Articles | Volume 11, issue 4
https://doi.org/10.5194/amt-11-2239-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-11-2239-2018
© Author(s) 2018. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
MAX-DOAS NO2 observations over Guangzhou, China; ground-based and satellite comparisons
Theano Drosoglou
CORRESPONDING AUTHOR
Laboratory of Atmospheric Physics, Aristotle University of
Thessaloniki, Thessaloniki, Greece
Maria Elissavet Koukouli
Laboratory of Atmospheric Physics, Aristotle University of
Thessaloniki, Thessaloniki, Greece
Natalia Kouremeti
Physikalisch-Meteorologisches Observatorium Davos, World Radiation
Center, Davos, Switzerland
Alkiviadis F. Bais
Laboratory of Atmospheric Physics, Aristotle University of
Thessaloniki, Thessaloniki, Greece
Irene Zyrichidou
Laboratory of Atmospheric Physics, Aristotle University of
Thessaloniki, Thessaloniki, Greece
Dimitris Balis
Laboratory of Atmospheric Physics, Aristotle University of
Thessaloniki, Thessaloniki, Greece
Ronald J. van der A
R&D Satellite Observations, Royal Netherlands Meteorological Institute (KNMI), De Bilt, the Netherlands
School of Atmospheric Physics, Nanjing University of Information Sciences and Technology, Nanjing, China
Jin Xu
Anhui Institute of Optics and Fine Mechanics Academy of Sciences
(AIOFM), Chinese Academy of Sciences (CAS), Hefei, China
Ang Li
Anhui Institute of Optics and Fine Mechanics Academy of Sciences
(AIOFM), Chinese Academy of Sciences (CAS), Hefei, China
Related authors
Theano Drosoglou, Ioannis-Panagiotis Raptis, Massimo Valeri, Stefano Casadio, Francesca Barnaba, Marcos Herreras-Giralda, Anton Lopatin, Oleg Dubovik, Gabriele Brizzi, Fabrizio Niro, Monica Campanelli, and Stelios Kazadzis
Atmos. Meas. Tech., 16, 2989–3014, https://doi.org/10.5194/amt-16-2989-2023, https://doi.org/10.5194/amt-16-2989-2023, 2023
Short summary
Short summary
Aerosol optical properties derived from sun photometers depend on the optical depth of trace gases absorbing solar radiation at specific spectral ranges. Various networks use satellite-based climatologies to account for this or neglect their effect. In this work, we evaluate the effect of NO2 absorption in aerosol retrievals from AERONET and SKYNET over two stations in Rome, Italy, with relatively high NO2 spatiotemporal variations, using NO2 data from the Pandora network and the TROPOMI sensor.
Dimitris Karagkiozidis, Alkiviadis Bais, Katerina Garane, Michel Van Roozendael, Dimitris Nikolis, Manuel Roca, and Dimitris Balis
EGUsphere, https://doi.org/10.5194/egusphere-2025-5627, https://doi.org/10.5194/egusphere-2025-5627, 2026
This preprint is open for discussion and under review for Atmospheric Measurement Techniques (AMT).
Short summary
Short summary
In this study, we measured the total ozone in the atmosphere over Thessaloniki, Greece, using remote-sensing techniques. Our approach, applied in both ultraviolet and visible regions, produced results highly consistent with reference instruments. It consistently captured daily and seasonal ozone patterns across both spectral regions under varying atmospheric conditions. This research enhances ground-based ozone monitoring and supports long-term observations and satellite validation.
Christos Spyrou, Ilias Fountoulakis, Stavros Solomos, Nikolaos Papadimitriou, Alkiviadis Bais, Julian Gröbner, Daniela Meloni, and Christos Zerefos
Atmos. Meas. Tech., 18, 7717–7734, https://doi.org/10.5194/amt-18-7717-2025, https://doi.org/10.5194/amt-18-7717-2025, 2025
Short summary
Short summary
Dust particles originating from desert areas of the planet have significant radiative impacts on the ground and atmospheric column. The magnitude of the dust radiative effect is dependent on their optical properties and mineralogical content. Therefore, we upgrade the METAL-WRF model to incorporate the direct radiative impact of the minerals in dust. The capabilities of the model to simulate the chemical composition and associated impacts is significantly improved.
Angelos Karanikolas, Benjamin Torres, Masahiro Momoi, Marcos Herreras Giralda, Natalia Kouremeti, Julian Gröbner, Lionel Doppler, and Stelios Kazadzis
Atmos. Meas. Tech., 18, 7651–7677, https://doi.org/10.5194/amt-18-7651-2025, https://doi.org/10.5194/amt-18-7651-2025, 2025
Short summary
Short summary
Several techniques retrieve of the aerosol size distribution. The Generalized Retrieval of Atmosphere and Surface Properties algorithm can retrieve aerosol size distribution parameters using only aerosol optical depth (AOD) as input that is continuously observed by sun photometers worldwide. In this study, we apply the algorithm to AOD measured by sun photometers and spectroradiometers to assess the performance and limitations of such retrievals and investigate the effect of the spectral range.
Anna Maria Neroladaki, Maria Tsagkaraki, Kyriaki Papoutsidaki, Kalliopi Tavernaraki, Filothei Boufidou, Pavlos Zarmpas, Irini Tsiodra, Eleni Liakakou, Aikaterini Bougiatioti, Giorgos Kouvarakis, Nikos Kalivitis, Christos Kaltsonoudis, Athanasios Karagioras, Dimitrios Balis, Konstantinos Michailidis, Konstantinos Kourtidis, Stelios Myriokefalitakis, Nikos Hatzianastassiou, Spyros N. Pandis, Athanasios Nenes, Nikolaos Mihalopoulos, and Maria Kanakidou
Atmos. Chem. Phys., 25, 17953–17971, https://doi.org/10.5194/acp-25-17953-2025, https://doi.org/10.5194/acp-25-17953-2025, 2025
Short summary
Short summary
Aerosol acidity affects aerosol composition and properties, and therefore climate, human health and ecosystems. We use summer and winter fine aerosol observations at 6 sites across Greece, and a thermodynamic model to calculate the spatial and seasonal variability of aerosol acidity. Aerosols were acidic to moderately acidic and more acidic during summer than winter. The importance of organics for aerosol acidity was small. Depending on location different factors controlled aerosol acidity.
Hannes Witt, Ronald J. van der A, Jieying Ding, Jeroen Kuenen, and Margreet C. van Zanten
EGUsphere, https://doi.org/10.5194/egusphere-2025-6036, https://doi.org/10.5194/egusphere-2025-6036, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
Short summary
Short summary
We present a detailed comparison of NOx emissions from the Dutch national emission inventory with completely independent emission data derived from satellite observations with the DECSO algorithm. We find good agreement in overall emission levels, regional emissions, and the 5-year emission trend. Our results demonstrate the robustness of the national inventory and the satellite-derived emissions and might serve as a use-case for the adoption of similar methods in other countries.
Ilias Fountoulakis, Kyriaki Papachristopoulou, Stelios Kazadzis, Gregor Hülsen, Julian Gröbner, Ioannis-Panagiotis Raptis, Dimitra Kouklaki, Akriti Masoom, Natalia Kouremeti, Charalampos Kontoes, and Christos S. Zerefos
Geosci. Model Dev., 18, 7451–7473, https://doi.org/10.5194/gmd-18-7451-2025, https://doi.org/10.5194/gmd-18-7451-2025, 2025
Short summary
Short summary
The UVIOS2 model has been evaluated at Davos, Switzerland during the UVCIII campaign. The accuracy in the modelled UV indices has been assessed for different combinations of model inputs. A good overall agreement between UVIOS2 and the world reference spectroradiometer QASUME was found (average ratio of ~ 1 between the modelled and measured UV index), although the variability in the ratio can be large under cloudy conditions.
Yutao Chen, Ronald J. van der A, Jieying Ding, Henk Eskes, Felipe Cifuentes, and Pieternel F. Levelt
EGUsphere, https://doi.org/10.5194/egusphere-2025-4490, https://doi.org/10.5194/egusphere-2025-4490, 2025
Short summary
Short summary
The SO2 gridded point emissions calculated from satellite measurements appear spread out around the source. This is inherent to the inversion method and the resolution of the satellite measurements. We made a new deconvolution algorithm to reverse the spreading and make the emission signal clearer. With this method, the effective resolution is improved. Known sources can be located more precisely, and new ones can be found from space. The same approach also works for other gases like NOx.
Sara Herrero-Anta, Sabine Eckhardt, Nikolaos Evangeliou, Stefania Gilardoni, Sandra Graßl, Dominic Heslin-Rees, Stelios Kazadzis, Natalia Kouremeti, Radovan Krejci, David Mateos, Mauro Mazzola, Christoph Ritter, Roberto Román, Kerstin Stebel, and Tymon Zielinski
EGUsphere, https://doi.org/10.5194/egusphere-2025-3423, https://doi.org/10.5194/egusphere-2025-3423, 2025
Short summary
Short summary
In summer 2019, unusually high aerosol levels were measured in the Arctic, linked to wildfires, volcanic eruptions, and anthropogenic pollution. Using various instruments and models, we traced their origins and found good agreement between methods. The particles were mostly non-absorbing, but still we found a reduction of the solar radiation reaching the surface. This study shows that combining different measurements improves our understanding of how distant events affect the Arctic climate.
Simone Pulimeno, Angelo Lupi, Vito Vitale, Claudia Frangipani, Carlos Toledano, Stelios Kazadzis, Natalia Kouremeti, Christoph Ritter, Sandra Graßl, Kerstin Stebel, Vitali Fioletov, Ihab Abboud, Sandra Blindheim, Lynn Ma, Norm O’Neill, Piotr Sobolewski, Pawan Gupta, Elena Lind, Thomas F. Eck, Antti Hyvärinen, Veijo Aaltonen, Rigel Kivi, Janae Csavina, Dmitry Kabanov, Sergey M. Sakerin, Olga R. Sidorova, Robert S. Stone, Hagen Telg, Laura Riihimaki, Raul R. Cordero, Martin Radenz, Ronny Engelmann, Michel Van Roozendal, Anatoli Chaikovsky, Philippe Goloub, Junji Hisamitsu, and Mauro Mazzola
EGUsphere, https://doi.org/10.5194/egusphere-2025-2527, https://doi.org/10.5194/egusphere-2025-2527, 2025
Short summary
Short summary
This study analyzed aerosols optical properties over the Arctic and Antarctic to measure them even during long periods of darkness. It found that pollution in the Arctic is decreasing, likely due to European emission regulations, while wildfires are becoming a more important source of particles. In Antarctica, particle levels are higher near the coast than inland, and vary by season. These results help us better understand how air pollution and climate are changing at the Earth’s poles.
