Articles | Volume 14, issue 5
https://doi.org/10.5194/amt-14-3953-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/amt-14-3953-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
28 May 2021
Research article |
| 28 May 2021
| 28 May 2021
Systematic comparison of vectorial spherical radiative transfer models in limb scattering geometry
Daniel Zawada
CORRESPONDING AUTHOR
Institute of Space and Atmospheric Studies, University of Saskatchewan, Saskatchewan, Canada
Ghislain Franssens
Royal Belgian Institute for Space Aeronomy, Brussels, Belgium
Robert Loughman
Department of Atmospheric and Planetary Sciences, Hampton University, Hampton, Virginia, USA
Antti Mikkonen
Finnish Meteorological Institute, Helsinki, Finland
Alexei Rozanov
Institute of Environmental Physics, University of Bremen, Bremen, Germany
Claudia Emde
Meteorological Institute, Ludwig-Maximilians-Universität, Munich, Germany
Adam Bourassa
Institute of Space and Atmospheric Studies, University of Saskatchewan, Saskatchewan, Canada
Seth Dueck
Institute of Space and Atmospheric Studies, University of Saskatchewan, Saskatchewan, Canada
Hannakaisa Lindqvist
Finnish Meteorological Institute, Helsinki, Finland
Didier Ramon
HYGEOS, Lille, France
Vladimir Rozanov
Institute of Environmental Physics, University of Bremen, Bremen, Germany
Emmanuel Dekemper
Royal Belgian Institute for Space Aeronomy, Brussels, Belgium
Erkki Kyrölä
Finnish Meteorological Institute, Helsinki, Finland
John P. Burrows
Institute of Environmental Physics, University of Bremen, Bremen, Germany
Didier Fussen
Royal Belgian Institute for Space Aeronomy, Brussels, Belgium
Doug Degenstein
Institute of Space and Atmospheric Studies, University of Saskatchewan, Saskatchewan, Canada
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Linlu Mei, Vladimir Rozanov, Alexei Rozanov, and John P. Burrows
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Phuc Thi Minh Ha, Yugo Kanaya, Kazuyo Yamaji, Syuichi Itahashi, Satoru Chatani, Takashi Sekiya, Maria Dolores Andrés Hernández, John Philip Burrows, Hans Schlager, Michael Lichtenstern, Mira Poehlker, and Bruna Holanda
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Antti Kukkurainen, Antti Mikkonen, Antti Arola, Antti Lipponen, Ville Kolehmainen, and Neus Sabater
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Zhihong Zhuo, Xinyue Wang, Yunqian Zhu, Wandi Yu, Ewa M. Bednarz, Eric Fleming, Peter R. Colarco, Shingo Watanabe, David Plummer, Georgiy Stenchikov, William Randel, Adam Bourassa, Valentina Aquila, Takashi Sekiya, Mark R. Schoeberl, Simone Tilmes, Jun Zhang, Paul J. Kushner, and Francesco S. R. Pausata
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The 2022 Hunga eruption caused unprecedented stratospheric water injection, triggering unique atmospheric impacts. This study combines observations and model simulations, projecting a stratospheric water vapor anomaly lasting 4–7 years, with significant temperature variations and ozone depletion in the upper atmosphere lasting 7–10 years. These findings offer critical insights into the role of stratospheric water vapor in shaping climate and atmospheric chemistry.
Rolf Müller, Lennart Bengtsson, John Birks, John Burrows, Ruprecht Jaenicke, and Richard S. Stolarski
Hist. Geo Space. Sci., 16, 31–40, https://doi.org/10.5194/hgss-16-31-2025, https://doi.org/10.5194/hgss-16-31-2025, 2025
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This paper reports a few anecdotes from the life of Paul J. Crutzen that were contributed by friends and colleagues. Taken together, these anecdotes should shed some light on the person that Paul was, as this is perhaps sometimes obscured when focusing solely on his many scientific achievements.
Ella Kivimäki, Maria Tenkanen, Tuula Aalto, Michael Buchwitz, Kari Luojus, Jouni Pulliainen, Kimmo Rautiainen, Oliver Schneising, Anu-Maija Sundström, Johanna Tamminen, Aki Tsuruta, and Hannakaisa Lindqvist
Biogeosciences, 22, 5193–5230, https://doi.org/10.5194/bg-22-5193-2025, https://doi.org/10.5194/bg-22-5193-2025, 2025
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We study how environmental variables influencing natural methane fluxes explain the seasonal variability in satellite-observed methane in Northern Hemisphere high-latitude wetland areas. Using two atmospheric model set-ups, we assess consistency with satellite data. Methane loss through reaction with hydroxyl radicals and links with snow cover, temperature, and snowmelt had the strongest influence. Our study highlights the value of satellite observations for understanding large-scale wetland emissions.
Meghan Brehon, Susann Tegtmeier, Adam Bourassa, Sean M. Davis, Udo Grabowski, Tobias Kerzenmacher, and Gabriele Stiller
EGUsphere, https://doi.org/10.5194/egusphere-2025-4457, https://doi.org/10.5194/egusphere-2025-4457, 2025
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We used satellite-based water vapour data to estimate vertical transport rates in the tropical stratosphere for 1995 to 2020. These estimates were compared with other upwelling datasets and used to analyze stratospheric variability. Our results find good agreement between the datasets and reveal that variability in upwelling is mainly driven by known climate patterns like the QBO and ENSO with a clear signal in the upwelling time series coinciding with the QBO disruptions of 2015/16 and 2019/20.
Anna Lange, Ulrike Niemeier, Alexei Rozanov, and Christian von Savigny
Atmos. Chem. Phys., 25, 11673–11688, https://doi.org/10.5194/acp-25-11673-2025, https://doi.org/10.5194/acp-25-11673-2025, 2025
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Our paper investigates whether it is possible to observe continuous injections of 1 and 2 Tg S y-1 (sulfur per year) into the stratosphere with the currently active satellite occultation instruments. The calculations show that, considering the natural variability and the assumptions made here, the stratospheric aerosols formed from continuous emissions of 1 and 2 Tg S y-1 in the quasi-steady-state phase can be detected, which is not the case in the first month of the 2-year initial phase.
Tea Thum, Javier Pacheco-Labrador, Mika Aurela, Alan Barr, Marika Honkanen, Bruce Johnson, Hannakaisa Lindqvist, Troy Magney, Mirco Migliavacca, Zoe Amie Pierrat, Tristan Quaife, Jochen Stutz, and Sönke Zaehle
EGUsphere, https://doi.org/10.5194/egusphere-2025-4432, https://doi.org/10.5194/egusphere-2025-4432, 2025
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Solar-induced chlorophyll fluorescence (SIF) is an optical signal emitted by plants, connected to the biochemical status of the plants. Therefore it helps to unveil what happens inside plants and since it can be observed with remote sensing, it provides a global view of plant activity. We included SIF module in a terrestrial biosphere model and examined how to best describe movement of the SIF signal in the forest. Our work will help to model SIF in boreal coniferous forests.
Viktoria F. Sofieva, Alexandra Laeng, Thomas von Clarmann, Gabriele Stiller, Michael Kiefer, Johanna Tamminen, Alexey Rozanov, Carlo Arosio, Nathaniel Livesey, Robert Damadeo, Patrick Sheese, Kaley A. Walker, Doug Degenstein, Daniel Zawada, Natalya A. Kramarova, and Arno Keppens
EGUsphere, https://doi.org/10.5194/egusphere-2025-2830, https://doi.org/10.5194/egusphere-2025-2830, 2025
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For satellite measurements of atmospheric composition, the random uncertainty estimates provided by retrieval algorithms might be imperfect due to various approximations used in the retrievals or presence of unknown error sources. This paper presents an overview of the methods used for validation of random uncertainty estimates. All methods discussed in this study are categorized, and assumptions and limitations of each method are discussed.
Björn Linder, Jörg Gumbel, Donal P. Murtagh, Linda Megner, Lukas Krasauskas, Doug Degenstein, Ole Martin Christensen, and Nickolay Ivchenko
Atmos. Meas. Tech., 18, 4453–4466, https://doi.org/10.5194/amt-18-4453-2025, https://doi.org/10.5194/amt-18-4453-2025, 2025
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In this study, the primary instrument carried by the satellite MATS is compared to the OSIRIS instrument on board the Odin satellite. A total of 36 close approaches between December 2022 and February 2023 were identified and analysed. The comparison reveals that the two instruments have good structural agreement and that MATS detects a signal that is ~20 % stronger than what is measured by OSIRIS.
Miriam Latsch, Andreas Richter, John P. Burrows, and Hartmut Bösch
Atmos. Meas. Tech., 18, 4373–4395, https://doi.org/10.5194/amt-18-4373-2025, https://doi.org/10.5194/amt-18-4373-2025, 2025
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This study presents our advanced methods to qualitatively detect ship-related nitrogen dioxide (NO2) signals in TROPOMI satellite data. By applying filtering techniques, we identify numerous global shipping routes, including previously undetected ones, as well as emissions from offshore platforms. Additionally, we compare the filtered satellite data with high-pass-filtered CAMS global model data to estimate the differences between observed and modeled NO2 emissions.
Gloria Klein, Xavier Ceamanos, Jérôme Vidot, Didier Ramon, and Mustapha Moulana
EGUsphere, https://doi.org/10.5194/egusphere-2025-3263, https://doi.org/10.5194/egusphere-2025-3263, 2025
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This work investigates the impact of the Earth's sphericity on geostationary satellite observations, particularly in the context of the operational estimation of aerosol and land surface properties from the Meteosat Third Generation-Imager's Flexible Combined Imager. We demonstrate that the plane-parallel approximation widely used in fast radiative transfer codes can introduce significant biases in certain situations, mainly depending on the observing geometry and wavelength.
Oke Huhs, Jakob Borchardt, Sven Krautwurst, Konstantin Gerilowski, Heinrich Bovensmann, Hartmut Bösch, and John Philip Burrows
EGUsphere, https://doi.org/10.5194/egusphere-2025-2953, https://doi.org/10.5194/egusphere-2025-2953, 2025
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Stray light is an error source in all optical instruments. In passive remote sensing observations of greenhouse gases, it creates false patterns in gas concentration maps. In this work, a post-flight stray light correction for MAMAP2D-Light is developed, improving the full processing chain from measured spectra, retrieved concentration maps, to emission rate estimates using real and simulated data. Additionally, a hardware improvement mitigates stray light for onward missions.
Michael Weimer, Michael Hilker, Stefan Noël, Max Reuter, Michael Buchwitz, Blanca Fuentes Andrade, Rüdiger Lang, Bernd Sierk, Yasjka Meijer, Heinrich Bovensmann, John P. Burrows, and Hartmut Bösch
Atmos. Meas. Tech., 18, 3321–3340, https://doi.org/10.5194/amt-18-3321-2025, https://doi.org/10.5194/amt-18-3321-2025, 2025
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Optical detectors have a maximum signal (saturation). Exceedance means that the measurement has to be discarded. We investigate where saturation will occur for the future European satellite mission dedicated to CO2 monitoring (CO2M) and strategies to avoid saturation. Saturation impacts coverage and precision, both of which are important for estimation of local CO2 emissions. We find that taking two pictures per sampling should be sufficient to avoid saturation for CO2M, with some impact on CO2 precision.
Carlo Arosio, Viktoria Sofieva, Andrea Orfanoz-Cheuquelaf, Alexei Rozanov, Klaus-Peter Heue, Diego Loyola, Edward Malina, Ryan M. Stauffer, David Tarasick, Roeland Van Malderen, Jerry R. Ziemke, and Mark Weber
Atmos. Meas. Tech., 18, 3247–3265, https://doi.org/10.5194/amt-18-3247-2025, https://doi.org/10.5194/amt-18-3247-2025, 2025
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Tropospheric ozone affects air quality and climate, being a pollutant and a greenhouse gas. We analyze satellite data of tropospheric ozone columns obtained by combining two types of observations: one providing stratospheric and the other total ozone. We compare common climatological features and study the influence of the tropopause (troposphere to stratosphere boundary) on the results. We also examine trends over the last 20 years and compare satellite data with ozonesondes to identify drifts.
Clair Duchamp, Bernard Legras, Aurélien Podglajen, Pasquale Sellitto, Adam E. Bourassa, Alexei Rozanov, Ghassan Taha, and Daniel J. Zawada
EGUsphere, https://doi.org/10.5194/egusphere-2025-3355, https://doi.org/10.5194/egusphere-2025-3355, 2025
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We analyzed the stratospheric aerosol plume from the 2022 Hunga eruption using satellite lidar data. We implemented a method to retrieve some aerosol properties, as standard products failed in this case. We found very high optical depth values in the days following the eruption, which decreased rapidly but remained elevated for months. Our results are broadly validated, though some satellite products underestimate the values due, in part, to the unusual aerosol size distribution in the plume.
Wolfgang Knorr, Matthew Williams, Tea Thum, Thomas Kaminski, Michael Voßbeck, Marko Scholze, Tristan Quaife, T. Luke Smallman, Susan C. Steele-Dunne, Mariette Vreugdenhil, Tim Green, Sönke Zaehle, Mika Aurela, Alexandre Bouvet, Emanuel Bueechi, Wouter Dorigo, Tarek S. El-Madany, Mirco Migliavacca, Marika Honkanen, Yann H. Kerr, Anna Kontu, Juha Lemmetyinen, Hannakaisa Lindqvist, Arnaud Mialon, Tuuli Miinalainen, Gaétan Pique, Amanda Ojasalo, Shaun Quegan, Peter J. Rayner, Pablo Reyes-Muñoz, Nemesio Rodríguez-Fernández, Mike Schwank, Jochem Verrelst, Songyan Zhu, Dirk Schüttemeyer, and Matthias Drusch
Geosci. Model Dev., 18, 2137–2159, https://doi.org/10.5194/gmd-18-2137-2025, https://doi.org/10.5194/gmd-18-2137-2025, 2025
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When it comes to climate change, the land surface is where the vast majority of impacts happen. The task of monitoring those impacts across the globe is formidable and must necessarily rely on satellites – at a significant cost: the measurements are only indirect and require comprehensive physical understanding. We have created a comprehensive modelling system that we offer to the research community to explore how satellite data can be better exploited to help us capture the changes that happen on our lands.
Irina Petropavlovskikh, Jeannette D. Wild, Kari Abromitis, Peter Effertz, Koji Miyagawa, Lawrence E. Flynn, Eliane Maillard Barras, Robert Damadeo, Glen McConville, Bryan Johnson, Patrick Cullis, Sophie Godin-Beekmann, Gerard Ancellet, Richard Querel, Roeland Van Malderen, and Daniel Zawada
Atmos. Chem. Phys., 25, 2895–2936, https://doi.org/10.5194/acp-25-2895-2025, https://doi.org/10.5194/acp-25-2895-2025, 2025
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Observational records show that stratospheric ozone is recovering in accordance with the implementation of the Montreal Protocol and its amendments. Natural ozone variability complicates the detection of small trends. This study optimizes a statistical model fit in ground-station-based observational records by adding parameters that interpret seasonal and long-term changes in atmospheric circulation and airmass mixing, which reduces uncertainties in detecting the stratospheric ozone recovery.
Timo H. Virtanen, Anu-Maija Sundström, Elli Suhonen, Antti Lipponen, Antti Arola, Christopher O'Dell, Robert R. Nelson, and Hannakaisa Lindqvist
Atmos. Meas. Tech., 18, 929–952, https://doi.org/10.5194/amt-18-929-2025, https://doi.org/10.5194/amt-18-929-2025, 2025
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We find that small particles suspended in the air (aerosols) affect the satellite observations of carbon dioxide (CO2) made by the Orbiting Carbon Observatory-2 satellite instrument. Satellite estimates of CO2 appear to be too high for clean areas and too low for polluted areas. Our results show that CO2 and aerosols are often co-emitted, and this is partly masked out in the current retrievals. Correctly accounting for the aerosol effect is important for CO2 emission estimates by satellites.
