period 2006 to 2019. The MOPITT products from different detector pixels and channels are compared with ground-based measurements from the Polar Environment Atmospheric Research Laboratory (PEARL) in Eureka, Nunavut, Canada. These results show good consistency between the satellite and ground-based measurements and provide guidance on the usage of these MOPITT data at high latitudes.
Gerald Wetzel, Michael Höpfner, Hermann Oelhaf, Felix Friedl-Vallon, Anne Kleinert, Guido Maucher, Miriam Sinnhuber, Janna Abalichin, Angelika Dehn, and Piera Raspollini
Atmos. Meas. Tech., 15, 6669–6704, https://doi.org/10.5194/amt-15-6669-2022, https://doi.org/10.5194/amt-15-6669-2022, 2022
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Satellite measurements of stratospheric trace gases are essential for monitoring distributions and trends of these species on a global scale. Here, we compare the final MIPAS ESA Level 2 version 8 data (temperature and trace gases) with measurements obtained with the balloon version of MIPAS in terms of data agreement of both sensors, including combined errors. For most gases, we find a 5 % to 20 % agreement of the retrieved vertical profiles of both MIPAS instruments in the lower stratosphere.
Maximilian Rißmann, Jia Chen, Gregory Osterman, Xinxu Zhao, Florian Dietrich, Moritz Makowski, Frank Hase, and Matthäus Kiel
Atmos. Meas. Tech., 15, 6605–6623, https://doi.org/10.5194/amt-15-6605-2022, https://doi.org/10.5194/amt-15-6605-2022, 2022
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The Orbiting Carbon Observatory 2 (OCO-2) measures atmospheric concentrations of the most potent greenhouse gas, CO2, globally. By comparing its measurements to a ground-based monitoring network in Munich (MUCCnet), we find that the satellite is able to reliably detect urban CO2 concentrations. Furthermore, spatial CO2 differences captured by OCO-2 and MUCCnet are strongly correlated, which indicates that OCO-2 could be helpful in determining urban CO2 emissions from space.
Sarah A. Strode, Ghassan Taha, Luke D. Oman, Robert Damadeo, David Flittner, Mark Schoeberl, Christopher E. Sioris, and Ryan Stauffer
Atmos. Meas. Tech., 15, 6145–6161, https://doi.org/10.5194/amt-15-6145-2022, https://doi.org/10.5194/amt-15-6145-2022, 2022
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We use a global atmospheric chemistry model simulation to generate scaling factors that account for the daily cycle of NO2 and ozone. These factors facilitate comparisons between sunrise and sunset observations from SAGE III/ISS and observations from other instruments. We provide the scaling factors as monthly zonal means for different latitudes and altitudes. We find that applying these factors yields more consistent comparisons between observations from SAGE III/ISS and other instruments.
Kimberlee Dubé, Daniel Zawada, Adam Bourassa, Doug Degenstein, William Randel, David Flittner, Patrick Sheese, and Kaley Walker
Atmos. Meas. Tech., 15, 6163–6180, https://doi.org/10.5194/amt-15-6163-2022, https://doi.org/10.5194/amt-15-6163-2022, 2022
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Satellite observations are important for monitoring changes in atmospheric composition. Here we describe an improved version of the NO2 retrieval for the Optical Spectrograph and InfraRed Imager System. The resulting NO2 profiles are compared to those from the Atmospheric Chemistry Experiment – Fourier Transform Spectrometer and the Stratospheric Aerosol and Gas Experiment III on the International Space Station. All datasets agree within 20 % throughout the stratosphere.
Edward Malina, Kevin W. Bowman, Valentin Kantchev, Le Kuai, Thomas P. Kurosu, Kazuyuki Miyazaki, Vijay Natraj, Gregory B. Osterman, and Matthew D. Thill
EGUsphere, https://doi.org/10.5194/egusphere-2022-774, https://doi.org/10.5194/egusphere-2022-774, 2022
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Characterising the distribution of ozone in the atmosphere is a challenging problem, with current Earth Observation satellites using either Thermal Infrared (TIR) or Ultra Violet (UV) instruments, sensitive to different portions of the atmosphere, making it difficult to gain a full picture. In this work, we combine measurements from the TIR and UV instruments Suomi NPP CrIS and Sentinel 5P/TROPOMI, to improve sensitivity through the whole atmosphere, and improve knowledge of ozone distribution.
Helen M. Worden, Gene L. Francis, Susan S. Kulawik, Kevin W. Bowman, Karen Cady-Pereira, Dejian Fu, Jennifer D. Hegarty, Valentin Kantchev, Ming Luo, Vivienne H. Payne, John R. Worden, Róisín Commane, and Kathryn McKain
Atmos. Meas. Tech., 15, 5383–5398, https://doi.org/10.5194/amt-15-5383-2022, https://doi.org/10.5194/amt-15-5383-2022, 2022
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Satellite observations of global carbon monoxide (CO) are essential for understanding atmospheric chemistry and pollution sources. This paper describes a new data product using radiance measurements from the Cross-track Infrared Sounder (CrIS) instrument on the Suomi National Polar-orbiting Partnership (SNPP) satellite that provides vertical profiles of CO from single-field-of-view observations. We show how these satellite CO profiles compare to aircraft observations and evaluate their biases.
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Short summary
We validated two BTS-based systems in a longer-term TOC analysis in the 2019/2020 campaign at Hohenpeißenberg and Davos. The results showed a deviation of the BTS-Solar to Brewers of < 0.1 % with a k = 2 of < 1.5 %. Koherent showed a deviation of 1.7 % with a k = 2 of 2.7 %. Resultingly, the BTS-Solar performance is comparable to Brewers in Hohenpeißenberg. Koherent shows a seasonal variation in Davos due to the sensitivity of its TOC retrieval algorithm to stratospheric temperature.
We validated two BTS-based systems in a longer-term TOC analysis in the 2019/2020 campaign at...