Akriti Masoom, Stelios Kazadzis, Robin Lewis Modini, Martin Gysel-Beer, Julian Gröbner, Martine Collaud Coen, Francisco Navas-Guzman, Natalia Kouremeti, Benjamin Tobias Brem, Nora Kristina Nowak, Giovanni Martucci, Maxime Hervo, and Sophie Erb
EGUsphere, https://doi.org/10.5194/egusphere-2025-2755, https://doi.org/10.5194/egusphere-2025-2755, 2025
Short summary
Short summary
This article aims at providing details on the special aerosol properties observed during 2023 Canadian wildfire plume transport and exploring the synergism between remote sensing and in situ measurements for investigating the cause of the occurrence of the observations of special aerosol properties.
Roberto Román, Daniel González-Fernández, Juan Carlos Antuña-Sánchez, Celia Herrero del Barrio, Sara Herrero-Anta, África Barreto, Victoria E. Cachorro, Lionel Doppler, Ramiro González, Christoph Ritter, David Mateos, Natalia Kouremeti, Gustavo Copes, Abel Calle, María José Granados-Muñoz, Carlos Toledano, and Ángel M. de Frutos
Atmos. Meas. Tech., 18, 2847–2875, https://doi.org/10.5194/amt-18-2847-2025, https://doi.org/10.5194/amt-18-2847-2025, 2025
Short summary
Short summary
This paper presents a novel technique to extract starlight signals from all-sky images and retrieve aerosol optical depth (AOD). It is validated against lunar photometry, showing a strong correlation between data series. This innovative approach will expand nocturnal AOD measurements to more locations, as all-sky cameras are a simpler and more cost-effective alternative to stellar and lunar photometers.
Lena Feld, Pablo Schmid, Marios Mermigkas, Dimitrios Balis, Jochen Gross, Darko Dubravica, Carlos Alberti, Benedikt Herkommer, Stefan Versick, Roland Ruhnke, Frank Hase, and Peter Braesicke
EGUsphere, https://doi.org/10.5194/egusphere-2025-639, https://doi.org/10.5194/egusphere-2025-639, 2025
Short summary
Short summary
Our goal is to measure CO2 emissions from cities, to verify and improve our knowledge of reported anthropogenic emissions. We use atmospheric measurements and simulations of CO2 transport to find an independent estimate. This study investigates the CO2 emissions of the city of Thessaloniki, where the reported emissions differ. The data we collected indicates that the emissions are larger than stated by the ODIAC inventory, which we used for our simulations.
Jiangman Xu, Ang Li, Zhaokun Hu, Hairong Zhang, and Min Qin
Atmos. Meas. Tech., 18, 865–879, https://doi.org/10.5194/amt-18-865-2025, https://doi.org/10.5194/amt-18-865-2025, 2025
Short summary
Short summary
This article introduces an experimental system for rapidly acquiring trace gas profiles using multi-channel spectroscopy, significantly enhancing the time resolution of spectral collection. The fast synchronous multi-axis differential optical absorption spectroscopy (FS MAX-DOAS) successfully obtains gas profiles. This work can also be integrated with mobile platforms for navigational observation research, which is crucial for making mobile MAX-DOAS profile measurements.
Yutao Chen, Ronald J. van der A, Jieying Ding, Henk Eskes, Jason E. Williams, Nicolas Theys, Athanasios Tsikerdekis, and Pieternel F. Levelt
Atmos. Chem. Phys., 25, 1851–1868, https://doi.org/10.5194/acp-25-1851-2025, https://doi.org/10.5194/acp-25-1851-2025, 2025
Short summary
Short summary
There is a lack of local SO2 top-down emission inventories in India. With the improvement in the divergence method and the derivation of SO2 local lifetime, gridded SO2 emissions over a large area can be estimated efficiently. This method can be applied to any region in the world to derive SO2 emissions. Especially for regions with high latitudes, our methodology has the potential to significantly improve the top-down derivation of SO2 emissions.
Angelos Karanikolas, Natalia Kouremeti, Monica Campanelli, Victor Estellés, Masahiro Momoi, Gaurav Kumar, Stephan Nyeki, and Stelios Kazadzis
Atmos. Meas. Tech., 17, 6085–6105, https://doi.org/10.5194/amt-17-6085-2024, https://doi.org/10.5194/amt-17-6085-2024, 2024
Short summary
Short summary
Different sun photometer networks use different instruments, post-processing algorithms and calibration protocols for aerosol optical depth (AOD) retrieval. Such differences can affect the homogeneity and comparability of their measurements. In this study, we assess the homogeneity between the sun photometer networks GAW-PFR and SKYNET, analysing common measurements during three campaigns between 2017–2021, and investigate the main cause of the differences.
Jieying Ding, Ronald van der A, Henk Eskes, Enrico Dammers, Mark Shephard, Roy Wichink Kruit, Marc Guevara, and Leonor Tarrason
Atmos. Chem. Phys., 24, 10583–10599, https://doi.org/10.5194/acp-24-10583-2024, https://doi.org/10.5194/acp-24-10583-2024, 2024
Short summary
Short summary
Here we applied the existing Daily Emissions Constrained by Satellite Observations (DECSO) inversion algorithm to NH3 observations from the CrIS satellite instrument to estimate NH3 emissions. As NH3 in the atmosphere is influenced by NOx, we implemented DECSO to estimate NOx and NH3 emissions simultaneously. The emissions are derived over Europe for 2020 at a spatial resolution of 0.2° using daily observations from CrIS and TROPOMI. Results are compared to bottom-up emission inventories.
Mengyao Liu, Ronald van der A, Michiel van Weele, Lotte Bryan, Henk Eskes, Pepijn Veefkind, Yongxue Liu, Xiaojuan Lin, Jos de Laat, and Jieying Ding
Atmos. Meas. Tech., 17, 5261–5277, https://doi.org/10.5194/amt-17-5261-2024, https://doi.org/10.5194/amt-17-5261-2024, 2024
Short summary
Short summary
A new divergence method was developed and applied to estimate methane emissions from TROPOMI observations over the Middle East, where it is typically challenging for a satellite to measure methane due to its complicated orography and surface albedo. Our results show the potential of TROPOMI to quantify methane emissions from various sources rather than big emitters from space after objectively excluding the artifacts in the retrieval.
Monica Campanelli, Victor Estellés, Gaurav Kumar, Teruyuki Nakajima, Masahiro Momoi, Julian Gröbner, Stelios Kazadzis, Natalia Kouremeti, Angelos Karanikolas, Africa Barreto, Saulius Nevas, Kerstin Schwind, Philipp Schneider, Iiro Harju, Petri Kärhä, Henri Diémoz, Rei Kudo, Akihiro Uchiyama, Akihiro Yamazaki, Anna Maria Iannarelli, Gabriele Mevi, Annalisa Di Bernardino, and Stefano Casadio
Atmos. Meas. Tech., 17, 5029–5050, https://doi.org/10.5194/amt-17-5029-2024, https://doi.org/10.5194/amt-17-5029-2024, 2024
Short summary
Short summary
To retrieve columnar aerosol properties from sun photometers, some calibration factors are needed. The on-site calibrations, performed as frequently as possible to monitor changes in the machine conditions, allow operators to track and evaluate the calibration status on a continuous basis, reducing the data gaps incurred by the periodic shipments for performing centralized calibrations. The performance of the on-site calibration procedures was evaluated, providing very good results.
Ronald J. van der A, Jieying Ding, and Henk Eskes
Atmos. Chem. Phys., 24, 7523–7534, https://doi.org/10.5194/acp-24-7523-2024, https://doi.org/10.5194/acp-24-7523-2024, 2024
Short summary
Short summary
Using observations of the Sentinel-5P satellite and the latest version of the inversion algorithm DECSO, anthropogenic NOx emissions are derived for Europe for the years 2019–2022 with a spatial resolution of 0.2°. The results are compared with European emissions of the Copernicus Atmosphere Monitoring Service.
Adrianus de Laat, Jos van Geffen, Piet Stammes, Ronald van der A, Henk Eskes, and J. Pepijn Veefkind
Atmos. Chem. Phys., 24, 4511–4535, https://doi.org/10.5194/acp-24-4511-2024, https://doi.org/10.5194/acp-24-4511-2024, 2024
Short summary
Short summary
Removal of stratospheric nitrogen oxides is crucial for the formation of the ozone hole. TROPOMI satellite measurements of nitrogen dioxide reveal the presence of a not dissimilar "nitrogen hole" that largely coincides with the ozone hole. Three very distinct regimes were identified: inside and outside the ozone hole and the transition zone in between. Our results introduce a valuable and innovative application highly relevant for Antarctic ozone hole and ozone layer recovery.
Kyriakoula Papachristopoulou, Ilias Fountoulakis, Alkiviadis F. Bais, Basil E. Psiloglou, Nikolaos Papadimitriou, Ioannis-Panagiotis Raptis, Andreas Kazantzidis, Charalampos Kontoes, Maria Hatzaki, and Stelios Kazadzis
Atmos. Meas. Tech., 17, 1851–1877, https://doi.org/10.5194/amt-17-1851-2024, https://doi.org/10.5194/amt-17-1851-2024, 2024
Short summary
Short summary
The upgraded systems SENSE2 and NextSENSE2 focus on improving the quality of solar nowcasting and forecasting. SENSE2 provides real-time estimates of solar irradiance across a wide region every 15 min. NextSENSE2 offers short-term forecasts of irradiance up to 3 h ahead. Evaluation with actual data showed that the instantaneous comparison yields the most discrepancies due to the uncertainties of cloud-related information and satellite versus ground-based spatial representativeness limitations.
Antonio Fernando Almansa, África Barreto, Natalia Kouremeti, Ramiro González, Akriti Masoom, Carlos Toledano, Julian Gröbner, Rosa Delia García, Yenny González, Stelios Kazadzis, Stéphane Victori, Óscar Álvarez, Fabrice Maupin, Virgilio Carreño, Victoria Eugenia Cachorro, and Emilio Cuevas
Atmos. Meas. Tech., 17, 659–675, https://doi.org/10.5194/amt-17-659-2024, https://doi.org/10.5194/amt-17-659-2024, 2024
Short summary
Short summary
This paper applies sun photometer synergies to improve calibration transference between different sun photometers and also enhance their quality assurance and quality control. We have validated this technique using different instrumentation, the WMO-GAW and NASA-AERONET references, under different aerosol regimes using the standard Langley calibration method as a reference.