Diego Santaren, Janne Hakkarainen, Gerrit Kuhlmann, Erik Koene, Frédéric Chevallier, Iolanda Ialongo, Hannakaisa Lindqvist, Janne Nurmela, Johanna Tamminen, Laia Amorós, Dominik Brunner, and Grégoire Broquet
Atmos. Meas. Tech., 18, 211–239, https://doi.org/10.5194/amt-18-211-2025, https://doi.org/10.5194/amt-18-211-2025, 2025
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This study evaluates data-driven inversion methods for estimating CO2 emissions from local sources, such as power plants and cities, using meteorological data and XCO2 and NO2 satellite images rather than atmospheric transport modeling. We assess and compare the performance of five different methods using simulations of 1 year of satellite images, taken from the upcoming Copernicus CO2 Monitoring Mission, covering 15 power plants and the city of Berlin, Germany.
Maximilian Reuter, Michael Hilker, Stefan Noël, Antonio Di Noia, Michael Weimer, Oliver Schneising, Michael Buchwitz, Heinrich Bovensmann, John P. Burrows, Hartmut Bösch, and Ruediger Lang
Atmos. Meas. Tech., 18, 241–264, https://doi.org/10.5194/amt-18-241-2025, https://doi.org/10.5194/amt-18-241-2025, 2025
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Carbon dioxide (CO2) and methane (CH4) are the main anthropogenic greenhouse gases. The European Copernicus CO2 monitoring satellite mission CO2M will provide measurements of their atmospheric concentrations, but the accuracy requirements are demanding and conventional retrieval methods computationally expensive. We present a new retrieval algorithm based on artificial neural networks that has the potential to meet the stringent requirements of the CO2M mission with minimal computational effort.
Seunghwan Seo, Si-Wan Kim, Kyoung-Min Kim, Andreas Richter, Kezia Lange, John P. Burrows, Junsung Park, Hyunkee Hong, Hanlim Lee, Ukkyo Jeong, Jung-Hun Woo, and Jhoon Kim
Atmos. Meas. Tech., 18, 115–128, https://doi.org/10.5194/amt-18-115-2025, https://doi.org/10.5194/amt-18-115-2025, 2025
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Over the Seoul metropolitan area, tropospheric NO2 vertical column densities from the Geostationary Environment Monitoring Spectrometer show distinct seasonal features. Also, varying a priori data have substantial impacts on the observed NO2 columns. The a priori data from different chemical transport models resulted in differences of up to −18.3 %. Notably, diurnal patterns of observed NO2 columns are similar for all datasets, although their a priori data exhibit contrasting diurnal patterns.
Claudia Emde, Veronika Pörtge, Mihail Manev, and Bernhard Mayer
Atmos. Meas. Tech., 17, 6769–6789, https://doi.org/10.5194/amt-17-6769-2024, https://doi.org/10.5194/amt-17-6769-2024, 2024
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We introduce an innovative method to retrieve the cloud fraction and optical thickness of liquid water clouds over the ocean based on polarimetry. This is well suited for satellite observations providing multi-angle polarization measurements. Cloud fraction and cloud optical thickness can be derived from measurements at two viewing angles: one within the cloudbow and one in the sun glint region.
Alexei Rozanov, Christine Pohl, Carlo Arosio, Adam Bourassa, Klaus Bramstedt, Elizaveta Malinina, Landon Rieger, and John P. Burrows
Atmos. Meas. Tech., 17, 6677–6695, https://doi.org/10.5194/amt-17-6677-2024, https://doi.org/10.5194/amt-17-6677-2024, 2024
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We developed a new algorithm to retrieve vertical distributions of aerosol extinction coefficients in the stratosphere. The algorithm is applied to measurements of scattered solar light from the spaceborne OMPS-LP (Ozone Mapper and Profiler Suite Limb Profiler) instrument. The retrieval results are compared to data from other spaceborne instruments and used to investigate the evolution of the aerosol plume following the eruption of the Hunga Tonga–Hunga Ha'apai volcano in January 2022.
Kimberlee Dubé, Susann Tegtmeier, Adam Bourassa, Daniel Zawada, Douglas Degenstein, William Randel, Sean Davis, Michael Schwartz, Nathaniel Livesey, and Anne Smith
Atmos. Chem. Phys., 24, 12925–12941, https://doi.org/10.5194/acp-24-12925-2024, https://doi.org/10.5194/acp-24-12925-2024, 2024
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Greenhouse gas emissions that warm the troposphere also result in stratospheric cooling. The cooling rate is difficult to quantify above 35 km due to a deficit of long-term observational data with high vertical resolution in this region. We use satellite observations from several instruments, including a new temperature product from OSIRIS, to show that the upper stratosphere, from 35–60 km, cooled by 0.5 to 1 K per decade over 2005–2021 and by 0.6 K per decade over 1979–2021.
Viktoria F. Sofieva, Alexei Rozanov, Monika Szelag, John P. Burrows, Christian Retscher, Robert Damadeo, Doug Degenstein, Landon A. Rieger, and Adam Bourassa
Earth Syst. Sci. Data, 16, 5227–5241, https://doi.org/10.5194/essd-16-5227-2024, https://doi.org/10.5194/essd-16-5227-2024, 2024
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Climate-related studies need information about the distribution of stratospheric aerosols, which influence the energy balance of the Earth’s atmosphere. In this work, we present a merged dataset of vertically resolved stratospheric aerosol extinction coefficients, which is derived from data of six limb and occultation satellite instruments. The created aerosol climate record covers the period from October 1984 to December 2023. It can be used in various climate-related studies.
Swathi Maratt Satheesan, Kai-Uwe Eichmann, John P. Burrows, Mark Weber, Ryan Stauffer, Anne M. Thompson, and Debra Kollonige
Atmos. Meas. Tech., 17, 6459–6484, https://doi.org/10.5194/amt-17-6459-2024, https://doi.org/10.5194/amt-17-6459-2024, 2024
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CHORA, an advanced cloud convective differential technique, enhances the accuracy of tropospheric-ozone retrievals. Unlike the traditional Pacific cloud reference sector scheme, CHORA introduces a local-cloud reference sector and an alternative approach (CLCT) for precision. Analysing monthly averaged TROPOMI data from 2018 to 2022 and validating with SHADOZ ozonesonde data, CLCT outperforms other methods and so is the preferred choice, especially in future geostationary satellite missions.
Kezia Lange, Andreas Richter, Tim Bösch, Bianca Zilker, Miriam Latsch, Lisa K. Behrens, Chisom M. Okafor, Hartmut Bösch, John P. Burrows, Alexis Merlaud, Gaia Pinardi, Caroline Fayt, Martina M. Friedrich, Ermioni Dimitropoulou, Michel Van Roozendael, Steffen Ziegler, Simona Ripperger-Lukosiunaite, Leon Kuhn, Bianca Lauster, Thomas Wagner, Hyunkee Hong, Donghee Kim, Lim-Seok Chang, Kangho Bae, Chang-Keun Song, Jong-Uk Park, and Hanlim Lee
Atmos. Meas. Tech., 17, 6315–6344, https://doi.org/10.5194/amt-17-6315-2024, https://doi.org/10.5194/amt-17-6315-2024, 2024
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Instruments for air quality observations on geostationary satellites provide multiple observations per day and allow for the analysis of the diurnal variation of important air pollutants such as nitrogen dioxide (NO2) over large areas. The South Korean instrument GEMS, launched in February 2020, is the first instrument in geostationary orbit and covers a large part of Asia. Our investigations show the observed diurnal evolution of NO2 at different measurement sites.
Giulia Roccetti, Luca Bugliaro, Felix Gödde, Claudia Emde, Ulrich Hamann, Mihail Manev, Michael Fritz Sterzik, and Cedric Wehrum
Atmos. Meas. Tech., 17, 6025–6046, https://doi.org/10.5194/amt-17-6025-2024, https://doi.org/10.5194/amt-17-6025-2024, 2024
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The amount of sunlight reflected by the Earth’s surface (albedo) is vital for the Earth's radiative system. While satellite instruments offer detailed spatial and temporal albedo maps, they only cover seven wavelength bands. We generate albedo maps that fully span the visible and near-infrared range using a machine learning algorithm. These maps reveal how the reflectivity of different land surfaces varies throughout the year. Our dataset enhances the understanding of the Earth's energy balance.
Steffen Vanselow, Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Heinrich Bovensmann, Hartmut Boesch, and John P. Burrows
Atmos. Chem. Phys., 24, 10441–10473, https://doi.org/10.5194/acp-24-10441-2024, https://doi.org/10.5194/acp-24-10441-2024, 2024
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We developed an algorithm to automatically detect persistent methane source regions, to quantify their emissions and to determine their source types, by analyzing TROPOMI data from 2018–2021. The over 200 globally detected natural and anthropogenic source regions include small-scale point sources such as individual coal mines and larger-scale source regions such as wetlands and large oil and gas fields.
Falco Monsees, Alexei Rozanov, John P. Burrows, Mark Weber, Annette Rinke, Ralf Jaiser, and Peter von der Gathen
Atmos. Chem. Phys., 24, 9085–9099, https://doi.org/10.5194/acp-24-9085-2024, https://doi.org/10.5194/acp-24-9085-2024, 2024
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Cyclones strongly influence weather predictability but still cannot be fully characterised in the Arctic because of the sparse coverage of meteorological measurements. A potential approach to compensate for this is the use of satellite measurements of ozone, because cyclones impact the tropopause and therefore also ozone. In this study we used this connection to investigate the correlation between ozone and the tropopause in the Arctic and to identify cyclones with satellite ozone observations.
Christine Pohl, Felix Wrana, Alexei Rozanov, Terry Deshler, Elizaveta Malinina, Christian von Savigny, Landon A. Rieger, Adam E. Bourassa, and John P. Burrows
Atmos. Meas. Tech., 17, 4153–4181, https://doi.org/10.5194/amt-17-4153-2024, https://doi.org/10.5194/amt-17-4153-2024, 2024
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Knowledge of stratospheric aerosol characteristics is important for understanding chemical and climate aerosol feedbacks. Two particle size distribution parameters, the aerosol extinction coefficient and the effective radius, are obtained from SCIAMACHY limb observations. The aerosol characteristics show good agreement with independent data sets from balloon-borne and satellite observations. This data set expands the limited knowledge of stratospheric aerosol characteristics.
Oliver Schneising, Michael Buchwitz, Maximilian Reuter, Michael Weimer, Heinrich Bovensmann, John P. Burrows, and Hartmut Bösch
Atmos. Chem. Phys., 24, 7609–7621, https://doi.org/10.5194/acp-24-7609-2024, https://doi.org/10.5194/acp-24-7609-2024, 2024
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Large quantities of CO and CO2 are emitted during conventional steel production. As satellite-based estimates of CO2 emissions at the facility level are challenging, co-emitted CO can indicate the carbon footprint of steel plants. We estimate CO emissions for German steelworks and use CO2 emissions from emissions trading data to derive a sector-specific CO/CO2 emission ratio for the steel industry; it is a prerequisite to use CO as a proxy for CO2 emissions from similar steel production sites.
Basudev Swain, Marco Vountas, Aishwarya Singh, Nidhi L. Anchan, Adrien Deroubaix, Luca Lelli, Yanick Ziegler, Sachin S. Gunthe, Hartmut Bösch, and John P. Burrows
Atmos. Chem. Phys., 24, 5671–5693, https://doi.org/10.5194/acp-24-5671-2024, https://doi.org/10.5194/acp-24-5671-2024, 2024
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Arctic amplification (AA) accelerates the warming of the central Arctic cryosphere and affects aerosol dynamics. Limited observations hinder a comprehensive analysis. This study uses AEROSNOW aerosol optical density (AOD) data and GEOS-Chem simulations to assess AOD variability. Discrepancies highlight the need for improved observational integration into models to refine our understanding of aerosol effects on cloud microphysics, ice nucleation, and radiative forcing under evolving AA.
Matthew S. Johnson, Alexei Rozanov, Mark Weber, Nora Mettig, John Sullivan, Michael J. Newchurch, Shi Kuang, Thierry Leblanc, Fernando Chouza, Timothy A. Berkoff, Guillaume Gronoff, Kevin B. Strawbridge, Raul J. Alvarez, Andrew O. Langford, Christoph J. Senff, Guillaume Kirgis, Brandi McCarty, and Larry Twigg
Atmos. Meas. Tech., 17, 2559–2582, https://doi.org/10.5194/amt-17-2559-2024, https://doi.org/10.5194/amt-17-2559-2024, 2024
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Monitoring tropospheric ozone (O3), a harmful pollutant negatively impacting human health, is primarily done using ground-based measurements and ozonesondes. However, these observation types lack the coverage to fully understand tropospheric O3. Satellites can retrieve tropospheric ozone with near-daily global coverage; however, they are known to have biases and errors. This study uses ground-based lidars to validate multiple satellites' ability to observe tropospheric O3.
Richard Maier, Fabian Jakub, Claudia Emde, Mihail Manev, Aiko Voigt, and Bernhard Mayer
Geosci. Model Dev., 17, 3357–3383, https://doi.org/10.5194/gmd-17-3357-2024, https://doi.org/10.5194/gmd-17-3357-2024, 2024
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Based on the TenStream solver, we present a new method to accelerate 3D radiative transfer towards the speed of currently used 1D solvers. Using a shallow-cumulus-cloud time series, we evaluate the performance of this new solver in terms of both speed and accuracy. Compared to a 3D benchmark simulation, we show that our new solver is able to determine much more accurate irradiances and heating rates than a 1D δ-Eddington solver, even when operated with a similar computational demand.
Ilias Fountoulakis, Alexandra Tsekeri, Stelios Kazadzis, Vassilis Amiridis, Angelos Nersesian, Maria Tsichla, Emmanouil Proestakis, Antonis Gkikas, Kyriakoula Papachristopoulou, Vasileios Barlakas, Claudia Emde, and Bernhard Mayer
Atmos. Chem. Phys., 24, 4915–4948, https://doi.org/10.5194/acp-24-4915-2024, https://doi.org/10.5194/acp-24-4915-2024, 2024
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In our study we provide an assessment, through a sensitivity study, of the limitations of models to calculate the dust direct radiative effect (DRE) due to the underrepresentation of its size, refractive index (RI), and shape. Our results indicate the necessity of including more realistic sizes and RIs for dust particles in dust models, in order to derive better estimations of the dust direct radiative effects.
Stefan Noël, Michael Buchwitz, Michael Hilker, Maximilian Reuter, Michael Weimer, Heinrich Bovensmann, John P. Burrows, Hartmut Bösch, and Ruediger Lang
Atmos. Meas. Tech., 17, 2317–2334, https://doi.org/10.5194/amt-17-2317-2024, https://doi.org/10.5194/amt-17-2317-2024, 2024
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FOCAL-CO2M is one of the three operational retrieval algorithms which will be used to derive XCO2 and XCH4 from measurements of the forthcoming European CO2M mission. We present results of applications of FOCAL-CO2M to simulated spectra, from which confidence is gained that the algorithm is able to fulfil the challenging requirements on systematic errors for the CO2M mission (spatio-temporal bias ≤ 0.5 ppm for XCO2 and ≤ 5 ppb for XCH4).
Daniel Zawada, Kimberlee Dubé, Taran Warnock, Adam Bourassa, Susann Tegtmeier, and Douglas Degenstein
Atmos. Meas. Tech., 17, 1995–2010, https://doi.org/10.5194/amt-17-1995-2024, https://doi.org/10.5194/amt-17-1995-2024, 2024
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There remain large uncertainties in long-term changes of stratospheric–atmospheric temperatures. We have produced a time series of more than 20 years of satellite-based temperature measurements from the OSIRIS instrument in the upper–middle stratosphere. The dataset is publicly available and intended to be used for a better understanding of changes in stratospheric temperatures.
Andrea Orfanoz-Cheuquelaf, Carlo Arosio, Alexei Rozanov, Mark Weber, Annette Ladstätter-Weißenmayer, John P. Burrows, Anne M. Thompson, Ryan M. Stauffer, and Debra E. Kollonige
Atmos. Meas. Tech., 17, 1791–1809, https://doi.org/10.5194/amt-17-1791-2024, https://doi.org/10.5194/amt-17-1791-2024, 2024
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Valuable information on the tropospheric ozone column (TrOC) can be obtained globally by combining space-borne limb and nadir measurements (limb–nadir matching, LNM). This study describes the retrieval of TrOC from the OMPS instrument (since 2012) using the LNM technique. The OMPS-LNM TrOC was compared with ozonesondes and other satellite measurements, showing a good agreement with a negative bias within 1 to 4 DU. This new dataset is suitable for pollution studies.
Adrien Deroubaix, Marco Vountas, Benjamin Gaubert, Maria Dolores Andrés Hernández, Stephan Borrmann, Guy Brasseur, Bruna Holanda, Yugo Kanaya, Katharina Kaiser, Flora Kluge, Ovid Oktavian Krüger, Inga Labuhn, Michael Lichtenstern, Klaus Pfeilsticker, Mira Pöhlker, Hans Schlager, Johannes Schneider, Guillaume Siour, Basudev Swain, Paolo Tuccella, Kameswara S. Vinjamuri, Mihalis Vrekoussis, Benjamin Weyland, and John P. Burrows
EGUsphere, https://doi.org/10.5194/egusphere-2024-516, https://doi.org/10.5194/egusphere-2024-516, 2024
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This study assesses atmospheric composition using air quality models during aircraft campaigns in Europe and Asia, focusing on carbonaceous aerosols and trace gases. While carbon monoxide is well modeled, other pollutants have moderate to weak agreement with observations. Wind speed modeling is reliable for identifying pollution plumes, where models tend to overestimate concentrations. This highlights challenges in accurately modeling aerosol and trace gas composition, particularly in cities.
Adrien Deroubaix, Marco Vountas, Benjamin Gaubert, Maria Dolores Andrés Hernández, Stephan Borrmann, Guy Brasseur, Bruna Holanda, Yugo Kanaya, Katharina Kaiser, Flora Kluge, Ovid Oktavian Krüger, Inga Labuhn, Michael Lichtenstern, Klaus Pfeilsticker, Mira Pöhlker, Hans Schlager, Johannes Schneider, Guillaume Siour, Basudev Swain, Paolo Tuccella, Kameswara S. Vinjamuri, Mihalis Vrekoussis, Benjamin Weyland, and John P. Burrows
EGUsphere, https://doi.org/10.5194/egusphere-2024-521, https://doi.org/10.5194/egusphere-2024-521, 2024
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This study explores the proportional relationships between carbonaceous aerosols (black and organic carbon) and trace gases using airborne measurements from two campaigns in Europe and East Asia. Differences between regions were found, but air quality models struggled to reproduce them accurately. We show that these proportional relationships can help to constrain models and can be used to infer aerosol concentrations from satellite observations of trace gases, especially in urban areas.
Christian von Savigny, Anna Lange, Christoph G. Hoffmann, and Alexei Rozanov
Atmos. Chem. Phys., 24, 2415–2422, https://doi.org/10.5194/acp-24-2415-2024, https://doi.org/10.5194/acp-24-2415-2024, 2024
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It is well known that volcanic eruptions strongly affect the colours of the twilight sky. Typically, volcanic eruptions lead to enhanced reddish and violet twilight colours. In rare cases, however, volcanic eruptions can also lead to green sunsets. This study provides an explanation for the occurrence of these unusual green sunsets based on simulations with a radiative transfer model. Green volcanic sunsets require a sufficient stratospheric aerosol optical depth and specific aerosol sizes.
Blanca Fuentes Andrade, Michael Buchwitz, Maximilian Reuter, Heinrich Bovensmann, Andreas Richter, Hartmut Boesch, and John P. Burrows
Atmos. Meas. Tech., 17, 1145–1173, https://doi.org/10.5194/amt-17-1145-2024, https://doi.org/10.5194/amt-17-1145-2024, 2024
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We developed a method to estimate CO2 emissions from localized sources, such as power plants, using satellite data and applied it to estimate CO2 emissions from the Bełchatów Power Station (Poland). As the detection of CO2 emission plumes from satellite data is difficult, we used observations of co-emitted NO2 to constrain the emission plume region. Our results agree with CO2 emission estimations based on the power-plant-generated power and emission factors.
Basudev Swain, Marco Vountas, Adrien Deroubaix, Luca Lelli, Yanick Ziegler, Soheila Jafariserajehlou, Sachin S. Gunthe, Andreas Herber, Christoph Ritter, Hartmut Bösch, and John P. Burrows
Atmos. Meas. Tech., 17, 359–375, https://doi.org/10.5194/amt-17-359-2024, https://doi.org/10.5194/amt-17-359-2024, 2024
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Aerosols are suspensions of particles dispersed in the air. In this study, we use a novel retrieval of satellite data to investigate an optical property of aerosols, the aerosol optical depth, in the high Arctic to assess their direct and indirect roles in climate change. This study demonstrates that the presented approach shows good quality and very promising potential.
Jonas Hachmeister, Oliver Schneising, Michael Buchwitz, John P. Burrows, Justus Notholt, and Matthias Buschmann
Atmos. Chem. Phys., 24, 577–595, https://doi.org/10.5194/acp-24-577-2024, https://doi.org/10.5194/acp-24-577-2024, 2024
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We quantified changes in atmospheric methane concentrations using satellite data and a dynamic linear model approach. We calculated global annual methane increases for the years 2019–2022, which are in good agreement with other sources. For zonal methane growth rates, we identified strong inter-hemispheric differences in 2019 and 2022. For 2022, we could attribute decreases in the global growth rate to the Northern Hemisphere, possibly related to a reduction in anthropogenic emissions.
Lukas Fehr, Chris McLinden, Debora Griffin, Daniel Zawada, Doug Degenstein, and Adam Bourassa
Geosci. Model Dev., 16, 7491–7507, https://doi.org/10.5194/gmd-16-7491-2023, https://doi.org/10.5194/gmd-16-7491-2023, 2023
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This work highlights upgrades to SASKTRAN, a model that simulates sunlight interacting with the atmosphere to help measure trace gases. The upgrades were verified by detailed comparisons between different numerical methods. A case study was performed using SASKTRAN’s multidimensional capabilities, which found that ignoring horizontal variation in the atmosphere (a common practice in the field) can introduce non-negligible errors where there is snow or high pollution.
Anna Lange, Alexei Rozanov, and Christian von Savigny
Atmos. Chem. Phys., 23, 14829–14839, https://doi.org/10.5194/acp-23-14829-2023, https://doi.org/10.5194/acp-23-14829-2023, 2023
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We were able to demonstrate quantitatively that the blue colour of the sky cannot be solely attributed to Rayleigh scattering. The influence of ozone on the blue colour of the sky is calculated for different viewing geometries, total ozone columns and an enhanced stratospheric aerosol scenario. Furthermore, the effects of polarisation, surface albedo and observer height are investigated.
James Barry, Stefanie Meilinger, Klaus Pfeilsticker, Anna Herman-Czezuch, Nicola Kimiaie, Christopher Schirrmeister, Rone Yousif, Tina Buchmann, Johannes Grabenstein, Hartwig Deneke, Jonas Witthuhn, Claudia Emde, Felix Gödde, Bernhard Mayer, Leonhard Scheck, Marion Schroedter-Homscheidt, Philipp Hofbauer, and Matthias Struck
Atmos. Meas. Tech., 16, 4975–5007, https://doi.org/10.5194/amt-16-4975-2023, https://doi.org/10.5194/amt-16-4975-2023, 2023
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Measured power data from solar photovoltaic (PV) systems contain information about the state of the atmosphere. In this work, power data from PV systems in the Allgäu region in Germany were used to determine the solar irradiance at each location, using state-of-the-art simulation and modelling. The results were validated using concurrent measurements of the incoming solar radiation in each case. If applied on a wider scale, this algorithm could help improve weather and climate models.
Kimberlee Dubé, Susann Tegtmeier, Adam Bourassa, Daniel Zawada, Douglas Degenstein, Patrick E. Sheese, Kaley A. Walker, and William Randel
Atmos. Chem. Phys., 23, 13283–13300, https://doi.org/10.5194/acp-23-13283-2023, https://doi.org/10.5194/acp-23-13283-2023, 2023
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This paper presents a technique for understanding the causes of long-term changes in stratospheric composition. By using N2O as a proxy for stratospheric circulation in the model used to calculated trends, it is possible to separate the effects of dynamics and chemistry on observed trace gas trends. We find that observed HCl increases are due to changes in the stratospheric circulation, as are O3 decreases above 30 hPa in the Northern Hemisphere.
Michael Kiefer, Dale F. Hurst, Gabriele P. Stiller, Stefan Lossow, Holger Vömel, John Anderson, Faiza Azam, Jean-Loup Bertaux, Laurent Blanot, Klaus Bramstedt, John P. Burrows, Robert Damadeo, Bianca Maria Dinelli, Patrick Eriksson, Maya García-Comas, John C. Gille, Mark Hervig, Yasuko Kasai, Farahnaz Khosrawi, Donal Murtagh, Gerald E. Nedoluha, Stefan Noël, Piera Raspollini, William G. Read, Karen H. Rosenlof, Alexei Rozanov, Christopher E. Sioris, Takafumi Sugita, Thomas von Clarmann, Kaley A. Walker, and Katja Weigel
Atmos. Meas. Tech., 16, 4589–4642, https://doi.org/10.5194/amt-16-4589-2023, https://doi.org/10.5194/amt-16-4589-2023, 2023
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We quantify biases and drifts (and their uncertainties) between the stratospheric water vapor measurement records of 15 satellite-based instruments (SATs, with 31 different retrievals) and balloon-borne frost point hygrometers (FPs) launched at 27 globally distributed stations. These comparisons of measurements during the period 2000–2016 are made using robust, consistent statistical methods. With some exceptions, the biases and drifts determined for most SAT–FP pairs are < 10 % and < 1 % yr−1.
Bianca Zilker, Andreas Richter, Anne-Marlene Blechschmidt, Peter von der Gathen, Ilias Bougoudis, Sora Seo, Tim Bösch, and John Philip Burrows
Atmos. Chem. Phys., 23, 9787–9814, https://doi.org/10.5194/acp-23-9787-2023, https://doi.org/10.5194/acp-23-9787-2023, 2023
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During Arctic spring, near-surface ozone is depleted by bromine released from salty sea ice and/or snow-covered areas under certain meteorological conditions. To study this ozone depletion and the prevailing meteorological conditions, two ozone data sets from Ny-Ålesund, Svalbard, have been evaluated. We found that during ozone depletion events lower pressure over the Barents Sea and higher pressure in the Icelandic Low area led to a transport of cold polar air from the north to Ny-Ålesund.
Midhun George, Maria Dolores Andrés Hernández, Vladyslav Nenakhov, Yangzhuoran Liu, John Philip Burrows, Birger Bohn, Eric Förster, Florian Obersteiner, Andreas Zahn, Theresa Harlaß, Helmut Ziereis, Hans Schlager, Benjamin Schreiner, Flora Kluge, Katja Bigge, and Klaus Pfeilsticker
Atmos. Chem. Phys., 23, 7799–7822, https://doi.org/10.5194/acp-23-7799-2023, https://doi.org/10.5194/acp-23-7799-2023, 2023
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The applicability of photostationary steady-state (PSS) assumptions to estimate the amount of the sum of peroxy radicals (RO2*) during the EMeRGe airborne observations from the known radical chemistry and onboard measurements of RO2* precursors, photolysis frequencies, and other trace gases such as NOx and O3 was investigated. The comparison of the calculated RO2* with the actual measurements provides an insight into the main processes controlling their concentration in the air masses measured.
Ethan Runge, Jeff Langille, Daniel Zawada, Adam Bourassa, and Doug Degenstein
Atmos. Meas. Tech., 16, 3123–3139, https://doi.org/10.5194/amt-16-3123-2023, https://doi.org/10.5194/amt-16-3123-2023, 2023
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The Limb Imaging Fourier Transform Spectrometer Experiment (LIFE) instrument takes vertical images of limb radiance across a wide mid-infrared spectral band from a stratospheric balloon. Measurements are used to infer vertical-trace-gas-profile retrievals of H2O, O3, HNO3, CH4, and N2O. Nearly time-/space-coincident observations from the Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) and Microwave Limb Sounder (MLS) instruments are compared to the LIFE results.
Kameswara S. Vinjamuri, Marco Vountas, Luca Lelli, Martin Stengel, Matthew D. Shupe, Kerstin Ebell, and John P. Burrows
Atmos. Meas. Tech., 16, 2903–2918, https://doi.org/10.5194/amt-16-2903-2023, https://doi.org/10.5194/amt-16-2903-2023, 2023
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Clouds play an important role in Arctic amplification. Cloud data from ground-based sites are valuable but cannot represent the whole Arctic. Therefore the use of satellite products is a measure to cover the entire Arctic. However, the quality of such cloud measurements from space is not well known. The paper discusses the differences and commonalities between satellite and ground-based measurements. We conclude that the satellite dataset, with a few exceptions, can be used in the Arctic.
Basudev Swain, Marco Vountas, Adrien Deroubaix, Luca Lelli, Aishwarya Singh, Yanick Ziegler, Sachin S. Gunthe, and John P. Burrows
EGUsphere, https://doi.org/10.5194/egusphere-2023-730, https://doi.org/10.5194/egusphere-2023-730, 2023
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Aerosols are suspensions of particles distributed in the air. Depending on their chemical composition, they scatter and/or absorb sunlight and thus cool or warm the earth's atmosphere and its surface. They also provide as a surface in the atmosphere upon which ice or liquid clouds droplets nucleate and grow. In this study, we use satellite observations and model simulations to investigate the properties of aerosols with the goal of assessing their direct and indirect role in climate change.
Viktoria F. Sofieva, Monika Szelag, Johanna Tamminen, Carlo Arosio, Alexei Rozanov, Mark Weber, Doug Degenstein, Adam Bourassa, Daniel Zawada, Michael Kiefer, Alexandra Laeng, Kaley A. Walker, Patrick Sheese, Daan Hubert, Michel van Roozendael, Christian Retscher, Robert Damadeo, and Jerry D. Lumpe
Atmos. Meas. Tech., 16, 1881–1899, https://doi.org/10.5194/amt-16-1881-2023, https://doi.org/10.5194/amt-16-1881-2023, 2023
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The paper presents the updated SAGE-CCI-OMPS+ climate data record of monthly zonal mean ozone profiles. This dataset covers the stratosphere and combines measurements by nine limb and occultation satellite instruments (SAGE II, OSIRIS, MIPAS, SCIAMACHY, GOMOS, ACE-FTS, OMPS-LP, POAM III, and SAGE III/ISS). The update includes new versions of MIPAS, ACE-FTS, and OSIRIS datasets and introduces data from additional sensors (POAM III and SAGE III/ISS) and retrieval processors (OMPS-LP).