Alexandra Tsekeri, Anna Gialitaki, Marco Di Paolantonio, Davide Dionisi, Gian Luigi Liberti, Alnilam Fernandes, Artur Szkop, Aleksander Pietruczuk, Daniel Pérez-Ramírez, Maria J. Granados Muñoz, Juan Luis Guerrero-Rascado, Lucas Alados-Arboledas, Diego Bermejo Pantaleón, Juan Antonio Bravo-Aranda, Anna Kampouri, Eleni Marinou, Vassilis Amiridis, Michael Sicard, Adolfo Comerón, Constantino Muñoz-Porcar, Alejandro Rodríguez-Gómez, Salvatore Romano, Maria Rita Perrone, Xiaoxia Shang, Mika Komppula, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Diofantos Hadjimitsis, Francisco Navas-Guzmán, Alexander Haefele, Dominika Szczepanik, Artur Tomczak, Iwona S. Stachlewska, Livio Belegante, Doina Nicolae, Kalliopi Artemis Voudouri, Dimitris Balis, Athena A. Floutsi, Holger Baars, Linda Miladi, Nicolas Pascal, Oleg Dubovik, and Anton Lopatin
Atmos. Meas. Tech., 16, 6025–6050, https://doi.org/10.5194/amt-16-6025-2023, https://doi.org/10.5194/amt-16-6025-2023, 2023
Short summary
Short summary
EARLINET/ACTRIS organized an intensive observational campaign in May 2020, with the objective of monitoring the atmospheric state over Europe during the COVID-19 lockdown and relaxation period. The work presented herein focuses on deriving a common methodology for applying a synergistic retrieval that utilizes the network's ground-based passive and active remote sensing measurements and deriving the aerosols from anthropogenic activities over Europe.
Yuhang Zhang, Jintai Lin, Jhoon Kim, Hanlim Lee, Junsung Park, Hyunkee Hong, Michel Van Roozendael, Francois Hendrick, Ting Wang, Pucai Wang, Qin He, Kai Qin, Yongjoo Choi, Yugo Kanaya, Jin Xu, Pinhua Xie, Xin Tian, Sanbao Zhang, Shanshan Wang, Siyang Cheng, Xinghong Cheng, Jianzhong Ma, Thomas Wagner, Robert Spurr, Lulu Chen, Hao Kong, and Mengyao Liu
Atmos. Meas. Tech., 16, 4643–4665, https://doi.org/10.5194/amt-16-4643-2023, https://doi.org/10.5194/amt-16-4643-2023, 2023
Short summary
Short summary
Our tropospheric NO2 vertical column density product with high spatiotemporal resolution is based on the Geostationary Environment Monitoring Spectrometer (GEMS) and named POMINO–GEMS. Strong hotspot signals and NO2 diurnal variations are clearly seen. Validations with multiple satellite products and ground-based, mobile car and surface measurements exhibit the overall great performance of the POMINO–GEMS product, indicating its capability for application in environmental studies.
Julian Gröbner, Natalia Kouremeti, Gregor Hülsen, Ralf Zuber, Mario Ribnitzky, Saulius Nevas, Peter Sperfeld, Kerstin Schwind, Philipp Schneider, Stelios Kazadzis, África Barreto, Tom Gardiner, Kavitha Mottungan, David Medland, and Marc Coleman
Atmos. Meas. Tech., 16, 4667–4680, https://doi.org/10.5194/amt-16-4667-2023, https://doi.org/10.5194/amt-16-4667-2023, 2023
Short summary
Short summary
Spectral solar irradiance measurements traceable to the International System of Units (SI) allow for intercomparability between instruments and for their validation according to metrological standards. Here we also validate and reduce the uncertainties of the top-of-atmosphere TSIS-1 Hybrid Solar Reference Spectrum (HSRS). The management of large networks, e.g. AERONET or GAW-PFR, will benefit from reducing logistical overhead, improving their resilience and achieving metrological traceability.
Akriti Masoom, Ilias Fountoulakis, Stelios Kazadzis, Ioannis-Panagiotis Raptis, Anna Kampouri, Basil E. Psiloglou, Dimitra Kouklaki, Kyriakoula Papachristopoulou, Eleni Marinou, Stavros Solomos, Anna Gialitaki, Dimitra Founda, Vasileios Salamalikis, Dimitris Kaskaoutis, Natalia Kouremeti, Nikolaos Mihalopoulos, Vassilis Amiridis, Andreas Kazantzidis, Alexandros Papayannis, Christos S. Zerefos, and Kostas Eleftheratos
Atmos. Chem. Phys., 23, 8487–8514, https://doi.org/10.5194/acp-23-8487-2023, https://doi.org/10.5194/acp-23-8487-2023, 2023
Short summary
Short summary
We analyse the spatial and temporal aerosol spectral optical properties during the extreme wildfires of August 2021 in Greece and assess their effects on air quality and solar radiation quantities related to health, agriculture, and energy. Different aerosol conditions are identified (pure smoke, pure dust, dust–smoke together); the largest impact on solar radiation quantities is found for cases with mixed dust–smoke aerosols. Such situations are expected to occur more frequently in the future.
Theano Drosoglou, Ioannis-Panagiotis Raptis, Massimo Valeri, Stefano Casadio, Francesca Barnaba, Marcos Herreras-Giralda, Anton Lopatin, Oleg Dubovik, Gabriele Brizzi, Fabrizio Niro, Monica Campanelli, and Stelios Kazadzis
Atmos. Meas. Tech., 16, 2989–3014, https://doi.org/10.5194/amt-16-2989-2023, https://doi.org/10.5194/amt-16-2989-2023, 2023
Short summary
Short summary
Aerosol optical properties derived from sun photometers depend on the optical depth of trace gases absorbing solar radiation at specific spectral ranges. Various networks use satellite-based climatologies to account for this or neglect their effect. In this work, we evaluate the effect of NO2 absorption in aerosol retrievals from AERONET and SKYNET over two stations in Rome, Italy, with relatively high NO2 spatiotemporal variations, using NO2 data from the Pandora network and the TROPOMI sensor.
Xiaojuan Lin, Ronald van der A, Jos de Laat, Henk Eskes, Frédéric Chevallier, Philippe Ciais, Zhu Deng, Yuanhao Geng, Xuanren Song, Xiliang Ni, Da Huo, Xinyu Dou, and Zhu Liu
Atmos. Chem. Phys., 23, 6599–6611, https://doi.org/10.5194/acp-23-6599-2023, https://doi.org/10.5194/acp-23-6599-2023, 2023
Short summary
Short summary
Satellite observations provide evidence for CO2 emission signals from isolated power plants. We use these satellite observations to quantify emissions. We found that for power plants with multiple observations, the correlation of estimated and reported emissions is significantly improved compared to a single observation case. This demonstrates that accurate estimation of power plant emissions can be achieved by monitoring from future satellite missions with more frequent observations.
Xiumei Zhang, Ronald van der A, Jieying Ding, Xin Zhang, and Yan Yin
Atmos. Chem. Phys., 23, 5587–5604, https://doi.org/10.5194/acp-23-5587-2023, https://doi.org/10.5194/acp-23-5587-2023, 2023
Short summary
Short summary
We compiled a ship emission inventory based on automatic identification system (AIS) signals in the Jiangsu section of the Yangtze River. This ship emission inventory was compared with Chinese bottom-up inventories and the satellite-derived emissions from TROPOMI. The result shows a consistent spatial distribution, with riverine cities having high NOx emissions. Inland ship emissions of NOx are shown to contribute at least 40 % to air pollution along the river.
Ka Lok Chan, Pieter Valks, Klaus-Peter Heue, Ronny Lutz, Pascal Hedelt, Diego Loyola, Gaia Pinardi, Michel Van Roozendael, François Hendrick, Thomas Wagner, Vinod Kumar, Alkis Bais, Ankie Piters, Hitoshi Irie, Hisahiro Takashima, Yugo Kanaya, Yongjoo Choi, Kihong Park, Jihyo Chong, Alexander Cede, Udo Frieß, Andreas Richter, Jianzhong Ma, Nuria Benavent, Robert Holla, Oleg Postylyakov, Claudia Rivera Cárdenas, and Mark Wenig
Earth Syst. Sci. Data, 15, 1831–1870, https://doi.org/10.5194/essd-15-1831-2023, https://doi.org/10.5194/essd-15-1831-2023, 2023
Short summary
Short summary
This paper presents the theoretical basis as well as verification and validation of the Global Ozone Monitoring Experiment-2 (GOME-2) daily and monthly level-3 products.
Antonis Gkikas, Anna Gialitaki, Ioannis Binietoglou, Eleni Marinou, Maria Tsichla, Nikolaos Siomos, Peristera Paschou, Anna Kampouri, Kalliopi Artemis Voudouri, Emmanouil Proestakis, Maria Mylonaki, Christina-Anna Papanikolaou, Konstantinos Michailidis, Holger Baars, Anne Grete Straume, Dimitris Balis, Alexandros Papayannis, Tomasso Parrinello, and Vassilis Amiridis
Atmos. Meas. Tech., 16, 1017–1042, https://doi.org/10.5194/amt-16-1017-2023, https://doi.org/10.5194/amt-16-1017-2023, 2023
Short summary
Short summary
We perform an assessment analysis of the Aeolus Standard Correct Algorithm (SCA) backscatter coefficient retrievals against reference observations acquired at three Greek lidar stations (Athens, Thessaloniki and Antikythera) of the PANACEA network. Overall, 43 cases are analysed, whereas specific aerosol scenarios in the vicinity of Antikythera island (SW Greece) are emphasised. All key Cal/Val aspects and recommendations, and the ongoing related activities, are thoroughly discussed.
Konstantinos Michailidis, Maria-Elissavet Koukouli, Dimitris Balis, J. Pepijn Veefkind, Martin de Graaf, Lucia Mona, Nikolaos Papagianopoulos, Gesolmina Pappalardo, Ioanna Tsikoudi, Vassilis Amiridis, Eleni Marinou, Anna Gialitaki, Rodanthi-Elisavet Mamouri, Argyro Nisantzi, Daniele Bortoli, Maria João Costa, Vanda Salgueiro, Alexandros Papayannis, Maria Mylonaki, Lucas Alados-Arboledas, Salvatore Romano, Maria Rita Perrone, and Holger Baars
Atmos. Chem. Phys., 23, 1919–1940, https://doi.org/10.5194/acp-23-1919-2023, https://doi.org/10.5194/acp-23-1919-2023, 2023
Short summary
Short summary
Comparisons with ground-based correlative lidar measurements constitute a key component in the validation of satellite aerosol products. This paper presents the validation of the TROPOMI aerosol layer height (ALH) product, using archived quality assured ground-based data from lidar stations that belong to the EARLINET network. Comparisons between the TROPOMI ALH and co-located EARLINET measurements show good agreement over the ocean.