Kai Krause, Folkard Wittrock, Andreas Richter, Dieter Busch, Anton Bergen, John P. Burrows, Steffen Freitag, and Olesia Halbherr
Atmos. Meas. Tech., 16, 1767–1787, https://doi.org/10.5194/amt-16-1767-2023, https://doi.org/10.5194/amt-16-1767-2023, 2023
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Inland shipping is an important source of nitrogen oxides (NOx). The amount of emitted NOx depends on the characteristics of the individual vessels and the traffic density. Ship emissions are often characterised by the amount of emitted NOx per unit of burnt fuel, and further knowledge about fuel consumption is needed to quantify the total emissions caused by ship traffic. In this study, a new approach to derive absolute emission rates (in g s−1) from onshore measurements is presented.
Linlu Mei, Vladimir Rozanov, Alexei Rozanov, and John P. Burrows
Geosci. Model Dev., 16, 1511–1536, https://doi.org/10.5194/gmd-16-1511-2023, https://doi.org/10.5194/gmd-16-1511-2023, 2023
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This paper summarizes recent developments of aerosol, cloud and surface reflectance databases and models in the framework of the software package SCIATRAN. These updates and developments extend the capabilities of the radiative transfer modeling, especially by accounting for different kinds of vertical inhomogeneties. Vertically inhomogeneous clouds and different aerosol types can be easily accounted for within SCIATRAN (V4.6). The widely used surface models and databases are now available.
Kezia Lange, Andreas Richter, Anja Schönhardt, Andreas C. Meier, Tim Bösch, André Seyler, Kai Krause, Lisa K. Behrens, Folkard Wittrock, Alexis Merlaud, Frederik Tack, Caroline Fayt, Martina M. Friedrich, Ermioni Dimitropoulou, Michel Van Roozendael, Vinod Kumar, Sebastian Donner, Steffen Dörner, Bianca Lauster, Maria Razi, Christian Borger, Katharina Uhlmannsiek, Thomas Wagner, Thomas Ruhtz, Henk Eskes, Birger Bohn, Daniel Santana Diaz, Nader Abuhassan, Dirk Schüttemeyer, and John P. Burrows
Atmos. Meas. Tech., 16, 1357–1389, https://doi.org/10.5194/amt-16-1357-2023, https://doi.org/10.5194/amt-16-1357-2023, 2023
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We present airborne imaging DOAS and ground-based stationary and car DOAS measurements conducted during the S5P-VAL-DE-Ruhr campaign in the Rhine-Ruhr region. The measurements are used to validate spaceborne NO2 data products from the Sentinel-5 Precursor TROPOspheric Monitoring Instrument (TROPOMI). Auxiliary data of the TROPOMI NO2 retrieval, such as spatially higher resolved a priori NO2 vertical profiles, surface reflectivity, and cloud treatment are investigated to evaluate their impact.
Chuan-Yao Lin, Wan-Chin Chen, Yi-Yun Chien, Charles C. K. Chou, Chian-Yi Liu, Helmut Ziereis, Hans Schlager, Eric Förster, Florian Obersteiner, Ovid O. Krüger, Bruna A. Holanda, Mira L. Pöhlker, Katharina Kaiser, Johannes Schneider, Birger Bohn, Klaus Pfeilsticker, Benjamin Weyland, Maria Dolores Andrés Hernández, and John P. Burrows
Atmos. Chem. Phys., 23, 2627–2647, https://doi.org/10.5194/acp-23-2627-2023, https://doi.org/10.5194/acp-23-2627-2023, 2023
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During the EMeRGe campaign in Asia, atmospheric pollutants were measured on board the HALO aircraft. The WRF-Chem model was employed to evaluate the biomass burning (BB) plume transported from Indochina and its impact on the downstream areas. The combination of BB aerosol enhancement with cloud water resulted in a reduction in incoming shortwave radiation at the surface in southern China and the East China Sea, which potentially has significant regional climate implications.
Luca Lelli, Marco Vountas, Narges Khosravi, and John Philipp Burrows
Atmos. Chem. Phys., 23, 2579–2611, https://doi.org/10.5194/acp-23-2579-2023, https://doi.org/10.5194/acp-23-2579-2023, 2023
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Arctic amplification describes the recent period in which temperatures have been rising twice as fast as or more than the global average and sea ice and the Greenland ice shelf are approaching a tipping point. Hence, the Arctic ability to reflect solar energy decreases and absorption by the surface increases. Using 2 decades of complementary satellite data, we discover that clouds unexpectedly increase the pan-Arctic reflectance by increasing their liquid water content, thus cooling the Arctic.
Yi Wang, Mark Schoeberl, Ghassan Taha, Daniel Zawada, and Adam Bourassa
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2023-36, https://doi.org/10.5194/amt-2023-36, 2023
Revised manuscript not accepted
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The OMPS-LP satellite instrument measures aerosol scattering properties across the atmospheric limb. Adopting an algorithm that uses extinction at two wavelengths, we retrieve vertical profiles of particle size and concentration. We demonstrate that these profiles are consistent with in-situ balloon and SAGE-III/ISS satellite measurements. We also show how aerosol size and concentration evolve during Reikoke and Hunga Tonga-Hunga Ha'apai eruptions.
Veronika Pörtge, Tobias Kölling, Anna Weber, Lea Volkmer, Claudia Emde, Tobias Zinner, Linda Forster, and Bernhard Mayer
Atmos. Meas. Tech., 16, 645–667, https://doi.org/10.5194/amt-16-645-2023, https://doi.org/10.5194/amt-16-645-2023, 2023
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In this work, we analyze polarized cloudbow observations by the airborne camera system specMACS to retrieve the cloud droplet size distribution defined by the effective radius (reff) and the effective variance (veff). Two case studies of trade-wind cumulus clouds observed during the EUREC4A field campaign are presented. The results are combined into maps of reff and veff with a very high spatial resolution (100 m × 100 m) that allow new insights into cloud microphysics.
Oliver Schneising, Michael Buchwitz, Jonas Hachmeister, Steffen Vanselow, Maximilian Reuter, Matthias Buschmann, Heinrich Bovensmann, and John P. Burrows
Atmos. Meas. Tech., 16, 669–694, https://doi.org/10.5194/amt-16-669-2023, https://doi.org/10.5194/amt-16-669-2023, 2023
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Methane and carbon monoxide are important constituents of the atmosphere in the context of climate change and air pollution. We present the latest advances in the TROPOMI/WFMD algorithm to simultaneously retrieve atmospheric methane and carbon monoxide abundances from space. The changes in the latest product version are described in detail, and the resulting improvements are demonstrated. An overview of the products is provided including a discussion of annual increases and validation results.
Paul S. Jeffery, Kaley A. Walker, Chris E. Sioris, Chris D. Boone, Doug Degenstein, Gloria L. Manney, C. Thomas McElroy, Luis Millán, David A. Plummer, Niall J. Ryan, Patrick E. Sheese, and Jiansheng Zou
Atmos. Chem. Phys., 22, 14709–14734, https://doi.org/10.5194/acp-22-14709-2022, https://doi.org/10.5194/acp-22-14709-2022, 2022
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The upper troposphere–lower stratosphere is one of the most variable regions in the atmosphere. To improve our understanding of water vapour and ozone concentrations in this region, climatologies have been developed from 14 years of measurements from three Canadian satellite instruments. Horizontal and vertical coordinates have been chosen to minimize the effects of variability. To aid in analysis, model simulations have been used to characterize differences between instrument climatologies.
Miriam Latsch, Andreas Richter, Henk Eskes, Maarten Sneep, Ping Wang, Pepijn Veefkind, Ronny Lutz, Diego Loyola, Athina Argyrouli, Pieter Valks, Thomas Wagner, Holger Sihler, Michel van Roozendael, Nicolas Theys, Huan Yu, Richard Siddans, and John P. Burrows
Atmos. Meas. Tech., 15, 6257–6283, https://doi.org/10.5194/amt-15-6257-2022, https://doi.org/10.5194/amt-15-6257-2022, 2022
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The article investigates different S5P TROPOMI cloud retrieval algorithms for tropospheric trace gas retrievals. The cloud products show differences primarily over snow and ice and for scenes under sun glint. Some issues regarding across-track dependence are found for the cloud fractions as well as for the cloud heights.
Kimberlee Dubé, Daniel Zawada, Adam Bourassa, Doug Degenstein, William Randel, David Flittner, Patrick Sheese, and Kaley Walker
Atmos. Meas. Tech., 15, 6163–6180, https://doi.org/10.5194/amt-15-6163-2022, https://doi.org/10.5194/amt-15-6163-2022, 2022
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Satellite observations are important for monitoring changes in atmospheric composition. Here we describe an improved version of the NO2 retrieval for the Optical Spectrograph and InfraRed Imager System. The resulting NO2 profiles are compared to those from the Atmospheric Chemistry Experiment – Fourier Transform Spectrometer and the Stratospheric Aerosol and Gas Experiment III on the International Space Station. All datasets agree within 20 % throughout the stratosphere.
Christian von Savigny, Anna Lange, Anne Hemkendreis, Christoph G. Hoffmann, and Alexei Rozanov
Clim. Past, 18, 2345–2356, https://doi.org/10.5194/cp-18-2345-2022, https://doi.org/10.5194/cp-18-2345-2022, 2022
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This study investigates the possibility of inferring information on aerosol optical depth from photographs of historic paintings. The idea – which has been applied in previous studies – is very interesting because it would provide an archive of the atmospheric aerosol loading covering many centuries. We show that twilight colours depend not only on the aerosol optical thickness, but also on several other parameters, making a quantitative estimate of aerosol optical depth very difficult.
Carlo Arosio, Alexei Rozanov, Victor Gorshelev, Alexandra Laeng, and John P. Burrows
Atmos. Meas. Tech., 15, 5949–5967, https://doi.org/10.5194/amt-15-5949-2022, https://doi.org/10.5194/amt-15-5949-2022, 2022
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This paper characterizes the uncertainties affecting the ozone profiles retrieved at the University of Bremen through OMPS limb satellite observations. An accurate knowledge of the uncertainties is relevant for the validation of the product and to correctly interpret the retrieval results. We investigate several sources of uncertainties, estimate a total random and systematic component, and verify the consistency of the combined OMPS-MLS total uncertainty.
Huan Yu, Claudia Emde, Arve Kylling, Ben Veihelmann, Bernhard Mayer, Kerstin Stebel, and Michel Van Roozendael
Atmos. Meas. Tech., 15, 5743–5768, https://doi.org/10.5194/amt-15-5743-2022, https://doi.org/10.5194/amt-15-5743-2022, 2022
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In this study, we have investigated the impact of 3D clouds on the tropospheric NO2 retrieval from UV–visible sensors. We applied standard NO2 retrieval methods including cloud corrections to synthetic data generated by the 3D radiative transfer model. A sensitivity study was done for synthetic data, and dependencies on various parameters were investigated. Possible mitigation strategies were investigated and compared based on 3D simulations and observed data.
Sophie Godin-Beekmann, Niramson Azouz, Viktoria F. Sofieva, Daan Hubert, Irina Petropavlovskikh, Peter Effertz, Gérard Ancellet, Doug A. Degenstein, Daniel Zawada, Lucien Froidevaux, Stacey Frith, Jeannette Wild, Sean Davis, Wolfgang Steinbrecht, Thierry Leblanc, Richard Querel, Kleareti Tourpali, Robert Damadeo, Eliane Maillard Barras, René Stübi, Corinne Vigouroux, Carlo Arosio, Gerald Nedoluha, Ian Boyd, Roeland Van Malderen, Emmanuel Mahieu, Dan Smale, and Ralf Sussmann
Atmos. Chem. Phys., 22, 11657–11673, https://doi.org/10.5194/acp-22-11657-2022, https://doi.org/10.5194/acp-22-11657-2022, 2022
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An updated evaluation up to 2020 of stratospheric ozone profile long-term trends at extrapolar latitudes based on satellite and ground-based records is presented. Ozone increase in the upper stratosphere is confirmed, with significant trends at most latitudes. In this altitude region, a very good agreement is found with trends derived from chemistry–climate model simulations. Observed and modelled trends diverge in the lower stratosphere, but the differences are non-significant.
John T. Sullivan, Arnoud Apituley, Nora Mettig, Karin Kreher, K. Emma Knowland, Marc Allaart, Ankie Piters, Michel Van Roozendael, Pepijn Veefkind, Jerry R. Ziemke, Natalya Kramarova, Mark Weber, Alexei Rozanov, Laurence Twigg, Grant Sumnicht, and Thomas J. McGee
Atmos. Chem. Phys., 22, 11137–11153, https://doi.org/10.5194/acp-22-11137-2022, https://doi.org/10.5194/acp-22-11137-2022, 2022
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A TROPOspheric Monitoring Instrument (TROPOMI) validation campaign (TROLIX-19) was held in the Netherlands in September 2019. The research presented here focuses on using ozone lidars from NASA’s Goddard Space Flight Center to better evaluate the characterization of ozone throughout TROLIX-19 as compared to balloon-borne, space-borne and ground-based passive measurements, as well as a global coupled chemistry meteorology model.
Kristof Bognar, Susann Tegtmeier, Adam Bourassa, Chris Roth, Taran Warnock, Daniel Zawada, and Doug Degenstein
Atmos. Chem. Phys., 22, 9553–9569, https://doi.org/10.5194/acp-22-9553-2022, https://doi.org/10.5194/acp-22-9553-2022, 2022
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We quantify recent changes in stratospheric ozone (outside the polar regions) using a combination of three satellite datasets. We find that upper stratospheric ozone have increased significantly since 2000, although the recovery shows an unexpected pause in the Northern Hemisphere. Combined with the likely decrease in ozone in the lower stratosphere, this presents an interesting challenge for predicting the future of the ozone layer.
Jonas Hachmeister, Oliver Schneising, Michael Buchwitz, Alba Lorente, Tobias Borsdorff, John P. Burrows, Justus Notholt, and Matthias Buschmann
Atmos. Meas. Tech., 15, 4063–4074, https://doi.org/10.5194/amt-15-4063-2022, https://doi.org/10.5194/amt-15-4063-2022, 2022
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Sentinel-5P trace gas retrievals rely on elevation data in their calculations. Outdated or inaccurate data can lead to significant errors in e.g. dry-air mole fractions of methane (XCH4). We show that the use of inadequate elevation data leads to strong XCH4 anomalies in Greenland. Similar problems can be expected for other regions with inaccurate elevation data. However, we expect these to be more localized. We show that updating elevation data used in the retrieval solves this issue.
Ovid O. Krüger, Bruna A. Holanda, Sourangsu Chowdhury, Andrea Pozzer, David Walter, Christopher Pöhlker, Maria Dolores Andrés Hernández, John P. Burrows, Christiane Voigt, Jos Lelieveld, Johannes Quaas, Ulrich Pöschl, and Mira L. Pöhlker
Atmos. Chem. Phys., 22, 8683–8699, https://doi.org/10.5194/acp-22-8683-2022, https://doi.org/10.5194/acp-22-8683-2022, 2022
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The abrupt reduction in human activities during the first COVID-19 lockdown created unprecedented atmospheric conditions. We took the opportunity to quantify changes in black carbon (BC) as a major anthropogenic air pollutant. Therefore, we measured BC on board a research aircraft over Europe during the lockdown and compared the results to measurements from 2017. With model simulations we account for different weather conditions and find a lockdown-related decrease in BC of 41 %.
Anna Lange, Gerd Baumgarten, Alexei Rozanov, and Christian von Savigny
Ann. Geophys., 40, 407–419, https://doi.org/10.5194/angeo-40-407-2022, https://doi.org/10.5194/angeo-40-407-2022, 2022
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We investigate the influence of different parameters on the colour of noctilucent clouds (highest clouds in the atmosphere), using radiative transfer calculations. We determined the effect of the particle size, optical depth, single scattering/multiple scattering and ozone. For sufficiently large optical depth and for specific viewing geometries, ozone plays only a minor role in the blueish colour of noctilucent clouds (new result).
Arve Kylling, Claudia Emde, Huan Yu, Michel van Roozendael, Kerstin Stebel, Ben Veihelmann, and Bernhard Mayer
Atmos. Meas. Tech., 15, 3481–3495, https://doi.org/10.5194/amt-15-3481-2022, https://doi.org/10.5194/amt-15-3481-2022, 2022
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Atmospheric trace gases such as nitrogen dioxide (NO2) may be measured by satellite instruments sensitive to solar ultraviolet–visible radiation reflected from Earth and its atmosphere. For a single pixel, clouds in neighbouring pixels may affect the radiation and hence the retrieved trace gas amount. We found that for a solar zenith angle less than about 40° this cloud-related NO2 bias is typically below 10 %, while for larger solar zenith angles the NO2 bias is on the order of tens of percent.
William G. Read, Gabriele Stiller, Stefan Lossow, Michael Kiefer, Farahnaz Khosrawi, Dale Hurst, Holger Vömel, Karen Rosenlof, Bianca M. Dinelli, Piera Raspollini, Gerald E. Nedoluha, John C. Gille, Yasuko Kasai, Patrick Eriksson, Christopher E. Sioris, Kaley A. Walker, Katja Weigel, John P. Burrows, and Alexei Rozanov
Atmos. Meas. Tech., 15, 3377–3400, https://doi.org/10.5194/amt-15-3377-2022, https://doi.org/10.5194/amt-15-3377-2022, 2022
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This paper attempts to provide an assessment of the accuracy of 21 satellite-based instruments that remotely measure atmospheric humidity in the upper troposphere of the Earth's atmosphere. The instruments made their measurements from 1984 to the present time; however, most of these instruments began operations after 2000, and only a few are still operational. The objective of this study is to quantify the accuracy of each satellite humidity data set.
Stefan Noël, Maximilian Reuter, Michael Buchwitz, Jakob Borchardt, Michael Hilker, Oliver Schneising, Heinrich Bovensmann, John P. Burrows, Antonio Di Noia, Robert J. Parker, Hiroshi Suto, Yukio Yoshida, Matthias Buschmann, Nicholas M. Deutscher, Dietrich G. Feist, David W. T. Griffith, Frank Hase, Rigel Kivi, Cheng Liu, Isamu Morino, Justus Notholt, Young-Suk Oh, Hirofumi Ohyama, Christof Petri, David F. Pollard, Markus Rettinger, Coleen Roehl, Constantina Rousogenous, Mahesh Kumar Sha, Kei Shiomi, Kimberly Strong, Ralf Sussmann, Yao Té, Voltaire A. Velazco, Mihalis Vrekoussis, and Thorsten Warneke
Atmos. Meas. Tech., 15, 3401–3437, https://doi.org/10.5194/amt-15-3401-2022, https://doi.org/10.5194/amt-15-3401-2022, 2022
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We present a new version (v3) of the GOSAT and GOSAT-2 FOCAL products.
In addition to an increased number of XCO2 data, v3 also includes products for XCH4 (full-physics and proxy), XH2O and the relative ratio of HDO to H2O (δD). For GOSAT-2, we also present first XCO and XN2O results. All FOCAL data products show reasonable spatial distribution and temporal variations and agree well with TCCON. Global XN2O maps show a gradient from the tropics to higher latitudes on the order of 15 ppb.
Mark Weber, Carlo Arosio, Melanie Coldewey-Egbers, Vitali E. Fioletov, Stacey M. Frith, Jeannette D. Wild, Kleareti Tourpali, John P. Burrows, and Diego Loyola
Atmos. Chem. Phys., 22, 6843–6859, https://doi.org/10.5194/acp-22-6843-2022, https://doi.org/10.5194/acp-22-6843-2022, 2022
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Long-term trends in column ozone have been determined from five merged total ozone datasets spanning the period 1978–2020. We show that ozone recovery due to the decline in stratospheric halogens after the 1990s (as regulated by the Montreal Protocol) is evident outside the tropical region and amounts to half a percent per decade. The ozone recovery in the Northern Hemisphere is however compensated for by the negative long-term trend contribution from atmospheric dynamics since the year 2000.
Nora Mettig, Mark Weber, Alexei Rozanov, John P. Burrows, Pepijn Veefkind, Anne M. Thompson, Ryan M. Stauffer, Thierry Leblanc, Gerard Ancellet, Michael J. Newchurch, Shi Kuang, Rigel Kivi, Matthew B. Tully, Roeland Van Malderen, Ankie Piters, Bogumil Kois, René Stübi, and Pavla Skrivankova
Atmos. Meas. Tech., 15, 2955–2978, https://doi.org/10.5194/amt-15-2955-2022, https://doi.org/10.5194/amt-15-2955-2022, 2022
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Vertical ozone profiles from combined spectral measurements in the UV and IR spectral ranges were retrieved by using data from TROPOMI/S5P and CrIS/Suomi-NPP. The vertical resolution and accuracy of the ozone profiles are improved by combining both wavelength ranges compared to retrievals limited to UV or IR spectral data only. The advancement of our TOPAS algorithm for combined measurements is required because in the UV-only retrieval the vertical resolution in the troposphere is very limited.
M. Dolores Andrés Hernández, Andreas Hilboll, Helmut Ziereis, Eric Förster, Ovid O. Krüger, Katharina Kaiser, Johannes Schneider, Francesca Barnaba, Mihalis Vrekoussis, Jörg Schmidt, Heidi Huntrieser, Anne-Marlene Blechschmidt, Midhun George, Vladyslav Nenakhov, Theresa Harlass, Bruna A. Holanda, Jennifer Wolf, Lisa Eirenschmalz, Marc Krebsbach, Mira L. Pöhlker, Anna B. Kalisz Hedegaard, Linlu Mei, Klaus Pfeilsticker, Yangzhuoran Liu, Ralf Koppmann, Hans Schlager, Birger Bohn, Ulrich Schumann, Andreas Richter, Benjamin Schreiner, Daniel Sauer, Robert Baumann, Mariano Mertens, Patrick Jöckel, Markus Kilian, Greta Stratmann, Christopher Pöhlker, Monica Campanelli, Marco Pandolfi, Michael Sicard, José L. Gómez-Amo, Manuel Pujadas, Katja Bigge, Flora Kluge, Anja Schwarz, Nikos Daskalakis, David Walter, Andreas Zahn, Ulrich Pöschl, Harald Bönisch, Stephan Borrmann, Ulrich Platt, and John P. Burrows
Atmos. Chem. Phys., 22, 5877–5924, https://doi.org/10.5194/acp-22-5877-2022, https://doi.org/10.5194/acp-22-5877-2022, 2022
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EMeRGe provides a unique set of in situ and remote sensing airborne measurements of trace gases and aerosol particles along selected flight routes in the lower troposphere over Europe. The interpretation uses also complementary collocated ground-based and satellite measurements. The collected data help to improve the current understanding of the complex spatial distribution of trace gases and aerosol particles resulting from mixing, transport, and transformation of pollution plumes over Europe.
Claudia Emde, Huan Yu, Arve Kylling, Michel van Roozendael, Kerstin Stebel, Ben Veihelmann, and Bernhard Mayer
Atmos. Meas. Tech., 15, 1587–1608, https://doi.org/10.5194/amt-15-1587-2022, https://doi.org/10.5194/amt-15-1587-2022, 2022
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Retrievals of trace gas concentrations from satellite observations can be affected by clouds in the vicinity, either by shadowing or by scattering of radiation from clouds in the clear region. We used a Monte Carlo radiative transfer model to generate synthetic satellite observations, which we used to test retrieval algorithms and to quantify the error of retrieved NO2 vertical column density due to cloud scattering.
Julia Koch, Adam Bourassa, Nick Lloyd, Chris Roth, and Christian von Savigny
Atmos. Chem. Phys., 22, 3191–3202, https://doi.org/10.5194/acp-22-3191-2022, https://doi.org/10.5194/acp-22-3191-2022, 2022
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The mesopause, the region of the earth's atmosphere between 85 and 100 km, is hard to access by direct measurements. Therefore we look for parameters that can be measured using satellite or ground-based measurements. In this study we researched sodium airglow, a phenomenon that occurs when sodium atoms are excited by chemical reactions. We compared satellite measurements of the airglow and resulting sodium concentration profiles to gain a better understanding of the sodium in that region.
Patrick E. Sheese, Kaley A. Walker, Chris D. Boone, Adam E. Bourassa, Doug A. Degenstein, Lucien Froidevaux, C. Thomas McElroy, Donal Murtagh, James M. Russell III, and Jiansheng Zou
Atmos. Meas. Tech., 15, 1233–1249, https://doi.org/10.5194/amt-15-1233-2022, https://doi.org/10.5194/amt-15-1233-2022, 2022
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This study analyzes the quality of two versions (v3.6 and v4.1) of ozone concentration measurements from the ACE-FTS (Atmospheric Chemistry Experiment Fourier Transform Spectrometer), by comparing with data from five satellite instruments between 2004 and 2020. It was found that although the v3.6 data exhibit a better agreement than v4.1 with respect to the other instruments, v4.1 exhibits much better stability over time than v3.6. The stability of v4.1 makes it suitable for ozone trend studies.
Kezia Lange, Andreas Richter, and John P. Burrows
Atmos. Chem. Phys., 22, 2745–2767, https://doi.org/10.5194/acp-22-2745-2022, https://doi.org/10.5194/acp-22-2745-2022, 2022
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In this study, we investigated short time variability of NOx emissions and lifetimes on a global scale. We combined 2 years of satellite Sentinel-5P TROPOMI tropospheric NO2 column data with wind data. Fifty NOx sources distributed around the world are analyzed. The retrieved emissions show a clear seasonal dependence. NOx lifetime shows a latitudinal dependence but only a week seasonal dependence. NOx emissions show a clear weekly pattern which in contrast is not visible for NOx lifetimes.
Thomas E. Taylor, Christopher W. O'Dell, David Crisp, Akhiko Kuze, Hannakaisa Lindqvist, Paul O. Wennberg, Abhishek Chatterjee, Michael Gunson, Annmarie Eldering, Brendan Fisher, Matthäus Kiel, Robert R. Nelson, Aronne Merrelli, Greg Osterman, Frédéric Chevallier, Paul I. Palmer, Liang Feng, Nicholas M. Deutscher, Manvendra K. Dubey, Dietrich G. Feist, Omaira E. García, David W. T. Griffith, Frank Hase, Laura T. Iraci, Rigel Kivi, Cheng Liu, Martine De Mazière, Isamu Morino, Justus Notholt, Young-Suk Oh, Hirofumi Ohyama, David F. Pollard, Markus Rettinger, Matthias Schneider, Coleen M. Roehl, Mahesh Kumar Sha, Kei Shiomi, Kimberly Strong, Ralf Sussmann, Yao Té, Voltaire A. Velazco, Mihalis Vrekoussis, Thorsten Warneke, and Debra Wunch
Earth Syst. Sci. Data, 14, 325–360, https://doi.org/10.5194/essd-14-325-2022, https://doi.org/10.5194/essd-14-325-2022, 2022
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We provide an analysis of an 11-year record of atmospheric carbon dioxide (CO2) concentrations derived using an optimal estimation retrieval algorithm on measurements made by the GOSAT satellite. The new product (version 9) shows improvement over the previous version (v7.3) as evaluated against independent estimates of CO2 from ground-based sensors and atmospheric inversion systems. We also compare the new GOSAT CO2 values to collocated estimates from NASA's Orbiting Carbon Observatory-2.
Tobias Küchler, Stefan Noël, Heinrich Bovensmann, John Philip Burrows, Thomas Wagner, Christian Borger, Tobias Borsdorff, and Andreas Schneider
Atmos. Meas. Tech., 15, 297–320, https://doi.org/10.5194/amt-15-297-2022, https://doi.org/10.5194/amt-15-297-2022, 2022
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We applied the air-mass-corrected differential optical absorption spectroscopy (AMC-DOAS) method to derive total column water vapour (TCWV) from Sentinel-5P measurements and compared it to independent data sets. The correlation coefficients of typically more than 0.9 and the small deviations up to 2.5 kg m−2 reveal good agreement between our data product and other TCWV data sets. In particular for the different Sentinel-5P water vapour products, the deviations are around 1 kg m−2.
Debora Griffin, Chris A. McLinden, Enrico Dammers, Cristen Adams, Chelsea E. Stockwell, Carsten Warneke, Ilann Bourgeois, Jeff Peischl, Thomas B. Ryerson, Kyle J. Zarzana, Jake P. Rowe, Rainer Volkamer, Christoph Knote, Natalie Kille, Theodore K. Koenig, Christopher F. Lee, Drew Rollins, Pamela S. Rickly, Jack Chen, Lukas Fehr, Adam Bourassa, Doug Degenstein, Katherine Hayden, Cristian Mihele, Sumi N. Wren, John Liggio, Ayodeji Akingunola, and Paul Makar
Atmos. Meas. Tech., 14, 7929–7957, https://doi.org/10.5194/amt-14-7929-2021, https://doi.org/10.5194/amt-14-7929-2021, 2021
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Satellite-derived NOx emissions from biomass burning are estimated with TROPOMI observations. Two common emission estimation methods are applied, and sensitivity tests with model output were performed to determine the accuracy of these methods. The effect of smoke aerosols on TROPOMI NO2 columns is estimated and compared to aircraft observations from four different aircraft campaigns measuring biomass burning plumes in 2018 and 2019 in North America.
Sandip S. Dhomse, Carlo Arosio, Wuhu Feng, Alexei Rozanov, Mark Weber, and Martyn P. Chipperfield
Earth Syst. Sci. Data, 13, 5711–5729, https://doi.org/10.5194/essd-13-5711-2021, https://doi.org/10.5194/essd-13-5711-2021, 2021
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High-quality long-term ozone profile data sets are key to estimating short- and long-term ozone variability. Almost all the satellite (and chemical model) data sets show some kind of bias with respect to each other. This is because of differences in measurement methodologies as well as simplified processes in the models. We use satellite data sets and chemical model output to generate 42 years of ozone profile data sets using a random-forest machine-learning algorithm that is named ML-TOMCAT.
Sven Krautwurst, Konstantin Gerilowski, Jakob Borchardt, Norman Wildmann, Michał Gałkowski, Justyna Swolkień, Julia Marshall, Alina Fiehn, Anke Roiger, Thomas Ruhtz, Christoph Gerbig, Jaroslaw Necki, John P. Burrows, Andreas Fix, and Heinrich Bovensmann
Atmos. Chem. Phys., 21, 17345–17371, https://doi.org/10.5194/acp-21-17345-2021, https://doi.org/10.5194/acp-21-17345-2021, 2021
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Quantification of anthropogenic CH4 emissions remains challenging, but it is essential for near-term climate mitigation strategies. We use airborne remote sensing observations to assess bottom-up estimates of coal mining emissions from one of Europe's largest CH4 emission hot spots located in Poland. The analysis reveals that emissions from small groups of shafts can be disentangled, but caution is advised when comparing observations to commonly reported annual emissions.
Anqi Li, Chris Z. Roth, Adam E. Bourassa, Douglas A. Degenstein, Kristell Pérot, Ole Martin Christensen, and Donal P. Murtagh
Earth Syst. Sci. Data, 13, 5115–5126, https://doi.org/10.5194/essd-13-5115-2021, https://doi.org/10.5194/essd-13-5115-2021, 2021
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The nightglow emission originating from the vibrationally excited hydroxyl layer (about 85 km altitude) has been measured by the infrared imager (IRI) on the Odin satellite for more than 15 years. In this study, we document the retrieval steps, the resulting volume emission rates and the layer characteristics. Finally, we use the monthly zonal averages to demonstrate the fidelity of the data set. This unique, long-term data set will be valuable for studying various topics near the mesopause.