Katerina Garane, Ka Lok Chan, Maria-Elissavet Koukouli, Diego Loyola, and Dimitris Balis
Atmos. Meas. Tech., 16, 57–74, https://doi.org/10.5194/amt-16-57-2023, https://doi.org/10.5194/amt-16-57-2023, 2023
Short summary
Short summary
In this work, 2.5 years of TROPOMI/S5P Total Column Water Vapor (TCWV) observations retrieved from the blue wavelength band are validated against co-located precipitable water measurements from NASA AERONET, which uses Cimel Sun photometers globally. Overall, the TCWV product agrees well on a global scale with the ground-based dataset (Pearson correl. coefficient 0.909) and has a mean relative bias of −2.7 ± 4.9 % with respect to the AERONET observations for moderate albedo and cloudiness.
Angelos Karanikolas, Natalia Kouremeti, Julian Gröbner, Luca Egli, and Stelios Kazadzis
Atmos. Meas. Tech., 15, 5667–5680, https://doi.org/10.5194/amt-15-5667-2022, https://doi.org/10.5194/amt-15-5667-2022, 2022
Short summary
Short summary
The aim of this work is to investigate the limitations of calculating long-term trends of a parameter that quantifies the overall effect of atmospheric aerosols on the solar radiation. A main finding is that even instruments with good agreement between their observations can show significantly different linear trends. By calculating time-varying trends, the trend agreement is shown to improve. We also show that different methods of trend estimation can result in significant trend differences.
Kostas Eleftheratos, John Kapsomenakis, Ilias Fountoulakis, Christos S. Zerefos, Patrick Jöckel, Martin Dameris, Alkiviadis F. Bais, Germar Bernhard, Dimitra Kouklaki, Kleareti Tourpali, Scott Stierle, J. Ben Liley, Colette Brogniez, Frédérique Auriol, Henri Diémoz, Stana Simic, Irina Petropavlovskikh, Kaisa Lakkala, and Kostas Douvis
Atmos. Chem. Phys., 22, 12827–12855, https://doi.org/10.5194/acp-22-12827-2022, https://doi.org/10.5194/acp-22-12827-2022, 2022
Short summary
Short summary
We present the future evolution of DNA-active ultraviolet (UV) radiation in view of increasing greenhouse gases (GHGs) and decreasing ozone depleting substances (ODSs). It is shown that DNA-active UV radiation might increase after 2050 between 50° N–50° S due to GHG-induced reductions in clouds and ozone, something that is likely not to happen at high latitudes, where DNA-active UV radiation will continue its downward trend mainly due to stratospheric ozone recovery from the reduction in ODSs.
Hanqing Kang, Bin Zhu, Gerrit de Leeuw, Bu Yu, Ronald J. van der A, and Wen Lu
Atmos. Chem. Phys., 22, 10623–10634, https://doi.org/10.5194/acp-22-10623-2022, https://doi.org/10.5194/acp-22-10623-2022, 2022
Short summary
Short summary
This study quantified the contribution of each urban-induced meteorological effect (temperature, humidity, and circulation) to aerosol concentration. We found that the urban heat island (UHI) circulation dominates the UHI effects on aerosol. The UHI circulation transports aerosol and its precursor gases from the warmer lower boundary layer to the colder lower free troposphere and promotes the secondary formation of ammonium nitrate aerosol in the cold atmosphere.
Xin Zhang, Yan Yin, Ronald van der A, Henk Eskes, Jos van Geffen, Yunyao Li, Xiang Kuang, Jeff L. Lapierre, Kui Chen, Zhongxiu Zhen, Jianlin Hu, Chuan He, Jinghua Chen, Rulin Shi, Jun Zhang, Xingrong Ye, and Hao Chen
Atmos. Chem. Phys., 22, 5925–5942, https://doi.org/10.5194/acp-22-5925-2022, https://doi.org/10.5194/acp-22-5925-2022, 2022
Short summary
Short summary
The importance of convection to the ozone and nitrogen oxides (NOx) produced from lightning has long been an open question. We utilize the high-resolution chemistry model with ozonesondes and space observations to discuss the effects of convection over southeastern China, where few studies have been conducted. Our results show the transport and chemistry contributions for various storms and demonstrate the ability of TROPOMI to estimate the lightning NOx production over small-scale convection.
Maria-Elissavet Koukouli, Konstantinos Michailidis, Pascal Hedelt, Isabelle A. Taylor, Antje Inness, Lieven Clarisse, Dimitris Balis, Dmitry Efremenko, Diego Loyola, Roy G. Grainger, and Christian Retscher
Atmos. Chem. Phys., 22, 5665–5683, https://doi.org/10.5194/acp-22-5665-2022, https://doi.org/10.5194/acp-22-5665-2022, 2022
Short summary
Short summary
Volcanic eruptions eject large amounts of ash and trace gases into the atmosphere. The use of space-borne instruments enables the global monitoring of volcanic SO2 emissions in an economical and risk-free manner. The main aim of this paper is to present its extensive verification, accomplished within the ESA S5P+I: SO2LH project, over major recent volcanic eruptions, against collocated space-borne measurements, as well as assess its impact on the forecasts provided by CAMS.
Dimitris Karagkiozidis, Martina Michaela Friedrich, Steffen Beirle, Alkiviadis Bais, François Hendrick, Kalliopi Artemis Voudouri, Ilias Fountoulakis, Angelos Karanikolas, Paraskevi Tzoumaka, Michel Van Roozendael, Dimitris Balis, and Thomas Wagner
Atmos. Meas. Tech., 15, 1269–1301, https://doi.org/10.5194/amt-15-1269-2022, https://doi.org/10.5194/amt-15-1269-2022, 2022
Short summary
Short summary
In this study we focus on the retrieval of aerosol, NO2, and HCHO vertical profiles from multi-axis differential optical absorption spectroscopy (MAX-DOAS) observations for the first time over Thessaloniki, Greece. We use two independent inversion algorithms for the profile retrievals. We evaluate their performance, we intercompare their results, and we validate their products with ancillary data, measured by other co-located reference instruments.
Antje Inness, Melanie Ades, Dimitris Balis, Dmitry Efremenko, Johannes Flemming, Pascal Hedelt, Maria-Elissavet Koukouli, Diego Loyola, and Roberto Ribas
Geosci. Model Dev., 15, 971–994, https://doi.org/10.5194/gmd-15-971-2022, https://doi.org/10.5194/gmd-15-971-2022, 2022
Short summary
Short summary
This paper describes the way that the Copernicus Atmosphere Monitoring Service (CAMS) produces forecasts of volcanic SO2. These forecasts are provided routinely every day. They are created by blending SO2 data from satellite instruments (TROPOMI and GOME-2) with the CAMS model. We show that the quality of the CAMS SO2 forecasts can be improved if additional information about the height of volcanic plumes is provided in the satellite data.
Song Liu, Pieter Valks, Gaia Pinardi, Jian Xu, Ka Lok Chan, Athina Argyrouli, Ronny Lutz, Steffen Beirle, Ehsan Khorsandi, Frank Baier, Vincent Huijnen, Alkiviadis Bais, Sebastian Donner, Steffen Dörner, Myrto Gratsea, François Hendrick, Dimitris Karagkiozidis, Kezia Lange, Ankie J. M. Piters, Julia Remmers, Andreas Richter, Michel Van Roozendael, Thomas Wagner, Mark Wenig, and Diego G. Loyola
Atmos. Meas. Tech., 14, 7297–7327, https://doi.org/10.5194/amt-14-7297-2021, https://doi.org/10.5194/amt-14-7297-2021, 2021
Short summary
Short summary
In this work, an improved tropospheric NO2 retrieval algorithm from TROPOMI measurements over Europe is presented. The stratospheric estimation is implemented with correction for the dependency of the stratospheric NO2 on the viewing geometry. The AMF calculation is implemented using improved surface albedo, a priori NO2 profiles, and cloud correction. The improved tropospheric NO2 data show good correlations with ground-based MAX-DOAS measurements.
Xin Tian, Yang Wang, Steffen Beirle, Pinhua Xie, Thomas Wagner, Jin Xu, Ang Li, Steffen Dörner, Bo Ren, and Xiaomei Li
Atmos. Chem. Phys., 21, 12867–12894, https://doi.org/10.5194/acp-21-12867-2021, https://doi.org/10.5194/acp-21-12867-2021, 2021
Short summary
Short summary
The performances of two MAX-DOAS inversion algorithms were evaluated for various aerosol pollution scenarios. One inversion algorithm is based on optimal estimation; the other uses a parameterized approach. In this analysis, three types of profile shapes for aerosols and NO2 were considered: exponential, Boltzmann, and Gaussian. The evaluation results can effectively guide the application of the two inversion algorithms in the actual atmosphere and improve the accuracy of the actual inversion.
Isabelle De Smedt, Gaia Pinardi, Corinne Vigouroux, Steven Compernolle, Alkis Bais, Nuria Benavent, Folkert Boersma, Ka-Lok Chan, Sebastian Donner, Kai-Uwe Eichmann, Pascal Hedelt, François Hendrick, Hitoshi Irie, Vinod Kumar, Jean-Christopher Lambert, Bavo Langerock, Christophe Lerot, Cheng Liu, Diego Loyola, Ankie Piters, Andreas Richter, Claudia Rivera Cárdenas, Fabian Romahn, Robert George Ryan, Vinayak Sinha, Nicolas Theys, Jonas Vlietinck, Thomas Wagner, Ting Wang, Huan Yu, and Michel Van Roozendael
Atmos. Chem. Phys., 21, 12561–12593, https://doi.org/10.5194/acp-21-12561-2021, https://doi.org/10.5194/acp-21-12561-2021, 2021
Short summary
Short summary
This paper assess the performances of the TROPOMI formaldehyde observations compared to its predecessor OMI at different spatial and temporal scales. We also use a global network of MAX-DOAS instruments to validate both satellite datasets for a large range of HCHO columns. The precision obtained with daily TROPOMI observations is comparable to monthly OMI observations. We present clear detection of weak HCHO column enhancements related to shipping emissions in the Indian Ocean.