Yu-Wen Chen, Yi-Chun Chen, Charles C.-K. Chou, Hui-Ming Hung, Shih-Yu Chang, Lisa Eirenschmalz, Michael Lichtenstern, Helmut Ziereis, Hans Schlager, Greta Stratmann, Katharina Kaiser, Johannes Schneider, Stephan Borrmann, Florian Obersteiner, Eric Förster, Andreas Zahn, Wei-Nai Chen, Po-Hsiung Lin, Shuenn-Chin Chang, Maria Dolores Andrés Hernández, Pao-Kuan Wang, and John P. Burrows
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-788, https://doi.org/10.5194/acp-2021-788, 2021
Preprint withdrawn
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By presenting an approach using EMeRGe-Asia airborne field measurements and surface observations, this study shows that the fraction of OH reactivity due to SO2-OH reaction has a significant correlation with the sulfate concentration. Approximately 30 % of sulfate is produced by SO2-OH reaction. Our results underline the importance of SO2-OH gas-phase oxidation in sulfate formation, and demonstrate that the method can be applied to other regions and under different meteorological conditions.
Anu Kauppi, Antti Kukkurainen, Antti Lipponen, Marko Laine, Antti Arola, Hannakaisa Lindqvist, and Johanna Tamminen
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2021-328, https://doi.org/10.5194/amt-2021-328, 2021
Revised manuscript not accepted
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We present a methodology in Bayesian framework for retrieving atmospheric aerosol optical depth and aerosol type from the pre-computed look-up tables (LUTs). Especially, we consider Bayesian model averaging and uncertainty originating from aerosol model selection and imperfect forward modelling. Our aim is to get more realistic uncertainty estimates. We have applied the methodology to TROPOMI/S5P satellite observations and evaluated the results against ground-based data from the AERONET.
Marc Schwaerzel, Dominik Brunner, Fabian Jakub, Claudia Emde, Brigitte Buchmann, Alexis Berne, and Gerrit Kuhlmann
Atmos. Meas. Tech., 14, 6469–6482, https://doi.org/10.5194/amt-14-6469-2021, https://doi.org/10.5194/amt-14-6469-2021, 2021
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NO2 maps from airborne imaging remote sensing often appear much smoother than one would expect from high-resolution model simulations of NO2 over cities, despite the small ground-pixel size of the sensors. Our case study over Zurich, using the newly implemented building module of the MYSTIC radiative transfer solver, shows that the 3D effect can explain part of the smearing and that building shadows cause a noticeable underestimation and noise in the measured NO2 columns.
Elizaveta Malinina, Alexei Rozanov, Ulrike Niemeier, Sandra Wallis, Carlo Arosio, Felix Wrana, Claudia Timmreck, Christian von Savigny, and John P. Burrows
Atmos. Chem. Phys., 21, 14871–14891, https://doi.org/10.5194/acp-21-14871-2021, https://doi.org/10.5194/acp-21-14871-2021, 2021
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In the paper, changes in the stratospheric aerosol loading after the 2018 Ambae eruption were analyzed using OMPS-LP observations. The eruption was also simulated with the MAECHAM5-HAM global climate model. Generally, the model and observations agree very well. We attribute the good consistency of the results to a precisely determined altitude and mass of the volcanic injection, as well as nudging of the meteorological data. The radiative forcing from the eruption was estimated to be −0.13 W m−2.
Nora Mettig, Mark Weber, Alexei Rozanov, Carlo Arosio, John P. Burrows, Pepijn Veefkind, Anne M. Thompson, Richard Querel, Thierry Leblanc, Sophie Godin-Beekmann, Rigel Kivi, and Matthew B. Tully
Atmos. Meas. Tech., 14, 6057–6082, https://doi.org/10.5194/amt-14-6057-2021, https://doi.org/10.5194/amt-14-6057-2021, 2021
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TROPOMI is a nadir-viewing satellite that has observed global atmospheric trace gases at unprecedented spatial resolution since 2017. The retrieval of ozone profiles with high accuracy has been demonstrated using the TOPAS (Tikhonov regularised Ozone Profile retrievAl with SCIATRAN) algorithm and applying appropriate spectral corrections to TROPOMI UV data. Ozone profiles from TROPOMI were compared to ozonesonde and lidar profiles, showing an agreement to within 5 % in the stratosphere.
Kai Krause, Folkard Wittrock, Andreas Richter, Stefan Schmitt, Denis Pöhler, Andreas Weigelt, and John P. Burrows
Atmos. Meas. Tech., 14, 5791–5807, https://doi.org/10.5194/amt-14-5791-2021, https://doi.org/10.5194/amt-14-5791-2021, 2021
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Ships are an important source of key pollutants. Usually, these are measured aboard the ship or on the coast using in situ instruments. This study shows how active optical remote sensing can be used to measure ship emissions and how to determine emission rates of individual ships out of those measurements. These emission rates are valuable input for the assessment of the influence of shipping emissions in regions close to the shipping lanes.
Andrea Orfanoz-Cheuquelaf, Alexei Rozanov, Mark Weber, Carlo Arosio, Annette Ladstätter-Weißenmayer, and John P. Burrows
Atmos. Meas. Tech., 14, 5771–5789, https://doi.org/10.5194/amt-14-5771-2021, https://doi.org/10.5194/amt-14-5771-2021, 2021
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OMPS/NPP (2012–present) allows obtaining the tropospheric ozone column by combining ozone data from limb and nadir observations from the same instrument platform. In a first step, the retrieval of the total ozone column from the OMPS Nadir Mapper using the weighting function fitting approach (WFFA) is described here. The OMPS total ozone was compared with ground-based and other satellite measurements, showing agreement within 2.5 %.
Lily N. Zhang, Susan Solomon, Kane A. Stone, Jonathan D. Shanklin, Joshua D. Eveson, Steve Colwell, John P. Burrows, Mark Weber, Pieternel F. Levelt, Natalya A. Kramarova, and David P. Haffner
Atmos. Chem. Phys., 21, 9829–9838, https://doi.org/10.5194/acp-21-9829-2021, https://doi.org/10.5194/acp-21-9829-2021, 2021
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In the 1980s, measurements at the British Antarctic Survey station in Halley, Antarctica, led to the discovery of the ozone hole. The Halley total ozone record continues to be uniquely valuable for studies of long-term changes in Antarctic ozone. Environmental conditions in 2017 forced a temporary cessation of operations, leading to a gap in the historic record. We develop and test a method for filling in the Halley record using satellite data and find evidence to further support ozone recovery.
Quentin Errera, Emmanuel Dekemper, Noel Baker, Jonas Debosscher, Philippe Demoulin, Nina Mateshvili, Didier Pieroux, Filip Vanhellemont, and Didier Fussen
Atmos. Meas. Tech., 14, 4737–4753, https://doi.org/10.5194/amt-14-4737-2021, https://doi.org/10.5194/amt-14-4737-2021, 2021
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ALTIUS is a micro-satellite which will measure the distribution of the ozone layer. Micro-satellites are intended to be cost-effective, but does this make the ALTIUS measurements any less valuable? To answer this, we simulated ALTIUS data and measured how it could constrain a model of the ozone layer; we then compared these results with those obtained from the state-of-the-art NASA Aura MLS satellite ozone measurements. The outcome shows us that the ALTIUS
budgetinstrument is indeed valuable.
Linlu Mei, Vladimir Rozanov, Christine Pohl, Marco Vountas, and John P. Burrows
The Cryosphere, 15, 2757–2780, https://doi.org/10.5194/tc-15-2757-2021, https://doi.org/10.5194/tc-15-2757-2021, 2021
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This paper presents a new snow property retrieval algorithm from satellite observations. This is Part 1 of two companion papers and shows the method description and sensitivity study. The paper investigates the major factors, including the assumptions of snow optical properties, snow particle distribution and atmospheric conditions (cloud and aerosol), impacting snow property retrievals from satellite observation.
Linlu Mei, Vladimir Rozanov, Evelyn Jäkel, Xiao Cheng, Marco Vountas, and John P. Burrows
The Cryosphere, 15, 2781–2802, https://doi.org/10.5194/tc-15-2781-2021, https://doi.org/10.5194/tc-15-2781-2021, 2021
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This paper presents a new snow property retrieval algorithm from satellite observations. This is Part 2 of two companion papers and shows the results and validation. The paper performs the new retrieval algorithm on the Sea and Land
Surface Temperature Radiometer (SLSTR) instrument and compares the retrieved snow properties with ground-based measurements, aircraft measurements and other satellite products.
Stefan Noël, Maximilian Reuter, Michael Buchwitz, Jakob Borchardt, Michael Hilker, Heinrich Bovensmann, John P. Burrows, Antonio Di Noia, Hiroshi Suto, Yukio Yoshida, Matthias Buschmann, Nicholas M. Deutscher, Dietrich G. Feist, David W. T. Griffith, Frank Hase, Rigel Kivi, Isamu Morino, Justus Notholt, Hirofumi Ohyama, Christof Petri, James R. Podolske, David F. Pollard, Mahesh Kumar Sha, Kei Shiomi, Ralf Sussmann, Yao Té, Voltaire A. Velazco, and Thorsten Warneke
Atmos. Meas. Tech., 14, 3837–3869, https://doi.org/10.5194/amt-14-3837-2021, https://doi.org/10.5194/amt-14-3837-2021, 2021
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We present the first GOSAT and GOSAT-2 XCO2 data derived with the FOCAL retrieval algorithm. Comparisons of the GOSAT-FOCAL product with other data reveal long-term agreement within about 1 ppm over 1 decade, differences in seasonal variations of about 0.5 ppm, and a mean regional bias to ground-based TCCON data of 0.56 ppm with a mean scatter of 1.89 ppm. GOSAT-2-FOCAL data are preliminary only, but first comparisons show that they compare well with the GOSAT-FOCAL results and TCCON.
Michaela I. Hegglin, Susann Tegtmeier, John Anderson, Adam E. Bourassa, Samuel Brohede, Doug Degenstein, Lucien Froidevaux, Bernd Funke, John Gille, Yasuko Kasai, Erkki T. Kyrölä, Jerry Lumpe, Donal Murtagh, Jessica L. Neu, Kristell Pérot, Ellis E. Remsberg, Alexei Rozanov, Matthew Toohey, Joachim Urban, Thomas von Clarmann, Kaley A. Walker, Hsiang-Jui Wang, Carlo Arosio, Robert Damadeo, Ryan A. Fuller, Gretchen Lingenfelser, Christopher McLinden, Diane Pendlebury, Chris Roth, Niall J. Ryan, Christopher Sioris, Lesley Smith, and Katja Weigel
Earth Syst. Sci. Data, 13, 1855–1903, https://doi.org/10.5194/essd-13-1855-2021, https://doi.org/10.5194/essd-13-1855-2021, 2021
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An overview of the SPARC Data Initiative is presented, to date the most comprehensive assessment of stratospheric composition measurements spanning 1979–2018. Measurements of 26 chemical constituents obtained from an international suite of space-based limb sounders were compiled into vertically resolved, zonal monthly mean time series. The quality and consistency of these gridded datasets are then evaluated using a climatological validation approach and a range of diagnostics.
Viktoria F. Sofieva, Monika Szeląg, Johanna Tamminen, Erkki Kyrölä, Doug Degenstein, Chris Roth, Daniel Zawada, Alexei Rozanov, Carlo Arosio, John P. Burrows, Mark Weber, Alexandra Laeng, Gabriele P. Stiller, Thomas von Clarmann, Lucien Froidevaux, Nathaniel Livesey, Michel van Roozendael, and Christian Retscher
Atmos. Chem. Phys., 21, 6707–6720, https://doi.org/10.5194/acp-21-6707-2021, https://doi.org/10.5194/acp-21-6707-2021, 2021
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The MErged GRIdded Dataset of Ozone Profiles is a long-term (2001–2018) stratospheric ozone profile climate data record with resolved longitudinal structure that combines the data from six limb satellite instruments. The dataset can be used for various analyses, some of which are discussed in the paper. In particular, regionally and vertically resolved ozone trends are evaluated, including trends in the polar regions.
Nellie Wullenweber, Anna Lange, Alexei Rozanov, and Christian von Savigny
Clim. Past, 17, 969–983, https://doi.org/10.5194/cp-17-969-2021, https://doi.org/10.5194/cp-17-969-2021, 2021
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This study investigates the physical processes leading to the rare phenomenon of the sun appearing blue or green. The phenomenon is caused by anomalous scattering by, e.g., volcanic or forest fire aerosols. Unlike most other studies, our study includes a full treatment of the effect of Rayleigh scattering on the colour of the sun. We investigate different factors and revisit a historic example, i.e. the Canadian forest fires in 1950, that led to blue sun events in different European countries.
Michael Buchwitz, Maximilian Reuter, Stefan Noël, Klaus Bramstedt, Oliver Schneising, Michael Hilker, Blanca Fuentes Andrade, Heinrich Bovensmann, John P. Burrows, Antonio Di Noia, Hartmut Boesch, Lianghai Wu, Jochen Landgraf, Ilse Aben, Christian Retscher, Christopher W. O'Dell, and David Crisp
Atmos. Meas. Tech., 14, 2141–2166, https://doi.org/10.5194/amt-14-2141-2021, https://doi.org/10.5194/amt-14-2141-2021, 2021
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The COVID-19 pandemic resulted in reduced anthropogenic carbon dioxide (CO2) emissions during 2020 in large parts of the world. We have used a small ensemble of satellite retrievals of column-averaged CO2 (XCO2) to find out if a regional-scale reduction of atmospheric CO2 can be detected from space. We focus on East China and show that it is challenging to reliably detect and to accurately quantify the emission reduction, which only results in regional XCO2 reductions of about 0.1–0.2 ppm.
Patrick E. Sheese, Kaley A. Walker, Chris D. Boone, Doug A. Degenstein, Felicia Kolonjari, David Plummer, Douglas E. Kinnison, Patrick Jöckel, and Thomas von Clarmann
Atmos. Meas. Tech., 14, 1425–1438, https://doi.org/10.5194/amt-14-1425-2021, https://doi.org/10.5194/amt-14-1425-2021, 2021
Short summary
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Output from climate chemistry models (CMAM, EMAC, and WACCM) is used to estimate the expected geophysical variability of ozone concentrations between coincident satellite instrument measurement times and geolocations. We use the Canadian ACE-FTS and OSIRIS instruments as a case study. Ensemble mean estimates are used to optimize coincidence criteria between the two instruments, allowing for the use of more coincident profiles while providing an estimate of the geophysical variation.
Jakob Borchardt, Konstantin Gerilowski, Sven Krautwurst, Heinrich Bovensmann, Andrew K. Thorpe, David R. Thompson, Christian Frankenberg, Charles E. Miller, Riley M. Duren, and John Philip Burrows
Atmos. Meas. Tech., 14, 1267–1291, https://doi.org/10.5194/amt-14-1267-2021, https://doi.org/10.5194/amt-14-1267-2021, 2021
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The AVIRIS-NG hyperspectral imager has been used successfully to identify and quantify anthropogenic methane sources utilizing different retrieval and inversion methods. Here, we examine the adaption and application of the WFM-DOAS algorithm to AVIRIS-NG measurements to retrieve local methane column enhancements, compare the results with other retrievals, and quantify the uncertainties resulting from the retrieval method. Additionally, we estimate emissions from five detected methane plumes.
Ghassan Taha, Robert Loughman, Tong Zhu, Larry Thomason, Jayanta Kar, Landon Rieger, and Adam Bourassa
Atmos. Meas. Tech., 14, 1015–1036, https://doi.org/10.5194/amt-14-1015-2021, https://doi.org/10.5194/amt-14-1015-2021, 2021
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This work describes the newly released OMPS LP aerosol extinction profile multi-wavelength Version 2.0 algorithm and dataset. It is shown that the V2.0 aerosols exhibit significant improvements in OMPS LP retrieval performance in the Southern Hemisphere and at lower altitudes. The new product is compared to the SAGE III/ISS, OSIRIS and CALIPSO missions and shown to be of good quality and suitable for scientific studies.
Kimberlee Dubé, Adam Bourassa, Daniel Zawada, Douglas Degenstein, Robert Damadeo, David Flittner, and William Randel
Atmos. Meas. Tech., 14, 557–566, https://doi.org/10.5194/amt-14-557-2021, https://doi.org/10.5194/amt-14-557-2021, 2021
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SAGE III/ISS measures profiles of NO2; however the algorithm to convert raw measurements to NO2 concentration neglects variations caused by changes in chemistry over the course of a day. We devised a procedure to account for these diurnal variations and assess their impact on NO2 measurements from SAGE III/ISS. We find that the new NO2 concentration is more than 10 % lower than NO2 from the standard algorithm below 30 km, showing that this effect is important to consider at lower altitudes.
Soheila Jafariserajehlou, Vladimir V. Rozanov, Marco Vountas, Charles K. Gatebe, and John P. Burrows
Atmos. Meas. Tech., 14, 369–389, https://doi.org/10.5194/amt-14-369-2021, https://doi.org/10.5194/amt-14-369-2021, 2021
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In this work, we study retrieval of snow grain morphologies and their impact on the reflectance in a coupled snow–atmosphere system. We present a sensitivity study to highlight the importance of having adequate information about snow and atmosphere. A novel two-stage algorithm for retrieving the size and shape of snow grains is presented. The reflectance simulation results are compared to that of airborne measurements; high correlations of 0.98 at IR and 0.88–0.98 at VIS are achieved.
Maximilian Reuter, Heinrich Bovensmann, Michael Buchwitz, Jakob Borchardt, Sven Krautwurst, Konstantin Gerilowski, Matthias Lindauer, Dagmar Kubistin, and John P. Burrows
Atmos. Meas. Tech., 14, 153–172, https://doi.org/10.5194/amt-14-153-2021, https://doi.org/10.5194/amt-14-153-2021, 2021
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CO2 measurements from a small unmanned aircraft system (sUAS) can provide a cost-effective way to complement and validate satellite-based measurements of anthropogenic CO2 emissions. We introduce an sUAS which is capable of determining atmospheric CO2 mass fluxes from its own sensor data. We show results of validation flights at the ICOS atmospheric station in Steinkimmen and from demonstration flights downwind a CO2-emitting natural gas processing facility.
Cited articles
Arosio, C., Rozanov, A., Malinina, E., Eichmann, K.-U., von Clarmann, T., and Burrows, J. P.: Retrieval of ozone profiles from OMPS limb scattering observations, Atmos. Meas. Tech., 11, 2135–2149, https://doi.org/10.5194/amt-11-2135-2018, 2018. a, b
Bernath, P. F., McElroy, C. T., Abrams, M. C., Boone, C. D., Butler, M.,
Camy-Peyret, C., Carleer, M., Clerbaux, C., Coheur, P. F., Colin, R., DeCola,
P., DeMazière, M., Drummond, J. R., Dufour, D., Evans, W. F., Fast, H.,
Fussen, D., Gilbert, K., Jennings, D. E., Llewellyn, E. J., Lowe, R. P.,
Mahieu, E., McConnell, J. C., McHugh, M., McLeod, S. D., Michaud, R.,
Midwinter, C., Nassar, R., Nichitiu, F., Nowlan, C., Rinsland, C. P., Rochon,
Y. J., Rowlands, N., Semeniuk, K., Simon, P., Skelton, R., Sloan, J. J.,
Soucy, M. A., Strong, K., Tremblay, P., Turnbull, D., Walker, K. A., Walkty,
I., Wardle, D. A., Wehrle, V., Zander, R., and Zou, J.: Atmospheric chemistry
experiment (ACE): Mission overview, Geophys. Res. Lett., 32,
L15S01, https://doi.org/10.1029/2005GL022386, 2005. a
Bourassa, A. E., Degenstein, D. A., Gattinger, R. L., and Llewellyn, E. J.:
Stratospheric aerosol retrieval with optical spectrograph and infrared
imaging system limb scatter measurements, J. Geophys. Res.,
112, D10217, https://doi.org/10.1029/2006JD008079, 2007. a, b
Bourassa, A. E., Degenstein, D. A., and Llewellyn, E. J.: SASKTRAN: A
spherical geometry radiative transfer code for efficient estimation of limb
scattered sunlight, J. Quant. Spectrosc. Ra., 109, 52–73, https://doi.org/10.1016/j.jqsrt.2007.07.007, 2008. a, b
Bovensmann, H.: SCIAMACHY: Mission objectives and measurement modes,
J. Atmos. Sci., 56, 127–150, 1999. a
Brion, J., Chakir, A., Daumont, D., Malicet, J., and Parisse, C.:
High-resolution laboratory absorption cross section of O3. Temperature
effect, Chem. Phys. Lett., 213, 610–612, 1993. a
Buras, R. and Mayer, B.: Efficient unbiased variance reduction techniques for
Monte Carlo simulations of radiative transfer in cloudy atmospheres:
The solution, J. Quant. Spectrosc. Ra.,
112, 434–447, https://doi.org/10.1016/j.jqsrt.2010.10.005, 2011. a
Butz, A., Bösch, H., Camy-Peyret, C., Chipperfield, M., Dorf, M., Dufour, G., Grunow, K., Jeseck, P., Kühl, S., Payan, S., Pepin, I., Pukite, J., Rozanov, A., von Savigny, C., Sioris, C., Wagner, T., Weidner, F., and Pfeilsticker, K.: Inter-comparison of stratospheric O3 and NO2 abundances retrieved from balloon borne direct sun observations and Envisat/SCIAMACHY limb measurements, Atmos. Chem. Phys., 6, 1293–1314, https://doi.org/10.5194/acp-6-1293-2006, 2006. a
Chowdhary, J., Zhai, P.-W., Boss, E., Dierssen, H., Frouin, R., Ibrahim, A.,
Lee, Z., Remer, L. A., Twardowski, M., Xu, F., Zhang, X., Ottaviani, M.,
Espinosa, W. R., and Ramon, D.: Modeling Atmosphere-Ocean Radiative
Transfer: A PACE Mission Perspective, Front. Earth Sci.,
7, https://doi.org/10.3389/feart.2019.00100, 2019. a
Chowdhary, J., Zhai, P.-W., Xu, F., Frouin, R., and Ramon, D.: Testbed results
for scalar and vector radiative transfer computations of light in
atmosphere-ocean systems, J. Quant. Spectrosc. Ra., 242, 106717, https://doi.org/10.1016/j.jqsrt.2019.106717, 2020. a
Cisewski, M., Zawodny, J., Gasbarre, J., Eckman, R., Topiwala, N.,
Rodriguez-Alvarez, O., Cheek, D., and Hall, S.: The Stratospheric Aerosol
and Gas Experiment (SAGE III) on the International Space
Station (ISS) Mission, in: Sensors, Systems, and Next-Generation
Satellites XVIII, SPIE Remote Sensing, Proc. SPIE 9241, 924107, https://doi.org/10.1117/12.2073131, 2014. a
Daumont, D., Brion, J., Charbonnier, J., and Malicet, J.: Ozone UV
spectroscopy I: Absorption cross-sections at room temperature, J.
Atmos. Chem., 15, 145–155, 1992. a
Degenstein, D. A., Bourassa, A. E., Roth, C. Z., and Llewellyn, E. J.: Limb scatter ozone retrieval from 10 to 60 km using a multiplicative algebraic reconstruction technique, Atmos. Chem. Phys., 9, 6521–6529, https://doi.org/10.5194/acp-9-6521-2009, 2009. a, b
Dueck, S. R., Bourassa, A. E., and Degenstein, D. A.: An efficient algorithm
for polarization in the SASKTRAN radiative transfer framework, J.
Quant. Spectrosc. Ra., 199, 1–11,
https://doi.org/10.1016/j.jqsrt.2017.05.016, 2017. a, b
Elash, B., Bourassa, A., Rieger, L., Dueck, S., Zawada, D., and Degenstein, D.:
The sensitivity to polarization in stratospheric aerosol retrievals from limb
scattered sunlight measurements, J. Quant. Spectrosc.
Ra., 189, 75–85, https://doi.org/10.1016/j.jqsrt.2016.11.014, 2017. a
Elash, B. J., Bourassa, A. E., Loewen, P. R., Lloyd, N. D., and Degenstein, D. A.: The Aerosol Limb Imager: acousto-optic imaging of limb-scattered sunlight for stratospheric aerosol profiling, Atmos. Meas. Tech., 9, 1261–1277, https://doi.org/10.5194/amt-9-1261-2016, 2016. a
Emde, C. and Mayer, B.: Simulation of solar radiation during a total eclipse: a challenge for radiative transfer, Atmos. Chem. Phys., 7, 2259–2270, https://doi.org/10.5194/acp-7-2259-2007, 2007. a
Emde, C., Buras, R., Mayer, B., and Blumthaler, M.: The impact of aerosols on polarized sky radiance: model development, validation, and applications, Atmos. Chem. Phys., 10, 383–396, https://doi.org/10.5194/acp-10-383-2010, 2010. a
Emde, C., Buras, R., and Mayer, B.: ALIS: An efficient method to compute
high spectral resolution polarized solar radiances using the Monte Carlo
approach, J. Quant. Spectrosc. Ra., 112,
1622–1631, https://doi.org/10.1016/j.jqsrt.2011.03.018, 2011. a
Emde, C., Barlakas, V., Cornet, C., Evans, F., Korkin, S., Ota, Y., Labonnote,
L. C., Lyapustin, A., Macke, A., Mayer, B., and Wendisch, M.: IPRT
polarized radiative transfer model intercomparison project – Phase A,
J. Quant. Spectrosc. Ra., 164, 8–36,
https://doi.org/10.1016/j.jqsrt.2015.05.007, 2015. a, b, c
Emde, C., Buras-Schnell, R., Kylling, A., Mayer, B., Gasteiger, J., Hamann, U., Kylling, J., Richter, B., Pause, C., Dowling, T., and Bugliaro, L.: The libRadtran software package for radiative transfer calculations (version 2.0.1), Geosci. Model Dev., 9, 1647–1672, https://doi.org/10.5194/gmd-9-1647-2016, 2016. a
Emde, C., Buras-Schnell, R., Sterzik, M., and Bagnulo, S.: Influence of
aerosols, clouds, and sunglint on polarization spectra of Earthshine,
Astron. Astrophys., 605, A2, https://doi.org/10.1051/0004-6361/201629948,
2017. a
Emde, C., Barlakas, V., Cornet, C., Evans, F., Wang, Z., Labonotte, L. C.,
Macke, A., Mayer, B., and Wendisch, M.: IPRT polarized radiative transfer
model intercomparison project – Three-dimensional test cases (phase B),
J. Quant. Spectrosc. Ra., 209, 19–44,
https://doi.org/10.1016/J.JQSRT.2018.01.024, 2018. a
Flynn, L. E., Seftor, C. J., Larsen, J. C., and Xu, P.: The ozone mapping and
profiler suite, in: Earth science satellite remote sensing,
Springer, Berlin, Heidelberg, 279–296, 2006. a
Fussen, D., Baker, N., Debosscher, J., Dekemper, E., Demoulin, P., Errera, Q.,
Franssens, G., Mateshvili, N., Pereira, N., Pieroux, D., and Vanhellemont,
F.: The ALTIUS atmospheric limb sounder, J. Quant.
Spectrosc. Ra., 238, 106542,
https://doi.org/10.1016/j.jqsrt.2019.06.021, 2019. a
Herman, B. M., Ben-David, A., and Thome, K. J.: Numerical technique for solving
the radiative transfer equation for a spherical shell atmosphere, Appl.
Optics, 33, 1760–1770, https://doi.org/10.1364/AO.33.001760, 1994. a
Herman, B. M., Caudill, T. R., Flittner, D. E., Thome, K. J., and Ben-David,
A.: Comparison of the Gauss–Seidel spherical polarized radiative
transfer code with other radiative transfer codes, Appl. Optics, 34,
4563–4572, https://doi.org/10.1364/AO.34.004563, 1995. a
Hovenier, J. W., Mee, van der Mee, C. V. M., and Domke, H.: Transfer of Polarized
Light in Planetary Atmospheres: Basic Concepts and Practical
Methods, Astrophysics and Space Science Library, Springer,
the Netherlands, https://doi.org/10.1007/978-1-4020-2856-4, 2004. a, b
Kokhanovsky, A. A., Budak, V. P., Cornet, C., Duan, M., Emde, C., Katsev,
I. L., Klyukov, D. A., Korkin, S. V., C-Labonnote, L., Mayer, B., Min, Q.,
Nakajima, T., Ota, Y., Prikhach, A. S., Rozanov, V. V., Yokota, T., and Zege,
E. P.: Benchmark results in vector atmospheric radiative transfer, J.
Quant. Spectrosc. Ra., 111, 1931–1946,
https://doi.org/10.1016/j.jqsrt.2010.03.005, 2010. a
Korkin, S., Yang, E.-S., Spurr, R., Emde, C., Krotkov, N., Vasilkov, A.,
Haffner, D., Mok, J., and Lyapustin, A.: Revised and extended benchmark
results for Rayleigh scattering of sunlight in spherical atmospheres,
J. Quant. Spectrosc. Ra., 254, 107181,
https://doi.org/10.1016/j.jqsrt.2020.107181, 2020. a
Kozun, M., Bourassa, A., Degenstein, D., and Loewen, P.: A multi-spectral
polarimetric imager for atmospheric profiling of aerosol and thin cloud:
Prototype design and sub-orbital performance, Rev. Sci.
Instrum., 91, 103106, https://doi.org/10.1063/5.0016129, 2020. a
Kyrölä, E., Tamminen, J., Leppelmeier, G. W., Sofieva, V., Hassinen, S.,
Bertaux, J. L., Hauchecorne, A., Dalaudier, F., Cot, C., Korablev, O.,
Fanton d'Andon, O., Barrot, G., Mangin, A., Théodore, B., Guirlet, M.,
Etanchaud, F., Snoeij, P., Koopman, R., Saavedra, L., Fraisse, R., Fussen,
D., and Vanhellemont, F.: GOMOS on Envisat: An overview, Adv.
Space Res., 33, 1020–1028, https://doi.org/10.1016/S0273-1177(03)00590-8,
2004. a
Llewellyn, E. J., Lloyd, N. D., Degenstein, D. A., Gattinger, R. L., Petalina,
S. V., Bourassa, A. E., Wiensz, J. T., Ivanov, E. V., McDade, I. C., Solheim,
B. H., McConnell, J. C., Haley, C. S., Savigny, C. v., Sioris, C. E.,
McLinden, C. A., Griffioen, E., Kaminski, J., Evans, W. F. J., Puckrin, E.,
Strong, K., Wehrle, V., Hum, R. H., Kendall, D. J. W., Matsushita, J.,
Murtagh, D. P., Brohede, S., Stegman, J., Witt, G., Barnes, G., Payne, W. F.,
Piche, L., Smith, K., Warshaw, G., Deslauniers, D. L., Marchand, P.,
Richardson, E. H., King, R. A., Wevers, I., McCreath, W., Kyrölä, E.,
Oikarinen, L., Leppelmeier, G. W., Auvinen, H., Megle, G., Hauchecorne, A.,
Lefevre, F., de La Noe, J., Ricaud, P., Frisk, U., Sjoberg, F., Scheele,
F. v., and Nordh, L.: The OSIRIS instrument on the Odin spacecraft,
Can. J. Phys., 82, 411–422, 2004. a, b
Loughman, R., Flittner, D., Nyaku, E., and Bhartia, P. K.: Gauss–Seidel limb scattering (GSLS) radiative transfer model development in support of the Ozone Mapping and Profiler Suite (OMPS) limb profiler mission, Atmos. Chem. Phys., 15, 3007–3020, https://doi.org/10.5194/acp-15-3007-2015, 2015. a, b, c, d, e, f
Loughman, R. P., Griffioen, E., Oikarinen, L., Postylyakov, O. V., Rozanov, A.,
Flittner, D. E., and Rault, D. F.: Comparison of radiative transfer models
for limb-viewing scattered sunlight measurements, J. Geophys.