Panagiotis G. Kosmopoulos, Stelios Kazadzis, Alois W. Schmalwieser, Panagiotis I. Raptis, Kyriakoula Papachristopoulou, Ilias Fountoulakis, Akriti Masoom, Alkiviadis F. Bais, Julia Bilbao, Mario Blumthaler, Axel Kreuter, Anna Maria Siani, Kostas Eleftheratos, Chrysanthi Topaloglou, Julian Gröbner, Bjørn Johnsen, Tove M. Svendby, Jose Manuel Vilaplana, Lionel Doppler, Ann R. Webb, Marina Khazova, Hugo De Backer, Anu Heikkilä, Kaisa Lakkala, Janusz Jaroslawski, Charikleia Meleti, Henri Diémoz, Gregor Hülsen, Barbara Klotz, John Rimmer, and Charalampos Kontoes
Atmos. Meas. Tech., 14, 5657–5699, https://doi.org/10.5194/amt-14-5657-2021, https://doi.org/10.5194/amt-14-5657-2021, 2021
Short summary
Short summary
Large-scale retrievals of the ultraviolet index (UVI) in real time by exploiting the modern Earth observation data and techniques are capable of forming operational early warning systems that raise awareness among citizens of the health implications of high UVI doses. In this direction a novel UVI operating system, the so-called UVIOS, was introduced for massive outputs, while its performance was tested against ground-based measurements revealing a dependence on the input quality and resolution.
Cheng Fan, Zhengqiang Li, Ying Li, Jiantao Dong, Ronald van der A, and Gerrit de Leeuw
Atmos. Chem. Phys., 21, 7723–7748, https://doi.org/10.5194/acp-21-7723-2021, https://doi.org/10.5194/acp-21-7723-2021, 2021
Short summary
Short summary
Emission control policy in China has resulted in the decrease of nitrogen dioxide concentrations, which however leveled off and stabilized in recent years, as shown from satellite data. The effects of the further emission reduction during the COVID-19 lockdown in 2020 resulted in an initial improvement of air quality, which, however, was offset by chemical and meteorological effects. The study shows the regional dependence over east China, and results have a wider application than China only.
Wannan Wang, Ronald van der A, Jieying Ding, Michiel van Weele, and Tianhai Cheng
Atmos. Chem. Phys., 21, 7253–7269, https://doi.org/10.5194/acp-21-7253-2021, https://doi.org/10.5194/acp-21-7253-2021, 2021
Short summary
Short summary
We developed a method to determine the type of photochemical regime of ozone formation by using only satellite observations of formaldehyde and nitrogen dioxide as well as ozone measurements on the ground. It was found that many cities in China, because of their high level of air pollution, are in the so-called VOC-limited photochemical regime. This means that the current reductions of nitrogen dioxide resulted in higher levels of photochemical smog in these cities.
Ioanna Skoulidou, Maria-Elissavet Koukouli, Astrid Manders, Arjo Segers, Dimitris Karagkiozidis, Myrto Gratsea, Dimitris Balis, Alkiviadis Bais, Evangelos Gerasopoulos, Trisevgeni Stavrakou, Jos van Geffen, Henk Eskes, and Andreas Richter
Atmos. Chem. Phys., 21, 5269–5288, https://doi.org/10.5194/acp-21-5269-2021, https://doi.org/10.5194/acp-21-5269-2021, 2021
Short summary
Short summary
The performance of LOTOS-EUROS v2.2.001 regional chemical transport model NO2 simulations is investigated over Greece from June to December 2018. Comparison with in situ NO2 measurements shows a spatial correlation coefficient of 0.86, while the model underestimates the concentrations mostly during daytime (12 to 15:00 local time). Further, the simulated tropospheric NO2 columns are evaluated against ground-based MAX-DOAS NO2 measurements and S5P/TROPOMI observations for July and December 2018.
Nicola Zoppetti, Simone Ceccherini, Bruno Carli, Samuele Del Bianco, Marco Gai, Cecilia Tirelli, Flavio Barbara, Rossana Dragani, Antti Arola, Jukka Kujanpää, Jacob C. A. van Peet, Ronald van der A, and Ugo Cortesi
Atmos. Meas. Tech., 14, 2041–2053, https://doi.org/10.5194/amt-14-2041-2021, https://doi.org/10.5194/amt-14-2041-2021, 2021
Short summary
Short summary
The new platforms for Earth observation from space will provide an enormous amount of data that can be hard to exploit as a whole. The Complete Data Fusion algorithm can reduce the data volume while retaining the information of the full dataset. In this work, we applied the Complete Data Fusion algorithm to simulated ozone profiles, and the results show that the fused products are characterized by higher information content compared to individual L2 products.
Konstantinos Michailidis, Maria-Elissavet Koukouli, Nikolaos Siomos, Dimitris Balis, Olaf Tuinder, L. Gijsbert Tilstra, Lucia Mona, Gelsomina Pappalardo, and Daniele Bortoli
Atmos. Chem. Phys., 21, 3193–3213, https://doi.org/10.5194/acp-21-3193-2021, https://doi.org/10.5194/acp-21-3193-2021, 2021
Short summary
Short summary
The aim of this study is to investigate the potential of the GOME-2 instrument aboard the MetOp-A, MetOp-B and MetOp-C platforms to deliver accurate geometrical features of lofted aerosol layers. For this purpose, we use archived ground-based data from lidar stations available from the EARLINET database. We show that for this well-developed and spatially well-spread aerosol layer, most GOME-2 retrievals fall within 1 km of the exact temporally collocated lidar observation.
Wannan Wang, Tianhai Cheng, Ronald J. van der A, Jos de Laat, and Jason E. Williams
Atmos. Meas. Tech., 14, 1673–1687, https://doi.org/10.5194/amt-14-1673-2021, https://doi.org/10.5194/amt-14-1673-2021, 2021
Short summary
Short summary
This paper is an evaluation of the AIRS and MLS ozone (O3) algorithms via comparison with daytime and night-time O3 datasets. Results show that further refinements of the AIRS O3 algorithm are required for better surface emissivity retrievals and that cloud cover is another problem that needs to be solved. An inconsistency is found in the
AscDescModeflag of the MLS v4.20 standard O3 product for 90–60° S and 60–90° N, resulting in inconsistent O3 profiles in these regions before May 2015.
Maria-Elissavet Koukouli, Ioanna Skoulidou, Andreas Karavias, Isaak Parcharidis, Dimitris Balis, Astrid Manders, Arjo Segers, Henk Eskes, and Jos van Geffen
Atmos. Chem. Phys., 21, 1759–1774, https://doi.org/10.5194/acp-21-1759-2021, https://doi.org/10.5194/acp-21-1759-2021, 2021
Short summary
Short summary
In recent years, satellite observations have contributed to monitoring air quality. During the first COVID-19 lockdown, lower levels of nitrogen dioxide were observed over Greece by S5P/TROPOMI for March and April 2020 (than the preceding year) due to decreased transport emissions. Taking meteorology into account, using LOTOS-EUROS CTM simulations, the resulting decline due to the lockdown was estimated to range between 0 % and −37 % for the five largest Greek cities, with an average of ~ −10 %.
Tijl Verhoelst, Steven Compernolle, Gaia Pinardi, Jean-Christopher Lambert, Henk J. Eskes, Kai-Uwe Eichmann, Ann Mari Fjæraa, José Granville, Sander Niemeijer, Alexander Cede, Martin Tiefengraber, François Hendrick, Andrea Pazmiño, Alkiviadis Bais, Ariane Bazureau, K. Folkert Boersma, Kristof Bognar, Angelika Dehn, Sebastian Donner, Aleksandr Elokhov, Manuel Gebetsberger, Florence Goutail, Michel Grutter de la Mora, Aleksandr Gruzdev, Myrto Gratsea, Georg H. Hansen, Hitoshi Irie, Nis Jepsen, Yugo Kanaya, Dimitris Karagkiozidis, Rigel Kivi, Karin Kreher, Pieternel F. Levelt, Cheng Liu, Moritz Müller, Monica Navarro Comas, Ankie J. M. Piters, Jean-Pierre Pommereau, Thierry Portafaix, Cristina Prados-Roman, Olga Puentedura, Richard Querel, Julia Remmers, Andreas Richter, John Rimmer, Claudia Rivera Cárdenas, Lidia Saavedra de Miguel, Valery P. Sinyakov, Wolfgang Stremme, Kimberly Strong, Michel Van Roozendael, J. Pepijn Veefkind, Thomas Wagner, Folkard Wittrock, Margarita Yela González, and Claus Zehner
Atmos. Meas. Tech., 14, 481–510, https://doi.org/10.5194/amt-14-481-2021, https://doi.org/10.5194/amt-14-481-2021, 2021
Short summary
Short summary
This paper reports on the ground-based validation of the NO2 data produced operationally by the TROPOMI instrument on board the Sentinel-5 Precursor satellite. Tropospheric, stratospheric, and total NO2 columns are compared to measurements collected from MAX-DOAS, ZSL-DOAS, and PGN/Pandora instruments respectively. The products are found to satisfy mission requirements in general, though negative mean differences are found at sites with high pollution levels. Potential causes are discussed.
Cited articles
Aliwell, S., Van Roozendael, M., Johnston, P., Richter, A., Wagner, T., Arlander, D. W., Burrows, J. P., Fish, D. J., Jones, R. L., Tørnkvist, K. K., Lambert, J.-C., Pfeilsticker, K., and Pundt, I.: Analysis for BrO in zenith-sky spectra: An intercomparison exercise for analysis improvement, J. Geophys. Res., 107, 4199, https://doi.org/10.1029/2001JD000329, 2002.
Amiridis, V., Marinou, E., Tsekeri, A., Wandinger, U., Schwarz, A., Giannakaki, E., Mamouri, R., Kokkalis, P., Binietoglou, I., Solomos, S., Herekakis, T., Kazadzis, S., Gerasopoulos, E., Proestakis, E., Kottas, M., Balis, D., Papayannis, A., Kontoes, C., Kourtidis, K., Papagiannopoulos, N., Mona, L., Pappalardo, G., Le Rille, O., and Ansmann, A.: LIVAS: a 3-D multi-wavelength aerosol/cloud database based on CALIPSO and EARLINET, Atmos. Chem. Phys., 15, 7127–7153, https://doi.org/10.5194/acp-15-7127-2015, 2015.