Res.-Atmos., 109, D06303, https://doi.org/10.1029/2003JD003854, 2004. a, b, c, d, e, f, g
Loughman, R. P., Flittner, D. E., Herman, B. M., Bhartia, P. K., Hilsenrath,
E., and McPeters, R. D.: Description and sensitivity analysis of a limb
scattering ozone retrieval algorithm, J. Geophys. Res., 110,
D19301, https://doi.org/10.1029/2004JD005429, 2005. a
Malicet, J., Daumont, D., Charbonnier, J., Parisse, C., Chakir, A., and Brion,
J.: Ozone UV spectroscopy. II. Absorption cross-sections and
temperature dependence, J. Atmos. Chem., 21, 263–273,
1995. a
Malinina, E., Rozanov, A., Rozanov, V., Liebing, P., Bovensmann, H., and Burrows, J. P.: Aerosol particle size distribution in the stratosphere retrieved from SCIAMACHY limb measurements, Atmos. Meas. Tech., 11, 2085–2100, https://doi.org/10.5194/amt-11-2085-2018, 2018. a
Malinina, E., Rozanov, A., Rieger, L., Bourassa, A., Bovensmann, H., Burrows, J. P., and Degenstein, D.: Stratospheric aerosol characteristics from space-borne observations: extinction coefficient and Ångström exponent, Atmos. Meas. Tech., 12, 3485–3502, https://doi.org/10.5194/amt-12-3485-2019, 2019. a
Malinina, E., Rozanov, A., Niemeier, U., Peglow, S., Arosio, C., Wrana, F., Timmreck, C., von Savigny, C., and Burrows, J. P.: Changes in stratospheric aerosol extinction coefficient after the 2018 Ambae eruption as seen by OMPS-LP and ECHAM5-HAM, Atmos. Chem. Phys. Discuss. [preprint], https://doi.org/10.5194/acp-2020-749, in review, 2020. a
Marchuk, G. I., Mikhailov, G. A., Nazareliev, M., Darbinjan, R. A., Kargin,
B. A., and Elepov, B. S.: The Monte Carlo methods in atmospheric optics,
vol. 12, Springer-Verlag Berlin Heidelberg, available at: https://www.springer.com/gp/book/9783662135037 (last access: 22 May 2021), 2013. a
Mauldin, L. E., Salikhov, R., Habib, S., Vladimirov, A. G., Carraway, D.,
Petrenko, G., and Comella, J.: Meteor-3M(1)/Stratospheric Aerosol and
Gas Experiment III (SAGE III) jointly sponsored by the National
Aeronautics and Space Administration and the Russian Space
Agency, Proc. SPIE 3501, Optical Remote Sensing of the Atmosphere and Clouds,
https://doi.org/10.1117/12.317767, 1998. a
Mayer, B.: Radiative transfer in the cloudy atmosphere, EPJ Web of Conferences,
1, 75–99, https://doi.org/10.1140/epjconf/e2009-00912-1,
2009. a
Mayer, B. and Kylling, A.: Technical note: The libRadtran software package for radiative transfer calculations – description and examples of use, Atmos. Chem. Phys., 5, 1855–1877, https://doi.org/10.5194/acp-5-1855-2005, 2005. a
McLinden, C. A. and Bourassa, A. E.: A Systematic Error in
Plane-Parallel Radiative Transfer Calculations, J.
Atmos. Sci., 67, 1695–1699, https://doi.org/10.1175/2009JAS3322.1, 2010. a, b
McLinden, C. A., Haley, C. S., Lloyd, N. D., Hendrick, F., Rozanov, A.,
Sinnhuber, B.-M., Goutail, F., Degenstein, D. A., Llewellyn, E. J., Sioris,
C. E., Roozendael, M. V., Pommereau, J. P., Lotz, W., and Burrows, J. P.:
Odin/OSIRIS observations of stratospheric BrO: Retrieval methodology,
climatology, and inferred Bry, J. Geophys. Res.-Atmos., 115, D15308, https://doi.org/10.1029/2009JD012488, 2010. a
Mishchenko, M. I., Lacis, A. A., and Travis, L. D.: Errors induced by the
neglect of polarization in radiance calculations for rayleigh-scattering
atmospheres, J. Quant. Spectrosc. Ra., 51,
491–510, https://doi.org/10.1016/0022-4073(94)90149-X, 1994. a
Murtagh, D., Frisk, U., Merino, F., Ridal, M., Jonsson, A., Stegman, J., Witt,
G., Jiménez, C., Megie, G., Noë, J. D., Ricaud, P., Baron, P., Pardo,
J. R., Llewellyn, E. J., Degenstein, D. A., Gattinger, R. L., Lloyd, N. D.,
Evans, W. F. J., McDade, I. C., Haley, C. S., Sioris, C. E., Savigny, V.,
Solheim, B. H., McConnell, J. C., Richardson, E. H., Leppelmeier, G. W.,
Auvinen, H., and Oikarinen, L.: An overview of the Odin atmospheric
mission, Can. J. Phys., 80, 309–318, https://doi.org/10.1139/P01-157,
2002. a
Natraj, V. and Hovenier, J.: Polarized light reflected and transmitted by thick
Rayleigh scattering atmospheres, Astrophys. J., 748, 28,
https://doi.org/10.1088/0004-637X/748/1/28, 2012. a
Oikarinen, L.: Polarization of light in UV-visible limb radiance
measurements, J. Geophys. Res.-Atmos., 106, 1533–1544,
https://doi.org/10.1029/2000JD900442, 2001. a
Oikarinen, L.: Effect of surface albedo variations on UV-visible
limb-scattering measurements of the atmosphere, J. Geophys.
Res.-Atmos., 107, ACH 13-1–ACH 13-15,
https://doi.org/10.1029/2001JD001492, 2002. a
Palmer, K. F. and Williams, D.: Optical Constants of Sulfuric Acid;
Application to the Clouds of Venus?, Appl. Optics, 14, 208–219,
https://doi.org/10.1364/AO.14.000208, 1975. a
Postylyakov, O.: Linearized vector radiative transfer model MCC++ for a
spherical atmosphere, J. Quant. Spectrosc. Ra., 88, 297–317, https://doi.org/10.1016/j.jqsrt.2004.01.009, 2004. a
Ramon, D., Steinmetz, F., Jolivet, D., Compiègne, M., and Frouin, R.: Modeling
polarized radiative transfer in the ocean-atmosphere system with the
GPU-accelerated SMART-G Monte Carlo code, J. Quant.
Spectrosc. Ra., 222–223, 89–107,
https://doi.org/10.1016/j.jqsrt.2018.10.017, 2019. a, b
Rault, D. F.: Ozone profile retrieval from Stratospheric Aerosol and Gas
Experiment (SAGE III) limb scatter measurements, J. Geophys.
Res., 110, D09309, https://doi.org/10.1029/2004JD004970, 2005. a
Rault, D. F. and Loughman, R. P.: The OMPS Limb Profiler Environmental
Data Record Algorithm Theoretical Basis Document and Expected
Performance, IEEE Transactions on Geoscience and Remote Sensing, 51,
2505–2527, https://doi.org/10.1109/TGRS.2012.2213093, 2013. a
Rault, D. F. and Spurr, R.: The OMPS Limb Profiler instrument:
two-dimensional retrieval algorithm, Proc. SPIE, 7827, Remote Sensing of Clouds and the Atmosphere XV, 78270P, https://doi.org/10.1117/12.864799, 2010. a
Rieger, L. A., Malinina, E. P., Rozanov, A. V., Burrows, J. P., Bourassa, A. E., and Degenstein, D. A.: A study of the approaches used to retrieve aerosol extinction, as applied to limb observations made by OSIRIS and SCIAMACHY, Atmos. Meas. Tech., 11, 3433–3445, https://doi.org/10.5194/amt-11-3433-2018, 2018. a, b
Rieger, L. A., Zawada, D. J., Bourassa, A. E., and Degenstein, D. A.: A
Multiwavelength Retrieval Approach for Improved OSIRIS Aerosol
Extinction Retrievals, J. Geophys. Res.-Atmos., 124,
7286–7307, https://doi.org/10.1029/2018JD029897, 2019. a
Roth, C. Z., Degenstein, D. A., Bourassa, A. E., and Llewellyn, E. J.: The
retrieval of vertical profiles of the ozone number density using Chappuis
band absorption information and a multiplicative algebraic reconstruction
technique, Can. J. Phys., 85, 1225–1243,
https://doi.org/10.1139/p07-130, 2007. a
Rozanov, A., Rozanov, V., and Burrows, J. P.: A numerical radiative transfer
model for a spherical planetary atmosphere: combined differential–integral
approach involving the Picard iterative approximation, J.
Quantit. Spectrosc. Ra., 69, 491–512,
https://doi.org/10.1016/S0022-4073(00)00100-X, 2001. a
Rozanov, A., Eichmann, K.-U., von Savigny, C., Bovensmann, H., Burrows, J. P., von Bargen, A., Doicu, A., Hilgers, S., Godin-Beekmann, S., Leblanc, T., and McDermid, I. S.: Comparison of the inversion algorithms applied to the ozone vertical profile retrieval from SCIAMACHY limb measurements, Atmos. Chem. Phys., 7, 4763–4779, https://doi.org/10.5194/acp-7-4763-2007, 2007. a
Rozanov, A., Kühl, S., Doicu, A., McLinden, C., Puķīte, J., Bovensmann, H., Burrows, J. P., Deutschmann, T., Dorf, M., Goutail, F., Grunow, K., Hendrick, F., von Hobe, M., Hrechanyy, S., Lichtenberg, G., Pfeilsticker, K., Pommereau, J. P., Van Roozendael, M., Stroh, F., and Wagner, T.: BrO vertical distributions from SCIAMACHY limb measurements: comparison of algorithms and retrieval results, Atmos. Meas. Tech., 4, 1319–1359, https://doi.org/10.5194/amt-4-1319-2011, 2011a. a
Rozanov, A., Weigel, K., Bovensmann, H., Dhomse, S., Eichmann, K.-U., Kivi, R., Rozanov, V., Vömel, H., Weber, M., and Burrows, J. P.: Retrieval of water vapor vertical distributions in the upper troposphere and the lower stratosphere from SCIAMACHY limb measurements, Atmos. Meas. Tech., 4, 933–954, https://doi.org/10.5194/amt-4-933-2011, 2011b. a, b
Rozanov, V., Rozanov, A., Kokhanovsky, A., and Burrows, J.: Radiative transfer
through terrestrial atmosphere and ocean: Software package SCIATRAN,
J. Quant. Spectrosc. Ra., 133, 13–71,
https://doi.org/10.1016/J.JQSRT.2013.07.004, 2014. a
Sioris, C. E., Rieger, L. A., Lloyd, N. D., Bourassa, A. E., Roth, C. Z., Degenstein, D. A., Camy-Peyret, C., Pfeilsticker, K., Berthet, G., Catoire, V., Goutail, F., Pommereau, J.-P., and McLinden, C. A.: Improved OSIRIS NO2 retrieval algorithm: description and validation, Atmos. Meas. Tech., 10, 1155–1168, https://doi.org/10.5194/amt-10-1155-2017, 2017. a, b
Taha, G., Rault, D. F., Loughman, R. P., Bourassa, A. E., and von Savigny, C.: SCIAMACHY stratospheric aerosol extinction profile retrieval using the OMPS/LP algorithm, Atmos. Meas. Tech., 4, 547–556, https://doi.org/10.5194/amt-4-547-2011, 2011. a
Taha, G., Loughman, R., Zhu, T., Thomason, L., Kar, J., Rieger, L., and Bourassa, A.: OMPS LP Version 2.0 multi-wavelength aerosol extinction coefficient retrieval algorithm, Atmos. Meas. Tech., 14, 1015–1036, https://doi.org/10.5194/amt-14-1015-2021, 2021.
a
Thomason, L. W., Ernest, N., Millán, L., Rieger, L., Bourassa, A., Vernier, J.-P., Manney, G., Luo, B., Arfeuille, F., and Peter, T.: A global space-based stratospheric aerosol climatology: 1979–2016, Earth Syst. Sci. Data, 10, 469–492, https://doi.org/10.5194/essd-10-469-2018, 2018. a
von Savigny, C., Ernst, F., Rozanov, A., Hommel, R., Eichmann, K.-U., Rozanov, V., Burrows, J. P., and Thomason, L. W.: Improved stratospheric aerosol extinction profiles from SCIAMACHY: validation and sample results, Atmos. Meas. Tech., 8, 5223–5235, https://doi.org/10.5194/amt-8-5223-2015, 2015. a, b
Waters, J. W., Froidevaux, L., Harwood, R. S., Jarnot, R. F., Pickett, H. M.,
Read, W. G., Siegel, P. H., Cofield, R. E., Filipiak, M. J., Flower, D. A.,
Holden, J. R., Lau, G. K., Livesey, N. J., Manney, G. L., Pumphrey, H. C.,
Santee, M. L., Wu, D. L., Cuddy, D. T., Lay, R. R., Loo, M. S., Perun, V. S.,
Schwartz, M. J., Stek, P. C., Thurstans, R. P., Boyles, M. A., Chandra,
K. M., Chavez, M. C., Chen, G. S., Chudasama, B. V., Dodge, R., Fuller,
R. A., Girard, M. A., Jiang, J. H., Jiang, Y., Knosp, B. W., Labelle, R. C.,
Lam, J. C., Lee, K. A., Miller, D., Oswald, J. E., Patel, N. C., Pukala,
D. M., Quintero, O., Scaff, D. M., Van Snyder, W., Tope, M. C., Wagner,
P. A., and Walch, M. J.: The Earth Observing System Microwave Limb
Sounder (EOS MLS) on the aura satellite, IEEE T.
Geosci. Remote, 44, 1075–1092,
https://doi.org/10.1109/TGRS.2006.873771, 2006. a
Wiscombe, W. J.: Improved Mie scattering algorithms, Appl. Optics, 19,
1505–1509, 1980. a
Zawada, D., Franssens, G., Loughman, R., Mikkonen, A., Rozanov, A., Emde, C.,
Bourassa, A., Dueck, S., Lindqvist, H., Ramon, D., Rozanov, V., Dekemper, E.,
Kyrölä, E., Burrows, J. P., Fussen, D., and Degenstein, D.: Radiance data
for “Systematic Comparison of Vectorial Spherical Radiative Transfer Models
in Limb Scattering Geometry” by Zawada et al., Zenodo, https://doi.org/10.5281/zenodo.4292303,
2020. a, b
Zawada, D. J., Rieger, L. A., Bourassa, A. E., and Degenstein, D. A.: Tomographic retrievals of ozone with the OMPS Limb Profiler: algorithm description and preliminary results, Atmos. Meas. Tech., 11, 2375–2393, https://doi.org/10.5194/amt-11-2375-2018, 2018. a
Short summary
Satellite measurements of atmospheric composition often rely on computer tools known as radiative transfer models to model the propagation of sunlight within the atmosphere. Here we have performed a detailed inter-comparison of seven different radiative transfer models in a variety of conditions. We have found that the models agree remarkably well, at a level better than previously reported. This result provides confidence in our understanding of atmospheric radiative transfer.
Satellite measurements of atmospheric composition often rely on computer tools known as...