Boersma, K. F., Eskes, H. J., and Brinksma, E. J.: Error Analysis for Tropospheric NO2 Retrieval from Space, J. Geophys. Res., 109, D04311, https://doi.org/10.1029/2003JD003962, 2004.
Boersma, K. F., Eskes, H. J., Dirksen, R. J., van der A, R. J., Veefkind, J. P., Stammes, P., Huijnen, V., Kleipool, Q. L., Sneep, M., Claas, J., Leitão, J., Richter, A., Zhou, Y., and Brunner, D.: An improved tropospheric NO2 column retrieval algorithm for the Ozone Monitoring Instrument, Atmos. Meas. Tech., 4, 1905–1928, https://doi.org/10.5194/amt-4-1905-2011, 2011.
Brinksma, E. J., Pinardi, G., Volten, H., Braak, R., Richter, A., Schönhardt, A., van Roozendael, M., Fayt, C., Hermans, C., Dirksen, R. J., Vlemmix, T., Berkhout, A. J. C., Swart, D. P. J., Oetjen, H., Wittrock, F., Wagner, T., Ibrahim, O. W., de Leeuw, G., Moerman, M., Curier, R. L., Celarier, E. A., Cede, A., Knap, W. H., Veefkind, J. P., Eskes, H. J., Allaart, M., Rothe, R., Piters, A. J. M., and Levelt, P. F.: The 2005 and 2006 DANDELIONS NO2 and aerosol intercomparison campaigns, J. Geophys. Res., 113, D16S46, https://doi.org/10.1029/2007JD008808, 2008.
Buras R., Dowling T., and Emde C.: New secondary-scattering correction in DISORT with increased efficiency for forward scattering, J. Quant. Spectrosc. Ra., 112, 2028–2034, 2011.
Celarier, E. A., Brinksma, E. J., Gleason, J. F., Veefkind, J. P., Cede, A., Herman, J. R., Ionov, D., Goutail, F., Pommereau, J. P., Lambert, J. C., van Roozendael, M., Pinardi, G., Wittrock, F., Schönhardt, A., Richter, A., Ibrahim, O. W., Wagner, T., Bojkov, B., Mount, G., Spinei, E., Chen, C. M., Pongetti, T. J., Sander, S. P., Bucsela, E. J., Wenig, M. O., Swart, D. P. J., Volten, H., Kroon, M., and Levelt, P. F.: Validation of Ozone Monitoring Instrument nitrogen dioxide columns, J. Geophys. Res., 113, D15S15, https://doi.org/10.1029/2007JD008908, 2008.
Chan, C. K. and Yao, X.: Air pollution in mega cities in China, Atmos. Environ., 42, 1–42, https://doi.org/10.1016/j.atmosenv.2007.09.003, 2008.
Chan, K. L., Hartl, A., Lam, Y. F., Xie, P. H., Liu, W. Q., Cheung, H. M., Lampel, J., Pöhler, D., Li, A., Xu, J., Zhou, H. J., Ning, Z., and Wenig, M. O.: Observations of tropospheric NO2 using ground based MAX-DOAS and OMI measurements during the Shanghai World Expo 2010, Atmos. Environ., 119, 45–58, 2015.
Chance, K. and Spurr, R. J. D.: Ring effect studies: Rayleigh scattering, including molecular parameters for rotational Raman scattering and the Fraunhofer spectrum, Appl. Opt., 36, 5224–5230, 1997.
Chen, D., Zhou, B., Beirle, S., Chen, L. M., and Wagner, T.: Tropospheric NO2 column densities deduced from zenith-sky DOAS measurements in Shanghai, China, and their application to satellite validation, Atmos. Chem. Phys., 9, 3641–3662, https://doi.org/10.5194/acp-9-3641-2009, 2009.
Clémer, K., Van Roozendael, M., Fayt, C., Hendrick, F., Hermans, C., Pinardi, G., Spurr, R., Wang, P., and De Mazière, M.: Multiple wavelength retrieval of tropospheric aerosol optical properties from MAXDOAS measurements in Beijing, Atmos. Meas. Tech., 3, 863–878, https://doi.org/10.5194/amt-3-863-2010, 2010.
Danckaert, T., Fayt, C., Van Roozendael, M., De Smedt, I., Letocart, V., Merlaud, A., and Pinardi, G.: QDOAS software user manual Version 2.111, IASB/BIRA, Uccle, Belgium, 2016.
De Smedt, I., Stavrakou, T., Hendrick, F., Danckaert, T., Vlemmix, T., Pinardi, G., Theys, N., Lerot, C., Gielen, C., Vigouroux, C., Hermans, C., Fayt, C., Veefkind, P., Müller, J.-F., and Van Roozendael, M.: Diurnal, seasonal and long-term variations of global formaldehyde columns inferred from combined OMI and GOME-2 observations, Atmos. Chem. Phys., 15, 12519–12545, https://doi.org/10.5194/acp-15-12519-2015, 2015.
Ding, J., van der A, R. J., Mijling, B., Levelt, P. F., and Hao, N.: NOx emission estimates during the 2014 Youth Olympic Games in Nanjing, Atmos. Chem. Phys., 15, 9399–9412, https://doi.org/10.5194/acp-15-9399-2015, 2015.
Drosoglou, T., Bais, A. F., Zyrichidou, I., Kouremeti, N., Poupkou, A., Liora, N., Giannaros, C., Koukouli, M. E., Balis, D., and Melas, D.: Comparisons of ground-based tropospheric NO2 MAX-DOAS measurements to satellite observations with the aid of an air quality model over the Thessaloniki area, Greece, Atmos. Chem. Phys., 17, 5829–5849, https://doi.org/10.5194/acp-17-5829-2017, 2017.
EPA: Air Quality Index-A Guide to Air Quality and Your Health, United States Environmental Protection Agency, Washington, DC20460, EPA-454/R-00-005, 2000.
Eskes, H. J. and Boersma, K. F.: Averaging kernels for DOAS total-column satellite retrievals, Atmos. Chem. Phys., 3, 1285–1291, https://doi.org/10.5194/acp-3-1285-2003, 2003.
Feister, U. and Grewe, R.: Spectral albedo measurements in the UV and visible region over different types of surface, Photochem. Photobiol., 62, 736–744, 1995.
Finlayson-Pitts, B. J. and Pitts, J. N.: Chemistry of the Upper and Lower Atmosphere, Academic Press, San Diego, 2000.
Frieß, U., Monks, P., Remedios, J., Rozanov, A., Sinreich, R., Wagner, T., and Platt, U.: MAX-DOAS O4 measurements: A new technique to derive information on atmospheric aerosols: 2. Modeling studies, J. Geophys. Res., 111, D14203, https://doi.org/10.1029/2005JD006618, 2006.
Frieß, U., Sihler, H., Sander, R., Pöhler, D., Yilmaz, S., and Platt, U.: The vertical distribution of BrO and aerosols in the Arctic: Measurements by active and passive differential optical absorption spectroscopy, J. Geophys. Res., 116, D00R04, https://doi.org/10.1029/2011JD015938, 2011.
Frieß, U., Klein Baltink, H., Beirle, S., Clémer, K., Hendrick, F., Henzing, B., Irie, H., de Leeuw, G., Li, A., Moerman, M. M., van Roozendael, M., Shaiganfar, R., Wagner, T., Wang, Y., Xie, P., Yilmaz, S., and Zieger, P.: Intercomparison of aerosol extinction profiles retrieved from MAX-DOAS measurements, Atmos. Meas. Tech., 9, 3205–3222, https://doi.org/10.5194/amt-9-3205-2016, 2016.
Fu, G. Q., Xu, W. Y., Yang, R. F., Li, J. B., and Zhao, C. S.: The distribution and trends of fog and haze in the North China Plain over the past 30 years, Atmos. Chem. Phys., 14, 11949–11958, https://doi.org/10.5194/acp-14-11949-2014, 2014.
Guo, H., Jiang, F., Cheng, H. R., Simpson, I. J., Wang, X. M., Ding, A. J., Wang, T. J., Saunders, S. M., Wang, T., Lam, S. H. M., Blake, D. R., Zhang, Y. L., and Xie, M.: Concurrent observations of air pollutants at two sites in the Pearl River Delta and the implication of regional transport, Atmos. Chem. Phys., 9, 7343–7360, https://doi.org/10.5194/acp-9-7343-2009, 2009.
Han, K. M., Lee, S., Chang, L. S., and Song, C. H.: A comparison study between CMAQ-simulated and OMI-retrieved NO2 columns over East Asia for evaluation of NOx emission fluxes of INTEX-B, CAPSS, and REAS inventories, Atmos. Chem. Phys., 15, 1913–1938, https://doi.org/10.5194/acp-15-1913-2015, 2015.
Hassinen, S., Balis, D., Bauer, H., Begoin, M., Delcloo, A., Eleftheratos, K., Gimeno Garcia, S., Granville, J., Grossi, M., Hao, N., Hedelt, P., Hendrick, F., Hess, M., Heue, K.-P., Hovila, J., Jønch-Sørensen, H., Kalakoski, N., Kauppi, A., Kiemle, S., Kins, L., Koukouli, M. E., Kujanpää, J., Lambert, J.-C., Lang, R., Lerot, C., Loyola, D., Pedergnana, M., Pinardi, G., Romahn, F., van Roozendael, M., Lutz, R., De Smedt, I., Stammes, P., Steinbrecht, W., Tamminen, J., Theys, N., Tilstra, L. G., Tuinder, O. N. E., Valks, P., Zerefos, C., Zimmer, W., and Zyrichidou, I.: Overview of the O3M SAF GOME-2 operational atmospheric composition and UV radiation data products and data availability, Atmos. Meas. Tech., 9, 383–407, https://doi.org/10.5194/amt-9-383-2016, 2016.
Heckel, A., Kim, S.-W., Frost, G. J., Richter, A., Trainer, M., and Burrows, J. P.: Influence of low spatial resolution a priori data on tropospheric NO2 satellite retrievals, Atmos. Meas. Tech., 4, 1805–1820, https://doi.org/10.5194/amt-4-1805-2011, 2011.
Hendrick, F., Müller, J.-F., Clémer, K., Wang, P., De Mazière, M., Fayt, C., Gielen, C., Hermans, C., Ma, J. Z., Pinardi, G., Stavrakou, T., Vlemmix, T., and Van Roozendael, M.: Four years of ground-based MAX-DOAS observations of HONO and NO2 in the Beijing area, Atmos. Chem. Phys., 14, 765–781, https://doi.org/10.5194/acp-14-765-2014, 2014.
Herman, J., Cede, A., Spinei, E., Mount, G., Tzortziou, M., and Abuhassan, N.: NO2 column amounts from groundbased Pandora and MFDOAS spectrometers using the direct-sun DOAS technique: Intercomparisons and application to OMI validation, J. Geophys. Res., 114, D13307, https://doi.org/10.1029/2009JD011848, 2009.
Hilboll, A., Richter, A., and Burrows, J. P.: Long-term changes of tropospheric NO2 over megacities derived from multiple satellite instruments, Atmos. Chem. Phys., 13, 4145–4169, https://doi.org/10.5194/acp-13-4145-2013, 2013.
Hönninger, G., von Friedeburg, C., and Platt, U.: Multi axis differential optical absorption spectroscopy (MAX-DOAS), Atmos. Chem. Phys., 4, 231–254, https://doi.org/10.5194/acp-4-231-2004, 2004.
Huang, H., Ho, K., Lee, S., Tsang, P., Ho, S., Zou, C., Zou, S., Cao, J., and Xu, H.: Characteristics of carbonaceous aerosol in PM2.5: Pearl Delta River region, China, Atmos. Res., 104–105, 227–236, 2012.
Huang, R.-J., Zhang, Y., Bozzetti, C., Ho, K.-F., Cao, J., Han, Y., Dällenbach, K. R., Slowik, J. G., Platt, S. M., Canonaco, F., Zotter, P., Wolf, R., Pieber, S. M., Bruns, E. A., Crippa, M., Ciarelli, G., Piazzalunga, A., Schwikowski, M., Abbaszade, G., Schnelle-Kreis, J., Zimmermann, R., An, Z., Szidat, S., Baltensperger, U., Haddad, I. E., and Prévôt, A. S. H.: High secondary aerosol contribution to particulate pollution during haze events in China, Nature, 514, 218–222, 2014.
Irie, H., Kanaya, Y., Akimoto, H., Iwabuchi, H., Shimizu, A., and Aoki, K.: First retrieval of tropospheric aerosol profiles using MAX-DOAS and comparison with lidar and sky radiometer measurements, Atmos. Chem. Phys., 8, 341–350, https://doi.org/10.5194/acp-8-341-2008, 2008.
Irie, H., Takashima, H., Kanaya, Y., Boersma, K. F., Gast, L., Wittrock, F., Brunner, D., Zhou, Y., and Van Roozendael, M.: Eight-component retrievals from ground-based MAX-DOAS observations, Atmos. Meas. Tech., 4, 1027–1044, https://doi.org/10.5194/amt-4-1027-2011, 2011.
Irie, H., Boersma, K. F., Kanaya, Y., Takashima, H., Pan, X., and Wang, Z. F.: Quantitative bias estimates for tropospheric NO2 columns retrieved from SCIAMACHY, OMI, and GOME-2 using a common standard for East Asia, Atmos. Meas. Tech., 5, 2403–2411, https://doi.org/10.5194/amt-5-2403-2012, 2012.
Jiang, C., Wang, H., Zhao, T., Li, T., and Che, H.: Modeling study of PM2.5 pollutant transport across cities in China's Jing-Jin-Ji region during a severe haze episode in December 2013, Atmos. Chem. Phys., 15, 5803–5814, https://doi.org/10.5194/acp-15-5803-2015, 2015.
Jin, J., Ma, J., Lin, W., Zhao, H., Shaiganfar, R., Beirle, S., and Wagner, T.: MAX-DOAS measurements and satellite validation of tropospheric NO2 and SO2 vertical column densities at a rural site of North China, Atmos. Environ, 133, 12–25, https://doi.org/10.1016/j.atmosenv.2016.03.031, 2016.
Kouremeti, N., Bais, A. F., Balis, D., and Zyrichidou, I., and Phaethon, A.: System for the Validation of Satellite Derived Atmospheric Columns of Trace Gases, in: Advances in Meteorology, Climatology and Atmospheric Physics, edited by: Helmis, C. G. and Nastos, P. T., 1081–1088, Springer Berlin Heidelberg, https://doi.org/10.1007/978-3-642-29172-2_151, 2013.
Kramer, L. J., Leigh, R. J., Remedios, J. J., and Monks, P. S.: Comparison of OMI and ground-based in situ and MAX-DOAS measurements of tropospheric nitrogen dioxide in an urban area, J. Geophys. Res., 113, D16S39, https://doi.org/10.1029/2007JD009168, 2008.
Leitão, J., Richter, A., Vrekoussis, M., Kokhanovsky, A., Zhang, Q. J., Beekmann, M., and Burrows, J. P.: On the improvement of NO2 satellite retrievals – aerosol impact on the airmass factors, Atmos. Meas. Tech., 3, 475–493, https://doi.org/10.5194/amt-3-475-2010, 2010.
Levelt, P., Joiner, J., Tamminen, J., Veefkind, P., Bhartia, P. K., Stein Zweers, D., Duncan, B. N., Streets, D. G., Eskes, H., van der A, R., McLinden, C., Fioletov, V., Carn, S., de Laat, J., DeLand, M., Marchenko, S., McPeters, R., Ziemke, J., Fu, D., Liu, X., Pickering, K., Apituley, A., Gonzáles Abad, G., Arola, A., Boersma, F., Chan Miller, C., Chance, K., de Graaf, M., Hakkarainen, J., Hassinen, S., Ialongo, I., Kleipool, Q., Krotkov, N., Li, C., Lamsal, L., Newman, P., Nowlan, C., Suileiman, R., Tilstra, L. G., Torres, O., Wang, H., and Wargan, K.: The Ozone Monitoring Instrument: Overview of twelve years in space, Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2017-487, in review, 2017.
Levelt P. F., van den Oord, G. H. J., Dobber, M. R., Malkki, A., Visser, H., de Vries, J., Stammes, P., Lundell, J. O. V., and Saari, H.: The Ozone Monitoring Instrument, IEEE T. Geosci. Remote, 44, 1093–1101, 2006.
Li, X., Brauers, T., Hofzumahaus, A., Lu, K., Li, Y. P., Shao, M., Wagner, T., and Wahner, A.: MAX-DOAS measurements of NO2, HCHO and CHOCHO at a rural site in Southern China, Atmos. Chem. Phys., 13, 2133–2151, https://doi.org/10.5194/acp-13-2133-2013, 2013.
Li, Z., Chen, H., Cribb, M., Dickerson, R., Holben, B., Li, C., Lu, D., Luo, Y., Maring, H., and Shi, G.: Preface to special section on East Asian Studies of Tropospheric Aerosols: An International Regional Experiment (EAST-AIRE), J. Geophys. Res., 112, D22S00, https://doi.org/10.1029/2007JD008479, 2007.
Lin, J.-T., Martin, R. V., Boersma, K. F., Sneep, M., Stammes, P., Spurr, R., Wang, P., Van Roozendael, M., Clémer, K., and Irie, H.: Retrieving tropospheric nitrogen dioxide from the Ozone Monitoring Instrument: effects of aerosols, surface reflectance anisotropy, and vertical profile of nitrogen dioxide, Atmos. Chem. Phys., 14, 1441–1461, https://doi.org/10.5194/acp-14-1441-2014, 2014.
Lin, J.-T., Liu, M.-Y., Xin, J.-Y., Boersma, K. F., Spurr, R., Martin, R., and Zhang, Q.: Influence of aerosols and surface reflectance on satellite NO2 retrieval: seasonal and spatial characteristics and implications for NOx emission constraints, Atmos. Chem. Phys., 15, 11217–11241, https://doi.org/10.5194/acp-15-11217-2015, 2015.
Liu, F., Beirle, S., Zhang, Q., van der A, R. J., Zheng, B., Tong, D., and He, K.: NOx emission trends over Chinese cities estimated from OMI observations during 2005 to 2015, Atmos. Chem. Phys., 17, 9261–9275, https://doi.org/10.5194/acp-17-9261-2017, 2017.
Liu, H., Wang, X., Zhang, J., He, K., Wu, Y., and Xu, J.: Emission controls and changes in air quality in Guangzhou during the Asian Games, Atmos. Environ., 76, 81–93, 2013.
Ma, J. Z., Beirle, S., Jin, J. L., Shaiganfar, R., Yan, P., and Wagner, T.: Tropospheric NO2 vertical column densities over Beijing: results of the first three years of ground-based MAX-DOAS measurements (2008–2011) and satellite validation, Atmos. Chem. Phys., 13, 1547–1567, https://doi.org/10.5194/acp-13-1547-2013, 2013.
Mayer, B. and Kylling, A.: Technical note: The libRadtran software package for radiative transfer calculations – description and examples of use, Atmos. Chem. Phys., 5, 1855–1877, https://doi.org/10.5194/acp-5-1855-2005, 2005.
Mebust, A. K. and Cohen, R. C.: Space-based observations of fire NOx emission coefficients: a global biome-scale comparison, Atmos. Chem. Phys., 14, 2509–2524, https://doi.org/10.5194/acp-14-2509-2014, 2014.
Munro, R., Lang, R., Klaes, D., Poli, G., Retscher, C., Lindstrot, R., Huckle, R., Lacan, A., Grzegorski, M., Holdak, A., Kokhanovsky, A., Livschitz, J., and Eisinger, M.: The GOME-2 instrument on the Metop series of satellites: instrument design, calibration, and level 1 data processing – an overview, Atmos. Meas. Tech., 9, 1279–1301, https://doi.org/10.5194/amt-9-1279-2016, 2016.
Olivier, J. G. J. and Berdowski, J. J. M.: Global emissions sources and sinks, in: The Climate System, edited by: Berdowski, J., Guicherit, R., and Heij, B. J., A.A. Balkema Publishers/Swets & Zeitlinger Publishers, Lisse, The Netherlands, ISBN: 90 5809 255 0, 33–78, 2001.
Ozone Monitoring Instrument (OMI): Data User's Guide, available at: https://docserver.gesdisc.eosdis.nasa.gov/repository/Mission/OMI/3.3_ScienceDataProductDocumentation/3.3.2_ProductRequirements_Designs/README.OMI_DUG.pdf (last access: 16 April 2018), 2012.
Platt, U.: Differential optical absorption spectroscopy (DOAS), in Air Monitoring by Spectroscopic Techniques, Chem. Anal. Ser., John Wiley, New York, 127, 27–84, 1994.
Platt, U. and Stutz, J.: Differential Optical Absorption Spectroscopy, Principles and Applications, Springer, Physics of Earth and Space Environments, ISBN: 978-3-540-21193-8, 2008.
Qin, M., Xie, P., Su, H., Gu, J., Peng, F., Li, S., Zeng, L., Liu, J., Liu, W., and Zhang, Y.: An observational study of the HONO-NO2 coupling at an urban site in Guangzhou City, South China, Atmos. Environ., 43, 5731–5742, https://doi.org/10.1016/j.atmosenv.2009.08.017, 2009.
Richter, A., Burrows, J. P., Nüß, H., Granier, C., and Niemeier, U.: Increase in tropospheric nitrogen dioxide over China observed from space, Nature, 437, 129–132, 2005.
Rothman, L. S., Gordon, I. E., Barber, R. J., Dothe, H., Gamache, R. R., Goldman, A., Perevalov, V., Tashkun, S. A., and Tennyson, J.: HITEMP, the high temperature molecular spectroscopic database, J. Quant. Spectrosc. Ra., 111, 2139–2150, 2010.
Schneider, P. and van der A, R. J.: A global single-sensor analysis of 2002–2011 tropospheric nitrogen dioxide trends observed from space, J. Geophys. Res., 117, 1–17, https://doi.org/10.1029/2012JD017571, 2012.
Schumann, U. and Huntrieser, H.: The global lightning-induced nitrogen oxides source, Atmos. Chem. Phys., 7, 3823–3907, https://doi.org/10.5194/acp-7-3823-2007, 2007.
Seinfeld, J. H. and Pandis, S. N.: Atmospheric Chemistry and Physics: From Air Pollution to Climate Change, J. Wiley, New York, 1998.
Serdyuchenko, A., Gorshelev, V., Weber, M., Chehade, W., and Burrows, J. P.: High spectral resolution ozone absorption cross-sections – Part 2: Temperature dependence, Atmos. Meas. Tech., 7, 625–636, https://doi.org/10.5194/amt-7-625-2014, 2014.
Shao, M., Zhang, Y., Zeng, L., Tang, X., Zhang, J., Zhong, L., and Wang, B.: Ground-level ozone in the Pearl River Delta and the roles of VOC and NOx in its production, J. Environ. Manage., 90, 512–518, 2009.
Solomon, S., Portmann, R. W., Sanders, R. W., Daniel, J. S., Madsen, W., Bartram, B., and Dutton E. G: On the role of nitrogen dioxide in the absorption of solar radiation, J. Geophys. Res., 104, 12047–12058, 1999.
Thalman, R. and Volkamer, R.: Temperature dependent absorption cross-sections of O2-O2 collision pairs between 340 and 630 nm and at atmospherically relevant pressure, Phys. Chem. Chem. Phys., 15, 15371, https://doi.org/10.1039/c3cp50968k, 2013.
Theys, N., De Smedt, I., Gent, J., Danckaert, T., Wang, T., Hendrick, F., Stavrakou, T., Bauduin, S., Clarisse, L., Li, C., Krotkov, N., Yu, H., Brenot, H., and Van Roozendael, M.: Sulfur dioxide vertical column DOAS retrievals from the Ozone Monitoring Instrument: Global observations and comparison to ground-based and satellite data, J. Geophys. Res.-Atmos., 120, 2470–2491, 2015.
Vandaele A. C., Hermans, C., Simon, P. C., Carleer, M., Colins, R., Fally, S., Mérienne, M. F., Jenouvrier, A., and Coquart, B.: Measurements of the NO2 absorption cross-sections from 42000 cm−1 to 10000 cm−1 (238–1000 nm) at 220 K and 294 K, J. Quant. Spectrosc. Ra., 59, 171–184, 1998.
van der A, R. J., Mijling, B., Ding, J., Koukouli, M. E., Liu, F., Li, Q., Mao, H., and Theys, N.: Cleaning up the air: effectiveness of air quality policy for SO2 and NOx emissions in China, Atmos. Chem. Phys., 17, 1775–1789, https://doi.org/10.5194/acp-17-1775-2017, 2017.
Van Roozendael, M., Fayt, C., Post, P., Hermans, C., and Lambert, J.-C.: Retrieval of BrO and NO2 from UV-Visible Observations, in: Sounding the troposphere from space: a new Era for Atmospheric Chemistry, The TROPOSAT Final Report, edited by: Borrell, P., Borrell, P. M., Burrows, J. P., and Platt, U., Springer Verlag, Berlin, Heidelberg, 155–166, 2003.
Velders, G. J. M., Granier, C., Portmann, R. W., Pfeilsticker, K., Wenig, M., Wagner, T., Platt, U., Richter, A., and Burrows, J. P.: Global tropospheric NO2 column distributions: Comparing 3-D model calculations with GOME measurements, J. Geophys. Res., 106, 12643–12660, 2001.
Vinken, G. C. M., Boersma, K. F., Maasakkers, J. D., Adon, M., and Martin, R. V.: Worldwide biogenic soil NOx emissions inferred from OMI NO2 observations, Atmos. Chem. Phys., 14, 10363–10381, https://doi.org/10.5194/acp-14-10363-2014, 2014.
Wang, J., Wang, C., Lai, C., Chang, C., Zhang, Y., Liu, S., and Shao, M.: Characterization of ozone precursors in the Pearl River Delta by time series observation of non-methane hydrocarbons, Atmos. Environ., 42, 6233–6246, https://doi.org/10.1016/j.atmosenv.2008.01.050, 2008.
Wang, X., Carmichael, G., Chen, D., Tang, Y., and Wang, T.: Impacts of different emission sources on air quality during March 2001 in the Pearl River Delta (PRD) region, Atmos. Environ, 39, 5227–5241, https://doi.org/10.1016/j.atmosenv.2005.04.035, 2005.
Wang, Y., Lampel, J., Xie, P., Beirle, S., Li, A., Wu, D., and Wagner, T.: Ground-based MAX–DOAS observations of tropospheric aerosols, NO2, SO2 and HCHO in Wuxi, China, from 2011 to 2014, Atmos. Chem. Phys., 17, 2189–2215, https://doi.org/10.5194/acp-17-2189-2017, 2017a.
Wang, Y., Beirle, S., Lampel, J., Koukouli, M., De Smedt, I., Theys, N., Li, A., Wu, D., Xie, P., Liu, C., Van Roozendael, M., Stavrakou, T., Müller, J.-F., and Wagner, T.: Validation of OMI, GOME-2A and GOME-2B tropospheric NO2, SO2 and HCHO products using MAX-DOAS observations from 2011 to 2014 in Wuxi, China: investigation of the effects of priori profiles and aerosols on the satellite products, Atmos. Chem. Phys., 17, 5007–5033, https://doi.org/10.5194/acp-17-5007-2017, 2017b.
Wagner, T., Dix, B., Friedeburg, C. C., Frieß, U., Sanghavi, S., Sinreich, R., and Platt, U.: MAX-DOAS O4 measurements: A new technique to derive information on atmospheric aerosols – Principles and information content, J. Geophys. Res., 109, D22205, https://doi.org/10.1029/2004JD004904, 2004.
Wagner, T., Beirle, S., Brauers, T., Deutschmann, T., Frieß, U., Hak, C., Halla, J. D., Heue, K. P., Junkermann, W., Li, X., Platt, U., and Pundt-Gruber, I.: Inversion of tropospheric profiles of aerosol extinction and HCHO and NO2 mixing ratios from MAX-DOAS observations in Milano during the summer of 2003 and comparison with independent data sets, Atmos. Meas. Tech., 4, 2685–2715, https://doi.org/10.5194/amt-4-2685-2011, 2011.
Webb, A. R., Stromberg, I. M., Li, H., and Bartlett, L. M.: Airborne spectral measurements of surface reflectivity at ultraviolet and visible wavelengths, J. Geophys. Res., 105, 4945–4948, 2000.
WHO: Review of evidence on health aspects of air pollution – REVIHAAP Project, Technical Report, World Health Organization, Regional Office for Europe, Copenhagen, Denmark, 2013.
Wittrock, F., Oetjen, H., Richter, A., Fietkau, S., Medeke, T., Rozanov, A., and Burrows, J. P.: MAX-DOAS measurements of atmospheric trace gases in Ny-Ålesund – Radiative transfer studies and their application, Atmos. Chem. Phys., 4, 955–966, https://doi.org/10.5194/acp-4-955-2004, 2004.
Wu, F. C., Xie, P. H., Li, A., Chan, K. L., Hartl, A., Wang, Y., Si, F. Q., Zeng, Y., Qin, M., Xu, J., Liu, J. G., Liu, W. Q., and Wenig, M.: Observations of SO2 and NO2 by mobile DOAS in the Guangzhou eastern area during the Asian Games 2010, Atmos. Meas. Tech., 6, 2277–2292, https://doi.org/10.5194/amt-6-2277-2013, 2013.
Xia, X., Li, Z., Holben, B., Wang, P., Eck, T., Chen, H., Cribb, M., and Zhao, Y.: Aerosol optical properties and radiative effects in the Yangtze Delta region of China, J. Geophys. Res., 112, D22S12, https://doi.org/10.1029/2007JD008859, 2007.
Zhang, Q., Streets, D. G., He, K., Wang, Y., Richter, A., Burrows, J. P., Uno, I., Jang, C. J., Chen, D., Yao, Z., and Lei, Y.: NOx emission trends for China, 1995–2004: The view from the ground and the view from space, J. Geophys. Res., 112, D22306, https://doi.org/10.1029/2007JD008684, 2007.
Zhou, K., Ye, Y., Liu, Q., Liu, A., and Peng, S.: Evaluation of ambient air quality in Guangzhou, China, J. Environ. Sci., 19, 432–437, 2007.
Zyrichidou, I., Koukouli, M. E., Balis, D. S., Katragkou, E., Melas, D., Poupkou, A., Kioutsioukis, I., van der A, R., Boersma, F. K., van Roozendael, M., and Richter, A.: Satellite observations and model simulations of tropospheric NO2 columns over south-eastern Europe, Atmos. Chem. Phys., 9, 6119–6134, https://doi.org/10.5194/acp-9-6119-2009, 2009.
Short summary
A diurnal pattern of tropospheric NO2 with two maxima around late morning and late afternoon is revealed, reflecting high anthropogenic emissions, and a minimum at noon, due to photochemical destruction of tropospheric NO2. GOME-2B shows the smallest underestimation despite its large pixel size. The distance between the measurement location and the satellite pixel center affects mostly GOME-2B data selection. The effect of clouds is more profound on the selection of OMI overpass data.
A diurnal pattern of tropospheric NO2 with two maxima around late morning and late afternoon is...